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Nanostructuring of thermoelectric materials via high-energy nonequilibrium processes and their novel functions

Research Project

Project/Area Number 26289246
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypePartial Multi-year Fund
Section一般
Research Field Composite materials/Surface and interface engineering
Research InstitutionIbaraki University

Principal Investigator

Ikeda Teruyuki  茨城大学, 工学部, 教授 (40314421)

Co-Investigator(Kenkyū-buntansha) 鵜殿 治彦  茨城大学, 工学部, 助教授 (10282279)
太田 弘道  茨城大学, 工学部, 教授 (70168946)
永野 隆敏  茨城大学, 工学部, 講師 (70343621)
篠嶋 妥  茨城大学, 工学部, 教授 (80187137)
Project Period (FY) 2014-04-01 – 2018-03-31
Project Status Completed (Fiscal Year 2017)
Budget Amount *help
¥17,030,000 (Direct Cost: ¥13,100,000、Indirect Cost: ¥3,930,000)
Fiscal Year 2016: ¥1,040,000 (Direct Cost: ¥800,000、Indirect Cost: ¥240,000)
Fiscal Year 2015: ¥1,040,000 (Direct Cost: ¥800,000、Indirect Cost: ¥240,000)
Fiscal Year 2014: ¥14,950,000 (Direct Cost: ¥11,500,000、Indirect Cost: ¥3,450,000)
Keywords熱電特性 / ナノ構造 / 相変態 / 状態図 / 熱伝導率 / ギブス-トムソン効果 / 固溶度 / 複合組織 / 熱電変換材料 / 組織制御 / キャリア密度 / フォノン散乱 / ボールミル / 熱電変換 / ナノ材料 / ナノ構造化熱電材料 / バンド構造
Outline of Final Research Achievements

In this research, we searched novel strategies to improve thermoelectric properties via functions of nanostructuring thermoelectric materials which are abundant on the earth and environmentally friendly. Achievements of this project are as follows: 1) enhancement of carrier concentration from the Gibbs-Thomson effect by dispersion of nanoprecipitates in Si, 2) development of novel low temperature synthesis method for Mg2Si, 3) clarification of the condition for the formation of Si precipitates in plate shape in Mg2Si, and 4) development of an efficient method to study the relation among chemical composition-microstructure-thermoelectric properties.

Report

(5 results)
  • 2017 Annual Research Report   Final Research Report ( PDF )
  • 2016 Annual Research Report
  • 2015 Annual Research Report
  • 2014 Annual Research Report
  • Research Products

    (55 results)

All 2018 2017 2016 2015 2014 Other

All Journal Article (8 results) (of which Int'l Joint Research: 1 results,  Peer Reviewed: 4 results,  Open Access: 1 results,  Acknowledgement Compliant: 1 results) Presentation (45 results) (of which Int'l Joint Research: 10 results,  Invited: 7 results) Remarks (2 results)

  • [Journal Article] Phase-field simulation of the Si precipitation process in Mg2Si under an applied stress2018

    • Author(s)
      Bin Liu, Teruyuki Ikeda, Yasushi Sasajima
    • Journal Title

      Mater. Sci. Eng. B

      Volume: 229 Pages: 65-69

    • DOI

      10.1016/j.mseb.2017.12.022

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Thermal microscope measurement of thermal effusivity distribution in compositionally graded PbTe-Sb2Te3-Ag2Te alloy system2018

    • Author(s)
      Tsuyoshi Nishi, Suguru Yamamoto, Mori Okawa, Kimihito Hatori, Teruyuki Ikeda, Hiromichi Ohta
    • Journal Title

      Thermochimica Acta

      Volume: 659 Pages: 39-43

    • DOI

      10.1016/j.tca.2017.11.004

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Simulation of the Si Precipitation Process in Mg<sub>2</sub>Si Using a Phase-Field Kinetic Model2016

    • Author(s)
      Bin Liu, Teruyuki Ikeda, Yasushi Sasajima
    • Journal Title

      MATERIALS TRANSACTIONS

      Volume: 57 Issue: 6 Pages: 922-926

    • DOI

      10.2320/matertrans.M2015479

    • NAID

      130005153147

    • ISSN
      1345-9678, 1347-5320
    • Related Report
      2016 Annual Research Report 2015 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research / Acknowledgement Compliant
  • [Journal Article] 熱電材料の組織制御のために (1) 状態図と各種反応2015

    • Author(s)
      池田輝之
    • Journal Title

      日本熱電学会誌

      Volume: 11 Pages: 21-25

    • Related Report
      2015 Annual Research Report
  • [Journal Article] 熱電材料の組織制御のために (2) サイズと形態の制御2015

    • Author(s)
      池田輝之
    • Journal Title

      日本熱電学会誌

      Volume: 12 Pages: 20-24

    • NAID

      130008159683

    • Related Report
      2015 Annual Research Report
  • [Journal Article] 熱電材料の組織制御のために (3) 組織の定量化2015

    • Author(s)
      池田輝之
    • Journal Title

      日本熱電学会誌

      Volume: 12 Pages: 20-23

    • NAID

      130008159682

    • Related Report
      2015 Annual Research Report
  • [Journal Article] Applying Quantitative Microstructure Control in Advanced Functional Composites2014

    • Author(s)
      Nicholas A. Heinz , Teruyuki Ikeda , Yanzhong Pei , G. Jeffrey Snyder
    • Journal Title

      Advanced Functional Materials

      Volume: 24 Issue: 15 Pages: 2135-2153

    • DOI

      10.1002/adfm.201302899

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed
  • [Journal Article] バルク熱電材料のナノ構造化2014

    • Author(s)
      池田輝之
    • Journal Title

      まてりあ

      Volume: 53 Pages: 307-311

    • NAID

      130004647449

    • Related Report
      2014 Annual Research Report
  • [Presentation] High-thermoelectric performance of nanostructured doped Mg2Si2018

    • Author(s)
      Babak Alinejad, Teruyuki Ikeda
    • Organizer
      日本金属学会春期講演大会
    • Related Report
      2017 Annual Research Report
  • [Presentation] 一方向凝固を利用した熱電材料の組織探索2018

    • Author(s)
      齊藤明子, 西峯広智, 池田亜矢子, 池田輝之, 高際良樹
    • Organizer
      日本金属学会春期講演大会
    • Related Report
      2017 Annual Research Report
  • [Presentation] Si基熱電材料のキャリア濃度増大と耐用条件2018

    • Author(s)
      菅原龍太郎, 渡部紘介, 池田輝之
    • Organizer
      日本金属学会春期講演大会
    • Related Report
      2017 Annual Research Report
  • [Presentation] Low temperature rapid fabrication of Mg2Si via activated reactive consolidation2018

    • Author(s)
      Babak Alinejad, Teruyuki Ikeda
    • Organizer
      TMS 2018 147rd Annual Meeting & Exhibition
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Microstructure control of bulk thermoelectric materials via phase transformations2018

    • Author(s)
      Teruyuki Ikeda
    • Organizer
      SPARCA 2018
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Single-step low temperature solid state reaction for synthesis of high purity dense Mg2Si2017

    • Author(s)
      Babak Alinejad, Teruyuki Ikeda
    • Organizer
      日本金属学会春期講演大会
    • Place of Presentation
      首都大学東京南大沢キャンパス
    • Year and Date
      2017-03-17
    • Related Report
      2016 Annual Research Report
  • [Presentation] Mechanical alloying of the silicon-boron system2017

    • Author(s)
      叶洪,池田輝之
    • Organizer
      日本金属学会春期講演大会
    • Place of Presentation
      首都大学東京南大沢キャンパス
    • Year and Date
      2017-03-15
    • Related Report
      2016 Annual Research Report
  • [Presentation] Microstructural size and morphology control of Si base thermoelectric composites2017

    • Author(s)
      T. Ikeda
    • Organizer
      TMS 2017 146rd Annual Meeting & Exhibition
    • Place of Presentation
      San Diego, California
    • Year and Date
      2017-02-28
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] 熱物性顕微鏡を用いた鉄基合金系熱電変換材料の熱浸透率測定2017

    • Author(s)
      大川萌里, 西剛史, 池田輝之, 太田弘道, 羽鳥仁人
    • Organizer
      熱物性シンポジウム
    • Related Report
      2017 Annual Research Report
  • [Presentation] 新規熱電材料の開発における一方向凝固法の有効性2017

    • Author(s)
      齊藤明子,青野美南,西峯広智,池田輝之,高際良樹,長谷川靖洋
    • Organizer
      日本熱電学会
    • Related Report
      2017 Annual Research Report
  • [Presentation] Si-Sb熱電材料のナノ構造化とキャリア濃度および熱伝導率の関係2017

    • Author(s)
      菅原龍太郎,渡部紘介,池田輝之
    • Organizer
      日本熱電学会
    • Related Report
      2017 Annual Research Report
  • [Presentation] パルス通電焼結法による高密度Si焼結体の作製2017

    • Author(s)
      渡辺英和、池田輝之
    • Organizer
      日本熱電学会
    • Related Report
      2017 Annual Research Report
  • [Presentation] Microstructure tailoring of silicon-aluminum oxide nano-composite for thermoelectric applications2017

    • Author(s)
      Babak Alinejad, Teruyuki Ikeda
    • Organizer
      日本金属学会秋期講演大会
    • Related Report
      2017 Annual Research Report
  • [Presentation] Nanostructuring and its effects on thermoelectric properties of Si base composites2017

    • Author(s)
      T. Ikeda, K. Watanobe, Y. Hong
    • Organizer
      IUMRS-ICAM 2017
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Fabrication of highly pure, dense Mg2Si via single-step low temperature reactive consolidation2017

    • Author(s)
      B.Alinejad, T. Ikeda
    • Organizer
      IUMRS-ICAM 2017
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Macroscale thermoelectric materials with low dimensional nanoscale features2017

    • Author(s)
      Teruyuki Ikeda, Masayuki Murata, Takashi Komine, Hideyuki Kiue, and Yasuhiro Hasegawa
    • Organizer
      The 36th International Conference on Thermoelectrics
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Nanostructuring of Mg&#8322;Si and its thermoelectric properties2016

    • Author(s)
      T. Adachi, T. Ikeda, G. Jeffrey Snyder
    • Organizer
      The International Symposium of Quantum Beam Science at Ibaraki University
    • Place of Presentation
      Ibaraki University
    • Year and Date
      2016-11-19
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 応力下におけるMg2Si合金のSi析出相の成長過程のシミュレーション2016

    • Author(s)
      劉濱,篠嶋妥,池田輝之
    • Organizer
      軽金属学会第131回秋期大会
    • Place of Presentation
      茨城大学水戸キャンパス
    • Year and Date
      2016-11-05
    • Related Report
      2016 Annual Research Report
  • [Presentation] ギブズートムソン効果によるバルクシリコンの固溶度の変化2016

    • Author(s)
      渡部紘介,池田輝之
    • Organizer
      第13 回 ヤングメタラジスト研究交流会
    • Place of Presentation
      東京大学本郷キャンパス 山上会館
    • Year and Date
      2016-10-21
    • Related Report
      2016 Annual Research Report
  • [Presentation] 粉体焼結における高密度Si焼結体の作製とナノ構造化2016

    • Author(s)
      渡辺英和,池田輝之
    • Organizer
      第13 回 ヤングメタラジスト研究交流会
    • Place of Presentation
      東京大学本郷キャンパス 山上会館
    • Year and Date
      2016-10-21
    • Related Report
      2016 Annual Research Report
  • [Presentation] 熱物性顕微鏡を用いたPb30Sb10Ag10Te50熱電材料の局所熱浸透率測定2016

    • Author(s)
      西 剛史, 池田 輝之, 太田 弘道, 山本 俊, 大川 萌里, 羽鳥 仁人
    • Organizer
      日本金属学会秋期講演大会
    • Place of Presentation
      大阪大学豊中キャンパス
    • Year and Date
      2016-09-21
    • Related Report
      2016 Annual Research Report
  • [Presentation] "Fabrication of silicon-alumina nano-composite via ball milling-SPS method for thermoelectric applications"2016

    • Author(s)
      Babak ALINEJAD, Teruyuki IKEDA
    • Organizer
      日本金属学会秋期講演大会
    • Place of Presentation
      大阪大学豊中キャンパス
    • Year and Date
      2016-09-21
    • Related Report
      2016 Annual Research Report
  • [Presentation] シリコン熱電材料の焼結性及びナノ構造制御2016

    • Author(s)
      渡辺 英和,池田輝之
    • Organizer
      日本金属学会秋期講演大会
    • Place of Presentation
      大阪大学豊中キャンパス
    • Year and Date
      2016-09-21
    • Related Report
      2016 Annual Research Report
  • [Presentation] 組織制御熱電材料の現状とこれから2016

    • Author(s)
      池田輝之
    • Organizer
      応用物理学会秋季学術講演会
    • Place of Presentation
      朱鷺メッセ,新潟市
    • Year and Date
      2016-09-16
    • Related Report
      2016 Annual Research Report
    • Invited
  • [Presentation] バルクシリコンのナノ構造化とドーパント固溶度2016

    • Author(s)
      渡部紘介,池田輝之
    • Organizer
      日本熱電学会
    • Place of Presentation
      東京理科大学葛飾キャンパス
    • Year and Date
      2016-09-05
    • Related Report
      2016 Annual Research Report
  • [Presentation] Boron (phosphorus) doping of silicon by high-energy ball milling2016

    • Author(s)
      Hong Ye, Teruyuki Ikeda
    • Organizer
      日本熱電学会
    • Place of Presentation
      東京理科大学葛飾キャンパス
    • Year and Date
      2016-09-05
    • Related Report
      2016 Annual Research Report
  • [Presentation] Low dimensional approach to improved thermoelectric performance via powder metallurgy and crystal growth method2016

    • Author(s)
      Babak Alinejad, Takashi Inozaki, Akiko Saitoh, Teruyuki Ikeda
    • Organizer
      日本熱電学会
    • Place of Presentation
      東京理科大学葛飾キャンパス
    • Year and Date
      2016-09-05
    • Related Report
      2016 Annual Research Report
  • [Presentation] Mg2Si合金におけるSi析出相の成長過程に及ぼす外部応力の影響2016

    • Author(s)
      リュウ ビン,池田輝之 篠嶋妥
    • Organizer
      軽金属学会関東支部総会・講演会
    • Place of Presentation
      東工大蔵前会館 くらまえホール
    • Year and Date
      2016-08-29
    • Related Report
      2016 Annual Research Report
  • [Presentation] Nanostructuring thermoelectric materials and its functions in various aspects2016

    • Author(s)
      Kosuke Watanobe, Ye Hong, Tetsuya Adachi, Takashi Inozaki, Yasuharu Saruta, Naotoshi Uchida, Teruyuki Ikeda
    • Organizer
      The 35th International Conference & The 1st Asia Conference on Thermoelectrics
    • Place of Presentation
      Wuhan, China
    • Year and Date
      2016-05-29
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Nanostructuring thermoelectric materials and its functions in various aspects2016

    • Author(s)
      Kosuke Watanobe, Ye Hong, Tetsuya Adachi, Takashi Inozaki, Yasuharu Saruta, Naotoshi Uchida, Teruyuki Ikeda
    • Organizer
      International Conference on Thermoelectrics
    • Place of Presentation
      武漢 (中国)
    • Year and Date
      2016-05-29
    • Related Report
      2015 Annual Research Report
  • [Presentation] マルチ拡散対法による効率的な多元系状態図の作成2016

    • Author(s)
      池田亜矢子,池田輝之
    • Organizer
      日本金属学会春期講演大会
    • Place of Presentation
      東京理科大学葛飾キャンパス
    • Year and Date
      2016-03-23
    • Related Report
      2015 Annual Research Report
  • [Presentation] 高エネルギーボールミルによるシリコンおよびシリサイド熱電材料のナノ構造化と制御2016

    • Author(s)
      安達哲也,叶洪,渡部紘介,井野崎崇,池田輝之
    • Organizer
      日本金属学会春期講演大会
    • Place of Presentation
      東京理科大学葛飾キャンパス
    • Year and Date
      2016-03-23
    • Related Report
      2015 Annual Research Report
  • [Presentation] Mg2Si合金におけるSi析出相の成長過程のPhase-Field シミュレーション2016

    • Author(s)
      劉濱,池田輝之,篠嶋妥
    • Organizer
      日本金属学会春期講演大会
    • Place of Presentation
      東京理科大学葛飾キャンパス
    • Year and Date
      2016-03-23
    • Related Report
      2015 Annual Research Report
  • [Presentation] 熱電材料のナノ構造化とドーパント固溶限2016

    • Author(s)
      渡部紘介,池田輝之
    • Organizer
      日本金属学会春期講演大会
    • Place of Presentation
      東京理科大学葛飾キャンパス
    • Year and Date
      2016-03-23
    • Related Report
      2015 Annual Research Report
  • [Presentation] Nanostructuring silicon base materials and its impacts on the thermoelectric properties2016

    • Author(s)
      Teruyuki Ikeda
    • Organizer
      TMS 2016 145rd Annual Meeting & Exhibition
    • Place of Presentation
      Nashville, Tennessee
    • Year and Date
      2016-02-14
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Phase field simulation of precipitation process of Si in Mg2Si2015

    • Author(s)
      Bin LIU, Yasushi SASAJIMA, Teruyuki IKEDA
    • Organizer
      25th Annual Meeting of MRS-J
    • Place of Presentation
      Yokohama, Japan
    • Year and Date
      2015-12-08
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 熱物性顕微鏡を用いたハイスループットな手法への挑戦2015

    • Author(s)
      西 剛史、山本 俊、大川萌里、太田弘道
    • Organizer
      日本機械学会第7回マイクロ・ナノ工学シンポジウム
    • Place of Presentation
      朱鷺メッセ(新潟県新潟市)
    • Year and Date
      2015-10-30
    • Related Report
      2015 Annual Research Report
  • [Presentation] 熱物性顕微鏡によるコンビナトリアル熱電変換材料の熱浸透率測定2015

    • Author(s)
      山本俊,大川萌里,西剛史,池田輝之,太田弘道,羽鳥仁人
    • Organizer
      第36回日本熱物性シンポジウム
    • Place of Presentation
      東北大学片平さくらホール
    • Year and Date
      2015-10-19
    • Related Report
      2015 Annual Research Report
  • [Presentation] 周期加熱放射測温法による熱拡散率分布測定法の開発2015

    • Author(s)
      羽鳥仁人・粟野孝昭・野口秀則・篠原貴洸・西 剛史・太田弘道
    • Organizer
      第36回日本熱物性シンポジウム
    • Place of Presentation
      東北大学片平キャンパス
    • Year and Date
      2015-10-19
    • Related Report
      2015 Annual Research Report
  • [Presentation] バルクシリコンのナノ構造化と溶解度2015

    • Author(s)
      渡部紘介,池田輝之
    • Organizer
      日本金属学会秋期講演大会
    • Place of Presentation
      九州大学伊都キャンパス
    • Year and Date
      2015-09-16
    • Related Report
      2015 Annual Research Report
  • [Presentation] 一方向凝固組成傾斜試料を利用した熱電材料のハイスループットな研究法2015

    • Author(s)
      鈴木利弥,池田輝之
    • Organizer
      日本金属学会秋期講演大会
    • Place of Presentation
      九州大学伊都キャンパス
    • Year and Date
      2015-09-16
    • Related Report
      2015 Annual Research Report
  • [Presentation] 熱電材料研究の現状とこれから2015

    • Author(s)
      池田輝之
    • Organizer
      一般社団法人 資源・素材学会東北支部 平成27年度春季大会
    • Place of Presentation
      東北大学片平さくらホール
    • Year and Date
      2015-06-17
    • Related Report
      2015 Annual Research Report
    • Invited
  • [Presentation] Control and stability of nanostructures of thermoelectric materials2015

    • Author(s)
      Teruyuki Ikeda
    • Organizer
      TMS 2015 144rd Annual Meeting & Exhibition
    • Place of Presentation
      Orlando (Florida), USA
    • Year and Date
      2015-03-15 – 2015-03-19
    • Related Report
      2014 Annual Research Report
    • Invited
  • [Presentation] PbTe基化合物のナノ構造化と格子熱伝導率2014

    • Author(s)
      田丸祐也 池田輝之
    • Organizer
      日本熱電学会
    • Place of Presentation
      物質・材料研究機構
    • Year and Date
      2014-09-29 – 2014-09-30
    • Related Report
      2014 Annual Research Report
  • [Presentation] 一方向凝固を利用したバルク機能材料のハイスループットな研究法2014

    • Author(s)
      鈴木利弥,池田輝之
    • Organizer
      日本熱電学会
    • Place of Presentation
      物質・材料研究機構
    • Year and Date
      2014-09-29 – 2014-09-30
    • Related Report
      2014 Annual Research Report
  • [Remarks] 材料組織と機能の研究室

    • URL

      http://tematiu.web.fc2.com/index.html

    • Related Report
      2016 Annual Research Report
  • [Remarks] 茨城大学工学部マテリアル工学科池田研究室

    • URL

      http://tematiu.web.fc2.com/index.html

    • Related Report
      2015 Annual Research Report 2014 Annual Research Report

URL: 

Published: 2014-04-04   Modified: 2019-03-29  

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