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Space selective formation of porous structures inside glass by laser induced elemental migration

Research Project

Project/Area Number 26410240
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeMulti-year Fund
Section一般
Research Field Inorganic industrial materials
Research InstitutionKyoto University

Principal Investigator

Sakakura Masaaki  京都大学, 産官学連携本部, 特定准教授 (90402958)

Co-Investigator(Kenkyū-buntansha) 下間 靖彦  京都大学, 工学研究科, 准教授 (40378807)
三浦 清貴  京都大学, 工学研究科, 教授 (60418762)
Project Period (FY) 2014-04-01 – 2017-03-31
Project Status Completed (Fiscal Year 2016)
Budget Amount *help
¥5,070,000 (Direct Cost: ¥3,900,000、Indirect Cost: ¥1,170,000)
Fiscal Year 2016: ¥1,170,000 (Direct Cost: ¥900,000、Indirect Cost: ¥270,000)
Fiscal Year 2015: ¥1,300,000 (Direct Cost: ¥1,000,000、Indirect Cost: ¥300,000)
Fiscal Year 2014: ¥2,600,000 (Direct Cost: ¥2,000,000、Indirect Cost: ¥600,000)
Keywordsガラス / 超短パルスレーザー / 空間光変調器 / 微細加工 / レーザープロセッシング / レーザー / 空間光変調 / 組成分布 / 相分離 / 多孔質
Outline of Final Research Achievements

We elucidated that the transient temperature distribution, the shape of the molten region as well as the elemental distributions inside glasses can be controlled by parallel irradiation with focused ultrashort laser pulses at different repetition rates. We found that the result of the elemental distribution changes by laser irradiation can induce phase separation and precipitation of nanocrystals in the molten region inside glasses and that microstructures such as porous structures are formed by the phase separation and nanocrystal precipitation. In addition, the parallel laser irradiation system developed in this study and the simulation of heat accumulation enabled estimation of the flow of glass melt during laser irradiation and laser melting with suppression of residual strain in the heated region.

Report

(4 results)
  • 2016 Annual Research Report   Final Research Report ( PDF )
  • 2015 Research-status Report
  • 2014 Research-status Report
  • Research Products

    (29 results)

All 2017 2016 2015 2014 Other

All Journal Article (14 results) (of which Int'l Joint Research: 3 results,  Peer Reviewed: 12 results,  Open Access: 8 results,  Acknowledgement Compliant: 8 results) Presentation (14 results) (of which Int'l Joint Research: 4 results,  Invited: 3 results) Remarks (1 results)

  • [Journal Article] Molecular dynamics simulation of the Soret effect in a CaSiO<sub>3</sub> glass melt2017

    • Author(s)
      Masahiro Shimizu, Hiroshi Kato, Masayuki Nishi Daisuke Hanakawa, Kohji Nagashima, Heidy Visbal, Hiroki Itasaka, Masaaki Sakakura, Yasuhiko Shimotsuma, Kiyotaka Miura, Kazuyuki Hirao
    • Journal Title

      Journal of the Ceramic Society of Japan

      Volume: 125 Issue: 3 Pages: 180-184

    • DOI

      10.2109/jcersj2.16187

    • NAID

      130005401721

    • ISSN
      1348-6535, 1882-0743
    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] 超短パルスレーザーによるガラス内部の局所溶融技術2017

    • Author(s)
      坂倉政明、三浦清貴
    • Journal Title

      NEW GLASS

      Volume: 32 Pages: 24-28

    • Related Report
      2016 Annual Research Report
    • Acknowledgement Compliant
  • [Journal Article] Modification and Dynamics inside Diamond by Femtosecond Laser Double-Pulse Irradiation2016

    • Author(s)
      Masaaki Sakakura, Takuro Okada, Vibhav Bharadwaj, Bellen Sotillo, Shane M. Eaton, Roberta Ramponi, Ali Serpenguzel, Ulas S. Gokay, Yasuhiko Shimotsuma, and Kiyotaka Miura
    • Journal Title

      Journal of Laser Micro/Nanoengineering

      Volume: 11 Issue: 3 Pages: 346-351

    • DOI

      10.2961/jlmn.2016.03.0012

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research / Acknowledgement Compliant
  • [Journal Article] Self-organization of polarization-dependent periodic nanostructures embedded in III&#8211;V semiconductor materials2016

    • Author(s)
      Y. Shimotsuma, T. Sei, M. Mori, M. Sakakura, K. Miura
    • Journal Title

      Appl. Phys. A

      Volume: 122 Issue: 3 Pages: 159-159

    • DOI

      10.1007/s00339-016-9686-6

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Open Access / Acknowledgement Compliant
  • [Journal Article] Soret coefficients of alkali oxides in alkali borate glass melts2016

    • Author(s)
      Masahiro Shimizu, Daisuke Hanakawa, Masayuki Nishi, Kohji Nagashima, Visbal Heidy, Masaaki Sakakura, Yasuhiko Shimotsuma, Kazuyuki Hirao, and Kiyotaka Miura
    • Journal Title

      Journal of the Ceramic Society of Japan

      Volume: 124 Issue: 7 Pages: 774-776

    • DOI

      10.2109/jcersj2.16053

    • NAID

      130005161665

    • ISSN
      1348-6535, 1882-0743
    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Space-selective precipitation of ZnO crystals in glass by using high repetition rate femtosecond laser irradiation2016

    • Author(s)
      Xi Du, Masaaki Sakakura, Torataro Kurita, Hang Zhang, Yasuhiko Shimotsuma, Kiyotaka Hirao, Kiyotaka Miura and Jianrong Qiu
    • Journal Title

      Journal of Non-Crystalline Solids

      Volume: 448 Pages: 79-82

    • DOI

      10.1016/j.jnoncrysol.2016.06.042

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Nanogratings Embedded in Al2O3-Dy2O3 Glass by Femtosecond Laser Irradiation2016

    • Author(s)
      S. Mori, T. Kurita, Y. Shimotsuma, M. Sakakura, and K. Miura
    • Journal Title

      Journal of Laser Micro Nanoengineering

      Volume: 11 Issue: 1 Pages: 87-90

    • DOI

      10.2961/jlmn.2016.01.0016

    • Related Report
      2015 Research-status Report
    • Peer Reviewed / Open Access
  • [Journal Article] Direct laser-writing of ferroelectric single-crystal waveguide architectures in glass for 3D integrated optics2015

    • Author(s)
      A. Stone, H. Jain, V. Dierolf, M. Sakakura, Y. Shimotsuma, K. Miura, K. Hirao, J. Lapointe, and Raman Kashyap
    • Journal Title

      Scientific Reports

      Volume: 5 Issue: 1 Pages: 10391-10391

    • DOI

      10.1038/srep10391

    • NAID

      120005822789

    • Related Report
      2015 Research-status Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Control of Si-rich region inside a sodalime glass by parallel femtosecond laser focusing at multiple spots2015

    • Author(s)
      M. Sakakura, T. Kurita,K. Yoshimura, Y. Shimotsuma, N. Fukuda, and K. Miura
    • Journal Title

      Applied Physics B

      Volume: 119 Issue: 3 Pages: 485-492

    • DOI

      10.1007/s00340-015-6061-9

    • Related Report
      2015 Research-status Report 2014 Research-status Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Transient strain distributions during femtosecond laser-induced deformation inside LiF and MgO single crystals2015

    • Author(s)
      M. Sakakura, Y. Shimotsuma, N. Fukuda, and K. Miura
    • Journal Title

      Journal of Applied Physics

      Volume: 118 Issue: 2 Pages: 023106-023106

    • DOI

      10.1063/1.4926614

    • NAID

      120005670889

    • Related Report
      2015 Research-status Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Fast and Slow Dynamics in Femtosecond Laser-induced Crack Propagation inside a LiF Single Crystal2015

    • Author(s)
      M. Sakakura, T. Okada, Y. Shimotsuma, N. Fukuda, and K. Miura
    • Journal Title

      Journal of Laser Micro Nanoengineering

      Volume: 10 Issue: 3 Pages: 320-324

    • DOI

      10.2961/jlmn.2015.03.0015

    • Related Report
      2015 Research-status Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] フェムト秒レーザー加工での過渡応力分布の観測と多点同時照射による応力変調2015

    • Author(s)
      坂倉政明
    • Journal Title

      応用物理

      Volume: 84 Pages: 997-1001

    • NAID

      130007718723

    • Related Report
      2015 Research-status Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Modification of flow of glass melt and elemental distributions by parallel irradiation with femtosecond laser pulses2015

    • Author(s)
      坂倉政明、栗田寅太郎、吉村光平 他3名
    • Journal Title

      Proceedings of SPIE

      Volume: 9350 Pages: 935013-935013

    • DOI

      10.1117/12.2078610

    • Related Report
      2014 Research-status Report
    • Acknowledgement Compliant
  • [Journal Article] Condensation of Si-rich region inside soda-lime glass by parallel femtosecond laser irradiation2014

    • Author(s)
      坂倉政明、吉村光平、栗田寅太郎 その他3名
    • Journal Title

      Optics Express

      Volume: 22 Issue: 13 Pages: 16493-16503

    • DOI

      10.1364/oe.22.016493

    • Related Report
      2014 Research-status Report
    • Peer Reviewed / Open Access
  • [Presentation] ピコ秒パルス列の時間変調によるガラスの局所溶融現象とその抑制2017

    • Author(s)
      中村 晃直, 坂倉 政明, 下間 靖彦, 三浦 清貴
    • Organizer
      第64回応用物理学会 春季学術講演会
    • Place of Presentation
      パシフィコ横浜(神奈川県、横浜市)
    • Year and Date
      2017-03-14
    • Related Report
      2016 Annual Research Report
  • [Presentation] 水中レーザー誘起衝撃波の楕円面反射による局所バブル発生2017

    • Author(s)
      今若 宏亮, 坂倉 政明,下間 靖彦, 三浦 清貴
    • Organizer
      レーザー学会学術講演会 第36回年次大会講演
    • Place of Presentation
      徳島大学(徳島県、徳島市)
    • Year and Date
      2017-01-07
    • Related Report
      2016 Annual Research Report
  • [Presentation] Impact of multiple stress and heat sources in parallel laser bulk processing inside transparent materials2016

    • Author(s)
      Masaaki Sakakura, Takuro Okada, Yasuhiko Shimotsuma, Kiyotaka Miura
    • Organizer
      CerSJ-GOMD Joint Symposium on Glass Science and Technologies
    • Place of Presentation
      京都大学(京都府、京都市)
    • Year and Date
      2016-11-13
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Applications of parallel femtosecond laser writing inside glasses and observation of the dynamics2016

    • Author(s)
      Masaaki Sakakura, Yasuhiko Shimotsuma, Naoaki Fukuda, Kiyotaka Miura
    • Organizer
      Bragg Gratings, Photosensitivity, and Poling in Glass Waveguides (BGPP)
    • Place of Presentation
      シドニー(オーストラリア)
    • Year and Date
      2016-09-05
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Spatially modulated beam for investigation of femtosecond laser-induced modification in transparent materials2016

    • Author(s)
      Masaaki Sakakura, Takuro Okada, Yasuhiko Shimotsuma, Naoaki Fukuda, Kiyotaka Miura
    • Organizer
      The 17th International Symposium on Laser Precision Microfabrication
    • Place of Presentation
      西安市(中国)
    • Year and Date
      2016-05-23
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 転位により阻害されるLiF単結晶内部の集光フェムト秒レーザー誘起構造変化の時間分解観測2016

    • Author(s)
      坂倉政明, 福田直晃, 岡田拓郎, 下間靖彦, 三浦清貴
    • Organizer
      日本化学会第96春季年会
    • Place of Presentation
      同志社大学 京田辺キャンパス(京都府京田辺市)
    • Year and Date
      2016-03-27
    • Related Report
      2015 Research-status Report
  • [Presentation] レーザーが拓く未来技術2016

    • Author(s)
      坂倉政明
    • Organizer
      日本機械学会 関西支部第91期定時総会講演会
    • Place of Presentation
      大阪電気通信大学 寝屋川キャンパス(大阪府寝屋川市)
    • Year and Date
      2016-03-11
    • Related Report
      2015 Research-status Report
    • Invited
  • [Presentation] 多点同時レーザー照射による単結晶内部の亀裂進展過程の観測と亀裂阻害応力の消失2015

    • Author(s)
      坂倉政明, 福田直晃, 岡田拓郎, 下間靖彦, 三浦清貴
    • Organizer
      第17回破壊力学シンポジウム
    • Place of Presentation
      京都テルサ(京都府京都市)
    • Year and Date
      2015-10-14
    • Related Report
      2015 Research-status Report
  • [Presentation] 単結晶内部の亀裂や転位バンドに影響を受けるフェムト秒レーザー誘起構造変化の時間分解観測2015

    • Author(s)
      岡田拓郎, 坂倉政明, 下間靖彦, 福田直晃, 三浦清貴
    • Organizer
      第76回応用物理学会秋季学術講演会
    • Place of Presentation
      名古屋国際会議場(愛知県名古屋市)
    • Year and Date
      2015-09-13
    • Related Report
      2015 Research-status Report
  • [Presentation] Fast and slow dynamics in femtosecond laser-induced crack propagation inside a LiF single crystal2015

    • Author(s)
      M. Sakakura, T. Okada, Y. Shimotsuma, N. Fukuda, K. Miura
    • Organizer
      The 16th International Symposium on Laser Precision Microfabrication
    • Place of Presentation
      北九州国際会議場(福岡県北九州市)
    • Year and Date
      2015-05-26
    • Related Report
      2015 Research-status Report
    • Int'l Joint Research
  • [Presentation] Modification of flow of glass melt and elemental distributions by parallel irradiation with femtosecond laser pulses2015

    • Author(s)
      坂倉政明、栗田寅太郎、吉村光平 他3名
    • Organizer
      SPIE 2015 Photonics West, LASE
    • Place of Presentation
      The Moscone Center (米国サンフランシスコ)
    • Year and Date
      2015-02-12
    • Related Report
      2014 Research-status Report
  • [Presentation] 多点同時フェムト秒レーザー照射によるガラス融液の流動と構成元素の空間分布制御2015

    • Author(s)
      吉村光平、坂倉政明、栗田寅太郎 他3名
    • Organizer
      The 25th Meeting on Glasses for Photonics
    • Place of Presentation
      日本科学未来館(東京都江東区青海)
    • Year and Date
      2015-01-30
    • Related Report
      2014 Research-status Report
  • [Presentation] 多点同時フェムト秒レーザ照射によるガラス内部の 局所組成分布形成2015

    • Author(s)
      坂倉政明、福田直晃、下間靖彦、三浦清貴
    • Organizer
      第82回レーザ加工学会講演会
    • Place of Presentation
      独立行政法人 産業技術総合研究所 臨海副都心センター(東京都江東区青海)
    • Year and Date
      2015-01-14
    • Related Report
      2014 Research-status Report
    • Invited
  • [Presentation] Control of Si-rich region inside a sodalime glass by parallel femtosecond laser focusing at multiple spots2014

    • Author(s)
      坂倉政明、栗田寅太郎、吉村光平 その他3名
    • Organizer
      9th International Conference on Photo-Excited Processes and Application
    • Place of Presentation
      くにびきメッセ(島根県松江市)
    • Year and Date
      2014-09-30
    • Related Report
      2014 Research-status Report
  • [Remarks] 高繰り返しレーザー照射による熱蓄積の解析と構造変化のメカニズム

    • URL

      http://saci-hitz.saci.kyoto-u.ac.jp/sakakura/index.html

    • Related Report
      2016 Annual Research Report

URL: 

Published: 2014-04-04   Modified: 2018-03-22  

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