Project/Area Number |
25400367
|
Research Category |
Grant-in-Aid for Scientific Research (C)
|
Allocation Type | Multi-year Fund |
Section | 一般 |
Research Field |
Condensed matter physics II
|
Research Institution | Kyoto University |
Principal Investigator |
Maesato Mitsuhiko 京都大学, 理学(系)研究科(研究院), 准教授 (60324604)
|
Co-Investigator(Renkei-kenkyūsha) |
IMAKUBO Tatsurou 長岡技術科学大学, 工学部, 准教授 (60291332)
|
Research Collaborator |
Brooks James S. 米国フロリダ州立大学, 国立強磁場研究所, 教授
Collet Eric 仏国レンヌ大学, 教授
Ouahab Lahcene 仏国レンヌ大学, 教授
|
Project Period (FY) |
2013-04-01 – 2016-03-31
|
Project Status |
Completed (Fiscal Year 2015)
|
Budget Amount *help |
¥4,940,000 (Direct Cost: ¥3,800,000、Indirect Cost: ¥1,140,000)
Fiscal Year 2015: ¥1,170,000 (Direct Cost: ¥900,000、Indirect Cost: ¥270,000)
Fiscal Year 2014: ¥1,170,000 (Direct Cost: ¥900,000、Indirect Cost: ¥270,000)
Fiscal Year 2013: ¥2,600,000 (Direct Cost: ¥2,000,000、Indirect Cost: ¥600,000)
|
Keywords | 磁性伝導体 / π-d複合体 / 強磁場物性 / 分子性導体 / 磁性 / 伝導性 / 強相関電子系 |
Outline of Final Research Achievements |
Utilizing iodine-bonding interactions and a mixed-anion approach, we synthesized a series of molecular conductors (DIETSe)2FeBr4xCl4(1-x) [0 < x < 1] while keeping the isostructure. Physical property measurements of the high-quality single crystals at low temperatures down to 0.3 K and high magnetic fields up to 45 T demonstrated simultaneous control of both spin and charge degrees of freedom. We succeeded in introducing large hysteresis associated with a spin-flop transition in both magnetic moment and magnetoresistance in mixed-anion salts, which has never been observed in other π-d hybrid systems. We also found intriguing magnetic field-induced phase transitions and quantum oscillations at high fields.
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