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Investigation of spin glass quantum critical material and its quantum critical phenomena

Research Project

Project/Area Number 26400347
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeMulti-year Fund
Section一般
Research Field Condensed matter physics II
Research InstitutionTohoku University

Principal Investigator

Li Dexin  東北大学, 金属材料研究所, 助教 (40281985)

Co-Investigator(Kenkyū-buntansha) 本間 佳哉  東北大学, 金属材料研究所, 助教 (00260448)
山村 朝雄  東北大学, 金属材料研究所, 准教授 (20281983)
青木 大  東北大学, 金属材料研究所, 教授 (30359541)
本多 史憲  東北大学, 金属材料研究所, 准教授 (90391268)
Project Period (FY) 2014-04-01 – 2017-03-31
Project Status Completed (Fiscal Year 2016)
Budget Amount *help
¥4,810,000 (Direct Cost: ¥3,700,000、Indirect Cost: ¥1,110,000)
Fiscal Year 2016: ¥1,300,000 (Direct Cost: ¥1,000,000、Indirect Cost: ¥300,000)
Fiscal Year 2015: ¥1,560,000 (Direct Cost: ¥1,200,000、Indirect Cost: ¥360,000)
Fiscal Year 2014: ¥1,950,000 (Direct Cost: ¥1,500,000、Indirect Cost: ¥450,000)
Keywordsスピングラス / 量子臨界状態 / フラストレーション効果 / f電子系化合物 / 量子臨海状態 / f電子系化合物
Outline of Final Research Achievements

Evident effects of element composition and external magnetic field on the spin glass behavior are observed for many ternary uranium and rare earth compounds. In particular, spin glass system U2Pd1+xSi3-x polycrystals and Ce2CuSi3 single crystal are synthesized and their basic physical properties are measured down to 1.8 K. As a result, the spin glass transition temperature of U2Pd1+xSi3-x decreases as the Si content increases. The optimum Si content that is highly likely to achieve a quantum critical state for U2Pd1+xSi3-x is found. On the other hand, it is confirmed that the spin glass characteristics of Ce2CuSi3 is changed by the external magnetic field. The spin glass transition temperature of Ce2CuSi3 moves toward the low temperature side as the external magnetic field increases, and there is a large possibility to achieve a quantum critical state near 1.4 kOe.

Report

(4 results)
  • 2016 Annual Research Report   Final Research Report ( PDF )
  • 2015 Research-status Report
  • 2014 Research-status Report
  • Research Products

    (46 results)

All 2017 2016 2015 2014

All Journal Article (10 results) (of which Int'l Joint Research: 1 results,  Peer Reviewed: 9 results,  Acknowledgement Compliant: 4 results,  Open Access: 2 results) Presentation (36 results) (of which Int'l Joint Research: 3 results)

  • [Journal Article] Large Upper Critical Field of Superconductivity in the Single Crystal U6Co2016

    • Author(s)
      D. Aoki, A. Nakamura, F. Honda, D. X. Li, Y. Homma
    • Journal Title

      J. Phys. Soc. Jpn.

      Volume: 85 Issue: 7 Pages: 0737131-4

    • DOI

      10.7566/jpsj.85.073713

    • NAID

      210000133998

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Int'l Joint Research / Acknowledgement Compliant
  • [Journal Article] New heavy-fermion antiferromagnet UPd2Cd202016

    • Author(s)
      Y. Hirose, H. Doto, F. Honda, D. X. Li, D. Aoki, Y. Haga, R. Settai
    • Journal Title

      J. Phys.: Cond. Matt.

      Volume: 28 Issue: 42 Pages: 5256011-6

    • DOI

      10.1088/0953-8984/28/42/425601

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Pressure-Induced Valence Transition and Characteristic Electronic States in EuRh2Si22016

    • Author(s)
      F. Honda, K. Okauchi, A. Nakamura, D. X. Li, D. Aoki, H. Akamine, Y. Ashitomi, M. Hedo, T. Nakama, Y. Onuki
    • Journal Title

      J. Phys. Soc. Jpn.

      Volume: 85 Issue: 6 Pages: 063701-5

    • DOI

      10.7566/jpsj.85.063701

    • NAID

      210000133948

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Investigation of exotic electronic properties on rare-earth & actinide compounds under high pressure2016

    • Author(s)
      F. Honda, D. X. Li, K. Okauchi, Y. Homma, A. Nakamura and D. Aoki
    • Journal Title

      MSR Advances

      Volume: 1 Issue: 44 Pages: 2975-2986

    • DOI

      10.1557/adv.2016.373

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Low Temperature Spin-Glass Behavior in Nonmagnetic Atom Disorder Compound Pr2CuIn32015

    • Author(s)
      Dexin Li, Yoshiya Homma, Fuminori Honda, Tomoo Yamamura and Dai Aoki
    • Journal Title

      Physics Procedia

      Volume: 75 Pages: 703-710

    • DOI

      10.1016/j.phpro.2015.12.091

    • Related Report
      2015 Research-status Report
    • Peer Reviewed
  • [Journal Article] Large Magnetocaloric Effect and Magnetic Properties in ErCoAl2015

    • Author(s)
      Dexin Li, Yoshiya Homma, Fuminori Honda, Tomoo Yamamura and Dai Aoki
    • Journal Title

      Physics Procedia

      Volume: 75 Pages: 1300-1305

    • DOI

      10.1016/j.phpro.2015.12.145

    • Related Report
      2015 Research-status Report
    • Peer Reviewed
  • [Journal Article] Single crystal growth and electronic state of UPd2Cd202015

    • Author(s)
      Hiroshi Doto, Yusuke Hirose, Fuminori Honda, Dexin Li, Yoshiya Homma, Dai Aoki, and Rikio Settai
    • Journal Title

      Physics Procedia

      Volume: 75 Pages: 56-61

    • DOI

      10.1016/j.phpro.2015.12.009

    • Related Report
      2015 Research-status Report
  • [Journal Article] Large Cyclotron Effective Mass Detected by de Haas-van Alphen Effect in YbCu2Si22015

    • Author(s)
      Dai Aoki, Fuminori Honda, Yoshiya Homma, DeXin Li, Rikio Settai, Hisatomo Harima, Yoshichika Onuki
    • Journal Title

      J. Phys. Soc. Jpn.

      Volume: 84 Issue: 3 Pages: 0350021-2

    • DOI

      10.7566/jpsj.84.035002

    • NAID

      210000133490

    • Related Report
      2014 Research-status Report
    • Peer Reviewed / Open Access / Acknowledgement Compliant
  • [Journal Article] Single crystal growth and magnetic properties of RCu9Sn4 (R:rare earth metals)2015

    • Author(s)
      Yusuke Hirose, Shun Tomaru, Shoko Sato, Shunpei Ota, Shuhei Kurahashi, Tetsuya, Takeuchi, Fuminori Honda, Yoshiya Homma, Dexin Li, Dai Aoki, Rikio Settai
    • Journal Title

      J. Phys.: Conf. Sec.

      Volume: 592 Pages: 0120341-6

    • DOI

      10.1088/1742-6596/592/1/012034

    • Related Report
      2014 Research-status Report
    • Peer Reviewed
  • [Journal Article] Large reversible magnetocaloric effect in ferromagnetic semiconductor EuS2014

    • Author(s)
      D. X. Li, T. Yamamura, S. Nimori, Y. Homma, F. Honda, Y. Haga and D. Aoki
    • Journal Title

      Solid State Communs.

      Volume: 193 Pages: 6-10

    • Related Report
      2014 Research-status Report
    • Peer Reviewed
  • [Presentation] 電荷密度波転移を示す強磁性物質SmNiC2における強い磁気異方性2017

    • Author(s)
      李徳新, 本間佳哉, 仲村愛, 清水悠晴, 本多史憲, 山村朝雄, 青木大
    • Organizer
      日本物理学会第72回年次大会
    • Place of Presentation
      大阪大学
    • Year and Date
      2017-03-17
    • Related Report
      2016 Annual Research Report
  • [Presentation] 単結晶Ce2T3Ge5 (T=Ir, Co, Pd)の物性と圧力効果2017

    • Author(s)
      中村優希, 中島美帆, 天児寧, 仲村愛, 李徳新, 本多史憲, 青木大, 郷地順, 上床美也
    • Organizer
      日本物理学会第72回年次大会
    • Place of Presentation
      大阪大学
    • Year and Date
      2017-03-17
    • Related Report
      2016 Annual Research Report
  • [Presentation] 重い電子系反強磁性超伝導体UNi2Al3の強磁場磁化過程2017

    • Author(s)
      望月健生, 清水悠晴, 近藤晃弘, 本間佳哉, 李徳新, 青木大, 松尾晶, 金道浩一
    • Organizer
      日本物理学会第72回年次大会
    • Place of Presentation
      大阪大学
    • Year and Date
      2017-03-17
    • Related Report
      2016 Annual Research Report
  • [Presentation] UIrSi3の単結晶育成と物性2017

    • Author(s)
      本多史憲, Valenta Jaroslav, Valiska Michal, Bara Vondrackova, Petr Opletal, Jiri Kastil, Prchal Jiri, 李徳新, 青木大, Sechovsky Vladimir
    • Organizer
      日本物理学会第72回年次大会
    • Place of Presentation
      大阪大学
    • Year and Date
      2017-03-17
    • Related Report
      2016 Annual Research Report
  • [Presentation] ThCu2Si2の単結晶育成とドハース・ファンアルフェン効果2017

    • Author(s)
      仲村愛, 本多史憲, 本間佳哉, 李徳新, 清水悠晴, Arvind Maurya, 大貫惇睦, 播磨尚朝, 青木大
    • Organizer
      日本物理学会第72回年次大会
    • Place of Presentation
      大阪大学
    • Year and Date
      2017-03-17
    • Related Report
      2016 Annual Research Report
  • [Presentation] 多段磁気転移を示すEu1-xLaxAl4 (x=0, 0.2)のメスバウアー分光測定2017

    • Author(s)
      本間佳哉, 仲村愛, 清水悠晴, 李徳新, 本多史憲, 青木大, 仲間隆男, 大貫惇睦
    • Organizer
      日本物理学会第72回年次大会
    • Place of Presentation
      大阪大学
    • Year and Date
      2017-03-17
    • Related Report
      2016 Annual Research Report
  • [Presentation] 超伝導体U6Coの核磁気共鳴による研究2016

    • Author(s)
      真砂全宏, 石田憲二, 仲村愛, 本間佳哉, 李徳新, 本多史憲, 青木大
    • Organizer
      日本物理学会2016年秋季大会
    • Place of Presentation
      金沢大学
    • Year and Date
      2016-09-21
    • Related Report
      2016 Annual Research Report
  • [Presentation] ThSb2とThBi2の単結晶育成とドハース・ファンアルフェン効果2016

    • Author(s)
      仲村愛, 本多史憲, 本間佳哉, 李徳新, 清水悠晴, 大貫惇睦, 青木大
    • Organizer
      日本物理学会2016年秋季大会
    • Place of Presentation
      金沢大学
    • Year and Date
      2016-09-21
    • Related Report
      2016 Annual Research Report
  • [Presentation] Ho2PtSi3における強磁性クラスターグラス挙動および大きな磁気熱量効果2016

    • Author(s)
      李徳新, 本間佳哉, 仲村愛, 本多史憲, 山村朝雄, 青木大
    • Organizer
      日本物理学会2016年秋季大会
    • Place of Presentation
      金沢大学
    • Year and Date
      2016-09-21
    • Related Report
      2016 Annual Research Report
  • [Presentation] UNi4Bの電流磁気効果のNMRによる検証2016

    • Author(s)
      岸本恭来, 小手川恒, 藤秀樹, 齋藤開, 網塚浩, 本間佳哉, 仲村愛, 李徳新, 本多史憲, 青木大
    • Organizer
      日本物理学会2016年秋季大会
    • Place of Presentation
      金沢大学
    • Year and Date
      2016-09-21
    • Related Report
      2016 Annual Research Report
  • [Presentation] サイクロイド型磁気秩序を示すUPtGeのPt-NMRによる研究2016

    • Author(s)
      徳永陽, 仲村愛, 青木大, 服部泰佑, 酒井宏典, 神戸振作, 本多史憲, 本間佳哉, 李徳新, 清水悠晴
    • Organizer
      日本物理学会2016年秋季大会
    • Place of Presentation
      金沢大学
    • Year and Date
      2016-09-21
    • Related Report
      2016 Annual Research Report
  • [Presentation] EuRh2Si2単結晶および関連物質の圧力誘起価数転移と臨界終点2016

    • Author(s)
      本多史憲, 岡内啓悟, 仲村愛, 李徳新, 青木大, 赤嶺拡, 安次富洋介, 辺土正人, 仲間隆男, 大貫惇睦
    • Organizer
      日本物理学会2016年秋季大会
    • Place of Presentation
      金沢大学
    • Year and Date
      2016-09-21
    • Related Report
      2016 Annual Research Report
  • [Presentation] Re-entrant Spin Glass Behavior and Large Magnetocaloric Effect in Er2PtSi32016

    • Author(s)
      D. X. Li, Y. Homma, A. Nakamura, F. Honda, T. Yamamura, D. Aoki
    • Organizer
      International Conference on Strongly Correlated Electron Systems
    • Place of Presentation
      Hangzhou, China
    • Year and Date
      2016-05-08
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Single Crystal Growth and Superconductivity in Th7Ni3 and La7Ni3 without Inversion Symmetry2016

    • Author(s)
      A. Nakamura, F. Honda, Y. Homma, D. X. Li, D. Aoki, K. Nishimura, M. Kakihana, M. Hedo, T. Nakama, and Y. Onuki
    • Organizer
      International Conference on Strongly Correlated Electron Systems
    • Place of Presentation
      Hangzhou, China
    • Year and Date
      2016-05-08
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 擬三元系ウラン化合物U(Rh1-xIrx)Geにおける磁気フラストレーション状態の形成究2016

    • Author(s)
      李徳新,本間佳哉,仲村愛,本多史憲,山村朝雄,青木大
    • Organizer
      日本物理学会第71回年次大会
    • Place of Presentation
      東北学院大学 泉キャンパス
    • Year and Date
      2016-03-19
    • Related Report
      2015 Research-status Report
  • [Presentation] UPtGeの強磁場磁化過程2016

    • Author(s)
      三宅厚志,仲村愛,志村康成,本間佳哉,李徳新,本多史憲,徳永将史,青木大
    • Organizer
      日本物理学会第71回年次大会
    • Place of Presentation
      東北学院大学 泉キャンパス
    • Year and Date
      2016-03-19
    • Related Report
      2015 Research-status Report
  • [Presentation] UCo1-xFexAl (x=0.02, 0.04)単結晶の磁性2016

    • Author(s)
      本間佳哉,李徳新,仲村愛,本多史憲,青木大
    • Organizer
      日本物理学会第71回年次大会
    • Place of Presentation
      東北学院大学 泉キャンパス
    • Year and Date
      2016-03-19
    • Related Report
      2015 Research-status Report
  • [Presentation] U6Coの単結晶育成と超伝導2016

    • Author(s)
      青木大,仲村愛,本多史憲,本間佳哉,李徳新
    • Organizer
      日本物理学会第71回年次大会
    • Place of Presentation
      東北学院大学 泉キャンパス
    • Year and Date
      2016-03-19
    • Related Report
      2015 Research-status Report
  • [Presentation] Th7Ni3とLa7Ni3の単結晶育成と物性2016

    • Author(s)
      仲村愛,本多史憲,西村健吾,垣花将司,辺土正人,仲間隆男,大貫惇睦,本間佳哉,李徳新,青木大
    • Organizer
      日本物理学会第71回年次大会
    • Place of Presentation
      東北学院大学 泉キャンパス
    • Year and Date
      2016-03-19
    • Related Report
      2015 Research-status Report
  • [Presentation] U2T3Si5(T: Rh, Ir)の物性と圧力効果 II2016

    • Author(s)
      本多史憲,仲村愛,李徳新,本間佳哉,芳賀芳範,青木大
    • Organizer
      日本物理学会第71回年次大会
    • Place of Presentation
      東北学院大学 泉キャンパス
    • Year and Date
      2016-03-19
    • Related Report
      2015 Research-status Report
  • [Presentation] 強磁性半導体EuSにおける巨大な磁気熱量効果2015

    • Author(s)
      李徳新,本間佳哉,本多史憲,山村朝雄,芳賀芳範,青木大
    • Organizer
      日本物理学会2015年秋季大会
    • Place of Presentation
      関西大学 千里山キャンパス
    • Year and Date
      2015-09-16
    • Related Report
      2015 Research-status Report
  • [Presentation] EuCu9Sn4とEuZn13における圧力下電気抵抗測定2015

    • Author(s)
      佐藤翔子,広瀬雄介,都丸駿,倉橋秀平,竹内徹也,本多史憲,李徳新,青木大,松林和幸,上床美也,芳賀芳範,摂待力生
    • Organizer
      日本物理学会2015年秋季大会
    • Place of Presentation
      関西大学 千里山キャンパス
    • Year and Date
      2015-09-16
    • Related Report
      2015 Research-status Report
  • [Presentation] UCo1-xFexAlの57Feメスバウアー分光2015

    • Author(s)
      本間佳哉,李徳新,仲村愛,本多史憲,青木大
    • Organizer
      日本物理学会2015年秋季大会
    • Place of Presentation
      関西大学 千里山キャンパス
    • Year and Date
      2015-09-16
    • Related Report
      2015 Research-status Report
  • [Presentation] U2T3Si5(T:Rh, Ir)の物性と圧力効果2015

    • Author(s)
      本多史憲,仲村愛,李徳新,本間佳哉,芳賀芳範,青木大
    • Organizer
      日本物理学会2015年秋季大会
    • Place of Presentation
      関西大学 千里山キャンパス
    • Year and Date
      2015-09-16
    • Related Report
      2015 Research-status Report
  • [Presentation] UPd2Cd20の単結晶育成と電子状態の研究2015

    • Author(s)
      土塔寛,広瀬雄介,本多史憲,李徳新,本間佳哉,青木大,摂待力生
    • Organizer
      日本物理学会2015年秋季大会
    • Place of Presentation
      関西大学 千里山キャンパス
    • Year and Date
      2015-09-16
    • Related Report
      2015 Research-status Report
  • [Presentation] Pressure effect of EuCu9Sn4 and EuZn132015

    • Author(s)
      Takeuchi, Fuminori Honda, Dexin Li, Dai Aoki, Kazuyuki Matsubayashi, Yoshiya Uwatoko, Yoshinori Haga, Rikio Settai
    • Organizer
      20th International Conference on Magnetism
    • Place of Presentation
      Barcelona, Spain
    • Year and Date
      2015-07-05
    • Related Report
      2015 Research-status Report
    • Int'l Joint Research
  • [Presentation] RPt2Cd20(R = Rare Earth)の単結晶育成と電子状態の研究2015

    • Author(s)
      土塔寛,広瀬雄介,本多史憲,李徳新,青木大,摂待力生
    • Organizer
      日本物理学会第70回年次大会
    • Place of Presentation
      早稲田大学 早稲田キャンパス
    • Year and Date
      2015-03-21 – 2015-03-24
    • Related Report
      2014 Research-status Report
  • [Presentation] CeCu9Sn4及び関連物質の単結晶育成と磁性2015

    • Author(s)
      佐藤翔子,広瀬雄介,都丸駿,太田俊平,倉橋秀平,竹内徹也,本多史憲,本間佳哉,李徳新,青木大,松林和幸,上床美也,芳賀芳範,摂待力生
    • Organizer
      日本物理学会第70回年次大会
    • Place of Presentation
      早稲田大学 早稲田キャンパス
    • Year and Date
      2015-03-21 – 2015-03-24
    • Related Report
      2014 Research-status Report
  • [Presentation] 新規ウラン化合物U2Rh3Ge5における磁気的性2015

    • Author(s)
      李徳新,本間佳哉,本多史憲,山村朝雄,青木大
    • Organizer
      日本物理学会第70回年次大会
    • Place of Presentation
      早稲田大学 早稲田キャンパス
    • Year and Date
      2015-03-21 – 2015-03-24
    • Related Report
      2014 Research-status Report
  • [Presentation] URh1-xFexGeの57Feメスバウアー分光2015

    • Author(s)
      本間佳哉,李徳新,本多史憲,青木大
    • Organizer
      日本物理学会第70回年次大会
    • Place of Presentation
      早稲田大学 早稲田キャンパス
    • Year and Date
      2015-03-21 – 2015-03-24
    • Related Report
      2014 Research-status Report
  • [Presentation] Single crystal growth and electronic state of RT2X202014

    • Author(s)
      Y. Hirose, S. Tomaru, H. Doto, S. Ota, F. Honda, D. X. Li, Y. Homma, D. Aoki and R. Settai
    • Organizer
      International Symposium on Utilization of Research Reactors for Material Studies
    • Place of Presentation
      Sendai, Institute for Materials Research
    • Year and Date
      2014-12-11 – 2014-12-12
    • Related Report
      2014 Research-status Report
  • [Presentation] RCu9Sn4 ( R:希土類元素 ) の磁性と結晶場効果2014

    • Author(s)
      都丸駿,広瀬雄介,太田俊平,倉橋秀平,佐藤翔子,竹内徹也,本多史憲,本間佳哉,李徳新,青木大,摂待力生
    • Organizer
      日本物理学会2014年秋季大会
    • Place of Presentation
      中部大学春日井キャンパス
    • Year and Date
      2014-09-07 – 2014-09-10
    • Related Report
      2014 Research-status Report
  • [Presentation] CePt2In7のde Haas-van Alphen効果と強磁場物性2014

    • Author(s)
      太田俊平,倉橋秀平,都丸駿,広瀬雄介,本多史憲,李徳新,青木大,三宅厚志,徳永将史,Albin de Muer,Ilya Sheikin,摂待力生
    • Organizer
      日本物理学会2014年秋季大会
    • Place of Presentation
      中部大学春日井キャンパス
    • Year and Date
      2014-09-07 – 2014-09-10
    • Related Report
      2014 Research-status Report
  • [Presentation] (Eu1-xLax)Al4(x=0, 0.2)反磁性体の151Euメスバウアー分光2014

    • Author(s)
      本間佳哉,李徳新,本多史憲,仲村愛,辺土正人,仲間隆男,大貫惇睦,青木大
    • Organizer
      日本物理学会2014年秋季大会
    • Place of Presentation
      中部大学春日井キャンパス
    • Year and Date
      2014-09-07 – 2014-09-10
    • Related Report
      2014 Research-status Report
  • [Presentation] U2T3X5 (T: Rh, Ir, X: Si, Ge)の高圧下物性2014

    • Author(s)
      本多史憲,李徳新,本間佳哉,芳賀芳範,青木大
    • Organizer
      日本物理学会2014年秋季大会
    • Place of Presentation
      中部大学春日井キャンパス
    • Year and Date
      2014-09-07 – 2014-09-10
    • Related Report
      2014 Research-status Report
  • [Presentation] U2Ir3Si5単結晶の磁気的性質2014

    • Author(s)
      李徳新,本間佳哉,本多史憲,山村朝雄,青木大
    • Organizer
      日本物理学会2014年秋季大会
    • Place of Presentation
      中部大学春日井キャンパス
    • Year and Date
      2014-09-07 – 2014-09-10
    • Related Report
      2014 Research-status Report

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Published: 2014-04-04   Modified: 2020-05-15  

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