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Development of dynamic nuclear polarization magnetic resonance force microscope (DNP-MRFM)

Research Project

Project/Area Number 26287081
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypePartial Multi-year Fund
Section一般
Research Field Condensed matter physics II
Research InstitutionKobe University

Principal Investigator

OHMICHI EIji  神戸大学, 理学(系)研究科(研究院), 准教授 (00323634)

Co-Investigator(Renkei-kenkyūsha) OHTA Hitoshi  神戸大学, 分子フォトサイエンス研究センター, 教授 (70194173)
Project Period (FY) 2014-04-01 – 2017-03-31
Project Status Completed (Fiscal Year 2016)
Budget Amount *help
¥16,510,000 (Direct Cost: ¥12,700,000、Indirect Cost: ¥3,810,000)
Fiscal Year 2016: ¥1,820,000 (Direct Cost: ¥1,400,000、Indirect Cost: ¥420,000)
Fiscal Year 2015: ¥8,190,000 (Direct Cost: ¥6,300,000、Indirect Cost: ¥1,890,000)
Fiscal Year 2014: ¥6,500,000 (Direct Cost: ¥5,000,000、Indirect Cost: ¥1,500,000)
Keywordsカンチレバー / 電子スピン共鳴 / 磁気共鳴力顕微鏡 / DNP / 走査プローブ顕微鏡 / 物性実験 / 生物物理 / 磁気共鳴
Outline of Final Research Achievements

We developed ultrasensitive high-frequency electron spin resonance technique and terahertz magnetic resonance force microscopy. With use of fiber-optic Fabry-Perot interferometry, a tiny sample on the order of 100 ng could become possible. Our technique was applied to hemin, a model substance of hemoproteins in frequencies up to 0.5 THz, and precise determination of zero-field splliting parameters was made.
In addition, three-axis piezoelectric translational stage for low-temperature and high-field eperiments were developed. By sweeping a magnetic-tip holding cantilever over the sample surface, we succeeded in spatially resolved ESR measurements at liquid helium temperature.

Report

(4 results)
  • 2016 Annual Research Report   Final Research Report ( PDF )
  • 2015 Annual Research Report
  • 2014 Annual Research Report
  • Research Products

    (26 results)

All 2017 2016 2015 2014

All Journal Article (6 results) (of which Peer Reviewed: 6 results,  Acknowledgement Compliant: 5 results) Presentation (20 results) (of which Int'l Joint Research: 4 results,  Invited: 4 results)

  • [Journal Article] High-frequency electron paramagnetic resonance of metal-containing porphyrin compounds using a microcantilever2016

    • Author(s)
      Eiji Ohmichi, Tsubasa Okamoto, Masaaki Mitani, Hideyuki Takahashi, Hitoshi Ohta
    • Journal Title

      Journal of Inorganic Biochemistry

      Volume: 162 Pages: 190-193

    • DOI

      10.1016/j.jinorgbio.2016.04.016

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Multi-frequency force-detected electron spin resonance in the millimeter-wave region up to 150 GHz2016

    • Author(s)
      E. Ohmichi, Y. Tokuda, R. Tabuse, D. Tsubokura, T. Okamoto, and H. Ohta
    • Journal Title

      Review of Scientific Instruments

      Volume: 87 Issue: 7

    • DOI

      10.1063/1.4959152

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Development of Ultrasensitive Terahertz ESR Spectroscopy for Metalloprotein Using a Microcantilever2016

    • Author(s)
      T. Okamoto, H. Takahashi, E. Ohmichi, and H. Ohta
    • Journal Title

      Journal of Infrared, Millimeter, and Terahertz Waves

      Volume: 37 Issue: 12 Pages: 1173-1184

    • DOI

      10.1007/s10762-016-0305-6

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Wide-dynamic-range cantilever magnetometry using a fiber-optic interferometer and its application to high-frequency electron spin resonance spectroscopy2016

    • Author(s)
      Hideyuki Takahashi, Tsubasa Okamoto, Eiji Ohmichi, and Hitoshi Ohta
    • Journal Title

      Applied Physics Express

      Volume: 9 Issue: 12 Pages: 126701-126701

    • DOI

      10.7567/apex.9.126701

    • NAID

      210000138131

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Development of High-Pressure ESR System Using Micro-coil2015

    • Author(s)
      K. Kawasaki, T. Sakurai, E. Ohmichi, S. Okubo, H. Ohta, K. Matsubayashi, Y. Uwatoko
    • Journal Title

      Appl. Magn. Reson.

      Volume: 46 Issue: 9 Pages: 987-992

    • DOI

      10.1007/s00723-015-0650-y

    • Related Report
      2015 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Mechanical detection of electron spin resonance beyond 1 THz2015

    • Author(s)
      H. Takahashi, E. Ohmichi, H. Ohta
    • Journal Title

      Appl. Phys. Lett.

      Volume: 107 Issue: 18

    • DOI

      10.1063/1.4935204

    • NAID

      120005842525

    • Related Report
      2015 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Presentation] メンブレン型ピエゾ抵抗センサーを用いた微小試料の磁気測定2017

    • Author(s)
      大道英二
    • Organizer
      日本物理学会 第72回年次大会
    • Place of Presentation
      大阪大学(大阪府・豊中市)
    • Year and Date
      2017-03-18
    • Related Report
      2016 Annual Research Report
  • [Presentation] Development of mechanically detected terahertz electron spin resonance technique2017

    • Author(s)
      Eiji Ohmichi
    • Organizer
      Molecular Photo Research Center International Symposium "Recent Advances in Terahertz Molecular Science"
    • Place of Presentation
      Kobe University (Kobe, Hyogo)
    • Year and Date
      2017-03-06
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] マイクロカンチレバーを用いたテラヘルツ電子スピン共鳴測定とその応用2017

    • Author(s)
      大道英二
    • Organizer
      テラヘルツ波科学技術と産業開拓182委員会第30回研究会
    • Place of Presentation
      大阪産業大学梅田サテライトキャンパス(大阪府・大阪市)
    • Year and Date
      2017-02-03
    • Related Report
      2016 Annual Research Report
    • Invited
  • [Presentation] カンチレバーを用いたテラヘルツ領域における電子スピン共鳴測定2016

    • Author(s)
      大道英二
    • Organizer
      テラヘルツ技術セミナー「テラヘルツ分子科学の進展」
    • Place of Presentation
      ホテル北野プラザ六甲荘(兵庫県・神戸市)
    • Year and Date
      2016-10-26
    • Related Report
      2016 Annual Research Report
    • Invited
  • [Presentation] カンチレバーを用いた磁気共鳴法の現状2016

    • Author(s)
      大道英二
    • Organizer
      第三回西日本強磁場科学研究会
    • Place of Presentation
      福井大学(福井県・福井市)
    • Year and Date
      2016-09-12
    • Related Report
      2016 Annual Research Report
  • [Presentation] ピエゾ抵抗型マイクロカンチレバーを用いた力検出高周波ESR測定法の開発2016

    • Author(s)
      岡本翔, 高橋英幸, 大道英二, 太田仁
    • Organizer
      日本物理学会 第71回年次大会
    • Place of Presentation
      東北学院大学(宮城県・仙台市)
    • Year and Date
      2016-03-21
    • Related Report
      2015 Annual Research Report
  • [Presentation] ミリ波領域における力検出ESR用ピエゾ駆動ステージの作製2016

    • Author(s)
      宮崎晃和, 大道英二, 太田仁
    • Organizer
      日本物理学会 第71回年次大会
    • Place of Presentation
      東北学院大学(宮城県・仙台市)
    • Year and Date
      2016-03-19
    • Related Report
      2015 Annual Research Report
  • [Presentation] 静電容量型マイクロカンチレバーの作製と高周波ESR測定への応用2016

    • Author(s)
      三木俊裕, 大道英二, 太田仁
    • Organizer
      日本物理学会 第71回年次大会
    • Place of Presentation
      東北学院大学(宮城県・仙台市)
    • Year and Date
      2016-03-19
    • Related Report
      2015 Annual Research Report
  • [Presentation] Cantilever detection of electron spin resonance in the terahertz region2016

    • Author(s)
      H. Takahashi, E. Ohmichi, H. Ohta
    • Organizer
      APS March meeting 2016
    • Place of Presentation
      Baltimore(米国)
    • Year and Date
      2016-03-15
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 磁化検出高周波ESR測定法のタンパク質への応用2015

    • Author(s)
      岡本翔、高橋英幸、大道英二、太田仁
    • Organizer
      第54回電子スピンサイエンス学会年会(SEST2015)
    • Place of Presentation
      朱鷺メッセ新潟(新潟県・新潟市)
    • Year and Date
      2015-11-03
    • Related Report
      2015 Annual Research Report
  • [Presentation] 光ファイバー光学系を用いたカシミール力測定装置の作製2015

    • Author(s)
      大道英二、石川陽帆、太田仁
    • Organizer
      日本物理学会2015年秋季大会
    • Place of Presentation
      関西大学(大阪府・吹田市)
    • Year and Date
      2015-09-19
    • Related Report
      2015 Annual Research Report
  • [Presentation] 後進行波管を光源として用いた機械検出ESRの高周波化2015

    • Author(s)
      高橋英幸, 大道英二, 太田仁
    • Organizer
      日本物理学会2015年秋季大会
    • Place of Presentation
      関西大学(大阪府・吹田市)
    • Year and Date
      2015-09-17
    • Related Report
      2015 Annual Research Report
  • [Presentation] カスタムカンチレバーを用いた超高感度ESR測定法の開発2015

    • Author(s)
      三木俊裕, 岡本翔, 大道英二, 太田仁
    • Organizer
      日本物理学会2015年秋季大会
    • Place of Presentation
      関西大学(大阪府・吹田市)
    • Year and Date
      2015-09-17
    • Related Report
      2015 Annual Research Report
  • [Presentation] カンチレバーを用いたヘムタンパク質の高周波ESR測定装置の改良2015

    • Author(s)
      岡本翔, 高橋英幸, 大道英二, 太田仁
    • Organizer
      日本物理学会2015年秋季大会
    • Place of Presentation
      関西大学(大阪府・吹田市)
    • Year and Date
      2015-09-16
    • Related Report
      2015 Annual Research Report
  • [Presentation] Magnet-on-cantilever配置におけるカンチレバーESR測定法の開発2015

    • Author(s)
      宮崎晃和, 大道英二, 大田仁
    • Organizer
      日本物理学会2015年秋季大会
    • Place of Presentation
      関西大学(大阪府・吹田市)
    • Year and Date
      2015-09-16
    • Related Report
      2015 Annual Research Report
  • [Presentation] Development for ultrasensitive terahertz ESR of metal protein using a microcantilever2015

    • Author(s)
      T. Okamoto, H. Takahashi, E. Ohmichi, H. Ohta
    • Organizer
      The Second International Symposium on Frontiers in THz Technology(FTT2015)
    • Place of Presentation
      アクトシティ浜松(静岡県・浜松市)
    • Year and Date
      2015-08-30
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Development of cantilever-detected ESR technique for small-volume heme protein analysis2015

    • Author(s)
      T. Okamoto, E, Ohmichi, H Ohta
    • Organizer
      The 3rd Awaji International Workshop on Electron Spin Science & Technology
    • Place of Presentation
      淡路夢舞台(兵庫県・淡路市)
    • Year and Date
      2015-06-15
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research
  • [Presentation] バイメタルカンチレバーを用いた熱的検出 高周波ESR測定法の開発2015

    • Author(s)
      大道英二, 田伏諒, 太田仁
    • Organizer
      日本物理学会
    • Place of Presentation
      早稲田大学(東京)
    • Year and Date
      2015-03-23
    • Related Report
      2014 Annual Research Report
  • [Presentation] マイクロカンチレバーを用いた超高感度高周波ESR測定2015

    • Author(s)
      大道英二
    • Organizer
      日本物理学会
    • Place of Presentation
      早稲田大学(東京)
    • Year and Date
      2015-03-22
    • Related Report
      2014 Annual Research Report
    • Invited
  • [Presentation] Recent advances in cantilever-detected ESR technique2014

    • Author(s)
      E. Ohmichi, R. Tabuse, A. Ishikawa, T. Okamoto, and H. Ohta
    • Organizer
      APES-IES-SEST 2014
    • Place of Presentation
      東大寺総合文化センター(日本、奈良)
    • Year and Date
      2014-11-14
    • Related Report
      2014 Annual Research Report

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Published: 2014-04-04   Modified: 2020-05-15  

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