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Practical application of radionuclide decontamination technology from polluted soil in Fukushima

Research Project

Project/Area Number 26248045
Research Category

Grant-in-Aid for Scientific Research (A)

Allocation TypeSingle-year Grants
Section一般
Research Field Green/Environmental chemistry
Research InstitutionEhime University

Principal Investigator

Aono Hiromichi  愛媛大学, 理工学研究科(工学系), 教授 (00184052)

Co-Investigator(Kenkyū-buntansha) 板垣 吉晃  愛媛大学, 理工学研究科(工学系), 准教授 (30325146)
松枝 直人  愛媛大学, 農学研究科, 教授 (90199753)
Project Period (FY) 2014-06-27 – 2018-03-31
Project Status Completed (Fiscal Year 2017)
Budget Amount *help
¥42,640,000 (Direct Cost: ¥32,800,000、Indirect Cost: ¥9,840,000)
Fiscal Year 2017: ¥5,590,000 (Direct Cost: ¥4,300,000、Indirect Cost: ¥1,290,000)
Fiscal Year 2016: ¥7,410,000 (Direct Cost: ¥5,700,000、Indirect Cost: ¥1,710,000)
Fiscal Year 2015: ¥7,930,000 (Direct Cost: ¥6,100,000、Indirect Cost: ¥1,830,000)
Fiscal Year 2014: ¥21,710,000 (Direct Cost: ¥16,700,000、Indirect Cost: ¥5,010,000)
Keywordsゼオライト / 放射性核種 / セシウム除染 / 磁化ゼオライト / 磁石選別機 / 除染シート / モルデナイト / 除染 / セシウム / Na-P1型ゼオライト / 水質汚濁・土壌汚染防止・浄化 / セラミックス / 磁性材料 / 放射性セシウム除染 / 複合材料 / 土壌除染 / 放射性セシウム / シート化 / 濃縮
Outline of Final Research Achievements

We studied for the purpose of decontamination of radionuclides (Cs) in soil and liquid. The radionuclide of the soil is adsorbed to the developed zeolite-magnetite composite material and recovered by the magnetic separator. The practical application is difficult, because the decontamination rate from the soil to the zeolite has decreased considerably year by year and the high cost of the magnetic separator can not be improved. For sheeting of zeolite, a nonwoven fabric zeolite sheet was prototyped and tried to decontaminate in rice fields in Fukushima. However, the practical application was difficult, because a sufficient decontamination rate was not obtained. Good results was obtained for glass solidification after decontamination. Furthermore, the addition of sodium carbonate was very effective in reducing the firing temperature and suppressing the vaporization of cesium.

Report

(5 results)
  • 2017 Annual Research Report   Final Research Report ( PDF )
  • 2016 Annual Research Report
  • 2015 Annual Research Report
  • 2014 Annual Research Report
  • Research Products

    (33 results)

All 2018 2017 2016 2015 2014

All Journal Article (7 results) (of which Int'l Joint Research: 4 results,  Peer Reviewed: 6 results,  Open Access: 5 results,  Acknowledgement Compliant: 3 results) Presentation (26 results) (of which Int'l Joint Research: 3 results,  Invited: 10 results)

  • [Journal Article] Cs immobilization using the formation of the glassy phase by the heat-treatment of natural mordenite2018

    • Author(s)
      H. Aono, R.Takahashi, Y. Itagaki, E. Johan, and N. Matsue
    • Journal Title

      Journal of Nuclear Materials

      Volume: 印刷中

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Development of Magnetic Zeolites for the Purpose of Radionuclide Decontamination2017

    • Author(s)
      青野宏通
    • Journal Title

      Journal of the Society of Powder Technology, Japan

      Volume: 54 Issue: 8 Pages: 524-526

    • DOI

      10.4164/sptj.54.524

    • NAID

      130006038607

    • ISSN
      0386-6157, 1883-7239
    • Related Report
      2017 Annual Research Report
  • [Journal Article] FABRICATION OF HIGH PURITY SILICA FROM RICE HUSK AND ITS CONVERSION INTO ZSM-52016

    • Author(s)
      E. Johan, K.Ogami, N. Matsue, Y. Itagaki, H. Aono
    • Journal Title

      ARPN Journal of Engineering and Applied Sciences

      Volume: 11 Pages: 4006-4010

    • Related Report
      2015 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Synthesis of Mordenite and its Composite Material Using Chemical Reagents for Cs Decontamination2016

    • Author(s)
      H.Aono, N. Kaji, Y. Itagaki, E. Johan, and N. Matsue
    • Journal Title

      J. Ceram. Soc. Jpn.

      Volume: 124

    • NAID

      130005149953

    • Related Report
      2015 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research / Acknowledgement Compliant
  • [Journal Article] Preparation of mordenite and its composite material with nano-sized magnetite from diatomites for radioactive Cs decontamination2015

    • Author(s)
      Keizo YAMADA, Erni. JOHAN, Naoto MATSUE, Yoshiteru ITAGAKI, and Hiromichi AONO
    • Journal Title

      Journal of the Ceramic Society of Japan

      Volume: 123 Issue: 1435 Pages: 129-135

    • DOI

      10.2109/jcersj2.123.129

    • NAID

      130004951109

    • ISSN
      1348-6535, 1882-0743
    • Related Report
      2015 Annual Research Report 2014 Annual Research Report
    • Peer Reviewed / Open Access / Acknowledgement Compliant
  • [Journal Article] Adsorption Selectivity of Cs+ and Sr2+ by Zeolites Affected by Coexistence Cation in Relation to Radioactive Decontamination2015

    • Author(s)
      M. W. Munthali, E. Johan, H. Aono, and N. Matsue
    • Journal Title

      Journal of Asian Ceramic Societies

      Volume: 3 Issue: 3 Pages: 245-250

    • DOI

      10.1016/j.jascer.2015.04.002

    • Related Report
      2015 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Adsorption characteristics of Cs<sup>+</sup> onto artificial zeolites synthesized from coal fly ash and diatomite2015

    • Author(s)
      E. Johan, K. Yoshida, M. W. Munthali, N. Matsue, Y. Itagaki, H. Aono
    • Journal Title

      Journal of the Ceramic Society of Japan

      Volume: 123 Issue: 1444 Pages: 1065-1072

    • DOI

      10.2109/jcersj2.123.1065

    • NAID

      130005113119

    • ISSN
      1348-6535, 1882-0743
    • Related Report
      2015 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research / Acknowledgement Compliant
  • [Presentation] 土壌中の放射性セシウムの除染除去のためのシート化ゼオライト2018

    • Author(s)
      エルニジョハン, 青野宏通, 松枝直人
    • Organizer
      日本セラミックス協会2018年年会
    • Related Report
      2017 Annual Research Report
  • [Presentation] ゼオライトによるCsおよびSr固定化における焼成温度の低温化2017

    • Author(s)
      髙橋龍一郎、Erni Johan、松枝直人、板垣吉晃、青野宏通
    • Organizer
      第30回日本セラミックス協会秋季シンポジウム
    • Related Report
      2017 Annual Research Report
  • [Presentation] チャバザイトの人工合成とCs吸着特性2017

    • Author(s)
      竹内優太,Erni Johan, 板垣吉晃, 青野宏通
    • Organizer
      第24回ヤングセラミストミーティングin中四国
    • Related Report
      2017 Annual Research Report
  • [Presentation] Zeolites Embedded Sheets for Removing Toxic Metals from Water2017

    • Author(s)
      Erni JOHAN, Lester BOTOMAN, Hiromichi AONO, Naoto MATSUE
    • Organizer
      The 34th International Japan-Korea Seminar on Ceramics (J-K Ceramics 34)
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Industry of zeolites and its nanocomposites and their application in soils and environment2017

    • Author(s)
      Erni Johan, Lester Botoman, Hiromichi Aono, Naoto Matsue
    • Organizer
      Secretariat of The 3rd International Conference of Green Agro-Industry(3rd ICGAI 2017)
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Synthesis of mordenite using natural resources and their adsorption properties of Cs+ and heavy metals2016

    • Author(s)
      T.Kunimoto, E. Johan, N. Matsue, Y. Itagaki, H. Aono
    • Organizer
      第26回日本MRS年次大会
    • Place of Presentation
      横浜市開港記念会館(神奈川県・横浜市)
    • Year and Date
      2016-12-19
    • Related Report
      2016 Annual Research Report
  • [Presentation] ゼオライトによるCsおよびSrの固定化における焼成条件の影響2016

    • Author(s)
      ○高橋龍一郎・Erni Johan・松枝直人・板垣吉晃・青野宏通
    • Organizer
      日本セラミックス協会秋季シンポジウム
    • Place of Presentation
      広島大学(広島県・東広島市)
    • Year and Date
      2016-09-07
    • Related Report
      2016 Annual Research Report
  • [Presentation] セシウムの簡便・低コスト除染:天然モルデナイト付着シートの利用2016

    • Author(s)
      松枝直人, Botoman Lester, Erni Johan, 青野宏通, 森田昌敏
    • Organizer
      環境放射能除染学会 第5回研究発表会・国際シンポジウム
    • Place of Presentation
      福島県文化センター(福島県・福島市)
    • Year and Date
      2016-07-06
    • Related Report
      2016 Annual Research Report
  • [Presentation] 吸着剤付着シートによるセシウム汚染土壌の除染2015

    • Author(s)
      松枝直人・Munthali Moses Wazingwa・青野宏通・Erni Johan
    • Organizer
      2015 年度(第111 回)日本土壌肥料学会関西支部講演会
    • Place of Presentation
      愛媛大学・愛媛県・松山市
    • Year and Date
      2015-12-11
    • Related Report
      2015 Annual Research Report
    • Invited
  • [Presentation] 人工ゼオライトのCs吸着特性と固定化挙動2015

    • Author(s)
      吉田 昂平・エルニ ジョハン・松枝 直人・板垣 吉晃・青野 宏通
    • Organizer
      第25回日本MRS年次大会
    • Place of Presentation
      横浜市開港記念会館・神奈川県・横浜市
    • Year and Date
      2015-12-08
    • Related Report
      2015 Annual Research Report
    • Invited
  • [Presentation] セシウム除染を目的としたモルデナイト-マグネタイト複合材料の試薬を用いた合成2015

    • Author(s)
      鍛治紀彰・Erni Johan・松枝直人・板垣吉晃・青野宏通
    • Organizer
      第25回日本MRS年次大会
    • Place of Presentation
      横浜市開港記念会館・神奈川県・横浜市
    • Year and Date
      2015-12-08
    • Related Report
      2015 Annual Research Report
    • Invited
  • [Presentation] FABRICATION OF HIGH PURITY SILICA FROM RICE HUSK AND ITS CONVERSION INTO ZSM-52015

    • Author(s)
      E. Johan, K.Ogami, N. Matsue, Y. Itagaki, H. Aono
    • Organizer
      STECHNOVA 2015 -International Energy Conference-
    • Place of Presentation
      Yogyakarta(インドネシア)
    • Year and Date
      2015-11-25
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Cs吸着を目的としたサポナイトの合成と評価2015

    • Author(s)
      田中雄大・吉田昂平・Erni Johan・板垣吉晃・青野宏通
    • Organizer
      第22回ヤングセラミストミーティングin中四国
    • Place of Presentation
      高知大学・高知県・高知市
    • Year and Date
      2015-11-21
    • Related Report
      2015 Annual Research Report
    • Invited
  • [Presentation] 天然資源を用いたモルデナイトの人工合成とセシウム吸着評価2015

    • Author(s)
      國本太歩・鍛治紀彰・Erni Johan・尾上清利・松枝直人・板垣吉晃・青野宏通
    • Organizer
      セラミックス協会秋季シンポジウム
    • Place of Presentation
      富山大学・富山県・富山市
    • Year and Date
      2015-09-16
    • Related Report
      2015 Annual Research Report
    • Invited
  • [Presentation] 天然資源を原料とするモルデナイトの人工合成とセシウム吸着評価2015

    • Author(s)
      青野宏通・國本太歩・鍛治紀彰・Erni Johan・板垣吉晃・尾上清利・松枝直人
    • Organizer
      平成27年度資源・素材学会関係学協会合同秋季大会
    • Place of Presentation
      愛媛大学・愛媛県・松山市
    • Year and Date
      2015-09-08
    • Related Report
      2015 Annual Research Report
    • Invited
  • [Presentation] モルデナイト-マグネタイト複合材料の人工合成とセシウム吸着特性(2)2015

    • Author(s)
      青野宏通
    • Organizer
      人口ゼオライトフォーラム
    • Place of Presentation
      キャンパス・イノベーションセンター・東京都・港区
    • Year and Date
      2015-06-15
    • Related Report
      2015 Annual Research Report
    • Invited
  • [Presentation] 人工合成により得たNa-P1型ゼオライト及びモルデナイトのCs吸着評価2015

    • Author(s)
      吉田昂平, Erni Johan, 松枝直人, 板垣吉晃, 青野宏通
    • Organizer
      日本セラミックス協会秋季大会
    • Place of Presentation
      岡山大学(岡山県岡山市)
    • Year and Date
      2015-03-18 – 2015-03-20
    • Related Report
      2014 Annual Research Report
  • [Presentation] モルデナイト‐マグネタイト複合材料の合成とセシウム吸着及び磁場回収能2015

    • Author(s)
      鍛治紀彰, 國本太歩, Erni Johan, 松枝直人, 板垣吉晃, 青野宏通
    • Organizer
      日本セラミックス協会秋季大会
    • Place of Presentation
      岡山大学(岡山県岡山市)
    • Year and Date
      2015-03-18 – 2015-03-20
    • Related Report
      2014 Annual Research Report
  • [Presentation] Preparation of the composite material from diatomite for Cs decontamination and its immobilization using heat treatment2014

    • Author(s)
      K. Yoshida, E. Johan, N. Matsu), Y. Itagaki, and H. Aono
    • Organizer
      第24回日本MRS年次大会
    • Place of Presentation
      横浜市開港記念会館他(神奈川県横浜市)
    • Year and Date
      2014-12-10 – 2014-12-12
    • Related Report
      2014 Annual Research Report
  • [Presentation] Evaluation of Cs adsorption for artificial Na-P1 zeolite and mordenite2014

    • Author(s)
      K. Yamada, E. Johan, N. Matsue, Y. Itagaki, and H. Aono
    • Organizer
      第24回日本MRS年次大会
    • Place of Presentation
      横浜市開港記念会館他(神奈川県横浜市)
    • Year and Date
      2014-12-10 – 2014-12-12
    • Related Report
      2014 Annual Research Report
  • [Presentation] Natural Zeolites as Potential Materials for Decontamination of Radioactive Cs2014

    • Author(s)
      Erni Johan, Toshio Yamada, Moses Munthali Wazingwa, Ponyadira Kabwadza-Corner, Hiromichi Aono, Naoto Matsue
    • Organizer
      The 5th International Conference on Sustainable Future for Human Security (SUSTAIN 2014)
    • Place of Presentation
      Bali, INDONESIA
    • Year and Date
      2014-11-17 – 2014-11-19
    • Related Report
      2014 Annual Research Report
  • [Presentation] Na-P1型ゼオライト‐マグネタイト複合材料の作製条件による除染性能への影響2014

    • Author(s)
      溝口裕己, Erni Johan, 松枝直人, 板垣吉晃, 青野宏通
    • Organizer
      第21回 ヤングセラミスト・ミーティング in 中四国
    • Place of Presentation
      島根大学(島根県松江市)
    • Year and Date
      2014-11-15
    • Related Report
      2014 Annual Research Report
  • [Presentation] 機能性を有する人工ゼオライトの開発(除染材料および蛍光材料を例として)2014

    • Author(s)
      青野宏通
    • Organizer
      環境・材料セミナー
    • Place of Presentation
      長崎県窯業技術センター(長崎県東彼杵郡)
    • Year and Date
      2014-11-05
    • Related Report
      2014 Annual Research Report
    • Invited
  • [Presentation] モルデナイト-マグネタイト複合材料の人工合成とセシウム吸着特性2014

    • Author(s)
      青野宏通
    • Organizer
      人工ゼオライトフォーラム
    • Place of Presentation
      キャンパス・イノベーションセンター(東京都港区芝浦)
    • Year and Date
      2014-07-19
    • Related Report
      2014 Annual Research Report
    • Invited
  • [Presentation] バーミキュライトを模擬土壌とした最適なセシウム除染条件の検討2014

    • Author(s)
      吉田昂平, 板垣吉晃, 青野宏通
    • Organizer
      第3回環境放射能除染研究発表会
    • Place of Presentation
      郡山市民文化センター(福島県郡山市)
    • Year and Date
      2014-07-03 – 2014-07-04
    • Related Report
      2014 Annual Research Report
  • [Presentation] 磁選回収を目的としたモルデナイト-マグネタイト複合材料の開発とセシウム吸着能力2014

    • Author(s)
      山田啓三, Erni Johan, 松枝直人, 板垣吉晃, 青野宏通
    • Organizer
      第3回環境放射能除染研究発表会
    • Place of Presentation
      郡山市民文化センター(福島県郡山市)
    • Year and Date
      2014-07-03 – 2014-07-04
    • Related Report
      2014 Annual Research Report

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Published: 2014-11-20   Modified: 2019-03-29  

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