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Development of near-field transient absorption imaging spectrometer and its application to nex-generation organic solar cells

Research Project

Project/Area Number 25390061
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeMulti-year Fund
Section一般
Research Field Applied materials
Research InstitutionNational Institute of Advanced Industrial Science and Technology

Principal Investigator

MATSUZAKI HIROYUKI  国立研究開発法人産業技術総合研究所, 分析計測標準研究部門, 主任研究員 (80422400)

Project Period (FY) 2013-04-01 – 2016-03-31
Project Status Completed (Fiscal Year 2015)
Budget Amount *help
¥5,200,000 (Direct Cost: ¥4,000,000、Indirect Cost: ¥1,200,000)
Fiscal Year 2015: ¥910,000 (Direct Cost: ¥700,000、Indirect Cost: ¥210,000)
Fiscal Year 2014: ¥1,560,000 (Direct Cost: ¥1,200,000、Indirect Cost: ¥360,000)
Fiscal Year 2013: ¥2,730,000 (Direct Cost: ¥2,100,000、Indirect Cost: ¥630,000)
Keywordsフェムト秒過渡吸収分光 / 有機薄膜太陽電池 / バルクへテロ接合 / 顕微分光 / 近接場光学顕微鏡 / バルクヘテロ接合
Outline of Final Research Achievements

By combining the optical microscopy including near-filed optical microscopy and femtosecond time-resolved transient absorption spectroscopy, I have performed the development of the transient absorption absorption imaging spectrometer with high spatial resolution, and I am mow in the phase of its appplication to real materials and devices. In particular, I have achieved the development of the high-sensitive system which can detect very weak transient absorption signal (< 5×10-5). By utilizing such high sensitivity, I have succeeded in performing the femtosecond time-resolved transient absorption measurments of the organic thin-film solar cell undeer very low excitation density. Based on the result, I have calrified the details of charge generation processes in the organic thin-film solar cell.

Report

(4 results)
  • 2015 Annual Research Report   Final Research Report ( PDF )
  • 2014 Research-status Report
  • 2013 Research-status Report
  • Research Products

    (35 results)

All 2016 2015 2014 2013 Other

All Journal Article (19 results) (of which Int'l Joint Research: 1 results,  Peer Reviewed: 19 results,  Open Access: 1 results,  Acknowledgement Compliant: 8 results) Presentation (15 results) (of which Int'l Joint Research: 1 results,  Invited: 2 results) Patent(Industrial Property Rights) (1 results)

  • [Journal Article] 励起光波長の選択によってモット絶縁体を金属と電荷密度波に転換する ~相関電子系の新しい光相制御~2016

    • Author(s)
      松﨑弘幸, 岩野薫, 岡本博
    • Journal Title

      日本物理学会誌

      Volume: 71 Pages: 311-317

    • Related Report
      2015 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Photoinduced Switching to Metallic States in the Two-Dimensional Organic Mott Insulator Dimethylphenazine-Tetrafluorotetracyanoquinodimethane with Anisotropic Molecular Stacks2015

    • Author(s)
      H. Matsuzaki, M. Ohkura, Y. Ishige, Y. Nogami, and H. Okamoto
    • Journal Title

      Phys. Rev. B

      Volume: 91 Issue: 24

    • DOI

      10.1103/physrevb.91.245140

    • Related Report
      2015 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Modulation of Electron Injection Dynamics of Ru‐Based Dye/TiO2 System in the Presence of Three Different Organic Solvents: Role of Solvent Dipole Moment and Donor Number2015

    • Author(s)
      Subrata Mahanta, Hiroyuki Matsuzaki, Takurou N Murakami, Ryuzi Katoh, Hajime Matsumoto, Akihiro Furube
    • Journal Title

      ChemPhysChem

      Volume: 16 Pages: 1657-1662

    • Related Report
      2015 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] In situ picosecond transient diffuse reflectance spectroscopy of opaque TiO2 systems under microwave irradiation and influence of oxygen vacancies on the UV-driven/microwave-assisted TiO2 photocatalysis2015

    • Author(s)
      Satoshi Horikoshi, Hideya Tsutsumi, Hiroyuki Matsuzaki, Akihiro Furube, Alexei V Emeline, Nick Serpone
    • Journal Title

      Journal of Materials Chemistry C

      Volume: 3 Issue: 23 Pages: 5958-5969

    • DOI

      10.1039/c4tc02748e

    • Related Report
      2015 Annual Research Report
    • Peer Reviewed / Int'l Joint Research / Acknowledgement Compliant
  • [Journal Article] Ultrafast Charge and Lattice Dynamics in One-dimensional Mott insulator of CuO-chain Compound Ca2CuO3 Investigated by Femtosecond Absorption Spectroscopy2015

    • Author(s)
      H. Matsuzaki, H. Nishioka, H. Uemura, A. Sawa, S. Sota, T. Tohyama, and H. Okamoto
    • Journal Title

      Phys. Rev. B

      Volume: 91 Issue: 8

    • DOI

      10.1103/physrevb.91.081114

    • Related Report
      2014 Research-status Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Formation of relaxed charge-transfer excitons in donor-acceptor-type polymer solar cells2014

    • Author(s)
      J. Tsutsumi, H. Matsuzaki, N. Kanai, T. Yamada, and T. Hasegawa
    • Journal Title

      Jpn. J. Appl. Phys.

      Volume: 53 Issue: 5S3 Pages: 05HB12-05HB12

    • DOI

      10.7567/jjap.53.05hb12

    • Related Report
      2014 Research-status Report
    • Peer Reviewed
  • [Journal Article] Dye Aggregation Effect on Interfacial Electron-Transfer Dynamics in Zinc Phthalocyanine-Sensitized Solar Cells2014

    • Author(s)
      Hiroyuki Matsuzaki, Takurou N Murakami, Naruhiko Masaki, Akihiro Furube, Mutsumi Kimura, Shogo Mori
    • Journal Title

      The Journal of Physical Chemistry C

      Volume: 118 Issue: 31 Pages: 17205-17212

    • DOI

      10.1021/jp500798c

    • Related Report
      2014 Research-status Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Excitation-Photon-Energy Selectivity of Photoconversions in Halogen-Bridged Pd-Chain Compounds: Mott Insulator to Metal or Charge-Density-Wave State2014

    • Author(s)
      H. Matsuzaki, M. Iwata, T. Miyamoto, T. Terashige, K. Iwano, S. Takaishi, M. Takamura, S. Kumagai, M. Yamashita, R. Takahashi, Y. Wakabayashi, and H. Okamoto
    • Journal Title

      Phys. Rev. lett.

      Volume: 113 Issue: 9 Pages: 096403-096403

    • DOI

      10.1103/physrevlett.113.096403

    • Related Report
      2014 Research-status Report
    • Peer Reviewed
  • [Journal Article] Continuous Control of Optical Gaps in Quasi-One-Dimensional Bromide-Bridged Platinum Complexes by Utilizing Chemical Pressure2014

    • Author(s)
      Shohei Kumagai, Hiroaki Iguchi, Shinya Takaishi, Brian K Breedlove, Masahiro Yamashita, Hiroyuki Matsuzaki, Hiroshi Okamoto, Kenichi Kato, Masaki Takata
    • Journal Title

      Inorganic chemistry

      Volume: 53 Issue: 21 Pages: 11764-11769

    • DOI

      10.1021/ic502071u

    • Related Report
      2014 Research-status Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Electron transport in TTF-CA under high pressures2014

    • Author(s)
      R. Takehara, K. Miyagawa, K. Kanoda, T. Miyamoto, H. Matsuzaki, H. Okamoto, H. Taniguchi, K. Matsubayashi, Y. Uwatoko
    • Journal Title

      Physica B: Condensed Matter

      Volume: 460 Pages: 83-87

    • DOI

      10.1016/j.physb.2014.11.045

    • Related Report
      2014 Research-status Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Trapped State Sensitive Kinetics in LaTiO2N Solid Photocatalyst with and without Cocatalyst Loading2014

    • Author(s)
      Rupashree Balia Singh, Hiroyuki Matsuzaki, Yohichi Suzuki, Kazuhiko Seki, Tsutomu Minegishi, Takashi Hisatomi, Kazunari Domen, Akihiro Furube
    • Journal Title

      Journal of the American Chemical Society

      Volume: 136 Issue: 49 Pages: 17324-17331

    • DOI

      10.1021/ja5102823

    • Related Report
      2014 Research-status Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Kinetics of Distance-Dependent Recombination between Geminate Charge Carriers by Diffusion under Coulomb Interaction2014

    • Author(s)
      Yohichi Suzuki, Akihiro Furube, Rupashree Balia Singh, Hiroyuki Matsuzaki, Tsutomu Minegishi, Takashi Hisatomi, Kazunari Domen, Kazuhiko Seki
    • Journal Title

      The Journal of Physical Chemistry C

      Volume: 119 Issue: 10 Pages: 5364-5373

    • DOI

      10.1021/acs.jpcc.5b00417

    • Related Report
      2014 Research-status Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Photocarrier dynamics in anatase TiO2 investigated by pump-probe absorption spectroscopy2014

    • Author(s)
      Hiroyuki Matsuzaki, Yuta Matsui, Ryusuke Uchida, Hiroyuki Yada1, Tsubasa Terashige, B.-S. Li, Akihiro Sawa, Masashi Kawasaki, Yoshinori Tokura, and Hiroshi Okamoto
    • Journal Title

      JOURNAL OF APPLIED PHYSICS

      Volume: 115 Issue: 18

    • DOI

      10.1063/1.4829456

    • Related Report
      2013 Research-status Report
    • Peer Reviewed
  • [Journal Article] Excited-State dynamics in diketopyrrolopyrrole-based copolymer for organic photovoltaics investigated by transient optical spectroscopy2013

    • Author(s)
      Hiroyuki Matsuzaki、Akihiro Furube、Ryuzi Katoh, Samarendra P. Singh, Prashant Sonar, Evan Laurence Williams, Vijila Chellappan, Gomathy Sandhya Subramanian, Sergey Gorelik, and Jonathan Hobley
    • Journal Title

      JAPANESE JOURNAL OF APPLIED PHYSICS

      Volume: 53 Issue: 1S Pages: 01AB11-01AB11

    • DOI

      10.7567/jjap.53.01ab11

    • NAID

      210000143269

    • Related Report
      2013 Research-status Report
    • Peer Reviewed
  • [Journal Article] Charge separation of charge-transfer excitons in donor-acceptor polymer solar cells2013

    • Author(s)
      J. Tsutsumi, H. Matsuzaki, N. Kanai, T. Yamada, and T. Hasegawa
    • Journal Title

      J. Phys. Chem. C

      Volume: 117 Issue: 33 Pages: 16769-16769

    • DOI

      10.1021/jp404094e

    • Related Report
      2013 Research-status Report
    • Peer Reviewed
  • [Journal Article] Nanoscale phase domain structure and associated device performance of organic solar cells based on a diketopyrrolopyrrole polymer2013

    • Author(s)
      Evan L. Williams, Sergey Gorelik, InYee Phang, Michel Bosman, Chellappan Vijila, Gomathy Sandhya Subramanian, Prashant Sonar, Jonathan Hobley, Samarendra P. Singh, Hiroyuki Matsuzaki, Akihiro Furube, and Ryuzi Katoh
    • Journal Title

      RSC ADVANCES

      Volume: 3 Issue: 43 Pages: 20113-20124

    • DOI

      10.1039/c3ra42636j

    • Related Report
      2013 Research-status Report
    • Peer Reviewed
  • [Journal Article] Measurement of a photoinduced transition from a nonordered phase to a transient ordered phase in the organic quantum-paraelectric compound dimethyltetrathiafulvalene-dibromodichloro-p-benzoquinone using femtosecond laser irradiation2013

    • Author(s)
      T. Miyamoto, K. Kimura, T. Hamamoto, H. Uemura, H. Yada, H. Matsuzaki, S. Horiuchi, and H. Okamoto
    • Journal Title

      Physical Review Letters

      Volume: 111 Issue: 18

    • DOI

      10.1103/physrevlett.111.187801

    • Related Report
      2013 Research-status Report
    • Peer Reviewed
  • [Journal Article] Smallest Optical Gap for Quasi-One-Dimensional Iodo-bridged Platinum Compounds2013

    • Author(s)
      Minseob Shin, Shinya Takaishi, Shohei Kumagai, Yutaro Ueda, Brian K. Breedlove, Hiroyuki Matsuzaki, Hiroshi Okamoto, Yusuke Wakabayashi, and Masahiro Yamashita
    • Journal Title

      DALTON TRANSACTIONS

      Volume: 42 Issue: 18 Pages: 6277-6280

    • DOI

      10.1039/c3dt32890b

    • Related Report
      2013 Research-status Report
    • Peer Reviewed
  • [Journal Article] Molecular Design Rule of Phthalocyanine Dyes for Highly Efficient Near-IR Performance in Dye Sensitized Solar Cells2013

    • Author(s)
      Mutsumi Kimura, Hirotaka Nomoto, Hiroyuki Suzuki, Takuro Ikeuci, Hiroyuki Matsuzaki, Takuro N. Murakami, Dr. Akihiko Furube, Naruhiko Masaki, Matthew J. Griffith, and Shogo Mori
    • Journal Title

      CHEMISTRY-A EUROPEAN JOURNAL

      Volume: 19 Issue: 23 Pages: 7496-7502

    • DOI

      10.1002/chem.201300716

    • Related Report
      2013 Research-status Report
    • Peer Reviewed
  • [Presentation] Photoinduced switching to metallic states in a two-dimensional organic charge-transfer complex dimethylphenazine-tetrafluorotetracyanoquinodimethane with anisotropic molecular stacks2015

    • Author(s)
      Hiroyuki Matsuzaki, Masa-aki Ohkura, Yu Ishige, Yoshio Nogami, Hiroshi Okamoto
    • Organizer
      The International Chemical Congress of Pacific Basin Societies 2015 (Pacifichem 2015)
    • Place of Presentation
      ハワイ州ホノルル市(アメリカ合衆国)
    • Year and Date
      2015-12-15
    • Related Report
      2015 Annual Research Report
  • [Presentation] 一次元銅酸化物Ca2CuO3における超高速電荷・格子ダイナミクス2015

    • Author(s)
      松﨑弘幸, 西岡大毅, 上村紘崇, 澤彰仁, 曽田繁利, 遠山貴巳, 岡本博
    • Organizer
      日本物理学会2015年秋季大会
    • Place of Presentation
      関西大学 千里山キャンパス(大阪府吹田市)
    • Year and Date
      2015-09-16
    • Related Report
      2015 Annual Research Report
  • [Presentation] 超高速分光によるLaTiO2N・TaON混合光触媒におけるキャリアダイナミクス2015

    • Author(s)
      DHARMAPURA H. Murthy Krishna, 秋山誠治, 松﨑弘幸, 古部昭広, 関和彦, 鈴木洋一, Min Liu, 久富隆史, 嶺岸耕, 山田太郎, 堂免一成
    • Organizer
      2015年光化学討論会
    • Place of Presentation
      大阪市立大学 杉本キャンパス(大阪府住吉区杉本)
    • Year and Date
      2015-09-09
    • Related Report
      2015 Annual Research Report
  • [Presentation] 過渡吸収分光法を用いた有機多層膜中における劣化層の特定2015

    • Author(s)
      東遥介, 高橋永次, 藤原豊, 松﨑弘幸, 古部 昭広
    • Organizer
      有機EL討論会第20回例会
    • Place of Presentation
      千葉大学西千葉キャンパスけやき会館(千葉県千葉市稲毛区)
    • Year and Date
      2015-06-18
    • Related Report
      2015 Annual Research Report
  • [Presentation] Photoexcited-State Dynamics in Organic Solar Cells Utilizing Diketopyrrolopyrrole-Based Copolymer Investigated By Transient Optical Spectroscopy2015

    • Author(s)
      Hiroyuki Matsuzaki, Akihiro Furube, Ryuzi Katoh, Samarendra P. Singh, Prashant Sonar, Evan Laurence Williams, Vijila Chellappan, Gomathy Sandhya Subramanian, Sergey Gorelik, Jonathan Hobley
    • Organizer
      The 227th ECS Metting
    • Place of Presentation
      イリノイ州シカゴ市(アメリカ合衆国)
    • Year and Date
      2015-05-24
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] 一次元臭素架橋Pd錯体における励起光波長による選択的光相制御:モット絶縁体-金属転移とモット絶縁体-電荷密度波相転移2015

    • Author(s)
      松﨑 弘幸、寺重 翼、宮本辰也、岡本 博、熊谷翔平、高石慎也、山下 正廣、岩野薫、高橋亮、若林裕助
    • Organizer
      日本物理学会第70回年次大会
    • Place of Presentation
      早稲田大学 早稲田キャンパス(東京都新宿区)
    • Year and Date
      2015-03-21
    • Related Report
      2014 Research-status Report
  • [Presentation] パルスレーザ光照射による大気中光電子放出2015

    • Author(s)
      細貝 拓也、松﨑 弘幸、古部 昭広、中村 健
    • Organizer
      2015年第62回応用物理学会春季学術講演会
    • Place of Presentation
      東海大学湘南キャンパス(神奈川県平塚市)
    • Year and Date
      2015-03-14
    • Related Report
      2014 Research-status Report
  • [Presentation] 過渡吸収分光法による熱活性型遅延蛍光分子の励起状態の研究2014

    • Author(s)
      細貝 拓也、古部 昭広、松﨑 弘幸、徳丸克己、吉岡俊博、筒井哲夫、中野谷一、八尋正幸、安達千波矢
    • Organizer
      有機EL討論会第19回例会
    • Place of Presentation
      沖縄県市町村自治会館(沖縄県那覇市)
    • Year and Date
      2014-11-28 – 2014-11-29
    • Related Report
      2014 Research-status Report
  • [Presentation] ジケトピロロピロール骨格を有するドナー・アクセプター型コポリマーを用いた有機太陽電池における光励起状態ダイナミクス2014

    • Author(s)
      松﨑 弘幸、古部 昭広、加藤 隆二、Sergey Gorelik、Evan Laurence Williams、Vijila Chellappan、Gomathy Sandhya Subramanian、Jonathan Hobley、Prashant Sonar、Samarendra P. Singh
    • Organizer
      2014年第75回応用物理学会秋季学術講演会
    • Place of Presentation
      北海道大学札幌キャンパス(北海道札幌市)
    • Year and Date
      2014-09-17
    • Related Report
      2014 Research-status Report
  • [Presentation] Dye Aggregation Effect on Interfacial Electron-Transfer Dynamics in Zinc Phthalocyanine-Sensitized Solar Cells2014

    • Author(s)
      松崎 弘幸、村上 拓郎、正木 成彦、古部 昭広、木村 睦、森正悟
    • Organizer
      The 20th International Conference on Conversion and Storage of Solar Energy (IPS-20)
    • Place of Presentation
      マリティムホテル(ドイツ ベルリン市)
    • Year and Date
      2014-07-29
    • Related Report
      2014 Research-status Report
  • [Presentation] 亜鉛フタロシアニン錯体を用いた色素増感太陽電池における界面電子移動ダイナミクス

    • Author(s)
      松崎 弘幸、古部 昭広、村上 拓郎、正木 成彦、森 正悟、木村 睦
    • Organizer
      光化学討論会
    • Place of Presentation
      愛媛大学城北地区
    • Related Report
      2013 Research-status Report
  • [Presentation] 電荷移動錯体DBTTF-TCNQ結晶のフェムト秒ポンププローブ分光

    • Author(s)
      松崎 弘幸、堤 潤也、長谷川 達生
    • Organizer
      日本物理学会2013年秋季大会
    • Place of Presentation
      徳島大学常三島キャンパス
    • Related Report
      2013 Research-status Report
  • [Presentation] Femtosecond absorption spectroscopy of bulk heterojunction solar cells utilizing a diketopyrrolopyrrole polymer

    • Author(s)
      Hiroyuki Matsuzaki、Akihiro Furube、Ryuzi Katoh, Samarendra P. Singh, Prashant Sonar, Evan Laurence Williams, Vijila Chellappan, Gomathy Sandhya Subramanian, Sergey Gorelik, and Jonathan Hobley
    • Organizer
      第26回光化学に関する国際会議(ICP2013)
    • Place of Presentation
      ルーヴァン・カトリッ ク大学(ベルギー王国ルーヴァン市)
    • Related Report
      2013 Research-status Report
  • [Presentation] 可視-近赤外過渡吸収分光装置 ~色素増感太陽電池の開発に威力を発揮~

    • Author(s)
      松崎 弘幸
    • Organizer
      第3回次世代ものづくり基盤技術産業展(TECH Biz EXPO 2013)
    • Place of Presentation
      ボートメッセなごや
    • Related Report
      2013 Research-status Report
    • Invited
  • [Presentation] 新規Diketopyrrolopyrrole系OPV材料の電荷再結合過程:高感度過渡吸収分光による検討

    • Author(s)
      Ryuzi Katoh, Hiroyuki Matsuzaki, Akihiro Furube, Gomathy Sandhya Subramanian, Evan Laurence Williams, Vijila Chellappan, Sergey Gorelik, Jonathan Hobley and Samarendra P. Singh
    • Organizer
      光化学討論会
    • Place of Presentation
      愛媛大学城北地区
    • Related Report
      2013 Research-status Report
  • [Patent(Industrial Property Rights)] 多層膜の評価方法2015

    • Inventor(s)
      松﨑弘幸, 東遥介, 髙橋永次, 藤原豊
    • Industrial Property Rights Holder
      国立研究開発法人産業技術総合研究所, 株式会社住化分析センター
    • Industrial Property Rights Type
      特許
    • Industrial Property Number
      2015-231084
    • Filing Date
      2015-11-26
    • Related Report
      2015 Annual Research Report

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Published: 2014-07-25   Modified: 2019-07-29  

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