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In-situ observation of dewetting phenomena by multi-quantum beam irradiation and investigation of their mechanism

Research Project

Project/Area Number 26420661
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeMulti-year Fund
Section一般
Research Field Physical properties of metals/Metal-base materials
Research InstitutionHokkaido University

Principal Investigator

SHIBAYAMA TAMAKI  北海道大学, 工学研究院, 教授 (10241564)

Co-Investigator(Kenkyū-buntansha) 岸本 弘立  室蘭工業大学, 工学研究科, 教授 (30397533)
Co-Investigator(Renkei-kenkyūsha) YATSU Shigeo  北海道大学, 大学院工学研究院, 特任助教 (40111158)
Research Collaborator LEI Yanhua  
Project Period (FY) 2014-04-01 – 2017-03-31
Project Status Completed (Fiscal Year 2016)
Budget Amount *help
¥5,070,000 (Direct Cost: ¥3,900,000、Indirect Cost: ¥1,170,000)
Fiscal Year 2016: ¥1,430,000 (Direct Cost: ¥1,100,000、Indirect Cost: ¥330,000)
Fiscal Year 2015: ¥1,820,000 (Direct Cost: ¥1,400,000、Indirect Cost: ¥420,000)
Fiscal Year 2014: ¥1,820,000 (Direct Cost: ¥1,400,000、Indirect Cost: ¥420,000)
Keywordsナノ粒子 / 表面プラズモン共鳴 / ナノ構造 / ナノ材料 / 微細構造解析 / その場観察 / 超高圧電子顕微鏡 / 濡れ性非濡れ性遷移 / 局在表面プラズモン共鳴 / 量子ビーム / レーザー / 照射効果 / LIPSS / 複合量子ビーム / 同時照射
Outline of Final Research Achievements

In this study, to investigate the mechanism of quantum beam irradiation induced dewetting phenomenon by image analysis using Quantum Beam High Voltage Electron Microscope in Hokkaido University, in-situ observation under co-irradiation with 100keV Ar ions and nanosecond-pulsed laser with 532 nm, or each quantum beam irradiation were done.
As a result of experiments, we succeeded to observe the behavior of Rayleigh instability during quantum beam irradiation induced dewetting of the noble metal changing from a rectangular shape to a spherical shape. As decreasing the thickness of the noble metal thin film, the average particle diameter of the nanoparticles is getting smaller than that of thicker one after dewetting. A blue shift of the absorption spectrum in the visible light region was confirmed due to the quantum effects.

Report

(4 results)
  • 2016 Annual Research Report   Final Research Report ( PDF )
  • 2015 Research-status Report
  • 2014 Research-status Report
  • Research Products

    (22 results)

All 2017 2016 2015 2014 Other

All Journal Article (3 results) (of which Int'l Joint Research: 2 results,  Peer Reviewed: 3 results,  Open Access: 1 results,  Acknowledgement Compliant: 3 results) Presentation (16 results) (of which Int'l Joint Research: 8 results,  Invited: 1 results) Remarks (3 results)

  • [Journal Article] Ion beam surface nanostructuring of noble metal films with localized surface plasmon excitation2017

    • Author(s)
      Meng, X., Shibayama, T., Yu, R., Ishioka, J. and Watanabe, S.
    • Journal Title

      Current Opinion in Solid State and Materials Science

      Volume: 印刷中 Issue: 4 Pages: 177-188

    • DOI

      10.1016/j.cossms.2017.01.001

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Int'l Joint Research / Acknowledgement Compliant
  • [Journal Article] Synthesis of surfactant-free Cu-Pt dendritic heterostructures with highly electrocatalytic performance for methanol oxidation reaction2016

    • Author(s)
      Kang, S., Gao, G., Xie, X., Shibayama, T., Lei, Y., Wang, Y. and Cai, L.
    • Journal Title

      Materials Research Letters

      Volume: 4 Issue: 4 Pages: 212-218

    • DOI

      10.1080/21663831.2016.1179228

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research / Acknowledgement Compliant
  • [Journal Article] In-situ observation of self-assembly of quasi-two-dimensional Au nano-submicron particles on β-SiC substrates via nanosecond-pulsed laser irradiation-induced dewetting of thin Au films2016

    • Author(s)
      Y.H. Lei, R.X. Yu, T. Shibayama, J. Ishioka and S. Watanabe
    • Journal Title

      Materials Letters

      Volume: 164 Pages: 202-205

    • DOI

      10.1016/j.matlet.2015.11.004

    • Related Report
      2015 Research-status Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Presentation] イオン液体中半導体ZnS-AgInS2固溶体ナノ粒子の光誘起反応TEM内その場観察2016

    • Author(s)
      五十嵐直也, 石岡準也, 大藤功将, 小暮一馬, 鳥本司3¥, 柴山環樹
    • Organizer
      平成28年度公益社団法人日本顕微鏡学会北海道支部学術講演会ポスター講演
    • Place of Presentation
      北海道大学、札幌市
    • Year and Date
      2016-12-10
    • Related Report
      2016 Annual Research Report
  • [Presentation] “EBSDを用いたイオン照射材料の硬さ試験機による微小圧痕周りの残留ひずみ分布解析2016

    • Author(s)
      関口 亮, 柴山 環樹, 檜木 達也, 近藤 創介
    • Organizer
      日本金属学会2016年秋期講演大会
    • Place of Presentation
      大阪大学豊中キャンパス、豊中市
    • Year and Date
      2016-09-21
    • Related Report
      2016 Annual Research Report
  • [Presentation] 水封入セルを用いた液中光照射誘起反応のTEM内その場観察2016

    • Author(s)
      大藤 功将, 五十嵐 直也, 石岡 準也, Melbert Jeem, 柴山 環樹, 渡辺 精一
    • Organizer
      2016年度応用物理学会秋季学術講演会
    • Place of Presentation
      朱鷺メッセ、新潟市
    • Year and Date
      2016-09-13
    • Related Report
      2016 Annual Research Report
  • [Presentation] Development of laser-equipped muti-beam HVEM and application study on radiation effects in materials2016

    • Author(s)
      S. Watanabe and T. Shibayama
    • Organizer
      11th Polish-Japanese Joint Seminar on Micro and Nano Analysis
    • Place of Presentation
      Gniew, Poland
    • Year and Date
      2016-09-11
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Direct Observation of Photocorrosion of ZnO Crystals in Ionic Liquid by High-Voltage Electron Microscope2016

    • Author(s)
      J. Ishioka, K. Kogure, Kosuke Ofuji, K. Kawaguchi, M. Jeem, T. Shibayama, and S. Watanabe
    • Organizer
      11th Polish-Japanese Joint Seminar on Micro and Nano Analysis
    • Place of Presentation
      Gniew, Poland
    • Year and Date
      2016-09-11
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Dierectric constant change of glass substrate after ion irradiation and SPR measurements by STEM/EELS2016

    • Author(s)
      Ruixuan Yu, Junya Ishioka, Tamaki Shibayama, Sousuke Kondo and Tatsuya Hinoki
    • Organizer
      The 7th International Symposium of Advanced Energy Science - Frontiers of Zero Emission Energy -
    • Place of Presentation
      京都大学宇治キャンパス、宇治市
    • Year and Date
      2016-09-05
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 複合量子ビーム超高圧電子顕微鏡を用いた光照射誘起現象その場観察2016

    • Author(s)
      石岡 準也,大藤 功将,五十嵐 直也,柴山 環樹,渡辺精一
    • Organizer
      日本顕微鏡学会第72回学術講演会
    • Place of Presentation
      仙台国際センター、仙台市
    • Year and Date
      2016-06-14
    • Related Report
      2016 Annual Research Report
  • [Presentation] 複合量子ビーム超高圧電子顕微鏡を用いたガラス基板上の金ナノ構造形成その場観察2016

    • Author(s)
      于 睿ケン,石岡 準也,大久保 賢二,谷岡 隆志,大多 亮,柴山 環樹,渡辺 精一
    • Organizer
      日本顕微鏡学会第72回学術講演会
    • Place of Presentation
      仙台国際センター、仙台市
    • Year and Date
      2016-06-14
    • Related Report
      2016 Annual Research Report
  • [Presentation] In-situ observation of Au thin film dewetting on dielectric substrate (SiO2 glass and silicon nitride) during quantum beam irradiation2015

    • Author(s)
      Ruixuan Yu,Tamaki Shibayama,Yanhua Lei, Shigeo Yatsu,Junya Ishioka,Seiichi Watanabe
    • Organizer
      The 2nd East-Asia Microscopy Conference
    • Place of Presentation
      The Himeji Chamber of Commerce and Industry(HCCI), Himeji, Hyogo
    • Year and Date
      2015-11-24
    • Related Report
      2015 Research-status Report
    • Int'l Joint Research
  • [Presentation] Correlation between dielectric constant change of glass substrate after ion irradiation and LSPR wavelength2015

    • Author(s)
      Ruixuan Yu, Junya Ishioka,Shigeo Yatsu,Tamaki Shibayama,Sousuke Kondo and Tatsuya Hinoki
    • Organizer
      The 6th International Symposium of Advanced Energy Science
    • Place of Presentation
      Kyoto University, Uji, Kyoto
    • Year and Date
      2015-09-01
    • Related Report
      2015 Research-status Report
    • Int'l Joint Research
  • [Presentation] In-Situ Observation of Self-Organizing Au Nanoparticles on SiC Substrate via Pulsed Laser Induced Dwetting of thin Au film2015

    • Author(s)
      Y.H. Lei, R.X. Yu, J. Ishioka, T. Shibayama, S. Watanabe, S. Yatsu
    • Organizer
      1st International Conference on Applied Surface Science
    • Place of Presentation
      Riverside Oriental Hotel, Shanghai, P. R. China
    • Year and Date
      2015-07-27
    • Related Report
      2015 Research-status Report
    • Int'l Joint Research
  • [Presentation] In-situ observation of Au film nanostructuring on SiO2 glass substrate during nanosecond-pulsed laser irradiation2015

    • Author(s)
      Ruixuan Yu,Tamaki Shibayama,Yanhua Lei, Shigeo Yatsu,Junya
    • Organizer
      1st International Conference on Applied Surface Science
    • Place of Presentation
      Riverside Oriental Hotel, Shanghai, P. R. China
    • Year and Date
      2015-07-27
    • Related Report
      2015 Research-status Report
    • Int'l Joint Research
  • [Presentation] マルチ量子ビーム超高圧電子顕微鏡を用いたレーザー照射誘起 dewetting のその場観察2015

    • Author(s)
      于 睿ケン、柴山 環樹、谷津 茂男、石岡 準也、渡辺 精一
    • Organizer
      日本顕微鏡学会第 71 回学術講演会
    • Place of Presentation
      国立京都国際会館、京都
    • Year and Date
      2015-05-13
    • Related Report
      2015 Research-status Report
    • Int'l Joint Research
  • [Presentation] Ion and nanosecond-pulsed laser co-irradiation effects on the surface nanostructure of Au thin films on SiO2 glass substrates2014

    • Author(s)
      Ruixuan Yu, T. Shibayama, J. Ishioka, S. Yatsu and S. Watanabe
    • Organizer
      10th Japanese-Polish Joint Seminar on Micro and Nano Analysis
    • Place of Presentation
      Suzuki Memorial Hall, Faculty of Engineering, Hokkaido Univesity
    • Year and Date
      2014-10-25
    • Related Report
      2014 Research-status Report
  • [Presentation] In situ observation of dewetting process of Au thin film on the surface of SiC substrate by nanosecond pulsed laser irradiation2014

    • Author(s)
      Lei Yanhua, Ruixuan Yu, T. Shibayama, J. Ishioka, S. Yatsu and S. Watanabe
    • Organizer
      10th Japanese-Polish Joint Seminar on Micro and Nano Analysis
    • Place of Presentation
      Suzuki Memorial Hall, Faculty of Engineering, Hokkaido Univesity
    • Year and Date
      2014-10-25
    • Related Report
      2014 Research-status Report
  • [Presentation] イオンおよびナノ秒パルスレーザー同時照射によるAu/SiO2表面のナノ構造化とその光学特性2014

    • Author(s)
      于睿ケン,柴山環樹,谷津茂男,石岡準也,渡辺精一
    • Organizer
      第75回応用物理学会秋季学術講演会
    • Place of Presentation
      北海道大学札幌キャンパス
    • Year and Date
      2014-09-19
    • Related Report
      2014 Research-status Report
  • [Remarks] 論文・発表

    • URL

      http://labs.eng.hokudai.ac.jp/labo/ryoshi_carem/?page_id=23

    • Related Report
      2016 Annual Research Report
  • [Remarks] 北大院工学研究院エネルギー・マテリアル融合領域研究センター量子エネルギー変換材料分野 論文・発表

    • URL

      http://labs.eng.hokudai.ac.jp/labo/ryoshi_carem/?page_id=23

    • Related Report
      2015 Research-status Report
  • [Remarks] http://labs.eng.hokudai.ac.jp/labo/ryoshi_carem/

    • Related Report
      2014 Research-status Report

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Published: 2014-04-04   Modified: 2018-12-17  

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