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Variations of the decay modes of 235mU and 229mTh depending on the chemical environment

Research Project

Project/Area Number 25800150
Research Category

Grant-in-Aid for Young Scientists (B)

Allocation TypeMulti-year Fund
Research Field Particle/Nuclear/Cosmic ray/Astro physics
Research InstitutionOsaka University

Principal Investigator

Kasamatsu Yoshitaka  大阪大学, 理学(系)研究科(研究院), 講師 (70435593)

Research Collaborator SHIGEKAWA Yudai  大阪大学, 大学院理学研究科
YASUDA Yuki  大阪大学, 大学院理学研究科
Project Period (FY) 2013-04-01 – 2016-03-31
Project Status Completed (Fiscal Year 2015)
Budget Amount *help
¥4,290,000 (Direct Cost: ¥3,300,000、Indirect Cost: ¥990,000)
Fiscal Year 2015: ¥650,000 (Direct Cost: ¥500,000、Indirect Cost: ¥150,000)
Fiscal Year 2014: ¥1,560,000 (Direct Cost: ¥1,200,000、Indirect Cost: ¥360,000)
Fiscal Year 2013: ¥2,080,000 (Direct Cost: ¥1,600,000、Indirect Cost: ¥480,000)
Keywords229mTh / 235mU / 核異性体 / 内部転換 / 電子分光 / ガンマ線遷移 / 真空紫外線 / U-235m
Outline of Final Research Achievements

We developed the high-efficient spectrometer for low-energy electrons, the collection apparatus for recoil products, and the detection system for vacuum-ultraviolet photons from 229mTh. We prepared 235mU and 229mTh samples with several kinds of chemical forms and conducted electron detection for 235mU samples and photon detection for 229mTh samples using these apparatuses.
Variation of the electron spectrum in addition to the half-life depending on the chemical form was observed for 235mU. We were able to directly discuss the influence of the orbital elections on the nuclear decay of 235mU. For 229mTh, photons emitted from 229mTh were not observed although the Cherenkov light originating from the decays of the daughter nuclides of 229mTh was detected. This is important result to discuss the decay properties of 229mTh taking into account the results previously reported.

Report

(4 results)
  • 2015 Annual Research Report   Final Research Report ( PDF )
  • 2014 Research-status Report
  • 2013 Research-status Report
  • Research Products

    (9 results)

All 2016 2015 2014

All Journal Article (1 results) Presentation (8 results) (of which Int'l Joint Research: 2 results)

  • [Journal Article] Search for ultraviolet photons from precipitated 229mTh samples2015

    • Author(s)
      Y. Yasuda, Y. Kasamatsu, Y. Shigekawa, T. Ohtsuki, K. Takamiya, A. Shinohara
    • Journal Title

      KURRI PROGRESS REPORT 2014

      Volume: 2014 Pages: 139-139

    • Related Report
      2015 Annual Research Report
  • [Presentation] 化学状態に依存した235mUの半減期変化の測定2016

    • Author(s)
      重河優大、笠松良崇、安田勇輝、篠原厚
    • Organizer
      日本化学会第96春季年会
    • Place of Presentation
      京都、日本
    • Year and Date
      2016-03-24
    • Related Report
      2015 Annual Research Report
  • [Presentation] Developments of the collection apparatus for recoil products and spectrometer of low-energy internal-conversion electrons to study the deexcitation process of 235mU2015

    • Author(s)
      Y. Shigekawa, Y. Kasamatsu, A. Shinohara
    • Organizer
      International Chemical Congress of Pacific Basin Societies
    • Place of Presentation
      Hawaii, USA
    • Year and Date
      2015-12-15
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Spectroscopy of Low-energy Conversion Electrons to investigate the Deexcitation Process of 235mU2015

    • Author(s)
      Yudai Shigekawa, Yoshitaka Kasamatsu, Yuki Yasuda, Atsushi Shinohara
    • Organizer
      The 2nd International Symposium on Interactive Materials Science Cadet Program
    • Place of Presentation
      Osaka, Japan
    • Year and Date
      2015-11-18
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 低エネルギー励起核229mThの脱励起過程における真空紫外光測定2015

    • Author(s)
      安田勇輝、笠松良崇、重河優大、 髙宮幸一、大槻勤、三頭聰明、篠原厚
    • Organizer
      第59回放射化学討論会
    • Place of Presentation
      宮城、日本
    • Year and Date
      2015-09-25
    • Related Report
      2015 Annual Research Report
  • [Presentation] 235mUの壊変過程の解明を目指した低エネルギー内部転換電子分光測定2015

    • Author(s)
      重河優大、笠松良崇、安田勇輝、篠原厚
    • Organizer
      第59 回放射化学討論会
    • Place of Presentation
      宮城、日本
    • Year and Date
      2015-09-25
    • Related Report
      2015 Annual Research Report
  • [Presentation] Search for ultraviolet and visible rays from 229mTh2014

    • Author(s)
      Yoshitaka Kasamatsu, Yuki Yasuda, Yudai Shigekawa, Atsushi Shinohara, Koichi Takamiya, Tsutomu Ohtsuki
    • Organizer
      Fourth Joint Meeting of the Nuclear Physics Divisions of the American Physical Society and the Physical Society of Japan (Hawaii 2014)
    • Place of Presentation
      Hawaii, USA
    • Year and Date
      2014-10-07 – 2014-10-11
    • Related Report
      2014 Research-status Report
  • [Presentation] Development of the collection apparatus for recoil products for study of the deexcitation process of 235mU2014

    • Author(s)
      Yudai Shigekawa, Yoshitaka Kasamatsu, Atsushi Shinohara
    • Organizer
      Fourth Joint Meeting of the Nuclear Physics Divisions of the American Physical Society and the Physical Society of Japan (Hawaii 2014)
    • Place of Presentation
      Hawaii, USA
    • Year and Date
      2014-10-07 – 2014-10-11
    • Related Report
      2014 Research-status Report
  • [Presentation] U-235mの脱励起過程の研究に向けた反跳核捕集装置の開発2014

    • Author(s)
      重河優大、笠松良崇、篠原厚
    • Organizer
      第58回放射化学討論会
    • Place of Presentation
      名古屋、愛知
    • Year and Date
      2014-09-11 – 2014-09-13
    • Related Report
      2014 Research-status Report

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Published: 2014-07-25   Modified: 2019-07-29  

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