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Influence of properties of inorganic porous hollow fiber membranes on CO2 desorption from chemical absorbents in the membrane flash process

Research Project

Project/Area Number 26420762
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeMulti-year Fund
Section一般
Research Field Properties in chemical engineering process/Transfer operation/Unit operation
Research InstitutionShinshu University

Principal Investigator

TAKAHASHI Nobuhide  信州大学, 学術研究院繊維学系, 教授 (40377651)

Project Period (FY) 2014-04-01 – 2017-03-31
Project Status Completed (Fiscal Year 2016)
Budget Amount *help
¥5,070,000 (Direct Cost: ¥3,900,000、Indirect Cost: ¥1,170,000)
Fiscal Year 2016: ¥1,560,000 (Direct Cost: ¥1,200,000、Indirect Cost: ¥360,000)
Fiscal Year 2015: ¥1,560,000 (Direct Cost: ¥1,200,000、Indirect Cost: ¥360,000)
Fiscal Year 2014: ¥1,950,000 (Direct Cost: ¥1,500,000、Indirect Cost: ¥450,000)
KeywordsCO2化学吸収プロセス / 省エネルギー / アルミナ多孔質膜 / CO2放散 / 触媒効果 / 酸性官能基 / CO2化学吸収 / 減圧放散 / 多孔質中空糸膜 / アルミナ粒子 / 酸性官能基修飾 / 放散促進 / 放散エネルギー削減 / ナノ粒子析出多孔質膜による二酸化炭素の放散促進 / 膜材料の触媒効果による二酸化炭素の放散促進 / 地球温暖化 / 二酸化炭素回収貯留 / CO2分離 / 化学吸収 / 吸収液再生 / 多孔質膜
Outline of Final Research Achievements

Carbon capture and storage, CCS is expected to be a promising technology to mitigate the global warming. For its practical use, however, it is necessary to reduce the energy consumption in the solvent regeneration in the chemical absorption method. Then, this study focused on the membrane flash process using alumina porous hollow fiber membranes. This uses pressure control not much heat supply used in the conventional method to release CO2 from the rich solvent.
In this study, influence of physical and chemical properties of the membrane on CO2 desorption performance was experimentally investigated. The results showed that the contact time and area between the rich solvent and the membrane had great influence on the CO2 desorption rate and there was the appropriate membrane structure yielding a higher CO2 desorption rate. Also, it was found out that the introduction of acidic chemical groups like a phosphate group to the membrane surface was an effective way to promote CO2 desorption.

Report

(4 results)
  • 2016 Annual Research Report   Final Research Report ( PDF )
  • 2015 Research-status Report
  • 2014 Research-status Report
  • Research Products

    (12 results)

All 2017 2016 2015 2014 Other

All Journal Article (1 results) (of which Peer Reviewed: 1 results,  Open Access: 1 results,  Acknowledgement Compliant: 1 results) Presentation (9 results) (of which Int'l Joint Research: 5 results) Remarks (2 results)

  • [Journal Article] Influence of addition of functionalized alumina particles on CO2 stripping from amine solvents2017

    • Author(s)
      Nobuhide Takahashi, Satoko Miyakawa, Iori Shimada, Mitsumasa Osada, Hiroshi Fukunaga
    • Journal Title

      Energy procedia

      Volume: 印刷中 Pages: 2024-2029

    • DOI

      10.1016/j.egypro.2017.03.1336

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Open Access / Acknowledgement Compliant
  • [Presentation] クロスフロー型中空糸膜コンタクターのシェル側流れ方向の列数による対流物質移動への影響2017

    • Author(s)
      竹内一迅, 嶋田五百里, 長田光正, 福長博, 高橋伸英
    • Organizer
      化学工学会第82年会
    • Place of Presentation
      芝浦工業大学(東京都江東区)
    • Year and Date
      2017-03-06
    • Related Report
      2016 Annual Research Report
  • [Presentation] Influence of addition of functionalized alumina particles on CO2 stripping from amine solvents2016

    • Author(s)
      Nobuhide Takahashi, Satoko Miyakawa, Iori Shimada, Mitsumasa Osada, Hiroshi Fukunaga
    • Organizer
      13th International Conference on Greenhouse Gas Control Technologies, GHGT-13
    • Place of Presentation
      Lausanne, Switzerland
    • Year and Date
      2016-11-14
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Influence of addition of functionalized alumina particles on CO2 stripping from amine solvents2016

    • Author(s)
      Nobuhide Takahashi, Satoko Miyakawa, Iori Shimada, Mitsumasa Osada
    • Organizer
      13th Conference on Greenhouse Gas Control Technologies (GHGT)
    • Place of Presentation
      The SwissTech Convention Center (Lausanne, Switzerland)
    • Year and Date
      2016-11-14
    • Related Report
      2015 Research-status Report
    • Int'l Joint Research
  • [Presentation] Effects Of The Structure Of Inorganic Porous Hollow Fiber Membrane On CO2 Desorption Rate In A Membrane Flash Process2015

    • Author(s)
      Ayaka Yokomichi, Iori Shimada, Hiroshi Fukunaga, Nobuhide Takahashi
    • Organizer
      APCChE2015(Asian Pacific Confederation of Chemical Engineering)
    • Place of Presentation
      Melbourne Convention and Exhibition Centre, Melbourne, Australia
    • Year and Date
      2015-09-27 – 2015-10-01
    • Related Report
      2014 Research-status Report
  • [Presentation] Quantification of intrusion of chemical absorbent liquid into porous hollow fiber membrane and its influences on CO2 absorption rate in a membrane contactor2015

    • Author(s)
      Nobuhide Takahashi, Yuki Sakai, Iori Shimada, Mitsumasa Osada, Hiroshi Fukunaga
    • Organizer
      Asian Pacific Confederation of Chemical Engineering (APCChE) Congress 2015
    • Place of Presentation
      Melbourne Convention and Exhibition Centre (Melbourne, Australia)
    • Year and Date
      2015-09-27
    • Related Report
      2015 Research-status Report
    • Int'l Joint Research
  • [Presentation] Effects of the structure of inorganic porous hollow fiber membrane on CO2 desorption rate in a membrane flash process2015

    • Author(s)
      Ayaka Yokomichi, Iori Shimada, Mitsumasa Osada, Hiroshi Fukunaga, Nobuhide Takahashi
    • Organizer
      Asian Pacific Confederation of Chemical Engineering (APCChE) Congress 2015
    • Place of Presentation
      Melbourne Convention and Exhibition Centre (Melbourne, Australia)
    • Year and Date
      2015-09-27
    • Related Report
      2015 Research-status Report
    • Int'l Joint Research
  • [Presentation] CO2 desorption performance of amine-based solvents by membrane flash process2015

    • Author(s)
      Nobuhide Takahashi, Takuya Wada, Iori Shimada, Hiroshi Fukunaga
    • Organizer
      3rd Post Combustion Capture Conference (PCCC3)
    • Place of Presentation
      Hotel Delta Regina (Regina, Canada)
    • Year and Date
      2015-09-08
    • Related Report
      2015 Research-status Report
    • Int'l Joint Research
  • [Presentation] 金属酸化物粒子の化学的性質がCO2減圧放散速度に及ぼす影響2015

    • Author(s)
      保科有希, 嶋田五百里, 長田光正, 福長博, 高橋伸英
    • Organizer
      化学工学会第80年会
    • Place of Presentation
      芝浦工業大学豊洲キャンパス(東京都江東区)
    • Year and Date
      2015-03-19 – 2015-03-21
    • Related Report
      2014 Research-status Report
  • [Presentation] 無機多孔質中空糸膜の構造がCO2の減圧フラッシュ放散速度へ及ぼす影響2014

    • Author(s)
      横道礼果, 高橋伸英, 嶋田五百里, 福長博
    • Organizer
      化学工学会第46回秋季大会
    • Place of Presentation
      九州大学 伊都キャンパス(福岡県福岡市)
    • Year and Date
      2014-09-17 – 2014-09-19
    • Related Report
      2014 Research-status Report
  • [Remarks] 研究室ホームページ

    • URL

      http://www.fiber.shinshu-u.ac.jp/novhide-lab/Research.html

    • Related Report
      2016 Annual Research Report
  • [Remarks] 研究室ホームページ

    • URL

      http://www.fiber.shinshu-u.ac.jp/novhide-lab/index.html

    • Related Report
      2015 Research-status Report 2014 Research-status Report

URL: 

Published: 2014-04-04   Modified: 2018-03-22  

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