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Theoretical study of an isotope separation method with terahertz optical pulses

Research Project

Project/Area Number 26420875
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeMulti-year Fund
Section一般
Research Field Nuclear engineering
Research InstitutionJapan Atomic Energy Agency

Principal Investigator

ICHIHARA AKIRA  国立研究開発法人日本原子力研究開発機構, 原子力科学研究部門 原子力基礎工学研究センター, 研究主幹 (60354784)

Co-Investigator(Kenkyū-buntansha) 松岡 雷士  広島大学, 工学研究院, 助教 (50455276)
瀬川 悦生  東北大学, 情報科学研究科, 准教授 (30634547)
Project Period (FY) 2014-04-01 – 2017-03-31
Project Status Completed (Fiscal Year 2016)
Budget Amount *help
¥4,290,000 (Direct Cost: ¥3,300,000、Indirect Cost: ¥990,000)
Fiscal Year 2016: ¥650,000 (Direct Cost: ¥500,000、Indirect Cost: ¥150,000)
Fiscal Year 2015: ¥910,000 (Direct Cost: ¥700,000、Indirect Cost: ¥210,000)
Fiscal Year 2014: ¥2,730,000 (Direct Cost: ¥2,100,000、Indirect Cost: ¥630,000)
Keywords同位体分離 / テラヘルツ / 二原子分子 / 回転励起 / 分子解離 / 数理モデル / 量子ウォーク / 直交多項式 / 解離 / 直行多項式 / シミュレーション / 塩化リチウム / レーザー同位体分離
Outline of Final Research Achievements

We proposed a method for dissociating diatomic molecules isotope-selectively in the gas phase by using terahertz optical pulses. A pulse train composed of a few pulses was introduced to excite the selected isotope into the highly rotationally-excited state. With the computer simulation for lithium chloride molecules in the rotational temperature of 70 K, we demonstrated that the selected isotope molecules can be dissociated effectively by using the designed terahertz pulses. Moreover, we clarified the characteristics of rotational excitation induced by optical pulse trains through the analyses of mathematical models.

Report

(4 results)
  • 2016 Annual Research Report   Final Research Report ( PDF )
  • 2015 Research-status Report
  • 2014 Research-status Report
  • Research Products

    (32 results)

All 2017 2016 2015 2014 Other

All Int'l Joint Research (1 results) Journal Article (9 results) (of which Int'l Joint Research: 2 results,  Peer Reviewed: 8 results,  Acknowledgement Compliant: 8 results,  Open Access: 3 results) Presentation (21 results) (of which Int'l Joint Research: 8 results,  Invited: 1 results) Remarks (1 results)

  • [Int'l Joint Research] 韓京大学校(韓国)

    • Related Report
      2016 Annual Research Report
  • [Journal Article] Localization in Rotational Excitation of Diatomic Molecules Induced by a Train of Optical Pulses2017

    • Author(s)
      L. Matsuoka, E. Segawa
    • Journal Title

      Interdisciplinary Information Sciences

      Volume: 23 Issue: 1 Pages: 51-56

    • DOI

      10.4036/iis.2017.A.07

    • NAID

      130005519570

    • ISSN
      1340-9050, 1347-6157
    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Open Access / Acknowledgement Compliant
  • [Journal Article] Asymptotic behavior of a rotational population distribution in a molecular quantum-kicked rotor with ideal quantum resonance2017

    • Author(s)
      L. Matsuoka, E. Segawa, K. Yuki, N. Konno, N. Obata
    • Journal Title

      Physics Letters A

      Volume: 未定 Issue: 21 Pages: 1773-1779

    • DOI

      10.1016/j.physleta.2017.03.032

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Int'l Joint Research / Acknowledgement Compliant
  • [Journal Article] One-dimensional three-state quantum walks: Weak limits and localization2016

    • Author(s)
      C. K. Ko, E. Segawa, H. J. Yoo
    • Journal Title

      Infinite dimensional analysis, Quantum Probability and Related Topics

      Volume: 19 Issue: 04 Pages: 1650025-1650025

    • DOI

      10.1142/s0219025716500259

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Int'l Joint Research / Acknowledgement Compliant
  • [Journal Article] Generator of an abstract quantum walk2016

    • Author(s)
      E. Segawa, A. Suzuki
    • Journal Title

      Quantum Studies: Mathematics and Foundations

      Volume: 3 Issue: 1 Pages: 11-30

    • DOI

      10.1007/s40509-016-0070-1

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Unified parameter for localization in isotope-selective rotational excitation of diatomic molecules using a train of optical pulses2015

    • Author(s)
      L. Matsuoka
    • Journal Title

      Physical Review A

      Volume: 91 Issue: 4 Pages: 043420-043420

    • DOI

      10.1103/physreva.91.043420

    • Related Report
      2015 Research-status Report
    • Peer Reviewed / Open Access / Acknowledgement Compliant
  • [Journal Article] Spectral properties of weighted line digraphs2015

    • Author(s)
      E. Segawa
    • Journal Title

      RIMS Kokyuroku

      Volume: 1956 Pages: 16-28

    • Related Report
      2015 Research-status Report
  • [Journal Article] Quantum control of isotope-selective rovibrational excitation of diatomic molecules in the thermal distribution2015

    • Author(s)
      A. Ichihara. L. Matsuoka, Y. Kurosaki, K. Yokoyama
    • Journal Title

      Optical Review

      Volume: 22 Issue: 1 Pages: 153-156

    • DOI

      10.1007/s10043-015-0025-5

    • Related Report
      2014 Research-status Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Isotope-selective dissociation of diatomic molecules by terahertz optical pulses2015

    • Author(s)
      A. Ichihara, L. Matsuoka, E. Segawa and K. Yokoyama,
    • Journal Title

      Physical Review A

      Volume: 91 Issue: 4 Pages: 043404-043404

    • DOI

      10.1103/physreva.91.043404

    • Related Report
      2014 Research-status Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Trapping and spreading properties of quantum walk in homological structure2014

    • Author(s)
      Takuya Machida, Etsuo Segawa
    • Journal Title

      Quantum Information Processing

      Volume: online Issue: 5 Pages: 1539-1558

    • DOI

      10.1007/s11128-014-0819-6

    • Related Report
      2015 Research-status Report
    • Peer Reviewed / Open Access / Acknowledgement Compliant
  • [Presentation] Computer simulation of isotope-selective dissociation of lithium chloride molecules in the rotational temperature of 70 K by terahertz optical pulses2017

    • Author(s)
      A. Ichihara, L. Matsuoka
    • Organizer
      日本化学会第97春季年会
    • Place of Presentation
      慶應義塾大学 日吉キャンパス (神奈川県横浜市)
    • Year and Date
      2017-03-17
    • Related Report
      2016 Annual Research Report
  • [Presentation] 連続時間量子ウォークの描像に基づく二原子分子の回転励起の数理モデル解析2017

    • Author(s)
      松岡 雷士
    • Organizer
      日本物理学会第72回年次大会
    • Place of Presentation
      大阪大学 豊中キャンパス (大阪府豊中市)
    • Year and Date
      2017-03-17
    • Related Report
      2016 Annual Research Report
  • [Presentation] 量子ウォークを架け橋にした学際交流2017

    • Author(s)
      瀬川 悦生
    • Organizer
      数学パワーが世界を変える-統数研数学協働プログラム- CREST・さきがけ・数学協働プログラムの合同シンポジウム
    • Place of Presentation
      東京大学 駒場キャンパス (東京都目黒区)
    • Year and Date
      2017-02-26
    • Related Report
      2016 Annual Research Report
    • Invited
  • [Presentation] Sensitivity of a quantum walk to boundary2016

    • Author(s)
      H. Obuse, E. Segawa
    • Organizer
      Workshop of Quantum Simulation and Quantum Walks 2016
    • Place of Presentation
      Czech Technical University in Prague, Prague, (Czech Republic)
    • Year and Date
      2016-11-17
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 単位円周上の直交多項式・分散関係・統計的性質2016

    • Author(s)
      瀬川 悦生
    • Organizer
      統計数理研究所数学協働プログラムワークショップ「量子系の数理と物質制御への展開II:量子ウォークを架け橋に」
    • Place of Presentation
      横浜国立大学 常盤台キャンパス (神奈川県横浜市)
    • Year and Date
      2016-10-22
    • Related Report
      2016 Annual Research Report
  • [Presentation] 光パルス列による分子回転励起の数理モデル解析-数工連携の苦難と成果-2016

    • Author(s)
      松岡 雷士
    • Organizer
      統計数理研究所数学協働プログラムワークショップ「量子系の数理と物質制御への展開II:量子ウォークを架け橋に」
    • Place of Presentation
      横浜国立大学 常盤台キャンパス (神奈川県横浜市)
    • Year and Date
      2016-10-22
    • Related Report
      2016 Annual Research Report
  • [Presentation] 量子ウォークの縁への感受性2016

    • Author(s)
      瀬川 悦生
    • Organizer
      日本数学会 2016秋季統合分科会
    • Place of Presentation
      関西大学 千里山キャンパス (大阪府吹田市)
    • Year and Date
      2016-09-15
    • Related Report
      2016 Annual Research Report
  • [Presentation] Quantum walks on half line relate to orthogonal polynomials2016

    • Author(s)
      E. Segawa
    • Organizer
      International Workshop on IDAQP
    • Place of Presentation
      Chungbuk National University, Cheongju (Korea)
    • Year and Date
      2016-09-09
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Spectral and stochastic behaviors of Grover walks2016

    • Author(s)
      E. Segawa
    • Organizer
      The Japanese Conference on Combinatorics and Its Applications Mini Symposium : Spectral Graph Theory and Related Topics
    • Place of Presentation
      Kyoto Univeresity, Clock Tower Central Hall, Kyoto (Japan)
    • Year and Date
      2016-05-22
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 光学パルスを用いた塩化リチウム分子の同位体選択的振動励起の計算機シミュレーション2016

    • Author(s)
      市原 晃
    • Organizer
      日本化学会第96春季年会
    • Place of Presentation
      同志社大学 京田辺キャンパス (京都府京田辺市)
    • Year and Date
      2016-03-24
    • Related Report
      2015 Research-status Report
  • [Presentation] Localization in rotational excitation of diatomic molecules induced by a train of optical pulses2015

    • Author(s)
      L. Matsuoka, E. Segawa
    • Organizer
      Workshop of Quantum Simulation and Quantum Walks 2015
    • Place of Presentation
      Yokohama National University, Education and Culture Hall  (神奈川県横浜市)
    • Year and Date
      2015-11-16
    • Related Report
      2015 Research-status Report
    • Int'l Joint Research
  • [Presentation] Szego class and ballistic spreading of quantum walks2015

    • Author(s)
      E. Segawa
    • Organizer
      Workshop of Quantum Simulation and Quantum Walks 2015
    • Place of Presentation
      Yokohama National University, Education and Culture Hall  (神奈川県横浜市)
    • Year and Date
      2015-11-16
    • Related Report
      2015 Research-status Report
    • Int'l Joint Research
  • [Presentation] Generator of some quantum walks2015

    • Author(s)
      E. Segawa
    • Organizer
      11th Sendai Workshop on Infinite Dimensional Analysis and Quantum Probability
    • Place of Presentation
      東北大学 情報科学研究科棟 (宮城県仙台市)
    • Year and Date
      2015-10-26
    • Related Report
      2015 Research-status Report
    • Int'l Joint Research
  • [Presentation] 光パルス列による分子回転励起過程における磁気量子数の影響の数理解析2015

    • Author(s)
      松岡 雷士, 瀬川 悦生
    • Organizer
      第9回分子科学討論会
    • Place of Presentation
      東京工業大学 大岡山キャンパス (東京都目黒区)
    • Year and Date
      2015-09-16
    • Related Report
      2015 Research-status Report
  • [Presentation] 無限ツリー上のGrover walkの発生の固有空間2015

    • Author(s)
      瀬川 悦生
    • Organizer
      日本数学会 2015秋季統合分科会
    • Place of Presentation
      京都産業大学 (京都府京都市)
    • Year and Date
      2015-09-13
    • Related Report
      2015 Research-status Report
  • [Presentation] Mathematical study on quantum walks and its application2015

    • Author(s)
      E. Segawa
    • Organizer
      Moscow State Univ.-Tohoku Univ., 2nd IT Joint workshop
    • Place of Presentation
      Moskow State University, Moscow ( Russia)
    • Year and Date
      2015-09-07
    • Related Report
      2015 Research-status Report
    • Int'l Joint Research
  • [Presentation] Orthogonal polynomials and the limit distribution of induced quantum walks on the half line2015

    • Author(s)
      E. Segawa
    • Organizer
      10th Jikji Workshop on Infinite Dimensional Analysis and Quantum Probability
    • Place of Presentation
      Chungbuk National University, Jeonju (Korea)
    • Year and Date
      2015-07-29
    • Related Report
      2015 Research-status Report
    • Int'l Joint Research
  • [Presentation] A mathematical approach based on orthogonal polynomials for rotational excitation of diatomic molecules2015

    • Author(s)
      L. Matsuoka, E. Segawa
    • Organizer
      第31回化学反応討論会
    • Place of Presentation
      北海道大学 工学部フロンティア応用科学研究棟 (北海道札幌市)
    • Year and Date
      2015-06-03
    • Related Report
      2015 Research-status Report
  • [Presentation] 光学パルスによる塩化リチウム分子の同位体選択的振動励起の理論研究2015

    • Author(s)
      市原 晃、横山 啓一
    • Organizer
      日本化学会第95春季年会
    • Place of Presentation
      日本大学理工学部船橋キャンパス/薬学部(千葉県船橋市)
    • Year and Date
      2015-03-26 – 2015-03-29
    • Related Report
      2014 Research-status Report
  • [Presentation] 非共鳴光パルス列中での二原子分子の回転遷移過程の数理モデル2014

    • Author(s)
      松岡 雷士
    • Organizer
      第8回分子科学討論会
    • Place of Presentation
      広島大学東広島キャンパス(広島県東広島市)
    • Year and Date
      2014-09-21 – 2014-09-24
    • Related Report
      2014 Research-status Report
  • [Presentation] 光パルス列中での二原子分子の回転分布局在化の数理モデル2014

    • Author(s)
      松岡 雷士、市原 晃、瀬川 悦生、横山 啓一
    • Organizer
      第17回理論化学討論会
    • Place of Presentation
      名古屋大学東山キャンパス(愛知県名古屋市)
    • Year and Date
      2014-05-22 – 2014-05-24
    • Related Report
      2014 Research-status Report
  • [Remarks] プラズマ基礎科学研究室(難波・松岡研究室)

    • URL

      http://home.hiroshima-u.ac.jp/plasma/index.html

    • Related Report
      2016 Annual Research Report

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Published: 2014-04-04   Modified: 2018-03-22  

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