Local potential structure characterization of polar oxide interfaces by atomic-resolution electric field imaging STEM
Project/Area Number |
26289234
|
Research Category |
Grant-in-Aid for Scientific Research (B)
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Allocation Type | Partial Multi-year Fund |
Section | 一般 |
Research Field |
Inorganic materials/Physical properties
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Research Institution | The University of Tokyo |
Principal Investigator |
Shibata Naoya 東京大学, 工学(系)研究科(研究院), 准教授 (10376501)
|
Project Period (FY) |
2014-04-01 – 2017-03-31
|
Project Status |
Completed (Fiscal Year 2016)
|
Budget Amount *help |
¥16,120,000 (Direct Cost: ¥12,400,000、Indirect Cost: ¥3,720,000)
Fiscal Year 2016: ¥2,600,000 (Direct Cost: ¥2,000,000、Indirect Cost: ¥600,000)
Fiscal Year 2015: ¥8,840,000 (Direct Cost: ¥6,800,000、Indirect Cost: ¥2,040,000)
Fiscal Year 2014: ¥4,680,000 (Direct Cost: ¥3,600,000、Indirect Cost: ¥1,080,000)
|
Keywords | STEM / セラミックス / 電場 / 極性結晶 / 界面 / 極性界面 / ポテンシャル |
Outline of Final Research Achievements |
In this study, we tried to directly observe electric field structures at ceramic interfaces by atomic-resolution differential phase contrast scanning transmission electron microscopy (DPC STEM) to understand the fundamental mechanisms of interface properties in polar ceramic materials. First, we developed theory and experimental setups for quantitative DPC STEM. Then, we applied this new technique to various applications. We obtained the following main results. 1. We could directly observe local electric field variation at polar crystal interfaces related to their local potential structures. 2. We could directly observe pn junction in semiconductor materials in real space as an electric field variation. 3. We could observe atomic electric field within gold single atoms.
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Report
(4 results)
Research Products
(105 results)
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[Journal Article] Assessment of Strain-Generated Oxygen Vacancies Using SrTiO3 Bicrystals2015
Author(s)
SY. Choi, SD. Kim, M. Choi, HS. Lee, J. Ryu, N. Shibata, T. Mizoguchi, E. Tochigi, T. Yamamoto, SJL. Kang, Y. Ikuhara
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Journal Title
NANO LETTERS
Volume: 15
Issue: 6
Pages: 4129-4134
DOI
Related Report
Peer Reviewed / Int'l Joint Research
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[Journal Article] Photoelectrochemical Oxidation of Water Using BaTaO2N Photoanodes Prepared by Particle Transfer Method2015
Author(s)
K. Ueda, T. Minegishi, J. Clune, M. Nakabayashi, T. Hisatomi, H. Nishiyama, M. Katayama, N. Shibata, J. Kubota, T. Yamada, K. Domen
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Journal Title
J. Am. Chem. Soc.
Volume: 137
Issue: 6
Pages: 2227-2230
DOI
Related Report
Peer Reviewed
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[Journal Article] Spatially-resolved mapping of history-dependent coupled electrochemical and electronical behaviors of electroresistive NiO2014
Author(s)
I. Sugiyama, Y. Kim, S. Jesse, E. Strelcov, A. Kumar, A. Tselev, E.K. Rahani, V. B. Shenoy, T. Yamamoto, N. Shibata, Y. Ikuhara, S.V. Kalinin
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Journal Title
Scientific Reports
Volume: 4
Issue: 1
Pages: 6725-6725
DOI
Related Report
Peer Reviewed / Open Access / Acknowledgement Compliant
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[Journal Article] Enhancement of Solar Hydrogen Evolution from Water by Surface Modification with CdS and TiO2 on Porous CuInS2 Photocathodes Prepared by Electrodeposition-Sulfurization Method2014
Author(s)
J. Zhao, T. Minegishi, L. Zhang, M. Zhong, Gunawan, M. Nakabayashi, G. Ma, T. Hisatomi, M. Katayama, S. Ikeda, N. Shibata, T. Yamada, K. Domen
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Journal Title
Angew. Chem. Int. Ed.
Volume: 53
Issue: 44
Pages: 11808-11812
DOI
Related Report
Peer Reviewed
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[Journal Article] Large magnetoelectric coupling in magnetically short-range ordered Bi5Ti3FeO15 film2014
Author(s)
H. Zhao, H. Kimura, Z. Cheng, M. Osada, J. Wang, X. Wang, S. Dou, Y. Liu, J. Yu, T. Matsumoto, T. Tohei, N. Shibata, Y. Ikuhara
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Journal Title
Scientific Reports
Volume: 4
Issue: 1
Pages: 5255-1
DOI
Related Report
Peer Reviewed / Open Access
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[Journal Article] A New Sealed Lithium-Peroxide Battery with a Co-Doped Li2O Cathode in a Superconcentrated Lithium Bis(fluorosulfonyl)amide Electrolyte2014
Author(s)
S. Okuoka, Y. Ogasawara, Y. Suga, M. Hibino, T. Kudo, H. Ono, K. Yonehara, Y. Sumida, Y. Yamada, A. Yamada, M. Oshima, E. Tochigi, N. Shibata, Y. Ikuhara and N. Mizuno
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Journal Title
Scientific Reports
Volume: 4
Issue: 1
Pages: 5684-5684
DOI
Related Report
Peer Reviewed
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[Journal Article] Atomic structure of luminescent centers in high-efficiency Ce-doped w-AlN single crystal2014
Author(s)
R.Ishikawa, A.R.Lupini, F.Oba, S.D.Findlay, N.Shibata, T.Taniguchi, K.Watanabe, H.Hayashi, T.Sakai, I.Tanaka, Y.Ikuhara, and S.J.Pennycook
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Journal Title
Scientific Reports
Volume: 4
Issue: 1
Pages: 3778-3778
DOI
Related Report
Peer Reviewed / Open Access
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[Presentation] Direct electromagnetic structure observation by aberration-corrected differential phase contrast scanning transmission electron microscopy2016
Author(s)
N. Shibata, S.D. Findlay, T. Matsumoto, T. Seki, G.S. Santolino, Y. Kohno, H. Sawada, H. Sasaki, Y.G. So, R. Ishikawa and Y. Ikuhara
Organizer
Microscopy and Microanalysis 2016
Place of Presentation
USA, Ohio, Columbus
Year and Date
2016-07-26
Related Report
Int'l Joint Research / Invited
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