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muSR Study on the Electron Tranfser in Organic Solar Cell Materials

Research Project

Project/Area Number 25620155
Research Category

Grant-in-Aid for Challenging Exploratory Research

Allocation TypeMulti-year Fund
Research Field Energy-related chemistry
Research InstitutionThe Institute of Physical and Chemical Research

Principal Investigator

WATANABE Isao  独立行政法人理化学研究所, 仁科加速器研究センター, 専任研究員 (40260195)

Co-Investigator(Renkei-kenkyūsha) KAWASAKI Ikuto  独立行政法人理化学研究所, 仁科加速器研究センター, 基礎特別研究員 (90552307)
Project Period (FY) 2013-04-01 – 2015-03-31
Project Status Completed (Fiscal Year 2014)
Budget Amount *help
¥4,030,000 (Direct Cost: ¥3,100,000、Indirect Cost: ¥930,000)
Fiscal Year 2014: ¥1,950,000 (Direct Cost: ¥1,500,000、Indirect Cost: ¥450,000)
Fiscal Year 2013: ¥2,080,000 (Direct Cost: ¥1,600,000、Indirect Cost: ¥480,000)
Keywordsミュオンスピン緩和法 / 有機太陽光発電 / 電子伝達 / 汎関数密度計算 / 国際研究協力 / 国際研究者交流 / エネルギー問題 / 発電 / 半密度関数計算 / 国際研究者交流鵜 / μSR / 電子伝導 / 有機材料 / 低次元性
Outline of Final Research Achievements

The muon-spin relaxation (muSR) technique has been applied to organic solar-cell materials. The flush-lamp muSR technique by using a pulsed muon beam has been used for this research creating light-exited electrons in organic materials. Some possible organic solar-cell materials like Polythiophene, PC71BM, PTB7 and so on have been chosen. We have succeeded to observe the muon-spin depolarization behavior which is caused by light-exited electron when the flush lamp is turned on. This result opens a new research direction to use muSR as a microscopic method for the investigation of light-exited electrons in organic solar-cell materials from the microscopic viewpoint. In addition to this, the importance of the information of muon sites in materials has been found. This is a new valuable finding of the current research. Accordingly, we have newly started to develop a way to estimate muon sites in organic and related system by using the density functional theory.

Report

(3 results)
  • 2014 Annual Research Report   Final Research Report ( PDF )
  • 2013 Research-status Report
  • Research Products

    (16 results)

All 2014 2013

All Journal Article (6 results) (of which Peer Reviewed: 6 results) Presentation (10 results) (of which Invited: 5 results)

  • [Journal Article] Charge Carrier Dynamics of Active Material Solar Cell P3HT: ZnO Nanoparticles Studied by Muon Spin Relaxation (muSR)2014

    • Author(s)
      L. Safriani, Risdiana, A. Bahtiar, A. Aprilia, R.E. Siregar, R. Hidayat, T.P.I. Saragi, I. Kawasaki, and I. Watanabe
    • Journal Title

      Advanced Materials Research

      Volume: 896 Pages: 477-480

    • Related Report
      2014 Annual Research Report 2013 Research-status Report
    • Peer Reviewed
  • [Journal Article] An Effect of the Super-Cell Calculation on Muon Positions and Local Deformations of Crystal Structure in La2CuO42014

    • Author(s)
      B. Adiperdana, E. Suprayoga, N. Adam, Mohm-Tajudin S.S., Rozlan A.F., S. Sulaiman, M.I. Mohamed-Ibrahim, T. Kawamata, T. Adachi, I.A. Dharmawan, R.E. Siregar, Y. Koike, and I. Watanabe,
    • Journal Title

      J. Phys. Conf. Ser.

      Volume: 551

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Muon sites in Ce(Ru,Rh)2Al10 investigated by using Density Functional Theory from the view point of electronic potential2014

    • Author(s)
      N. Adam, E. Suprayoga, B. Adiperdana, H. Guo, H. Tanida, S.S. Mohd-Tajudin, R. Kobayashi, M. Sera, T. Nishioka, M. Matsumura, S. Sulaiman, M.I. Mohamed Ibrahim, and I. Watanabe,
    • Journal Title

      J. Phys. Conf. Ser.

      Volume: 551

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Search for Potential Minimum Positions in Metal-Organic Hybrids, (C2H5NH3)2CuCl4 and (C6H5CH2CH2NH3)2CuCl4, by Using Density Functional Theory2014

    • Author(s)
      E. Suprayoga, A.A. Nugroho, A.O. Polyakov, T.T.M. Palstra, and I. Watanabe,
    • Journal Title

      J. Phys. Conf. Ser.

      Volume: 551

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed
  • [Journal Article] An Investigation of Muon Sites in YBa2Cu3O6 by Using Density Functional Theory2014

    • Author(s)
      S.S. Mohd-Tajudin, S.N.A. Ahmad, D.F. Hasan-Baseri, E. Suprayoga, N. Adam, Rozlan A.F., S. Sulaiman, M.I. Mohamed-Ibrahim, and I. Watanabe,
    • Journal Title

      J. Phys. Conf. Ser. 551,

      Volume: 551

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Muon-Spin-Relaxation Study of Organic Semiconductor Spiro-Linked Compound2013

    • Author(s)
      T. P. I. Saragi, Risdiana, L. Safriani, I. Kawasaki, J. Salbeck and I. Watanabe
    • Journal Title

      Organic Electronics

      Volume: 14 Pages: 62-66

    • Related Report
      2013 Research-status Report
    • Peer Reviewed
  • [Presentation] Electronic Structure of CeRu2Al10 based on LSDA+U Calculations2014

    • Author(s)
      N. Adam、S. Sulaiman、M.I. Mohamed-Ibrahim、渡邊功雄
    • Organizer
      RIKEN Symposium: 1st RIKEN-Sophia Joint Syposium; Recent Progresses on the Muon-Site Estimation
    • Place of Presentation
      上智大学、東京
    • Year and Date
      2014-12-15 – 2014-12-16
    • Related Report
      2014 Annual Research Report
  • [Presentation] Electronic Structure and Hyperfine Interaction of Muonated La2CuO42014

    • Author(s)
      Rozlan A.F.、S. Sulaiman、M.I. Mohamed-Ibrahim、渡邊功雄
    • Organizer
      RIKEN Symposium: 1st RIKEN-Sophia Joint Syposium; Recent Progresses on the Muon-Site Estimation
    • Place of Presentation
      上智大学、東京
    • Year and Date
      2014-12-15 – 2014-12-16
    • Related Report
      2014 Annual Research Report
  • [Presentation] Search for Muon Stopping Positions in Organic-Inorganic Hybrids2014

    • Author(s)
      E. Suprayoga、A.A. Nugroho、A.O. Polyakov、T.T.M. Palstra、渡邊功雄
    • Organizer
      RIKEN Symposium: 1st RIKEN-Sophia Joint Syposium; Recent Progresses on the Muon-Site Estimation Based on Density Functional Theory
    • Place of Presentation
      上智大学、東京
    • Year and Date
      2014-12-15 – 2014-12-16
    • Related Report
      2014 Annual Research Report
  • [Presentation] Investigation of Muon Sites in YBa2Cu3O6 by Using Density Functional Theory2014

    • Author(s)
      S.S. Mohd-Tajudin、S.N.A. Ahmad、D.F. Hasan-Baseri、E. Suprayoga、N. Adam、Rozlan A.F.、S. Sulaiman、M.I. Mohamed-Ibrahim、渡邊功雄
    • Organizer
      RIKEN Symposium: 1st RIKEN-Sophia Joint Syposium; Recent Progresses on the Muon-Site Estimation
    • Place of Presentation
      上智大学、東京
    • Year and Date
      2014-12-15 – 2014-12-16
    • Related Report
      2014 Annual Research Report
  • [Presentation] Muon Site Estimation in La2CuO4 by the Density Functional Theory2014

    • Author(s)
      渡邊功雄
    • Organizer
      2nd International Conference on Functional Material Science 2014
    • Place of Presentation
      Lombok, Indonesia
    • Year and Date
      2014-11-12 – 2014-11-13
    • Related Report
      2014 Annual Research Report
    • Invited
  • [Presentation] Highlights of muSR at the RIKEN-RAL2014

    • Author(s)
      渡邊功雄
    • Organizer
      ITS Department Sminar
    • Place of Presentation
      Surabaya, Indonesia
    • Year and Date
      2014-07-07 – 2014-07-08
    • Related Report
      2014 Annual Research Report
    • Invited
  • [Presentation] Applications of a DC Muon Source to the Muon to Material Science2014

    • Author(s)
      渡邊功雄
    • Organizer
      RISP scientific Seminar
    • Place of Presentation
      韓国・太田市
    • Related Report
      2013 Research-status Report
    • Invited
  • [Presentation] Applications of Pulsed Muon Beam to Material Science at the RIKEN-RAL Muon Facility2014

    • Author(s)
      渡邊功雄
    • Organizer
      NTNU Science Seminar
    • Place of Presentation
      ノルウェー・NTNU
    • Related Report
      2013 Research-status Report
    • Invited
  • [Presentation] Applications of Pulsed Muon Beam to Material Science at the RIKEN-RAL Muon Facility2014

    • Author(s)
      渡邊功雄
    • Organizer
      3rd Workshop for Light/Quantum Beam Science Promotion
    • Place of Presentation
      東北大学
    • Related Report
      2013 Research-status Report
    • Invited
  • [Presentation] Charge Carrier Dynamics of Active Material Solar Cell P3HT: ZnO Nanoparticles Studied by Muon Spin Relaxation2013

    • Author(s)
      L.Safriani、Risdiana、A.Bahtiar、A.Aprilia、R.E.Siregar、R.Hidayat、T.P.I.Saragi、I.Kawasaki、I.Watanabe
    • Organizer
      The 2013 International Conference on Advanced Material Science and Technology (ICAMST2013)
    • Place of Presentation
      インドネシア・ジョグジャカルタ
    • Related Report
      2013 Research-status Report

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Published: 2014-07-25   Modified: 2019-07-29  

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