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Investigation of the functional domain interfaces in ferroelectrics by controlling domain wall density

Research Project

Project/Area Number 26400327
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeMulti-year Fund
Section一般
Research Field Condensed matter physics I
Research InstitutionNational Institutes for Quantum and Radiological Science and Technology (2016-2017)
Japan Atomic Energy Agency (2014-2015)

Principal Investigator

OHWADA KENJI  国立研究開発法人量子科学技術研究開発機構, 関西光科学研究所 放射光科学研究センター, 上席研究員(定常) (60343935)

Co-Investigator(Kenkyū-buntansha) 松浦 直人  一般財団法人総合科学研究機構(総合科学研究センター(総合科学研究室)及び中性子科学センター(研究開発, 中性子科学センター, 副主任研究員 (30376652)
岩田 真  名古屋工業大学, 工学(系)研究科(研究院), 教授 (40262886)
西松 毅  東北大学, 金属材料研究所, 助教 (70323095)
Project Period (FY) 2014-04-01 – 2018-03-31
Project Status Completed (Fiscal Year 2017)
Budget Amount *help
¥4,810,000 (Direct Cost: ¥3,700,000、Indirect Cost: ¥1,110,000)
Fiscal Year 2016: ¥650,000 (Direct Cost: ¥500,000、Indirect Cost: ¥150,000)
Fiscal Year 2015: ¥1,690,000 (Direct Cost: ¥1,300,000、Indirect Cost: ¥390,000)
Fiscal Year 2014: ¥2,470,000 (Direct Cost: ¥1,900,000、Indirect Cost: ¥570,000)
Keywords強誘電体 / 界面 / ドメイン / リラクサー強誘電体 / 電場 / 放射光 / 中性子散乱 / 分子動力学法
Outline of Final Research Achievements

We have investigated the dynamics of domain walls in BaTiO3, in which the density of domain walls is much increased by the domain engineering process. We have found out the Bragg rods scattering from the domain wall for the first time by the synchrotron X-ray scattering, and performed the quasi-elastic neutron scattering experiment by focusing on the Bragg Rods scattering. The intensity was rapidly decreased toward the transition temperature (393 K). This is due to the broadening of the domain wall width towards the transition temperature. The energy width of the Bragg rods scattering was resolution limited (~3 micro eV). The results indicate that the energy scale of the domain wall dynamics is lower than 3 micro eV.

Report

(5 results)
  • 2017 Annual Research Report   Final Research Report ( PDF )
  • 2016 Research-status Report
  • 2015 Research-status Report
  • 2014 Research-status Report
  • Research Products

    (30 results)

All 2018 2017 2016 2015 2014 Other

All Journal Article (9 results) (of which Int'l Joint Research: 2 results,  Peer Reviewed: 9 results,  Open Access: 2 results,  Acknowledgement Compliant: 3 results) Presentation (20 results) (of which Int'l Joint Research: 7 results,  Invited: 11 results) Remarks (1 results)

  • [Journal Article] Polarization rotation associated with phonon dynamics in monoclinic C phase near morphotropic phase boundary studied by diffuse and inelastic X-ray scattering from a Ti-composition-gradient Pb[(Mg1/3Nb2/3)1-xTix]O3 single crystal2018

    • Author(s)
      K. Ohwada, S. Tsukada, M. Matsuura, S. Tsutsui, A. Q. R. Baron, J. Mizuki, K. Namikawa
    • Journal Title

      Ferroelectrics

      Volume: -

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Relation between Fractal Inhomogeneity and In/Nb-Arrangement in Pb(In1/2Nb1/2)O32017

    • Author(s)
      24. S. Tsukada, K. Ohwada, H. Ohwa, S. Mori, S. Kojima, N. Yasuda, H. Terauchi, and Y. Akishige
    • Journal Title

      Scientific Reports

      Volume: 7 Issue: 1 Pages: 17508-17508

    • DOI

      10.1038/s41598-017-17349-3

    • NAID

      120007134601

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] COHERENT X-RAY DIFFRACTION FOR DOMAIN OBSERVATION II2017

    • Author(s)
      K. Ohwada, D. Shimizu, J. Mizuki, K. Fujiwara, T. Nagata, N. Ikeda, H. Ohwa, N. Yasuda and K. Namikawa
    • Journal Title

      Ferroelectrics

      Volume: 511-513

    • Related Report
      2016 Research-status Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Design of a prototype split-and-delay unit for XFEL pulses, and their evaluation by synchrotron radiation X-rays2017

    • Author(s)
      Jun’ya Sakamoto, Kenji Ohwada, Masahiko Ishino, Jun’ichiro Mizuki, Masami Ando and Kazumichi Namikawa
    • Journal Title

      Journal of Synchrotron Radiation

      Volume: 24 Issue: 1 Pages: 95-102

    • DOI

      10.1107/s1600577516017744

    • Related Report
      2016 Research-status Report
    • Peer Reviewed
  • [Journal Article] Influence of defects on ferroelectric and electrocaloric properties of BaTiO32016

    • Author(s)
      A. Grunebohm and T. Nishimatsu
    • Journal Title

      Physical Review B

      Volume: 93 Issue: 13 Pages: 134101-134101

    • DOI

      10.1103/physrevb.93.134101

    • Related Report
      2015 Research-status Report
    • Peer Reviewed / Int'l Joint Research / Acknowledgement Compliant
  • [Journal Article] Negative correlation between electrical response and domain size in a Ti-composition-gradient Pb[(Mg1/3Nb2/3)1-xTix]O3 crystal near the morphotropic phase boundary2015

    • Author(s)
      Daisuke Shimizu, Shinya Tsukada, Masato Matsuura, Jun'ya Sakamoto, Seiji Kojima, Kazumichi Namikawa, Jun'ichiro Mizuki, and Kenji Ohwada
    • Journal Title

      Physical Review B

      Volume: 92 Issue: 17

    • DOI

      10.1103/physrevb.92.174121

    • Related Report
      2015 Research-status Report
    • Peer Reviewed
  • [Journal Article] The Performance of TOF near Backscattering Spectrometer DNA in MLF, J-PARC2015

    • Author(s)
      K. Shibata, N. Takahashi, Y. Kawakita, M. Matsuura, T. Yamada, T. Tominaga, W. Kambara, M. Kobayashi, Y. Inamura, T. Nakatani, K. Nakajima, and M. Arai
    • Journal Title

      JPS Conference Proceedings

      Volume: 8 Pages: 036022-036022

    • DOI

      10.7566/jpscp.8.036022

    • Related Report
      2015 Research-status Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Temperature-field phase diagram under the electric field along [111]c direction in BaTiO32015

    • Author(s)
      M. Iwata, K. Ando, M. Maeda, and Y. Ishibashi
    • Journal Title

      Japanese Journal of Applied Physics

      Volume: 54 Issue: 5 Pages: 051501-051501

    • DOI

      10.7567/jjap.54.051501

    • NAID

      210000145122

    • Related Report
      2015 Research-status Report
    • Peer Reviewed
  • [Journal Article] Elastocaloric Response of PbTiO3 Predicted from a First-Principles Effective Hamiltonian2015

    • Author(s)
      Jordan A. Barr, S. P. Beckman and Takeshi Nishimatsu
    • Journal Title

      J. Phys. Soc. Jpn.

      Volume: 84 Issue: 2 Pages: 024716-024716

    • DOI

      10.7566/jpsj.84.024716

    • NAID

      210000133445

    • Related Report
      2014 Research-status Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Presentation] BaTiO3のドメイン境界ダイナミクス2018

    • Author(s)
      大和田 謙二
    • Organizer
      日本物理学会第73回年次大会(2018)
    • Related Report
      2017 Annual Research Report
  • [Presentation] Dynamics of domain walls in BaTiO3(発表確定)2018

    • Author(s)
      K. Ohwada, M. Matsuura, S. Tsukada, K. Deno, J. Mizuki, and M. Iwata
    • Organizer
      2018 ISAF-FMA-AMF-AMEC-PFM (IFAAP) Joint Conference
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Multiple length scales in relaxor ferroelectrics2017

    • Author(s)
      Kenji Ohwada, Jun'ichiro Mizuki, Kazumichi Namikawa
    • Organizer
      Th 14th International Meeting on Ferroelectricity
    • Place of Presentation
      San Antonio (Texas, USA)
    • Year and Date
      2017-09-04
    • Related Report
      2016 Research-status Report
    • Int'l Joint Research / Invited
  • [Presentation] スローダイナミクスの立場から核共鳴準弾性散乱への期待2017

    • Author(s)
      大和田 謙二
    • Organizer
      第10回SPRUC 核共鳴散乱研究会、第1回核共鳴準弾性散乱研究会
    • Place of Presentation
      グランパーク カンファレンス 303 中会議室(東京都港区)
    • Year and Date
      2017-02-24
    • Related Report
      2016 Research-status Report
    • Invited
  • [Presentation] Multiple Length Scales in Relaxor Ferroielectrics2017

    • Author(s)
      大和田 謙二, 水木 純一郎, 並河 一道
    • Organizer
      The 14th International Meeting on Ferroelectricity (IMF2017)
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] X線回折を利用したBaTiO3正方晶相のドメイン境界の研究 / X-ray diffraction study of domain boundaries in the tetragonal BaTiO32016

    • Author(s)
      大和田 謙二
    • Organizer
      第26回日本MRS年次大会
    • Place of Presentation
      産業貿易センター(神奈川県横浜市)
    • Year and Date
      2016-12-20
    • Related Report
      2016 Research-status Report
  • [Presentation] Domain/heterophase fluctuations in the relaxor ferroelectrics studied by coherent x-ray diffraction2016

    • Author(s)
      K. Ohwada, D. Shimizu, J. Mizuki and K. Namikawa
    • Organizer
      Joint RCBJSF-IWRF Conference
    • Place of Presentation
      くにびきメッセ(島根県松江市)
    • Year and Date
      2016-06-19
    • Related Report
      2016 Research-status Report
    • Int'l Joint Research
  • [Presentation] Heterogeneity and relaxors: A synchrotron x-ray scattering study2015

    • Author(s)
      K. Ohwada
    • Organizer
      Pacifichem2015
    • Place of Presentation
      Hawaii (USA)
    • Year and Date
      2015-12-15
    • Related Report
      2015 Research-status Report
    • Int'l Joint Research / Invited
  • [Presentation] Slow localized mode in the polar cluster of relaxor ferroelectrics near morphotropic phase boundary2015

    • Author(s)
      M. Matsuura, Z. Xu, G. Xu, P. M. Gehring, H. Endo, and K. Shibata
    • Organizer
      Pacifichem2015
    • Place of Presentation
      Hawaii (USA)
    • Year and Date
      2015-12-15
    • Related Report
      2015 Research-status Report
    • Int'l Joint Research / Invited
  • [Presentation] コヒーレントX線によるドメイン観察II2015

    • Author(s)
      大和田 謙二, 清水大輔, 水木純一郎, 藤原考将, 永田知子, 池田直, 並河一道
    • Organizer
      第25回日本MRS年次大会
    • Place of Presentation
      波止場会館(神奈川県横浜市)
    • Year and Date
      2015-12-08
    • Related Report
      2015 Research-status Report
  • [Presentation] MPB近傍のリラクサー強誘電体における分極振幅モード2015

    • Author(s)
      松浦直人, Z. Xu, G. Xu, P. M. Gehring, 柴田薫
    • Organizer
      第25回日本MRS年次大会
    • Place of Presentation
      波止場会館(神奈川県横浜市)
    • Year and Date
      2015-12-08
    • Related Report
      2015 Research-status Report
  • [Presentation] リラクサー強誘電体Pb[(Mg1/3Nb2/3)(1-x)Tix]O3濃度傾斜試料を用いたX線散漫散乱測定2015

    • Author(s)
      清水大輔, 大和田謙二, 坂本潤哉, 塚田真也, 松浦直人, 筒井智嗣, Alfred Q. R. Baron, E, 並河一道, 水木純一郎
    • Organizer
      日本物理学会2015年秋季大会(関西大学)
    • Place of Presentation
      関西大学(大阪府大阪市)
    • Year and Date
      2015-09-16
    • Related Report
      2015 Research-status Report
  • [Presentation] Molecular dynamics simulations of electrocaloric and elastocaloric effects in ferroelectrics2015

    • Author(s)
      T. Nishimatsu
    • Organizer
      2015 EMN SPAIN MEETING
    • Place of Presentation
      San Sebastian (Spain)
    • Year and Date
      2015-09-01
    • Related Report
      2015 Research-status Report
    • Int'l Joint Research / Invited
  • [Presentation] 高次構造とコヒーレントX線利用、次世代構造物性2015

    • Author(s)
      大和田謙二
    • Organizer
      PF研究会「次世代放射光光源を用いた構造物性研究への期待」
    • Place of Presentation
      KEK(つくば)
    • Year and Date
      2015-07-27
    • Related Report
      2015 Research-status Report
    • Invited
  • [Presentation] 不均質とリラクサー2015

    • Author(s)
      大和田謙二
    • Organizer
      第20回 中国・四国・北九州地区誘電体セミナ―
    • Place of Presentation
      島根大学(島根県松江市)
    • Year and Date
      2015-06-19
    • Related Report
      2015 Research-status Report
    • Invited
  • [Presentation] コヒーレントX線散乱で調べるリラクサー強誘電体PZN-9%PTのドメイン形成過程2015

    • Author(s)
      大和田謙二, 水木純一郎, 並河一道
    • Organizer
      日本物理学会
    • Place of Presentation
      早稲田大学(東京都新宿区)
    • Year and Date
      2015-03-21 – 2015-03-24
    • Related Report
      2014 Research-status Report
  • [Presentation] Higher-order Structures Near MPB2014

    • Author(s)
      Kenji OHWADA
    • Organizer
      International Workshop on Relaxor Ferroelectrics
    • Place of Presentation
      Stirin, Czech Republic
    • Year and Date
      2014-10-13 – 2014-10-16
    • Related Report
      2014 Research-status Report
    • Invited
  • [Presentation] Study of Relaxor Ferroelectrics by Using Coherent X-ray Scattering2014

    • Author(s)
      Kenji OHWADA
    • Organizer
      Workshop: CROSSroads of Users and J-PARC 第12回「不均一系における構造と機能」
    • Place of Presentation
      茨城量子ビーム研究センター(茨城県)
    • Year and Date
      2014-09-16 – 2014-09-17
    • Related Report
      2014 Research-status Report
    • Invited
  • [Presentation] Structural Aspect of Relaxor Ferroelectrics near Morphotropic Phase Boundary Studied by Synchrotron X-ray Scattering2014

    • Author(s)
      Kenji OHWADA
    • Organizer
      The 15th IUMRS-International Conference in Asia (IUMRS-ICA 2014)
    • Place of Presentation
      福岡大学(福岡市城南区)
    • Year and Date
      2014-08-24 – 2014-08-29
    • Related Report
      2014 Research-status Report
  • [Presentation] Self-organization of domains near morphotropic phase boundary studied by coherent X-ray scattering2014

    • Author(s)
      Kenji Ohwada, Jun'ichiro Mizuki, Mitsuyoshi Matsushita, Kazumichi Namikawa
    • Organizer
      The 10th Japan-Korea Conference on Ferroelectrics
    • Place of Presentation
      広島国際会議場(広島市中区)
    • Year and Date
      2014-08-17 – 2014-08-20
    • Related Report
      2014 Research-status Report
  • [Remarks] 物理学会直前ミニ研究会「第2回ドメインの物理 界面とフラクタル」

    • URL

      https://sourceforge.net/p/loto/wiki/Workshop/

    • Related Report
      2015 Research-status Report

URL: 

Published: 2014-04-04   Modified: 2020-05-15  

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