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Low temperature activation mechanism of plasma-catalysis and its applications

Research Project

Project/Area Number 26400539
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeMulti-year Fund
Section一般
Research Field Plasma science
Research InstitutionNational Institute of Advanced Industrial Science and Technology

Principal Investigator

Kim Hyun-Ha  国立研究開発法人産業技術総合研究所, 環境管理研究部門, 主任研究員 (20356893)

Co-Investigator(Kenkyū-buntansha) 寺本 慶之  国立研究開発法人産業技術総合研究所, 環境管理研究部門, 主任研究員 (00635328)
尾形 敦  国立研究開発法人産業技術総合研究所, 環境管理研究部門, 研究副部門長 (70356690)
Project Period (FY) 2014-04-01 – 2017-03-31
Project Status Completed (Fiscal Year 2016)
Budget Amount *help
¥3,510,000 (Direct Cost: ¥2,700,000、Indirect Cost: ¥810,000)
Fiscal Year 2016: ¥1,040,000 (Direct Cost: ¥800,000、Indirect Cost: ¥240,000)
Fiscal Year 2015: ¥1,300,000 (Direct Cost: ¥1,000,000、Indirect Cost: ¥300,000)
Fiscal Year 2014: ¥1,170,000 (Direct Cost: ¥900,000、Indirect Cost: ¥270,000)
Keywords低温プラズマ / 触媒 / VOC分解 / ストリーマ / プラズマー触媒 / サフェースストリマ / ゼオライト
Outline of Final Research Achievements

Plasma on the surface of catalyst was consisted of primary and secondary streamers. The different activities of Ag and Pt in plasma-catalysis were found to be correlated with the properties of streamer propagation. The propagation velocity of primary streamers was found to be dependent on the applied voltage and the type of catalyst. For the Ag/TiO2 catalyst-packed-bed reactor with a mesh-to-mesh configuration, the primary streamer reached about 660 km/s. Through successive steps, the partial discharge served as a staging point for primary streamers, and promoted their propagation toward the next catalyst bead. In contrast to primary streamers, secondary streamer velocities were almost completely independent of the applied voltage. These finding may provide some useful insight in understanding fundamental working mechanism of plasma-catalysis.

Report

(4 results)
  • 2016 Annual Research Report   Final Research Report ( PDF )
  • 2015 Research-status Report
  • 2014 Research-status Report
  • Research Products

    (21 results)

All 2017 2016 2015 2014 Other

All Int'l Joint Research (1 results) Journal Article (4 results) (of which Int'l Joint Research: 2 results,  Peer Reviewed: 4 results,  Acknowledgement Compliant: 4 results) Presentation (15 results) (of which Int'l Joint Research: 8 results,  Invited: 8 results) Book (1 results)

  • [Int'l Joint Research] KIMM(韓国)

    • Related Report
      2016 Annual Research Report
  • [Journal Article] Time-resolved imaging of positive pulsed corona-induced surface streamers on TiO2 and γ-Al2O3-supported Ag catalysts2016

    • Author(s)
      H.H. Kim, Y. Teramoto, A. Ogata
    • Journal Title

      J. Phys D: Appl. Phys

      Volume: 49 Issue: 41 Pages: 415204-415204

    • DOI

      10.1088/0022-3727/49/41/415204

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Plasma catalysis for environmental treatment and energy applications2016

    • Author(s)
      H.H. Kim, Y. Teramoto, T. Nanba, H. Takagi, A. Ogata,
    • Journal Title

      Plasma Chemistry and Plasma Processing

      Volume: 36 Issue: 1 Pages: 45-72

    • DOI

      10.1007/s11090-015-9652-7

    • Related Report
      2015 Research-status Report
    • Peer Reviewed / Int'l Joint Research / Acknowledgement Compliant
  • [Journal Article] A multidisciplinary approach to understand the interactions of nonthermal plasma and catalyst: A Review2015

    • Author(s)
      H.H. Kim, Y. Teramoto, N. Negishi, A. Ogata
    • Journal Title

      Catalysis Today

      Volume: 256 Pages: 13-22

    • DOI

      10.1016/j.cattod.2015.04.009

    • Related Report
      2015 Research-status Report
    • Peer Reviewed / Int'l Joint Research / Acknowledgement Compliant
  • [Journal Article] Effects of Si/Al ratio on the interaction of nonthermal plasma and Ag/HY catalysts2015

    • Author(s)
      H.H. Kim, Y. Teramoto, T. Sano, N. Negishi, A. Ogata
    • Journal Title

      App, Cat. B: Environ

      Volume: 166-167 Pages: 9-17

    • DOI

      10.1016/j.apcatb.2014.11.008

    • Related Report
      2014 Research-status Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Presentation] Plasma-Catalysis for the Remediation of toxic gases pollutants2017

    • Author(s)
      H.H. Kim
    • Organizer
      2017 Conference on New Combustion Concepts
    • Place of Presentation
      KAUST (Saudi Arabia)
    • Year and Date
      2017-03-06
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] ICCD カメラによる触媒表面のサフェースストリーマの進展観察2016

    • Author(s)
      金 賢夏,寺本慶之,尾形 敦
    • Organizer
      静電気学学会全国大会
    • Place of Presentation
      群馬大学
    • Year and Date
      2016-09-28
    • Related Report
      2016 Annual Research Report
  • [Presentation] Plasma-Catalysis: From Catalyst Screening to NH3 Synthesis2016

    • Author(s)
      H.H. Kim, H. Takagi, T. Nanba, Y. Teramoto, A. Ogata
    • Organizer
      IWPEEA 2016
    • Place of Presentation
      Liverpool (イギリス)
    • Year and Date
      2016-08-23
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] LTP for Energy & Environmental Applications:2016

    • Author(s)
      H.H. Kim
    • Organizer
      NSF-LTP
    • Place of Presentation
      Washington DC (米国)
    • Year and Date
      2016-08-22
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Plasma-Catalysis: From Catalyst Screening to Gas Cleaning Process2016

    • Author(s)
      H.H. Kim, Y. Teramoto, A. Ogata
    • Organizer
      ISNTP-10
    • Place of Presentation
      Florianopolis(ブラジル)
    • Year and Date
      2016-08-01
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 低温プラズマと触媒の複合技術を利用したガス浄化とアンモニア合2016

    • Author(s)
      金賢夏
    • Organizer
      第29回環境工学連合講演会
    • Place of Presentation
      岩手大学
    • Year and Date
      2016-05-26
    • Related Report
      2016 Annual Research Report
  • [Presentation] ICCD Camera Imaging of Surface Streamers on the Surface of Catalyst2015

    • Author(s)
      H.H. Kim
    • Organizer
      PETEA 2015
    • Place of Presentation
      京都国際会館 (京都)
    • Year and Date
      2015-12-10
    • Related Report
      2015 Research-status Report
    • Int'l Joint Research
  • [Presentation] Plasma-Driven Catalysis: From fundamental to possible application2015

    • Author(s)
      H.H. Kim, Y.Teramoto, A. Ogata
    • Organizer
      AOTs-21
    • Place of Presentation
      Crown Plaza Hotel (San Diego、米国)
    • Year and Date
      2015-11-16
    • Related Report
      2015 Research-status Report
    • Int'l Joint Research / Invited
  • [Presentation] Plasma-driven catalysis for VOC removal2015

    • Author(s)
      H.H. Kim, Y.Teramoto, A. Ogata
    • Organizer
      ISNPEDADM 2015
    • Place of Presentation
      Hotel Le Recif (Le Union、 フランス)
    • Year and Date
      2015-10-26
    • Related Report
      2015 Research-status Report
    • Int'l Joint Research
  • [Presentation] 誘電体バリア放電の諸現象と目的反応に適した誘電体バリアの選び方2015

    • Author(s)
      金賢夏
    • Organizer
      日本学術振興会第153委員会 第123回研究会
    • Place of Presentation
      東京弘済会館(東京)
    • Year and Date
      2015-10-21
    • Related Report
      2015 Research-status Report
    • Invited
  • [Presentation] Plasma catalysis for Environmental and Energy applications2015

    • Author(s)
      H.H. Kim
    • Organizer
      ISPC-22
    • Place of Presentation
      Anterwerpen大学(Anterwerpen、ベルぎ)
    • Year and Date
      2015-07-06
    • Related Report
      2015 Research-status Report
    • Int'l Joint Research / Invited
  • [Presentation] Interaction of Plasma and Catalyst; Current Status and Road to Industrial Use2014

    • Author(s)
      金賢夏, 寺本慶之,根岸信彰、尾形敦
    • Organizer
      Plasma Conference 2014
    • Place of Presentation
      新潟朱鷺メッセ(新潟)
    • Year and Date
      2014-11-18 – 2014-11-21
    • Related Report
      2014 Research-status Report
  • [Presentation] Multidisciplinary approach to understand the Interaction of nonthermal plasma and catalyst2014

    • Author(s)
      Hyun-Ha Kim*UP, Yoshiyuki Teramoto, Nobuaki Negishi, Atsushi Ogata
    • Organizer
      ISPCEM-2014
    • Place of Presentation
      Tianjin University (Tianjin)
    • Year and Date
      2014-09-13 – 2014-09-16
    • Related Report
      2014 Research-status Report
    • Invited
  • [Presentation] 低温プラズマと銀担持ゼオライト触媒の相互作用2014

    • Author(s)
      金賢夏,寺本慶之、佐野泰三、根岸信彰, 尾形敦
    • Organizer
      静電気学会全国大会
    • Place of Presentation
      広島国際大学(広島)
    • Year and Date
      2014-09-08 – 2014-09-09
    • Related Report
      2014 Research-status Report
  • [Presentation] 大気圧プラズマと触媒複合反応のシナジー2014

    • Author(s)
      金賢夏
    • Organizer
      非平衡反応場の創出と化学合成プロセスへの応用
    • Place of Presentation
      東京工業大学(東京)
    • Year and Date
      2014-08-28
    • Related Report
      2014 Research-status Report
    • Invited
  • [Book] Plasma-Driven Catalysis for Volatile Organic Compounds (VOCs)2016

    • Author(s)
      H.H. Kim, Y. Teramoto, A. Ogata, N. Negishi,
    • Total Pages
      1578
    • Publisher
      CRC Press (Taylor & Francis Group)
    • Related Report
      2016 Annual Research Report

URL: 

Published: 2014-04-04   Modified: 2018-03-22  

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