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Selective separation of heat-generating nuclide from high-level liquid wastes and application of internal irradiation therapy of cancer

Research Project

Project/Area Number 25289349
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypePartial Multi-year Fund
Section一般
Research Field Nuclear engineering
Research InstitutionTohoku University

Principal Investigator

Kim Seong-Yun  東北大学, 工学(系)研究科(研究院), 准教授 (50574357)

Co-Investigator(Kenkyū-buntansha) FUNAKI Yoshihito  東北大学, サイクロトロン・ラジオアイソトープセンター, 講師 (50261491)
Xu Yuanlai  東北大学, サイクロトロン・ラジオアイソトープセンター, 助教 (10643992)
ISHII Keizo  東北大学, 工学研究科, 教授 (00134065)
MATSUYAMA Shigeo  東北大学, 工学研究科, 准教授 (70219525)
KIKUCHI Yohei  東北大学, 工学研究科, 准教授 (50359535)
ITO Tatsuya  東北大学, 工学研究科, 助教 (20757653)
Project Period (FY) 2013-04-01 – 2016-03-31
Project Status Completed (Fiscal Year 2015)
Budget Amount *help
¥17,030,000 (Direct Cost: ¥13,100,000、Indirect Cost: ¥3,930,000)
Fiscal Year 2015: ¥1,950,000 (Direct Cost: ¥1,500,000、Indirect Cost: ¥450,000)
Fiscal Year 2014: ¥9,750,000 (Direct Cost: ¥7,500,000、Indirect Cost: ¥2,250,000)
Fiscal Year 2013: ¥5,330,000 (Direct Cost: ¥4,100,000、Indirect Cost: ¥1,230,000)
Keywords保健物理 / 環境安全 / 放射性廃棄物 / 放射線医学 / 保険物理
Outline of Final Research Achievements

To separate Cs(I) and Sr(II), which are heat-generating nuclides, from high-level liquid waste (HLLW) generated from spent nuclear fuel reprocessing selectively and efficiently, an innovative separation process of the nuclides have been developed by using novel macroporous silica-based adsorbents based on extraction chromatography method. Moreover, a new purification process of the recovered nuclides based on extraction chromatography method was investigated and the process was used for internal irradiation therapy of cancer is proved and radiotherapy technique using a novel Y-labeled radiopharmaceutical.

Report

(4 results)
  • 2015 Annual Research Report   Final Research Report ( PDF )
  • 2014 Annual Research Report
  • 2013 Annual Research Report
  • Research Products

    (23 results)

All 2016 2015 2014 2013

All Journal Article (6 results) (of which Peer Reviewed: 5 results,  Acknowledgement Compliant: 2 results) Presentation (16 results) Funded Workshop (1 results)

  • [Journal Article] Adsorption behavior and Radiation Effects of a Silica-based (Calix[4]+Dodecanol)/SiO2-P Adsorbent for Selective Separation of Cs(I) from High Level Liquid Waste2016

    • Author(s)
      Tatsuya Ito, Yuanlai Xu, Seong-Yun Kim, Ryuji Nagaishi, Takaumi Kimura
    • Journal Title

      Separation Science and Technology

      Volume: 51 Issue: 1 Pages: 22-31

    • DOI

      10.1080/01496395.2015.1085877

    • Related Report
      2015 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Investigation on Selective Separation of Sr(II) from High Level Liquid Waste Using a Macroporous Silica-based Absorbent2015

    • Author(s)
      Seong-Yun Kim, Tatsuya Ito, Yuanlai Xu, Keitaro Hitomi, Keizo Ishii
    • Journal Title

      GLOBAL2015

      Volume: 5170 Pages: 1575-1581

    • Related Report
      2015 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Discussion on Applicability of Macroporous Silica-based Adsorbents to Multistep Partitioning Process of High Level Liquid Waste2015

    • Author(s)
      Tatsuya Ito, Seong-Yun Kim, Yuanlai Xu, Atsushi Yoshida, Keitaro Hitomi, Keizo Ishii
    • Journal Title

      GLOBAL2015

      Volume: 5173 Pages: 1590-1596

    • Related Report
      2015 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Adsorption behavior of trivalent americium and rare earth ions onto a macroporous silica-based isobutyl-BTP/SiO2-P adsorbent in nitric acid solution2014

    • Author(s)
      Yuanlai Xu, Seong-Yun Kim, Tatsuya Ito, Keitaro Hitomi, Etsushu Kuraoka, Shigekazu Usuda, Keizo Ishii
    • Journal Title

      Journal of Radioanalytical and Nuclear Chemistry

      Volume: 299 Issue: 1 Pages: 149-155

    • DOI

      10.1007/s10967-013-2747-9

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Extraction of Cesium and Strontium from Nitric Acid Solution using Ionic liquids2014

    • Author(s)
      Takahashi T., Kim S.-Y., Tokuda H., Hitomi K. and Ishii K.
    • Journal Title

      CYRIC Annual Report 2012-2013

      Volume: VI.5 Pages: 113-117

    • Related Report
      2014 Annual Research Report
  • [Journal Article] Adsorption and desorption behavior of tetravalent zirconium onto a silica-based macroporous TODGA adsorbent in HNO3 solution2013

    • Author(s)
      Yuanlai Xu, Seong-Yun Kim, Shigekazu Usuda, Yuezhou Wei, Keizo Ishii
    • Journal Title

      Journal of Radioanalytical and Nuclear Chemistry

      Volume: 297 Issue: 1 Pages: 91-96

    • DOI

      10.1007/s10967-012-2355-0

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Presentation] イオン液体を用いた高レベル放射性廃液の分離プロセスの開発(4)カリックスアレーンクラウン6 誘導体を用いた硝酸溶液からのセシウム(I)の選択的抽出2016

    • Author(s)
      高橋正幸、伊藤辰也、金聖潤
    • Organizer
      日本原子力学会「2016年春の年会」
    • Place of Presentation
      宮城県仙台市青葉区片平・東北大学川内キャンパス
    • Year and Date
      2016-03-26
    • Related Report
      2015 Annual Research Report
  • [Presentation] 高レベル放射性廃液中からの発熱性元素の高選択分離法の開発(1)カリックスクラウン含有イオン液体含浸吸着材による吸着・分離特性2016

    • Author(s)
      工藤達矢、伊藤辰也、金聖潤
    • Organizer
      日本原子力学会「2016年春の年会」
    • Place of Presentation
      宮城県仙台市青葉区片平・東北大学川内キャンパス
    • Year and Date
      2016-03-26
    • Related Report
      2015 Annual Research Report
  • [Presentation] 含浸吸着材を用いた高レべル放射性廃液中からのSr(II)の選択的分離とその医療応用2015

    • Author(s)
      金聖潤、伊藤辰也、長野宣道、人見啓太朗、石井慶造
    • Organizer
      2015年日本イオン交換学会・日本溶媒抽出学会連合年会
    • Place of Presentation
      石川県野々市市扇が丘・金沢工業大学 扇が丘キャンパス
    • Year and Date
      2015-10-23
    • Related Report
      2015 Annual Research Report
  • [Presentation] クラウンエーテル含有イオン液体抽出系を用いた硝酸溶液からのSr(II)の抽出特性2015

    • Author(s)
      高橋正幸、伊藤辰也、長野宣道、人見啓太朗、石井慶造、金聖潤、徳田玄明
    • Organizer
      2015年日本イオン交換学会・日本溶媒抽出学会連合年会
    • Place of Presentation
      石川県野々市市扇が丘・金沢工業大学 扇が丘キャンパス
    • Year and Date
      2015-10-23
    • Related Report
      2015 Annual Research Report
  • [Presentation] イオン液体を用いた高レベル放射性廃液の分離プロセスの開発;(3)DtBuCH18C6を用いたイオン液体抽出系における硝酸溶液からのストロンチウムの選択的分離2015

    • Author(s)
      高橋正幸、伊藤辰也、徳田玄明、長野宣道、人見啓太朗、石井慶造、金聖潤
    • Organizer
      日本原子力学会「2015年秋の大会」
    • Place of Presentation
      静岡県静岡市 駿河区大谷・静岡大学静岡キャンパス
    • Year and Date
      2015-09-09
    • Related Report
      2015 Annual Research Report
  • [Presentation] 多孔性シリカ担持型吸着材を用いたストロンチウムとイットリウムの分離に関する研究(I)2015

    • Author(s)
      田村知也、高橋正幸、徳田玄明、人見啓太郎、石井慶造、金聖潤
    • Organizer
      日本原子力学会「2015年春の年会」
    • Place of Presentation
      茨城大学日立キャンパス、茨城県日立市中成沢町
    • Year and Date
      2015-03-20 – 2015-03-22
    • Related Report
      2014 Annual Research Report
  • [Presentation] シリカ担持型吸着材を用いた高レベル放射性廃液の多段型核種分離プロセスの有用性検討;(2)シミュレーションによるプロセス評価2015

    • Author(s)
      伊藤辰也、吉田篤、金聖潤
    • Organizer
      日本原子力学会「2015年春の年会」
    • Place of Presentation
      茨城大学日立キャンパス、茨城県日立市中成沢町
    • Year and Date
      2015-03-20 – 2015-03-22
    • Related Report
      2014 Annual Research Report
  • [Presentation] イオン液体を用いた高レベル放射性廃液の分離プロセスの開発;(2)クラウンエーテルの化学修飾の違いによる抽出特性への影響2015

    • Author(s)
      高橋正幸、徳田玄明、人見啓太朗、石井慶造、金聖潤
    • Organizer
      日本原子力学会「2015年春の年会」
    • Place of Presentation
      茨城大学日立キャンパス、茨城県日立市中成沢町
    • Year and Date
      2015-03-20 – 2015-03-22
    • Related Report
      2014 Annual Research Report
  • [Presentation] Treatment of high level liquid waste using macroporous silica-based adsorbents2014

    • Author(s)
      Seong-Yun Kim
    • Organizer
      1st Korea-Japan Joint Technical Workshop on Energy Materials
    • Place of Presentation
      Pukyong National University, Busan, Korea
    • Year and Date
      2014-12-01 – 2014-12-02
    • Related Report
      2014 Annual Research Report
  • [Presentation] Feasibility of CT Imaging with Detection Module of High-Resolution CdTe-Semiconductor PET scanner2014

    • Author(s)
      Yohei Kikuchi, Seong-Yun Kim
    • Organizer
      World Molecular Imaging Congress 2014
    • Place of Presentation
      COEX Convention & Exhibition Center, Seoul, Korea
    • Year and Date
      2014-09-17 – 2014-09-20
    • Related Report
      2014 Annual Research Report
  • [Presentation] イオン液体を用いた高レベル放射性廃液の分離プロセスの開発;(1)分離プロセスの検討2014

    • Author(s)
      高橋正幸、徳田玄明、金聖潤、人見啓太郎、石井慶造
    • Organizer
      日本原子力学会「2014年秋の大会」
    • Place of Presentation
      京都大学、京都府京都市左京区吉田本町
    • Year and Date
      2014-09-08 – 2014-09-10
    • Related Report
      2014 Annual Research Report
  • [Presentation] シリカ担持型吸着材を用いた高レベル放射性廃液の多段型核種分離プロセスの有用性検討2014

    • Author(s)
      伊藤辰也、金聖潤、永石隆二、木村貴海
    • Organizer
      日本原子力学会「2014年秋の大会」
    • Place of Presentation
      京都大学、京都府京都市左京区吉田本町
    • Year and Date
      2014-09-08 – 2014-09-10
    • Related Report
      2014 Annual Research Report
  • [Presentation] 高レベル放射性廃液中(HLLW)からの発熱性核種の分離技術の開発2014

    • Author(s)
      船木善仁、菊池洋平、金聖潤
    • Organizer
      日本薬学会第134年会
    • Place of Presentation
      熊本大学黒髪キャンパス
    • Related Report
      2013 Annual Research Report
  • [Presentation] Study on Adsorption and Separation Behavior of Strontium and Yttrium with Macroporous Silica Based Adsorbents2013

    • Author(s)
      Yuanlai Xu, Seong-Yun Kim, Yoshihito Funaki, Keitaro Hitomi, Keizo Ishii
    • Organizer
      日本原子力学会「2013年秋の大会」
    • Place of Presentation
      八戸工業大学
    • Related Report
      2013 Annual Research Report
  • [Presentation] Selective Separation of Cesium from Simulated High Level Liquid Waste using a Silica-based (Calix[4] + Dodecanol)/SiO2-P Adsorbent2013

    • Author(s)
      Yuanlai Xu, Seong-Yun Kim, Tatsuya Ito, Haruki Tokuda, Tsutomu Tada, Keitaro Hitomi, Keizo Ishii
    • Organizer
      5th Asia-Pacific Symposium on Radiochemistry'13 (APSORC-13)
    • Place of Presentation
      金沢市文化ホール
    • Related Report
      2013 Annual Research Report
  • [Presentation] Adsorption and Separation Behavior of Strontium from Simulated High Level Liquid Waste using a Macroporous Silica-based DtBuCH18C6/SiO2-P Absorbent2013

    • Author(s)
      Yuanlai Xu, Seong-Yun Kim, Tatsuya Ito, Haruki Tokuda, Keitaro Hitomi, Keizo Ishii
    • Organizer
      The 4th International Symposium on Innovative Nuclear Energy Systems(INES-4)
    • Place of Presentation
      東工大蔵前会館・ロイヤルブルーホール
    • Related Report
      2013 Annual Research Report
  • [Funded Workshop] Global 20152015

    • Place of Presentation
      パリ(フランス)
    • Year and Date
      2015-09-19
    • Related Report
      2015 Annual Research Report

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Published: 2013-05-21   Modified: 2019-07-29  

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