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Fabrication of epitaxial thin film solid-state secondary batteries and interface research

Research Project

Project/Area Number 25420724
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeMulti-year Fund
Section一般
Research Field Inorganic materials/Physical properties
Research InstitutionNational Institute for Materials Science

Principal Investigator

Ohnishi Tsuyoshi  国立研究開発法人物質・材料研究機構, 国際ナノアーキテクトニクス研究拠点, MANA研究者 (80345230)

Project Period (FY) 2013-04-01 – 2016-03-31
Project Status Completed (Fiscal Year 2015)
Budget Amount *help
¥5,200,000 (Direct Cost: ¥4,000,000、Indirect Cost: ¥1,200,000)
Fiscal Year 2015: ¥1,040,000 (Direct Cost: ¥800,000、Indirect Cost: ¥240,000)
Fiscal Year 2014: ¥1,300,000 (Direct Cost: ¥1,000,000、Indirect Cost: ¥300,000)
Fiscal Year 2013: ¥2,860,000 (Direct Cost: ¥2,200,000、Indirect Cost: ¥660,000)
Keywords機能性セラミックス / 機能性セラミックス材料
Outline of Final Research Achievements

The final goal is to develop ultimately high-power solid-state Li-ion batteries. In order to achieve this, oxide epitaxial thin films of cathode materials, solid electrolytes and current collectors were synthesized, and fabrication of epitaxial thin film solid-state secondary batteries were attempted by lamination of these. A part of epitaxial thin film was abandoned since scheduled combination was not allowed due to extremely different growth conditions of each film. Still, some high-power thin film solid-state batteries were successfully fabricated by using amorphous solid electrolyte thin films.

Report

(4 results)
  • 2015 Annual Research Report   Final Research Report ( PDF )
  • 2014 Research-status Report
  • 2013 Research-status Report
  • Research Products

    (25 results)

All 2016 2015 2014 2013

All Journal Article (13 results) (of which Peer Reviewed: 13 results,  Acknowledgement Compliant: 3 results) Presentation (12 results) (of which Int'l Joint Research: 2 results,  Invited: 8 results)

  • [Journal Article] Influence of high deposition rate on LiCoO2 epitaxial films prepared by pulsed laser deposition2015

    • Author(s)
      K. Nishio, T. Ohnishi, M. Osada, N. Ohta, K. Wtanabe, K. Takada
    • Journal Title

      Solid State Ionics

      Volume: 286 Pages: 91-95

    • DOI

      10.1016/j.ssi.2015.06.006

    • Related Report
      2015 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] High Electron Mobility of Nb-Doped SrTiO3 Films Stemming from Rod-Type Sr Vacancy Clusters2015

    • Author(s)
      S. Kobayashi, Y. Mizumukai, T. Ohnishi, N. Shibata, Y. Ikuhara and T. Yamamoto
    • Journal Title

      ACS Nano

      Volume: 9 Issue: 11 Pages: 10769-10777

    • DOI

      10.1021/acsnano.5b05720

    • Related Report
      2015 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Epitaxy of Li3xLa2/3-xTiO3 films and the influence of la ordering on Li-ion conduction2015

    • Author(s)
      T. Ohnishi, K. Mitsuishi, K. Nishio, K. Takada
    • Journal Title

      Chemistry of Materials

      Volume: 27 Issue: 4 Pages: 1233-1241

    • DOI

      10.1021/cm504033r

    • Related Report
      2014 Research-status Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Composition controlled LiCoO2 epitaxial thin film growth by pulsed laser deposition2015

    • Author(s)
      T. Ohnishi, K. Nishio, K. Takada
    • Journal Title

      Proc. of SPIE

      Volume: 9364 Pages: 1-9

    • DOI

      10.1117/12.2076710

    • Related Report
      2014 Research-status Report
    • Peer Reviewed
  • [Journal Article] An amorphous Si film anode for all-solid-state lithium batteries2014

    • Author(s)
      R. Miyazaki, N. Ohta, T. Ohnishi, I, Sakaguchi, K. Takada
    • Journal Title

      Journal of Power Sources

      Volume: 272 Pages: 541-545

    • DOI

      10.1016/j.jpowsour.2014.08.109

    • Related Report
      2014 Research-status Report
    • Peer Reviewed
  • [Journal Article] Synthesis of LiCoO2 epitaxial thin films using a sol-gel method2014

    • Author(s)
      T. Kwon, T. Ohnishi, K. Mitsuishi, T.C. Ozawa, K. Takada
    • Journal Title

      Journal of Power Sources

      Volume: 274 Pages: 417-423

    • DOI

      10.1016/j.jpowsour.2014.10.070

    • Related Report
      2014 Research-status Report
    • Peer Reviewed
  • [Journal Article] Development of microscopy for lithium analysis using medium-energy2014

    • Author(s)
      小林峰、鴨志田敦史、秋山日出夫、渡邊賢、大西剛、高田和典、鈴木拓
    • Journal Title

      Applied Physics Express

      Volume: 7 Issue: 10 Pages: 1-4

    • DOI

      10.7567/apex.7.106601

    • Related Report
      2014 Research-status Report
    • Peer Reviewed
  • [Journal Article] Crystal orientation of epitaxial LiCoO2 films grown on SrTiO3 substrates2014

    • Author(s)
      K. Nishio, T. Ohnishi, K. Akatsuka, K. Takada
    • Journal Title

      Journal of Power Sources

      Volume: 247 Pages: 687-691

    • DOI

      10.1016/j.jpowsour.2013.08.132

    • Related Report
      2013 Research-status Report
    • Peer Reviewed
  • [Journal Article] Versatile van der Waals epitaxy-like growth of crystal films using two-dimensional nanosheets as a seed layer: Orientation tuning of SrTiO3 films along three important axes on glass substrates2014

    • Author(s)
      T. Shibata, H. Takano, Y. Ebina, D.S. Kim, T.C. Ozawa, K. Akatsuka, T. Ohnishi, K. Takada, T. Kogure, T. Sasaki
    • Journal Title

      Journal of Materials Chemistry C

      Volume: 2 Issue: 3 Pages: 441-449

    • DOI

      10.1039/c3tc31787k

    • Related Report
      2013 Research-status Report
    • Peer Reviewed
  • [Journal Article] High performance silicon-based anodes in solid-state lithium batteries2014

    • Author(s)
      R.B. Cervera, N. Suzuki, T. Ohnishi, M. Osada, K. Mitsuishi, T. Kambara, K. Takada
    • Journal Title

      Energy and Environmental Science

      Volume: 7 Issue: 2 Pages: 662-666

    • DOI

      10.1039/c3ee43306d

    • Related Report
      2013 Research-status Report
    • Peer Reviewed
  • [Journal Article] Corrigendum to "Crystal orientation of epitaxial LiCoO2 films grown on SrTiO3 substrates" [J. Power Sources 247 (2014) 687-691]2014

    • Author(s)
      K. Nishio, T. Ohnishi, K. Akatsuka, K. Takada
    • Journal Title

      Journal of Power Sources

      Volume: 0 Pages: 412-413

    • DOI

      10.1016/j.jpowsour.2014.03.067

    • Related Report
      2013 Research-status Report
    • Peer Reviewed
  • [Journal Article] Silicon nitride thin film electrode for lithium-ion batteries2013

    • Author(s)
      N. Suzuki, R.B. Cervera, T. Ohnishi, K. Takada
    • Journal Title

      J. Power Sources

      Volume: 231 Pages: 186-189

    • DOI

      10.1016/j.jpowsour.2012.12.097

    • Related Report
      2013 Research-status Report
    • Peer Reviewed
  • [Journal Article] Oriented film growth of Ba1-xSrxTiO3 dielectrics on glass substrates using 2D nanosheet seed layer2013

    • Author(s)
      C. Jung, T. Ohnishi, M. Osada, K. Takada, T. Sasaki
    • Journal Title

      ACS Applied Materials and Interfaces

      Volume: 5 Issue: 11 Pages: 4592-4596

    • DOI

      10.1021/am400849z

    • Related Report
      2013 Research-status Report
    • Peer Reviewed
  • [Presentation] Epitaxial Thin Film Growth for Interface Research on All Solid-State Li-Ion Batteries2016

    • Author(s)
      T. Ohnishi
    • Organizer
      BIT’s 2nd Annual World Congress of Smart Materials-2016
    • Place of Presentation
      Grand Copthorne Waterfront Hotel , Singapore
    • Year and Date
      2016-03-04
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] LLZ焼結体の表面2015

    • Author(s)
      大西剛、岩谷幸作、本林秀文、高田和典
    • Organizer
      第41回固体イオニクス討論会
    • Place of Presentation
      北海道大学工学部フロンティア応用科学研究棟
    • Year and Date
      2015-11-25
    • Related Report
      2015 Annual Research Report
  • [Presentation] パルスレーザー堆積法の理想と現実2015

    • Author(s)
      大西剛
    • Organizer
      第35回エレクトロセラミックス研究討論会
    • Place of Presentation
      東京工業大学大岡山キャンパス 蔵前会館
    • Year and Date
      2015-10-22
    • Related Report
      2015 Annual Research Report
    • Invited
  • [Presentation] Influence of La Ordering on Li-ion Conduction in Li3xLa2/3-xTiO3 Epitaxial Films2015

    • Author(s)
      T. Ohnishi, K. Mitsuishi, K. Nishio, K. Takada
    • Organizer
      The 9th International Conference on the Science and Technology for Advanced Ceramics (STAC-9)
    • Place of Presentation
      つくば国際会議場
    • Year and Date
      2015-10-19
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Solid-State Lithium Battery and Thin Film Technology2015

    • Author(s)
      Tsuyoshi, Ohnishi
    • Organizer
      11th International Conference on Ceramic Materials and Components for Energy and Environmental Applications
    • Place of Presentation
      Vancouver, BC, Canada
    • Year and Date
      2015-06-19
    • Related Report
      2014 Research-status Report
    • Invited
  • [Presentation] Influence of La Ordering in Li3xLa2/3−xTiO3 Epitaxial Films on Li-Ion Conduction2015

    • Author(s)
      T. Ohnishi, K. Mitsuishi, K. Nishio, K. Takada
    • Organizer
      20th International Conference on Solid State Ionics
    • Place of Presentation
      Keystone, Colorado, USA
    • Year and Date
      2015-06-15
    • Related Report
      2014 Research-status Report
  • [Presentation] High-rate growth of high-crystallinity LiCoO2 epitaxial thin films by pulsed laser deposition2015

    • Author(s)
      Tsuyoshi Ohnishi
    • Organizer
      SPIE OPTO
    • Place of Presentation
      San Francisco, California, USA
    • Year and Date
      2015-02-08
    • Related Report
      2014 Research-status Report
    • Invited
  • [Presentation] Thin film growth by pulsed laser deposition for interface research on all solid-state Li-ion batteries2014

    • Author(s)
      Tsuyoshi Ohnishi
    • Organizer
      Oxide Thin Films for Advanced Energy and Information Applications: Materials Chemistry of Thin Film Oxides
    • Place of Presentation
      Hilton Chicago Indian Lakes Resort, Chicago, USA
    • Year and Date
      2014-07-14
    • Related Report
      2014 Research-status Report
    • Invited
  • [Presentation] THIN FILM GROWTH BY PULSED LASER DEPOSITION FOR INTERFACE RESEARCH ON ALL SOLID-STATE Li-ION BATTERIES2014

    • Author(s)
      Tsuyoshi Ohnishi
    • Organizer
      Oxide Thin Films for Advanced Energy and Information Applications: Materials Chemistry of Thin Film Oxides
    • Place of Presentation
      Hilton Chicago Indian Lakes Resort, Chicago, USA
    • Related Report
      2013 Research-status Report
    • Invited
  • [Presentation] 全固体リチウムイオン電池と薄膜技術2013

    • Author(s)
      大西剛
    • Organizer
      第74回応用物理学会秋季学術講演会
    • Place of Presentation
      同志社大学京田辺キャンパス
    • Related Report
      2013 Research-status Report
    • Invited
  • [Presentation] 全固体リチウム電池と薄膜技術2013

    • Author(s)
      大西剛
    • Organizer
      2013電気化学秋季大会
    • Place of Presentation
      東京工業大学大岡山キャンパス
    • Related Report
      2013 Research-status Report
    • Invited
  • [Presentation] Li3xLa2/3-xTiO3エピタキシャル薄膜の組成制御2013

    • Author(s)
      大西剛、西尾和記、高田和典
    • Organizer
      第54回電池討論会
    • Place of Presentation
      大阪国際会議場
    • Related Report
      2013 Research-status Report

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Published: 2014-07-25   Modified: 2019-07-29  

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