Aqueous chemistry of the heaviest elements using a gas-filled recoil ion separator
| Project/Area Number |
26286082
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| Research Category |
Grant-in-Aid for Scientific Research (B)
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| Allocation Type | Partial Multi-year Fund |
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| Section | 一般 |
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| Research Field |
Quantum beam science
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| Research Institution | Institute of Physical and Chemical Research |
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Principal Investigator |
HABA HIROMITSU 国立研究開発法人理化学研究所, 仁科加速器研究センター, チームリーダー (60360624)
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| Co-Investigator(Kenkyū-buntansha) |
小森 有希子 国立研究開発法人理化学研究所, 仁科加速器研究センター, 特別研究員 (50726370)
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| Co-Investigator(Renkei-kenkyūsha) |
MORIMOTO Kouji 国立研究開発法人理化学研究所, 仁科加速器研究センター, チームリーダー (00332247)
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| Project Period (FY) |
2014-04-01 – 2018-03-31
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| Project Status |
Completed (Fiscal Year 2017)
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| Budget Amount *help |
¥16,120,000 (Direct Cost: ¥12,400,000、Indirect Cost: ¥3,720,000)
Fiscal Year 2016: ¥3,510,000 (Direct Cost: ¥2,700,000、Indirect Cost: ¥810,000)
Fiscal Year 2015: ¥6,110,000 (Direct Cost: ¥4,700,000、Indirect Cost: ¥1,410,000)
Fiscal Year 2014: ¥6,500,000 (Direct Cost: ¥5,000,000、Indirect Cost: ¥1,500,000)
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| Keywords | 超重元素 / 106番元素シーボーギウム / 107番元素ボーリウム / 気体充填型反跳核分離装置 / 溶媒抽出装置 / 単一原子化学 / 重イオン線形加速器 / 相対論効果 / 理研重イオン線形加速器 / シーボーギウム / ボーリウム / 理研重イオンリニアック |
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| Outline of Final Research Achievements |
A rapid chemical analysis system has been developed for superheavy elements by installing a gas-jet transport system, a continuous dissolution apparatus, a flow solvent extractor, and a flow liquid scintillation detector to the RIKEN gas-filled recoil ion separator. The present system is expected to realize aqueous chemistry of the heaviest elements such as element 106, seaborgium (Sg) and element 107 bohrium (Bh).
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Report
(5 results)
Research Products
(152 results)
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[Journal Article] Observation of the chemical reaction equilibria of element 104, rutherfordium: Solid-liquid extraction of Rf, Zr, Hf and Th with Aliquat 336 resin from HCl2017
Author(s)
T. Yokokita, Y. Kasamatsu, A. Kino, H. Haba, Y. Shigekawa, Y. Yasuda, K. Nakamura, K. Toyomura, Y. Komori, M. Murakami, T. Yoshimura, N. Takahashi, K. Morita, and A. Shinohara
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Journal Title
RIKEN Accel. Prog. Rep.
Volume: 50
Pages: 26-26
Related Report
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[Journal Article] On-line column chromatograpy of 88Nb with 52 wt% Aliquat 336 resin from HF media for Db experiment2017
Author(s)
D. Sato, M. Murakami, S. Goto, K. Ooe, R. Motoyama, K. Shirai, S. Tsuchiya, H. Haba, Y. Komori, S. Yano, A. Toyoshima, A. Mitsukai, H. Kikunaga, and H. Kudo
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Journal Title
RIKEN Accel. Prog. Rep.
Volume: 50
Pages: 246-246
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[Journal Article] On-line solvent extraction of Re with a rapid solvent extraction apparatus coupled to the GARIS gas-jet system2017
Author(s)
Y. Komori, H. Haba, K. Ooe, D. Kaji, Y. Kasamatsu, H. Kikunaga, A. Mitsukai, K. Morimoto, R. Motoyama, J. P. Omtvedt, Z. Qin, D. Sato, N. Sato, Y. Shigekawa, T. Tanaka, A. Toyoshima, K. Tsukada, Y. Wang, K. Watanabe, S. Wulff, S. Yamaki, S. Yano, and Y. Yasuda
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Journal Title
RIKEN Accel. Prog. Rep.
Volume: 50
Pages: 247-247
Related Report
Open Access / Int'l Joint Research
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[Journal Article] Batch solid-liquid extraction of Nb and Ta with 52 wt% Aliquat 336 resin from HF solutions2017
Author(s)
D. Sato, M. Murakami, K. Ooe, R. Motoyama, H. Haba, Y. Komori, A. Toyoshima, A. Mitsukai, H. Kikunaga, S. Goto, and H. Kudo
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Journal Title
RIKEN Accel. Prog. Rep.
Volume: 50
Pages: 249-249
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[Journal Article] Coprecipitation experiment with Sm hydroxide using a multitracer produced by nuclear spallation reaction: A tool for chemical studies with superheavy elements2017
Author(s)
Y. Kasamatsu, T. Yokokita, K. Toyomura, Y. Shigekawa, H. Haba, J. Kanaya, M. Huang, Y. Ezaki, T. Yoshimura, K. Morita, and A. Shinohara
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Journal Title
RIKEN Accel. Prog. Rep.
Volume: 50
Pages: 252-252
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[Journal Article] First online multi reflection time-of-flight mass measurements of isobaric chains produced by fusion-evaporation reactions: Toward identification of superheavy elements via mass spectroscopy2017
Author(s)
P.Schury, M.Wada, Y.Ito, D.Kaji, F.Arai, M.MacCormick, I.Murray, H.Haba, S.Jeong, S.Kimura, H.Koura, H.Miyatake, K.Morimoto, K.Morita, A.Ozawa, M. Reponen, P-A.Soederstroem, A.Takamine, T.Tanaka, H.Wollnik
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Journal Title
Physical Review C
Volume: 95
Issue: 1
Pages: 011305-011305
DOI
NAID
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[Journal Article] Study of the reaction 48Ca + 248Cm → 296Lv* at RIKEN-GARIS2017
Author(s)
D. Kaji, K. Morita, K. Morimoto, H. Haba, M. Asai, K. Fujita, Z. Gan, H. Geissel, H. Hasebe, S. Hofmann, M. Huang, Y. Komori, L. Ma, J. Maurer, M. Murakami, M. Takeyama, F. Tokanai, T. Tanaka, Y. Wakabayashi, T. Yamaguchi, S. Yamaki, and A. Yoshida
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Journal Title
J. Phys. Soc. Jpn.
Volume: 86
Issue: 3
Pages: 034201-034201
DOI
NAID
Related Report
Peer Reviewed / Int'l Joint Research
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[Journal Article] Coprecipitation experiment with Sm hydroxide using a multitracer produced by nuclear spallation reaction: A tool for chemical studies with superheavy elements Applied Radiation and Isotopes2016
Author(s)
Y. Kasamatsu, T. Yokokita, K. Toyomura, Y. Shigekawa, H. Haba, J. Kanaya, M. Huang, Y. Ezaki, T. Yoshimura, K. Morita, and A. Shinohara
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Journal Title
Appl. Radiat. Isot.
Volume: 118
Pages: 105-116
DOI
Related Report
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[Journal Article] Observation of the chemical reaction equilibria of element 104, rutherfordium: Solid-liquid extraction of Rf, Zr, Hf and Th with Aliquat 336 resin from HCl2016
Author(s)
T. Yokokita, Y. Kasamatsu, A. Kino, H. Haba, Y. Shigekawa, Y. Yasuda, K. Nakamura, K. Toyomura, Y. Komori, M. Murakami, T. Yoshimura, N. Takahashi, K. Morita, and A. Shinohara
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Journal Title
Dalton Trans.
Volume: 45
Issue: 47
Pages: 18827-18831
DOI
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[Journal Article] In-Situ Synthesis of Volatile Carbonyl Complexes with Short-Lived Nuclides2015
Author(s)
J. Even, D. Ackermann, M. Asai, M. Block, H. Brand, A. Di Nitto, Ch. E. Duellmann, R. Eichler, F. Fan, H. Haba, W. Hartmann, A. Huebner, F. P. Hessberger, M. Huang, E. Jaeger, D. Kaji, J. Kanaya, Y. Kaneya, J. Khuyagbaatar, B. Kindler, J. V. Kratz, J. Krier, Y. Kudou, N. Kurz, M. Laatiaoui, B. Lommel, J. Maurer et al.
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Journal Title
J. Radioanal. Nucl. Chem.
Volume: 303
Pages: 2457-2466
DOI
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[Journal Article] Development of an automated batch-type solid-liquid extraction apparatus and extraction of Zr, Hf, and Th by triisooctylamine from HCl solutions for chemistry of element 104, Rf2015
Author(s)
Kasamatsu,Y., Kino, A., Yokokita, T., Nakamura, K., Komori, Y., Toyomura, K., Yoshimura, T., Haba, H., Kanaya, J., Huang, M., Kudou, Y., Takahashi, N., and Shinohara, A.
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Journal Title
Radiochim. Acta
Volume: 103
Issue: 7
Pages: 513-521
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[Journal Article] Decomposition studies of group 6 hexacarbonyl complexes. Part 1: Production and decomposition of Mo(CO)6 and W(CO)62015
Author(s)
I. Usoltsev, R. Eichler, Y. Wang, J. Even, A. Yakushev, H. Haba, M. Asai, H. Brand, A. Di Nitto, Ch.E. Duellmann, F. Fangli, W. Hartmann, M. Huang, E. Jaeger, D. Kaji, J. Kanaya, Y. Kaneya, J. Khuyagbaatar, B. Kindler, J.V. Kratz, J. Krier, Y. Kudou, N. Kurz, B. Lommel, S. Miyashita et al.
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Journal Title
Radiochim. Acta
Volume: 104
Issue: 3
Pages: 141-151
DOI
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Organizer
日本物理学会 第72回年次大会（2017年）
Place of Presentation
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Year and Date
2017-03-20
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[Presentation] 50Ti,51V+248Cm反応における融合障壁分布の測定2017
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日本物理学会 第72回年次大会（2017年）
Place of Presentation
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Year and Date
2017-03-20
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[Presentation] 超重元素化学の現状と展望2017
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Place of Presentation
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Year and Date
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[Presentation] Liquid-liquid extraction of element 104, Rf, in Aliquat 336/HCl system2017
Author(s)
N. Kondo, Y. Kasamatsu, H. Haba, K. Ouchi, M. Nagase, Y. Yasuda, Y. Shigekawa, A. Kanda, Y. Kuboki, Y. Komori, S. Yano, N. Sato, T. Yokokita, and A. Shinohara
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ACTINIDES2017, July 9-14, 2017, Sendai, Japan
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[Presentation] Development of a rapid solvent extraction apparatus coupled to the GARIS gas-jet transport system for aqueous chemistry of the heaviest elements2017
Author(s)
Y. Komori, H. Haba, K. Ooe, D. Kaji, Y. Kasamatsu, H. Kikunaga, A. Mitsukai, K. Morimoto, R. Motoyama, J. P. Omtvedt, Z. Qin, D. Sato, N. Sato, Y. Shigekawa, T. Tanaka, A. Toyoshima, K. Tsukada, Y. Wang, K. Watanabe, S. Wulff, S. Yamaki, S. Yano, and Y. Yasuda
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[Presentation] Gas-phase chemistry of technetium and rhenium carbonyl complexes with short-lived isotopes2017
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Author(s)
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9th Workshop on the Chemistry of the Heaviest Elements, Oct. 8-11, 2017, Ascona, Switzerland
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[Presentation] Observation of the chemical reaction equilibria of rutherfordium2017
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[Presentation] Aliquat 336/HCl系におけるRfの溶媒抽出実験2017
Author(s)
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2017 Symposium on Nuclear Data, Nov. 16-17, 2017, Tokai-mura, Ibaraki, Japan
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9th International Conference on Nuclear and Radiochemistry (NRC9)
Place of Presentation
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Year and Date
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9th International Conference on Nuclear and Radiochemistry (NRC9)
Place of Presentation
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Year and Date
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[Presentation] Development of a rapid solvent extraction apparatus for aqueous chemistry of the heaviest elements2016
Author(s)
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Place of Presentation
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Year and Date
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Author(s)
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Place of Presentation
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Year and Date
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[Presentation] Solid-liquid and liquid-liquid extractions of Zr, Hf, Th and element 104, Rf, in an Aliquat 336/HCl system2015
Author(s)
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Organizer
International Chemical Congress of Pacific Basin Societies 2015 (Pacifichem 2015)
Place of Presentation
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Year and Date
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[Presentation] Extraction behavior of Mo and W from H2SO4 with Aliquat336 as homologues of seaborgium (Sg)2015
Author(s)
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Place of Presentation
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[Presentation] Liquid-liquid extraction behavior of zirconium and hafnium as homologs of element 104, rutherfordium using chelate extractants2015
Author(s)
K. Ooe, A. Tanaka, R. Yamada, H. Kikunaga, M. Murakami, Y. Komori, H. Haba, S. Goto, and H. Kudo
Organizer
International Chemical Congress of Pacific Basin Societies 2015 (Pacifichem 2015)
Place of Presentation
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Year and Date
2015-12-19
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[Presentation] 硫酸-Aliquat336系におけるMoならびにWの溶媒抽出挙動：超重元素Sgの硫酸錯体形成に向けたモデル実験2015
Author(s)
水飼秋菜, 豊嶋厚史, 金谷佑亮, 大江一弘, 佐藤大輔, 村上昌史, 小森有希子, 羽場宏光, 浅井雅人, 塚田和明, 佐藤哲也, 永目諭一郎
Organizer
2015日本放射化学会年会・第59回放射化学討論会
Place of Presentation
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Year and Date
2015-09-25
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[Presentation] Production of Radioisotopes of 261Rf, 262Db, 265Sg, and 266,267Bh for Superheavy Element Chemistry Using GARIS at RIKEN2015
Author(s)
H. Haba, R. Aono, D. Kaji, Y. Kasamatsu, H. Kikunaga, Y. Komori, H. Kudo, K. Morimoto, K. Morita, M. Murakami, K. Nishio, K. Ooe, A. Shinohara, M. Takeyama, T. Tanaka, A. Toyoshima, K. Tsukada, S. Tsuto, Y. Wakabayashi, S. Yamaki, T. Yokokita, and A. Yoneda
Organizer
5th International Conference on the Chemistry and Physics of the Transactinide Elements (TAN15)
Place of Presentation
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Year and Date
2015-05-29
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[Presentation] Coprecipitation Behavior of Rf with Sm Hydroxide2015
Author(s)
Y. Kasamatsu, K. Toyomura, T. Yokokita, Y. Shigekawa, H. Haba, Y. Komori, J. Kanaya, M. Huang, K. Morita, N. Takahashi, M. Murakami, H. Kikunaga, T. Mitsugashira, T. Yoshimura, T. Ohtsuki, K. Takamiya, and A. Shinohara
Organizer
5th International Conference on the Chemistry and Physics of the Transactinide Elements (TAN15)
Place of Presentation
裏磐梯ロイヤルホテル（福島県・耶麻郡）
Year and Date
2015-05-27
Related Report
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[Presentation] Solid-Liquid Extraction of Rf with Aliquat 336 from HCl2015
Author(s)
T. Yokokita, Y. Kasamatsu, Y. Shigekawa, Y. Yasuda, K. Nakamura, A. Kino, K. Toyomura, N. Takahashi, H. Haba, Y. Komori, M. Murakami, T. Yoshimura, and A. Shinohara
Organizer
5th International Conference on the Chemistry and Physics of the Transactinide Elements (TAN15)
Place of Presentation
裏磐梯ロイヤルホテル（福島県・耶麻郡）
Year and Date
2015-05-27
Related Report
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[Presentation] Developments towards Aqueous Phase Chemistry of Transactinide Elements2015
Author(s)
A. Toyoshima, K. Ooe, M. Asai, M.F. Attallah, N. Goto, N.S. Gupta, H. Haba, M. Kaneko, Y. Kaneya, Y. Kasamatsu, Y. Kitatsuji, Y. Kitayama, K. Koga, Y. Komori, T. Koyama, J.V. Kratz, H.V. Lerum, A. Mitsukai, S. Miyashita, Y. Oshimi, V. Pershina, D. Sato, T.K. Sato, Y. Shigekawa, A. Shinohara, A. Tanaka et al.
Organizer
5th International Conference on the Chemistry and Physics of the Transactinide Elements (TAN15)
Place of Presentation
裏磐梯ロイヤルホテル（福島県・耶麻郡）
Year and Date
2015-05-27
Related Report
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[Presentation] Excitation Functions of Db Isotopes Produced in 248Cm(19F,xn) Reaction2015
Author(s)
M. Murakami, S. Goto, K. Ooe, D. Sato, S. Tsuto, N. Goto, T. Koyama, R. Aono, H. Haba, M Huang, and H. Kudo
Organizer
5th International Conference on the Chemistry and Physics of the Transactinide Elements (TAN15)
Place of Presentation
裏磐梯ロイヤルホテル（福島県・耶麻郡）
Year and Date
2015-05-26
Related Report
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[Presentation] Extraction Behavior of Mo and W from H2SO4 with Aliquat336 as Homologs of Seaborgium (Sg)2015
Author(s)
A. Mitsukai, A. Toyoshima, A. Vascon, Y. Kaneya, M. Murakami, K. Ooe, N. Goto, D. Sato, Y. Komori, H. Haba, K. Tsukada, M. Asai, T.K. Sato, Y. Nagame, and M. Schaedel
Organizer
5th International Conference on the Chemistry and Physics of the Transactinide Elements (TAN15)
Place of Presentation
裏磐梯ロイヤルホテル（福島県・耶麻郡）
Year and Date
2015-05-26
Related Report
-
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[Presentation] Extraction Behavior of Rutherfordium as a Cationic Fluoride Complex with a TTA Chelate Extractant from HF/HNO3 Acidic Solutions2015
Author(s)
Y. Kitayama, Y. Fukuda, H. Haba, K. Tsukada, A. Toyoshima, H. Kikunaga, M. Murakami, Y. Komori, M.H. Huang, T. Taniguchi, S. Ueno, K. Hayashi, Y. Yatsu, I. Chiyonishio, K. Murakami, and A. Yokoyama
Organizer
5th International Conference on the Chemistry and Physics of the Transactinide Elements (TAN15)
Place of Presentation
裏磐梯ロイヤルホテル（福島県・耶麻郡）
Year and Date
2015-05-26
Related Report
-
[Presentation] Adsorption Behavior of Zr and Hf by TTA-reversed-phase Chromatography for Aqueous Chemistry of a Super-heavy Element, Rf2015
Author(s)
Y. Fukuda, Y. Kitayama, H. Haba, K. Tsukada, A. Toyoshima, H. Kikunaga, M.H. Huang, M. Murakami, Y. Komori, I. Chiyonishio, and A. Yokoyama
Organizer
5th International Conference on the Chemistry and Physics of the Transactinide Elements (TAN15)
Place of Presentation
裏磐梯ロイヤルホテル（福島県・耶麻郡）
Year and Date
2015-05-26
Related Report
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[Presentation] Development of a Rapid Flow-Type Solvent Extraction Apparatus for Extraction of Rf2015
Author(s)
Y. Kasamatsu, K. Nakamura, T. Yokokita, Y. Shigekawa, Y. Yasuda, N. Takahashi, Y. Kuboki, H. Haba, M. Murakami, T. Yoshimura, and A. Shinohara
Organizer
5th International Conference on the Chemistry and Physics of the Transactinide Elements (TAN15)
Place of Presentation
裏磐梯ロイヤルホテル（福島県・耶麻郡）
Year and Date
2015-05-26
Related Report
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