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Scaling in the correlations of inhomogeneous domains in functional materials

Research Project

Project/Area Number 25400355
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeMulti-year Fund
Section一般
Research Field Condensed matter physics II
Research Institution一般財団法人総合科学研究機構(総合科学研究センター(総合科学研究室)及び中性子科学センター(研究開発

Principal Investigator

Matsuura Masato  一般財団法人総合科学研究機構(総合科学研究センター(総合科学研究室)及び中性子科, 中性子科学センター, 副主任研究員 (30376652)

Co-Investigator(Renkei-kenkyūsha) ENDO HITOSHI  高エネルギー加速器研究機構, 物質構造科学研究所, 准教授 (40447313)
Research Collaborator KOREEDA AKITOSHI  立命館大学, 教授 (40323878)
Gehring Peter  NIST Center for Neutron Research, Researcher
Xu Guangyong  NIST Center for Neutron Research, Researcher
Project Period (FY) 2013-04-01 – 2017-03-31
Project Status Completed (Fiscal Year 2016)
Budget Amount *help
¥4,810,000 (Direct Cost: ¥3,700,000、Indirect Cost: ¥1,110,000)
Fiscal Year 2015: ¥650,000 (Direct Cost: ¥500,000、Indirect Cost: ¥150,000)
Fiscal Year 2014: ¥650,000 (Direct Cost: ¥500,000、Indirect Cost: ¥150,000)
Fiscal Year 2013: ¥3,510,000 (Direct Cost: ¥2,700,000、Indirect Cost: ¥810,000)
Keywords巨大応答 / 不均一構造 / 自己相似性 / フラクタル次元 / リラクサー強誘電体 / 中性子準弾性散乱 / 中性子小角散乱 / マイクロドメイン / スケーリング指数
Outline of Final Research Achievements

In order to reveal microscopic mechanism of the giant response in relaxor ferroelectrics and manganites, we have used neutron scattering to study correlations of inhomogeneous nano-sized domains which are commonly observed in these functional materials. From scaling analysis on the correlation of inhomogeneous domains, we have clarified that sparse correlation due to inhomogeneity is one of the key for giant responses. In addition, we have discovered novel relaxation mode with incommensurate wave vector from MEM analysis on the distribution of relaxation modes. Furthermore, we have found nano-sized domains with low-crystal symmetry only in the inhomogeneous compounds but not in the homogeneous compound. Thus, we have succeeded in evaluating correlations of inhomogeneous domains quantitatively and have found some key elements of inhomogeneous correlations for giant responses.

Report

(5 results)
  • 2016 Annual Research Report   Final Research Report ( PDF )
  • 2015 Research-status Report
  • 2014 Research-status Report
  • 2013 Research-status Report
  • Research Products

    (26 results)

All 2017 2016 2015 2014 Other

All Int'l Joint Research (4 results) Journal Article (4 results) (of which Int'l Joint Research: 2 results,  Peer Reviewed: 4 results,  Acknowledgement Compliant: 1 results,  Open Access: 1 results) Presentation (18 results) (of which Int'l Joint Research: 3 results,  Invited: 7 results)

  • [Int'l Joint Research] Korea Atomic Energy Research Institute(韓国)

    • Related Report
      2016 Annual Research Report
  • [Int'l Joint Research] NIST/Brookhaven National Laboratory(米国)

    • Related Report
      2016 Annual Research Report
  • [Int'l Joint Research] KAERI(韓国)

    • Related Report
      2015 Research-status Report
  • [Int'l Joint Research] NIST/Brookhaven national laboratory/University of California, Berkeley(米国)

    • Related Report
      2015 Research-status Report
  • [Journal Article] Temperature dependence of the small angle neutron scattering in the relaxor (1-x)Pb(Mg1/3Nb2/3)O3-xPbTiO3 (x=0.30)2017

    • Author(s)
      M. Matsuura, A. Koreeda, Tae-Hwan Kim, and Young-Soo Han
    • Journal Title

      Ferroelectrics

      Volume: -

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Int'l Joint Research / Acknowledgement Compliant
  • [Journal Article] Negative correlation between electrical response and domain size in a Ti-composition-gradient Pb[(Mg1/3Nb2/3)1-xTix]O3 crystal near the morphotropic phase boundary2015

    • Author(s)
      Daisuke Shimizu, Shinya Tsukada, Masato Matsuura, Jun'ya Sakamoto, Seiji Kojima, Kazumichi Namikawa, Jun'ichiro Mizuki, and Kenji Ohwada
    • Journal Title

      Physical Review B

      Volume: 92 Issue: 17

    • DOI

      10.1103/physrevb.92.174121

    • Related Report
      2015 Research-status Report
    • Peer Reviewed
  • [Journal Article] The Performance of TOF near Backscattering Spectrometer DNA in MLF, J-PARC2015

    • Author(s)
      K. Shibata, N. Takahashi, Y. Kawakita, M. Matsuura, T. Yamada, T. Tominaga, W. Kambara, M. Kobayashi, Y. Inamura, T. Nakatani, K. Nakajima, and M. Arai
    • Journal Title

      JPS Conference Proceedings

      Volume: 8 Pages: 036022-036022

    • DOI

      10.7566/jpscp.8.036022

    • Related Report
      2015 Research-status Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Phase diagram of the relaxor ferroelectric (1-x)Pb(Mg1/3Nb2/3)O3+xPbTiO3 revisited -a neutron powder diffraction study of the relaxor skin effect2015

    • Author(s)
      D. Phelan, E.E. Rodriguez, J. Gao, Y. Bing, Z.-G. Ye, Q. Huang, Jinsheng Wen, Guangyong Xu, C. Stock, M. Matsuura, and P.M. Gehring
    • Journal Title

      Phase Transitions

      Volume: 88 Issue: 3 Pages: 1-23

    • DOI

      10.1080/01411594.2014.989226

    • Related Report
      2014 Research-status Report
    • Peer Reviewed
  • [Presentation] 中性子散乱で見えるもの~中性子散乱の特徴と誘電体・磁性体・マルチフェロイクス研究への応用例~2016

    • Author(s)
      松浦直人
    • Organizer
      誘電体・磁性体若手 夏の学校
    • Place of Presentation
      ルーセントタカミヤ(山形県・山形市)
    • Year and Date
      2016-08-26
    • Related Report
      2016 Annual Research Report
    • Invited
  • [Presentation] Temperature and composition dependence of the small angle neutron scattering in the relaxor (1-x)Pb(Mg1/3Nb2/3)O3-xPbTiO3 (x= 0.30 and 0.37)2016

    • Author(s)
      Masato Matsuura, Tae-Hwan Kim, Young-Soo Han, and Akitoshi Koreeda
    • Organizer
      Joint RCBJSF-IWRF conference
    • Place of Presentation
      くにびきメッセ(島根県・松江市)
    • Year and Date
      2016-06-20
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] J-PARCにおけるスローダイナミクス計測の現在と未来~BL02 DNA を用いたダイナミクスの高精度測定~2016

    • Author(s)
      松浦直人, 山田武, 富永大輝, 小林誠, 川北至信, 柴田薫
    • Organizer
      豊田理研特定課題研究第4回研究会「マルチプローブ融合利用による新奇強誘電体材料の物性解明」
    • Place of Presentation
      関学梅田キャンパス(大阪)
    • Year and Date
      2016-02-22
    • Related Report
      2015 Research-status Report
    • Invited
  • [Presentation] 中性子散乱によるスローダイナミクス研究とMEMによる不均一緩和モード分布の可視化2016

    • Author(s)
      松浦直人
    • Organizer
      日本物理学会 2016年秋季大会
    • Place of Presentation
      金沢大学(石川県・金沢市)
    • Related Report
      2016 Annual Research Report
    • Invited
  • [Presentation] 中性子小角散乱によるリラクサー強誘電体(1-x)Pb(Mg1/3Nb2/3)O3-xPbTiO3におけるドメイン相関の研究2016

    • Author(s)
      松浦直人, Tae-Hwan Kim, and Young-Soo Han
    • Organizer
      第26回日本MRSJ年次大会
    • Place of Presentation
      横浜情報文化センター(神奈川県・横浜市)
    • Related Report
      2016 Annual Research Report
  • [Presentation] Slow localized mode in the polar cluster of relaxor ferroelectrics near morphotropic phase boundary2015

    • Author(s)
      M. Matsuura, Z. Xu, G. Xu, P. M. Gehring, H. Endo, and K. Shibata
    • Organizer
      Pacifichem2015
    • Place of Presentation
      Hawaii (USA)
    • Year and Date
      2015-12-15
    • Related Report
      2015 Research-status Report
    • Int'l Joint Research / Invited
  • [Presentation] MPB近傍のリラクサー強誘電体における分極振幅モード2015

    • Author(s)
      松浦直人, Z. Xu, G. Xu, P. M. Gehring, 柴田薫
    • Organizer
      第25回MRSJ年次大会
    • Place of Presentation
      波止場会館(横浜)
    • Year and Date
      2015-12-08
    • Related Report
      2015 Research-status Report
  • [Presentation] M. Matsuura, T. Tominaga, T. Yamada, K. Shibata, Y. Kawakita2015

    • Author(s)
      Mode distribution analysis of quasielastic neutron scattering in relaxor ferroelectrics
    • Organizer
      Future and Current Use of Neutron Spin-Echo Spectroscopy in Condensed Matter Research workshop
    • Place of Presentation
      Oak Ridge National Laboratory (USA)
    • Year and Date
      2015-05-13
    • Related Report
      2015 Research-status Report
    • Int'l Joint Research / Invited
  • [Presentation] 中性子準弾性散乱のMEM解析によるリラクサー強誘電体の不均一時間相関の研究2015

    • Author(s)
      松浦直人,富永大輝,山田武,柴田薫,川北至信
    • Organizer
      日本物理学会 第70回年次大会
    • Place of Presentation
      早稲田大学、東京
    • Year and Date
      2015-03-21 – 2015-03-24
    • Related Report
      2014 Research-status Report
  • [Presentation] SANS study of domain size distribution in relaxor ferroelectrics PMN-30%PT2015

    • Author(s)
      M. Matsuura, Tae-Hwan Kim, and Young-Soo Han
    • Organizer
      第14回日韓中性子科学研究会
    • Place of Presentation
      茨城量子ビーム研究センター, 茨城
    • Year and Date
      2015-01-07 – 2015-01-09
    • Related Report
      2014 Research-status Report
  • [Presentation] 中性子準弾性散乱のMEM解析によるリラクサー強誘電体の不均一時間相関の研究2014

    • Author(s)
      松浦直人, Tae-Hwan Kim, Young-Soo Han, 是枝聡肇
    • Organizer
      KEK-S課題 NSE研究会
    • Place of Presentation
      KEK, つくば
    • Year and Date
      2014-11-27
    • Related Report
      2014 Research-status Report
    • Invited
  • [Presentation] 中性子散乱によるリラクサー強誘電体の不均一空間・時間相関の研究2014

    • Author(s)
      松浦直人, Tae-Hwan Kim, Young-Soo Han, 是枝聡肇
    • Organizer
      第12回CROSSroads研究会「不均一系における構造と機能」
    • Place of Presentation
      茨城量子ビーム研究センター, 茨城
    • Year and Date
      2014-09-16 – 2014-09-17
    • Related Report
      2014 Research-status Report
  • [Presentation] Neutron small angle scattering studies of ferroelectric domains in relaxor ferroelectrics2014

    • Author(s)
      Masato Matsuura, Tae-Hwan Kim, Young-Soo Han, and Akitoshi Koreeda
    • Organizer
      International Union of Materials Research Societies (IUMRS) international conference in Asia 2014
    • Place of Presentation
      Fukuoka University, Fukuoka
    • Year and Date
      2014-08-24 – 2014-08-30
    • Related Report
      2014 Research-status Report
  • [Presentation] Neutron small angle scattering studies of ferroelectric domains in relaxor ferroelectrics2014

    • Author(s)
      Masato Matsuura, Tae-Hwan Kim, Young-Soo Han, and Akitoshi Koreeda
    • Organizer
      The 10th Japan-Korea Conference on Ferroelectrics
    • Place of Presentation
      International Conference Centre Hiroshima, Hiroshima
    • Year and Date
      2014-08-17 – 2014-08-20
    • Related Report
      2014 Research-status Report
  • [Presentation] SANS study of domain size distribution in relaxor ferroelectrics PMN-30%PT2014

    • Author(s)
      M. Matsuura, Tae-Hwan Kim, and Young-Soo Han
    • Organizer
      2014 Korea-Japan workshop: Materials Research Advanced by Neutron Scattering
    • Place of Presentation
      東北大学金属材料研究所
    • Year and Date
      2014-06-26
    • Related Report
      2014 Research-status Report
  • [Presentation] Wide Relaxation Time Distributions of Quasi-Elastic Neutron Scattering in relaxor ferroelectrics2014

    • Author(s)
      Masato Matsuura, T. Tominaga, T. Yamada, Y. Kawakita and K. Shibata
    • Organizer
      The 2nd International Symposium on Science at J-PARC
    • Place of Presentation
      Tsukuba International Congress Center, Tsukuba
    • Year and Date
      2014-06-12 – 2014-06-16
    • Related Report
      2014 Research-status Report
  • [Presentation] 中性子小角散乱によるリラクサーPMN-30%PTのドメインサイズ分布の研究2014

    • Author(s)
      松浦直人,Tae-Hwan Kim,Young-Soo Han,是枝聡肇
    • Organizer
      日本物理学会 第69回年次大会
    • Place of Presentation
      東海大学
    • Related Report
      2013 Research-status Report
  • [Presentation] 非鉛系リラクサー(Bi1/2Na1/2)TiO3における格子ダイナミクス2014

    • Author(s)
      松浦直人,飯田裕之, 廣田和馬, 大和田謙二, 野口祐二, 宮山勝
    • Organizer
      第21回日本MRSJシンポジウム
    • Place of Presentation
      横浜 波止場会館
    • Related Report
      2013 Research-status Report

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Published: 2014-07-25   Modified: 2022-02-16  

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