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Investigation of large magnetization and polarization in Bi(Fe,Co)O3 epitaxial thin films

Research Project

Project/Area Number 25600067
Research Category

Grant-in-Aid for Challenging Exploratory Research

Allocation TypeMulti-year Fund
Research Field Applied materials
Research InstitutionTohoku University

Principal Investigator

NAGANUMA Hiroshi  東北大学, 工学(系)研究科(研究院), 助教 (60434023)

Project Period (FY) 2013-04-01 – 2015-03-31
Project Status Completed (Fiscal Year 2014)
Budget Amount *help
¥4,030,000 (Direct Cost: ¥3,100,000、Indirect Cost: ¥930,000)
Fiscal Year 2014: ¥780,000 (Direct Cost: ¥600,000、Indirect Cost: ¥180,000)
Fiscal Year 2013: ¥3,250,000 (Direct Cost: ¥2,500,000、Indirect Cost: ¥750,000)
KeywordsBiFeO3 / マルチフェロイクス / BiCoO3 / 極薄膜 / マルチフェロイックス / エピタキシャル / 電気磁気効果 / 巨大自発分極 / ペロブスカイト
Outline of Final Research Achievements

BiFeO3 and BiCoO3 have a large polarization, and their solid solution of Bi (Fe, Co) O3 has a high spontaneous polarization/magnetization. Bi Fe(Co) O3 could maintain unsymmetrical crystal structure even if a film became ultrathin owing to epitaxial strain from single crystal SrTiO3 substrates. As a result of element specific XMCD measurements, was suggested that increasing the interfacial magnetization induced between BiFeO3 and CoFe. This may consider that electric charge formed at the interface by the large spontaneous polarization in the BiFeO3 which changing the angle of Fe of BiFeO3 and/or modulates the band structure of CoFe. This result suggested that we can expect the observation of the large tunnel electrical- and magneto-resistance effect using the Bi (Fe, Co) O3 a barrier material.

Report

(3 results)
  • 2014 Annual Research Report   Final Research Report ( PDF )
  • 2013 Research-status Report
  • Research Products

    (21 results)

All 2015 2014 2013

All Journal Article (6 results) (of which Peer Reviewed: 6 results,  Open Access: 3 results,  Acknowledgement Compliant: 5 results) Presentation (13 results) (of which Invited: 5 results) Book (1 results) Patent(Industrial Property Rights) (1 results)

  • [Journal Article] 100-nm-sized magnetic domain reversal by the magneto-electric effect in self-assembled BiFeO3/CoFe2O4 bilayer films2015

    • Author(s)
      Keita Sone, Hiroshi Naganuma, Masaki Ito, Takamichi Miyazaki, Takashi Nakajima, Soichiro Okamura
    • Journal Title

      Scientific Reports

      Volume: 5

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed / Open Access / Acknowledgement Compliant
  • [Journal Article] Evidence of rhombohedral structure within BiFeO3 thin film grown on SrTiO32015

    • Author(s)
      In-Tae Bae and Hiroshi Naganuma
    • Journal Title

      Applied Physics Express

      Volume: 8 Issue: 3 Pages: 031501-031501

    • DOI

      10.7567/apex.8.031501

    • NAID

      210000137418

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed / Open Access / Acknowledgement Compliant
  • [Journal Article] Preparation of monoclinic 0.9(BiFeO3)-0.1(BiCoO3) epitaxial films on orthorhombic YAlO3 (100) substrates by r.f. magnetron sputtering2015

    • Author(s)
      Hiroshi Naganuma, Koki Mukaiyama, Mikihiko Oogane, and Yasuo Ando
    • Journal Title

      Journal of Crystal Growth

      Volume: 409 Pages: 18-22

    • DOI

      10.1016/j.jcrysgro.2014.09.044

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Preparation of a heteroepitaxial LaxSryMnzO3/BiFeO3 bilayer by r.f. magnetron sputtering with various oxygen gas flow ratios2014

    • Author(s)
      Hiroshi Naganuma, Tomonose Ichinose, Husne. A. Begum, Seiya Sato, X. F. Han, Takamichi Miyazaki, In-Tae Bae, Mikihiko Oogane, Yasuo Ando
    • Journal Title

      AIP Advances

      Volume: 4 Issue: 8

    • DOI

      10.1063/1.4893998

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed / Open Access / Acknowledgement Compliant
  • [Journal Article] Multiferroic BiFeO3 glass-ceramics: Phase formation and physical property2014

    • Author(s)
      Y. Takahashi, K. Meguro, H. Naganuma, N. Terakado, T. Fujiwara
    • Journal Title

      Applied Physics Letters

      Volume: 104 Issue: 22

    • DOI

      10.1063/1.4881138

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Leakage current under high electric fields and magnetic properties in Co and Mn co-substituted BiFeO3 polycrystalline films2014

    • Author(s)
      Jun Miura, Takashi Nakajima, Hiroshi Naganuma, Soichiro Okamura
    • Journal Title

      Thin Solid Films

      Volume: 558 Pages: 194-199

    • DOI

      10.1016/j.tsf.2014.03.046

    • Related Report
      2013 Research-status Report
    • Peer Reviewed
  • [Presentation] マルチフェロイックスを障壁材料としたトンネル接合素子の展望2015

    • Author(s)
      永沼 博
    • Organizer
      セラミックス協会若手講演会
    • Place of Presentation
      岡山大学(岡山市)
    • Year and Date
      2015-03-17
    • Related Report
      2014 Annual Research Report
    • Invited
  • [Presentation] ペロブスカイトBiFeO3を用いたトンネル接合の伝導性2015

    • Author(s)
      永沼 博
    • Organizer
      『強誘電体障壁を有するFe4N基トンネル接合素子の開発』 第1回研究会
    • Place of Presentation
      東北大学電気通信研究所(仙台市)
    • Year and Date
      2015-02-20
    • Related Report
      2014 Annual Research Report
    • Invited
  • [Presentation] 菱面体晶BiFeO3を障壁層としたトンネル接合素子2015

    • Author(s)
      永沼 博
    • Organizer
      第283回応用セラミックス研究所講演会 「第4回材料構造講演会」
    • Place of Presentation
      東工大すずかけ台キャンパス(横浜市)
    • Year and Date
      2015-01-23
    • Related Report
      2014 Annual Research Report
    • Invited
  • [Presentation] BiFeO3を障壁層に用いたトンネル接合の作製2015

    • Author(s)
      一ノ瀬 智浩, 永沼 博, 大兼 幹彦, 安藤 康夫
    • Organizer
      誘電体スピントロニクス研究会
    • Place of Presentation
      東北大学
    • Year and Date
      2015-01-04
    • Related Report
      2014 Annual Research Report
    • Invited
  • [Presentation] SrTiO3[110]入射ナノビーム電子線回折によるBiFeO3エピタキシャル膜の構造解析2015

    • Author(s)
      佐藤 聖也, 永沼 博, Bae In-Tae, 一ノ瀬 智浩, 大兼 幹彦, 安藤 康夫
    • Organizer
      誘電体スピントロニクス研究会
    • Place of Presentation
      東北大学(仙台市)
    • Year and Date
      2015-01-04
    • Related Report
      2014 Annual Research Report
  • [Presentation] BiFeO3を障壁層としたマルチフェロイックトンネル接合素子2014

    • Author(s)
      永沼 博
    • Organizer
      スピニクス研究会 『最先端スピントロニクスと酸化物薄膜』
    • Place of Presentation
      東北大学さくらホール(仙台市)
    • Year and Date
      2014-12-12
    • Related Report
      2014 Annual Research Report
    • Invited
  • [Presentation] BiFeO3 を障壁層に用いたトンネル接合の作製2014

    • Author(s)
      一ノ瀬 智浩, 永沼 博, 大兼 幹彦, 安藤 康夫
    • Organizer
      応用物理学会東北支部学術講演会
    • Place of Presentation
      東北大学(仙台市)
    • Year and Date
      2014-12-04
    • Related Report
      2014 Annual Research Report
  • [Presentation] 電子線回折を用いたBiFeO3 エピタキシャル薄膜の結晶対称性評価2014

    • Author(s)
      佐藤 聖也, 永沼 博, Bae In-Tae, 一ノ瀬 智浩, 大兼 幹彦, 安藤 康夫
    • Organizer
      応用物理学会東北支部学術講演会
    • Place of Presentation
      東北大学(仙台市)
    • Year and Date
      2014-12-04
    • Related Report
      2014 Annual Research Report
  • [Presentation] LaSrMnO3/BiFeO3ヘテロ接合の作製2014

    • Author(s)
      一ノ瀬 智浩, 永沼 博, 大兼 幹彦, 安藤 康夫
    • Organizer
      応用物理学会学術講演会
    • Place of Presentation
      北海道大学(札幌市)
    • Year and Date
      2014-09-18
    • Related Report
      2014 Annual Research Report
  • [Presentation] 電子線回折によるBiFeO3エピタキシャル膜の構造解析2014

    • Author(s)
      佐藤 聖也, 永沼 博, Bae In-Tae, 一ノ瀬 智浩, 大兼 幹彦, 安藤 康夫
    • Organizer
      応用物理学会学術講演会
    • Place of Presentation
      北海道大学(札幌市)
    • Year and Date
      2014-09-17
    • Related Report
      2014 Annual Research Report
  • [Presentation] YAlO3(100)基板上に成長したBiFe0.9Co0.1O3エピタキシャル膜の構造と磁気特性2013

    • Author(s)
      一ノ瀬智浩,永沼博,大兼幹彦,安藤康夫
    • Organizer
      応用物理学会東北支部学術講演会
    • Place of Presentation
      山形大学米沢キャンパス
    • Related Report
      2013 Research-status Report
  • [Presentation] Monoclinic Bi(Fe0.9Co0.1)O3 epitaxial films grown on YAlO3 (100) substratesby r.f. magnetron sputtering2013

    • Author(s)
      Tomohiro Ichinose, Hiroshi Naganuma, Mikihiko Oogane and Yasuo Ando
    • Organizer
      応用物理学会秋季学術講演会
    • Place of Presentation
      同志社大学
    • Related Report
      2013 Research-status Report
  • [Presentation] Investigation of Dzyaloshinskii-Moriya interaction in rhombohedral and tetragonal BiFeO3/CoFe bilayers2013

    • Author(s)
      K. Mukaiyama, H. Naganuma, M. Oogane, Y. Ando
    • Organizer
      2013 Solid State Device and Materials
    • Place of Presentation
      ヒルトン福岡
    • Related Report
      2013 Research-status Report
  • [Book] Optical properties of Multiferroic BiFeO3 films2013

    • Author(s)
      Hiromi Shima, Hiroshi Naganuma, Soichiro Okamura
    • Total Pages
      549
    • Publisher
      Intech
    • Related Report
      2013 Research-status Report
  • [Patent(Industrial Property Rights)] マルチフェロイックトンネル接合素子および超高感度センサーデバイス2014

    • Inventor(s)
      永沼 博, 大兼 幹彦, 安藤 康夫, 一ノ瀬 智浩
    • Industrial Property Rights Holder
      永沼 博, 大兼 幹彦, 安藤 康夫, 一ノ瀬 智浩
    • Industrial Property Rights Type
      特許
    • Filing Date
      2014-12-03
    • Related Report
      2014 Annual Research Report

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Published: 2014-07-25   Modified: 2019-07-29  

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