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Source apportionment of highly chlorinated polycyclic aromatics in the environment

Research Project

Project/Area Number 26340015
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeMulti-year Fund
Section一般
Research Field Environmental dynamic analysis
Research InstitutionMeijo University

Principal Investigator

Ohura Takeshi  名城大学, 農学部, 教授 (60315851)

Co-Investigator(Kenkyū-buntansha) 濱本 博三  名城大学, 農学部, 准教授 (40365896)
Project Period (FY) 2014-04-01 – 2017-03-31
Project Status Completed (Fiscal Year 2016)
Budget Amount *help
¥4,940,000 (Direct Cost: ¥3,800,000、Indirect Cost: ¥1,140,000)
Fiscal Year 2016: ¥1,040,000 (Direct Cost: ¥800,000、Indirect Cost: ¥240,000)
Fiscal Year 2015: ¥2,860,000 (Direct Cost: ¥2,200,000、Indirect Cost: ¥660,000)
Fiscal Year 2014: ¥1,040,000 (Direct Cost: ¥800,000、Indirect Cost: ¥240,000)
Keywords塩素化多環芳香族炭化水素 / ClPAHs / 発生源 / 環境動態 / POPs / 高塩素化PAHs / 環境分析 / 環境残留性 / POPs候補 / 多環芳香族炭化水素 / 大気汚染 / 生体蓄積 / 塩素化多環芳香族類 / 発生源解析 / GC/MS / PAHs
Outline of Final Research Achievements

The purpose of this study is to reveal the environmental behaviors of high-chlorinated polycyclic aromatic hydrocarbons (ClPAHs). To achieve the purpose we first synthesized the ClPAHs with more than 3 chlorine atom to use as standards, resulted that four species of ClPAHs were newly obtained. Next we investigated the concentrations of ClPAHs in the environment, and evaluated the possible emission sources. Surveying ClPAHs in ambient particles, 24 species of ClPAHs were detected in the samples. Also, the concentrations of metals, hopanes that are typical indicators of combustion sources were also investigated in the air samples. The relationships of concentrations between ClPAHs and certain indicators showed the significant correlations, suggested that ClPAHs in the air are produced by anthropogenic sources such as industrial activities and traffic. Furthermore the photodecay tests of ClPAHs showed that a part of PAHs become stable with increasing the number of chlorine substituted.

Report

(4 results)
  • 2016 Annual Research Report   Final Research Report ( PDF )
  • 2015 Research-status Report
  • 2014 Research-status Report
  • Research Products

    (21 results)

All 2017 2016 2015 2014

All Journal Article (10 results) (of which Int'l Joint Research: 2 results,  Peer Reviewed: 10 results,  Open Access: 4 results,  Acknowledgement Compliant: 2 results) Presentation (11 results) (of which Int'l Joint Research: 2 results,  Invited: 1 results)

  • [Journal Article] Size distribution of chlorinated polycyclic aromatic hydrocarbons in atmospheric particles2017

    • Author(s)
      K. Kakimoto, H. Nagayoshi, Y. Konishi, K. Kajimura, T. Ohura, T. Nakano, M. Hata, M. Furuuchi, N. Tang, K. Hayakawa, A. Toriba
    • Journal Title

      Arch. Environ. Contam. Toxicol.

      Volume: 72 Issue: 1 Pages: 58-64

    • DOI

      10.1007/s00244-016-0327-z

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Source apportionment of chlorinated polycyclic aromatic hydrocarbons associated with ambient particles in a Japanese megacity2016

    • Author(s)
      Y. Kamiya, A. Iijima, F. Ikemori, T. Okuda, T. Ohura
    • Journal Title

      Sci. Rep.

      Volume: 6 Issue: 1 Pages: 38358-38358

    • DOI

      10.1038/srep38358

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Spatio-temporal distribution, source, and genotoxic potential of polycyclic aromatic hydrocarbons in estuarine and riverine sediments from southern India2016

    • Author(s)
      P. Goswami, T. Ohura, K. S. Guruge, M. Yoshioka, N. Yamanaka, M. Akiba, N. Munuswamy
    • Journal Title

      Ecotoxicol. Environ. Saf.

      Volume: 130 Pages: 113-123

    • DOI

      10.1016/j.ecoenv.2016.04.016

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Local and seasonal variations in concentrations of chlorinated polycyclic aromatic hydrocarbons associated with particles in a Japanese megacity2016

    • Author(s)
      T. Ohura, Y. Kamiya, F. Ikemor
    • Journal Title

      J. Hazard. Mater.

      Volume: 312 Pages: 254-261

    • DOI

      10.1016/j.jhazmat.2016.03.072

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Photochlorination of polycyclic aromatic hydrocarbons in acidic brine solution2016

    • Author(s)
      T. Ohura, M. Miwa
    • Journal Title

      Bull. Environ. Contam. Toxicol.

      Volume: 96 Issue: 4 Pages: 524-529

    • DOI

      10.1007/s00128-015-1723-1

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Identification and characterization of oxidative metabolites of 1-chloropyrene.2015

    • Author(s)
      Kakimoto, K., Nagayoshi, H., Inazumi, N., Tani, A., Konishi, Y., Kajimura, K., Ohura, T., Nakano, T., Tang, N., Hayakawa, K., Toriba, A.
    • Journal Title

      Chem. Res. Toxicol.

      Volume: 28(9) Issue: 9 Pages: 1728-1736

    • DOI

      10.1021/acs.chemrestox.5b00173

    • Related Report
      2015 Research-status Report
    • Peer Reviewed / Open Access / Int'l Joint Research / Acknowledgement Compliant
  • [Journal Article] Optimization of pretreatment and ionization for GC/MS analysis for the determination of chlorinated PAHs in atmospheric particulate samples2015

    • Author(s)
      Y. Kamiya, F. Ikemori, T. Ohura
    • Journal Title

      Int. J. Environ. Anal. Chem.

      Volume: 95 Issue: 12 Pages: 1157-1168

    • DOI

      10.1080/03067319.2015.1048439

    • Related Report
      2015 Research-status Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Spatial and vertical distributions of sedimentary halogenated polycyclic aromatic hydrocarbons in moderately polluted areas of Asia.2015

    • Author(s)
      Ohura, T., Sakakibara, H., Watanabe, I., Shim, W.J., Manage, P.M., Guruge, K.S.
    • Journal Title

      Environmental Pollution

      Volume: 196 Pages: 331-340

    • DOI

      10.1016/j.envpol.2014.10.028

    • Related Report
      2015 Research-status Report
    • Peer Reviewed
  • [Journal Article] Sex-dependent difference in the hepatic and pulmonary toxicological effects in mice administrated 7-chlorinated benz[a]anthracene2014

    • Author(s)
      Hiroyuki Sakakibara, Takashi Ohura, Yuta Kamiya, Noriko Yamanaka, Nobuaki Shimada, Kayoko Shimoi, Keerthi S. Guruge
    • Journal Title

      Fundamental Toxicological Sciences

      Volume: 1 Pages: 101-108

    • Related Report
      2014 Research-status Report
    • Peer Reviewed
  • [Journal Article] Atmospheric chlorinated polycyclic aromatic hydrocarbons in East Asia2014

    • Author(s)
      K. Kakimoto, H. Nagayoshi, Y. Konishi, K. Kajimura, T. Ohura, K. Hayakawa, A. Toriba
    • Journal Title

      Chemosphere

      Volume: 111 Pages: 40-46

    • DOI

      10.1016/j.chemosphere.2014.03.072

    • Related Report
      2014 Research-status Report
    • Peer Reviewed / Open Access
  • [Presentation] Distribution of PAHs and their genotoxic potentials in surface and core sediments from southern India2016

    • Author(s)
      Keerthi S. Guruge, Prasun Goswami, Takeshi Ohura, Miyako Yoshioka, Noriko Yamanaka, Masato Akiba, Natesan Munuswamy
    • Organizer
      第25回環境化学討論会
    • Place of Presentation
      新潟
    • Year and Date
      2016-06-08
    • Related Report
      2016 Annual Research Report
  • [Presentation] 海鳥における塩素化多環芳香族類の生体蓄積性2016

    • Author(s)
      大浦 健、髙柳茉友子、新妻靖章
    • Organizer
      第25回環境化学討論会
    • Place of Presentation
      新潟
    • Year and Date
      2016-06-06
    • Related Report
      2016 Annual Research Report
  • [Presentation] Determination of particle-associated PAH derivatives(ClPAHs, NPAHs, OPAHs) in ambient air and automobile exhaust by gas chromatography/mass spectrometry with negative chemical ionization,2015

    • Author(s)
      Kamiya,Y., Kameda, T., Ohura, T., Tohno, S.
    • Organizer
      2015 International Symposium on Polycyclic Aromatic Compounds
    • Place of Presentation
      Bordeaux, France
    • Year and Date
      2015-09-13
    • Related Report
      2015 Research-status Report
    • Int'l Joint Research
  • [Presentation] ヒトチトクロームP450によるクロロピレンのin vitro 代謝解析2015

    • Author(s)
      永吉晴奈、柿本健作、稲角直也、谷 篤史、小西良昌、梶村計志、大浦 健、中野 武、早川和一、鳥羽 陽
    • Organizer
      第24回環境化学討論会
    • Place of Presentation
      札幌
    • Year and Date
      2015-06-24
    • Related Report
      2015 Research-status Report
  • [Presentation] 塩素化多環芳香族炭化水素類のナノ粒子中における粒径分布の解明2015

    • Author(s)
      柿本健作、永吉晴奈、小西良昌、梶村計志、大浦 健、畑 光彦、古内正美、唐 寧、早川和一、鳥羽 陽
    • Organizer
      第24回環境化学討論会
    • Place of Presentation
      札幌
    • Year and Date
      2015-06-24
    • Related Report
      2015 Research-status Report
  • [Presentation] Measurement of chlorinated polycyclic aromatic hydrocarbons associated with PM2.5 in Japan2015

    • Author(s)
      Yuta Kamiya, Takayuki Kameda, Takeshi Ohura, Daisuke Nakajima, Kimiyo Kumagai, Fumikazu Ikemori Makoto Kinoshita, Susumu Tohno
    • Organizer
      9th Asian Aerosol Conference (AAC)
    • Place of Presentation
      Kanazawa
    • Year and Date
      2015-06-24
    • Related Report
      2015 Research-status Report
    • Int'l Joint Research
  • [Presentation] Chlorinated Polycyclic Aromatic Hydrocarbons in Air Particulates in North-East Asia2014

    • Author(s)
      K. KAKIMOTO, H. NAGAYOSHI, S. TAKAGI, Y. KONISHI, K. KAJIMURA, T. OHURA, K. HAYAKAWA, A. TORIBA
    • Organizer
      International Conference of Asian Environmental Chemistry (ICAEC2014)
    • Place of Presentation
      Bangkok , THAILAND
    • Year and Date
      2014-11-24 – 2014-11-26
    • Related Report
      2014 Research-status Report
  • [Presentation] 塩素化多環芳香族炭化水素類の大気内挙動解析2014

    • Author(s)
      神谷優太,亀田貴之,大浦 健,東野 達
    • Organizer
      第55回大気環境学会年会
    • Place of Presentation
      松山
    • Year and Date
      2014-09-17 – 2014-09-19
    • Related Report
      2014 Research-status Report
  • [Presentation] 東京湾集水域におけるハロゲン化多環芳香族炭化水素類の環境残留特性2014

    • Author(s)
      堀井勇一、神谷優太、大浦 健
    • Organizer
      第23回環境化学討論会
    • Place of Presentation
      京都
    • Year and Date
      2014-05-14 – 2014-05-16
    • Related Report
      2014 Research-status Report
  • [Presentation] 生体試料中の塩素化多環芳香族類分析における前処理法の検討2014

    • Author(s)
      鈴木里奈、大浦 健
    • Organizer
      第23回環境化学討論会
    • Place of Presentation
      京都
    • Year and Date
      2014-05-14 – 2014-05-16
    • Related Report
      2014 Research-status Report
  • [Presentation] 大気ハロゲン化PAHs研究の最前線 ~分析法から発生源解析まで~2014

    • Author(s)
      大浦 健
    • Organizer
      第23回環境化学討論会
    • Place of Presentation
      京都
    • Year and Date
      2014-05-14
    • Related Report
      2014 Research-status Report
    • Invited

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Published: 2014-04-04   Modified: 2018-03-22  

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