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Elucidation of the concentration and condensation mechanism of trace harmful metals to PM2.5 in coal combustion

Research Project

Project/Area Number 26420163
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeMulti-year Fund
Section一般
Research Field Thermal engineering
Research InstitutionKagawa University (2018)
Maizuru National College of Technology (2014-2017)

Principal Investigator

Okumura Yukihiko  香川大学, 創造工学部, 教授 (80262971)

Project Period (FY) 2014-04-01 – 2019-03-31
Project Status Completed (Fiscal Year 2018)
Budget Amount *help
¥4,940,000 (Direct Cost: ¥3,800,000、Indirect Cost: ¥1,140,000)
Fiscal Year 2018: ¥1,040,000 (Direct Cost: ¥800,000、Indirect Cost: ¥240,000)
Fiscal Year 2017: ¥650,000 (Direct Cost: ¥500,000、Indirect Cost: ¥150,000)
Fiscal Year 2016: ¥1,040,000 (Direct Cost: ¥800,000、Indirect Cost: ¥240,000)
Fiscal Year 2015: ¥650,000 (Direct Cost: ¥500,000、Indirect Cost: ¥150,000)
Fiscal Year 2014: ¥1,560,000 (Direct Cost: ¥1,200,000、Indirect Cost: ¥360,000)
Keywords灰 / 粒子状浮遊物質 / 炭種 / コークス / 多環芳香族 / バイオマス / アルカリ金属 / 微量金属(灰) / PM2.5 / 揮発分 / チャー / ガス化 / 燃焼 / 環境負荷低減 / 石炭燃焼 / 昇温速度 / 溶融・合体 / 焼結鉱
Outline of Final Research Achievements

Multiple types of coal were pyrolyzed to obtain coke particles with different properties (melting point, amount of ash, caking and agglomerating properties). The coke particles were arranged to form layers and they were combusted. The effects of various factors on PM formation were then investigated.
(1) PM 2.5 was easily formed in a low temperature atmosphere (below 1000°C).(2) Combustion of coke particles produced from ash with a low melting point (approximately 1230°C) resulted in formation of lower amounts of PM 2.5 than combustion of coke particles from ash with a high melting point (approximately 1450°C). This is because the melting and coalescence of ash particles were easier in the former ash than in the latter ash.(3) The PM 2.5 formation can be suppressed by blending coal containing ash with a low melting point. In addition, The PM 2.5 formation can be suppressed by blending coal with a high value of the indicator.

Academic Significance and Societal Importance of the Research Achievements

健康被害を抑えるためにも,大気中への飛散を低減するためにも,燃焼から発生する微粒子(PM2.5)の生成機構および石炭燃焼におけるPM灰への微量有害元素の濃縮・凝縮現象の解明が必須である.本研究においては,近接する層状のコークス粉の燃焼から発生するPMの生成機構を調査するために基礎的な実験を実施した.調査項目は,(i) PM生成に及ぼす温度の影響,(ii) PM生成に及ぼすコークス内の灰性状(灰融点,灰分量)の影響,(iii) PM生成に及ぼすコークス性状(粘結塊化性)の影響である.
加えて,石炭揮発分中の多環芳香族炭化水素(PAHs)を起源とするPM生成についても調査した.

Report

(6 results)
  • 2018 Annual Research Report   Final Research Report ( PDF )
  • 2017 Research-status Report
  • 2016 Research-status Report
  • 2015 Research-status Report
  • 2014 Research-status Report
  • Research Products

    (26 results)

All 2018 2017 2016 2015 2014 Other

All Journal Article (3 results) (of which Int'l Joint Research: 1 results,  Peer Reviewed: 3 results,  Open Access: 1 results,  Acknowledgement Compliant: 1 results) Presentation (21 results) (of which Int'l Joint Research: 5 results,  Invited: 1 results) Remarks (2 results)

  • [Journal Article] Dispersion State of Catalytic Metal Supported on Bio-Char Elucidated Using Energy Dispersive X-ray Spectroscopy: Effects of Catalyst Type and Heating Process2017

    • Author(s)
      Toshiaki HANAOKA,Yukihiko OKUMURA
    • Journal Title

      Journal of the Japan Institute of Energy

      Volume: 96 Issue: 3 Pages: 73-85

    • DOI

      10.3775/jie.96.73

    • NAID

      130005519405

    • ISSN
      0916-8753, 1882-6121
    • Related Report
      2017 Research-status Report
    • Peer Reviewed
  • [Journal Article] Effect of heating rate and coal type on the yield of functional tar components2017

    • Author(s)
      Yukihiko Okumura
    • Journal Title

      Proceedings of the Combustion Institute

      Volume: 36 Issue: 2 Pages: 2075-2082

    • DOI

      10.1016/j.proci.2016.09.020

    • Related Report
      2016 Research-status Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Prediction of the First Pyrolysis Product and Yield in Biomass Gasifier2014

    • Author(s)
      Yukihiko OKUMURA, Takuya OKADA, Ken OKAZAKI
    • Journal Title

      Proc. The Fifteenth International Heat Transfer Conference

      Volume: IHTC15-8963/RNE-C1-323 Pages: 1-12

    • DOI

      10.1615/ihtc15.rne.008963

    • Related Report
      2014 Research-status Report
    • Peer Reviewed / Open Access / Acknowledgement Compliant
  • [Presentation] Gasification mechanism of woody biomass-derived char with supported Fe catalysts2018

    • Author(s)
      Yukihiko Okumura
    • Organizer
      The 16thINTERNATIONAL HEAT TRANSFER CONFERENCE
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 環境保全を目指したバイオマス/石炭の高度利用2018

    • Author(s)
      奥村 幸彦
    • Organizer
      中四国熱科学・工学研究会(日本伝熱学会中四国支部主催,徳島大学理工学部)
    • Related Report
      2018 Annual Research Report
    • Invited
  • [Presentation] 炭素転換率に伴うバイオマスチャー構造に関する研究 - ガス化剤の影響 -2018

    • Author(s)
      奥村 幸彦
    • Organizer
      第56回燃焼シンポジウム講演論文集(日本燃焼学会主催)
    • Related Report
      2018 Annual Research Report
  • [Presentation] バイオマスからの一次揮発タール成分の詳細分析2018

    • Author(s)
      奥村 幸彦
    • Organizer
      第55回石炭科学会議(日本エネルギー学会主催)
    • Related Report
      2018 Annual Research Report
  • [Presentation] Effect of Gasifying Agents on the Gasification Rate of Biomass-Derived Char2017

    • Author(s)
      Yukihiko Okumura, Shuhei Ohtani
    • Organizer
      The Ninth JSME-KSME Thermal and Fluids Engineering Conference
    • Related Report
      2017 Research-status Report
    • Int'l Joint Research
  • [Presentation] Fe 触媒担持下におけるチャーのガス化機構2017

    • Author(s)
      奥村 幸彦
    • Organizer
      第54回石炭科学会議論文集(日本エネルギー学会主催,秋田ビューホテル)
    • Related Report
      2017 Research-status Report
  • [Presentation] ガス化の進行に伴うバイオマスチャー細孔の発達機構2017

    • Author(s)
      奥村 幸彦,大谷 周平,田中 裕也
    • Organizer
      第26回日本エネルギー学会大会講演論文集(日本エネルギー学会主催,ウィンクあいち)
    • Related Report
      2017 Research-status Report
  • [Presentation] 触媒担持によるバイオマスチャーのガス化速度向上機構に関する研究2017

    • Author(s)
      奥村 幸彦
    • Organizer
      第27回環境工学総合シンポジウム2017講演論文集(日本機械学会主催,アクトシティ浜松)
    • Related Report
      2017 Research-status Report
  • [Presentation] 熱分解タール成分およびPAH生成に及ぼす炭種の影響2016

    • Author(s)
      奥村 幸彦
    • Organizer
      第54回燃焼シンポジウム (日本燃焼学会主催)
    • Place of Presentation
      仙台国際センター
    • Year and Date
      2016-11-23
    • Related Report
      2016 Research-status Report
  • [Presentation] MECHANISM OF GASIFICATION RATE-ENHANCEMENT ELUCIDATED BY CROSS-SECTIONAL ANALYSIS OF CATALYST-SUPPORTING BIOCHARS2016

    • Author(s)
      Yukihiko Okumura
    • Organizer
      4th International Forum on Heat Transfer
    • Place of Presentation
      Sendai International Center
    • Year and Date
      2016-11-02
    • Related Report
      2016 Research-status Report
    • Int'l Joint Research
  • [Presentation] 高機能性タールの高収率化2016

    • Author(s)
      奥村 幸彦
    • Organizer
      第53回石炭科学会議論文集(日本エネルギー学会主催)
    • Place of Presentation
      福山市生涯学習プラザ
    • Year and Date
      2016-10-26
    • Related Report
      2016 Research-status Report
  • [Presentation] バイオマスの一次熱分解タール成分に及ぼす構成成分の影響2016

    • Author(s)
      奥村 幸彦
    • Organizer
      第25回日本エネルギー学会大会(日本エネルギー学会主催)
    • Place of Presentation
      工学院大学
    • Year and Date
      2016-08-09
    • Related Report
      2016 Research-status Report
  • [Presentation] A high-yield method for producing functional coal-tar component for use in advanced chemical applications2016

    • Author(s)
      Yukihiko Okumura
    • Organizer
      36th International Symposium on Combustion
    • Place of Presentation
      COEX, Seoul, Korea
    • Year and Date
      2016-07-31
    • Related Report
      2016 Research-status Report
    • Int'l Joint Research
  • [Presentation] 微粉コークス燃焼からのPM2.5生成とその抑制法 -焼結鉱製造に伴うPM生成-2015

    • Author(s)
      奥村 幸彦,朝日 貴哉
    • Organizer
      第53回燃焼シンポジウム講演論文集(日本燃焼学会主催)
    • Place of Presentation
      つくば国際会館
    • Year and Date
      2015-11-16
    • Related Report
      2015 Research-status Report
  • [Presentation] 微粉炭コークスの層状燃焼場におけるPM生成とその抑制法2015

    • Author(s)
      奥村 幸彦
    • Organizer
      第52回石炭科学会議論文集(日本エネルギー学会主催)
    • Place of Presentation
      伊勢市観光文化会館
    • Year and Date
      2015-10-28
    • Related Report
      2015 Research-status Report
  • [Presentation] 微粉炭コークスの層状燃焼場におけるPM生成2015

    • Author(s)
      奥村 幸彦、朝日 貴哉、國本 祐介
    • Organizer
      第24回日本エネルギー学会大会講演論文集(日本エネルギー学会主催)
    • Place of Presentation
      北海道コンベンションセンター
    • Year and Date
      2015-08-03
    • Related Report
      2015 Research-status Report
  • [Presentation] A HIGH-YIELD METHOD FOR PRODUCING FUNCTIONAL COAL TAR FOR USE IN ADVANCED APPLICATIONS2015

    • Author(s)
      Yukihiko OKUMURA
    • Organizer
      The 10th Asia Pacific Conference on Sustainable Energy & Environmental Technologies
    • Place of Presentation
      University of Seoul, Korea
    • Year and Date
      2015-07-02
    • Related Report
      2015 Research-status Report
    • Int'l Joint Research
  • [Presentation] 微粉炭燃焼におけるPM生成 - 燃焼温度,昇温速度,炭種の影響 -2014

    • Author(s)
      朝日 貴哉,國本 祐介,今川 賢信,奥村 幸彦
    • Organizer
      第52回燃焼シンポジウム講演論文集、(日本燃焼学会)
    • Place of Presentation
      岡山コンベンションセンター
    • Year and Date
      2014-12-03 – 2014-12-05
    • Related Report
      2014 Research-status Report
  • [Presentation] Effect of heating rate on first-tar component in coal pyrolysis2014

    • Author(s)
      Yukihiko OKUMURA
    • Organizer
      Proc. The 25th International Symposium on Transport Phenomena
    • Place of Presentation
      Krabi, Thailand
    • Year and Date
      2014-11-05 – 2014-11-07
    • Related Report
      2014 Research-status Report
  • [Presentation] 一次熱分解タール・PAH生成に及ぼす炭種の影響2014

    • Author(s)
      奥村 幸彦,朝日 貴哉
    • Organizer
      第51回石炭科学会議論文集 (日本エネルギー学会)
    • Place of Presentation
      東北大学
    • Year and Date
      2014-10-22 – 2014-10-23
    • Related Report
      2014 Research-status Report
  • [Presentation] バイオマスの一次熱分解タール成分に及ぼす昇温速度の影響2014

    • Author(s)
      奥村 幸彦
    • Organizer
      第23回日本エネルギー学会大会講演論文集 (日本エネルギー学会)
    • Place of Presentation
      九州大学
    • Year and Date
      2014-07-19 – 2014-07-20
    • Related Report
      2014 Research-status Report
  • [Remarks] 環境エネルギー工学研究室

    • URL

      http://www.eng.kagawa-u.ac.jp/~okumura/index0.html

    • Related Report
      2018 Annual Research Report
  • [Remarks] 環境エネルギー工学研究室

    • URL

      http://www.maizuru-ct.ac.jp/control/okumura/index0.html

    • Related Report
      2017 Research-status Report 2016 Research-status Report

URL: 

Published: 2014-04-04   Modified: 2020-03-30  

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