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Quantitative estimation of anthropogenic input of metallic elements to the environment using non-traditional isotope ratios

Research Project

Project/Area Number 26550020
Research Category

Grant-in-Aid for Challenging Exploratory Research

Allocation TypeMulti-year Fund
Research Field Environmental dynamic analysis
Research InstitutionKwansei Gakuin University (2015-2016)
Japan Agency for Marine-Earth Science and Technology (2014)

Principal Investigator

Tanimizu Masaharu  関西学院大学, 理工学部, 教授 (20373459)

Co-Investigator(Kenkyū-buntansha) 高橋 嘉夫  東京大学, 大学院理学系研究科(理学部), 教授 (10304396)
坂口 綾  筑波大学, 数理物質系, 准教授 (00526254)
Project Period (FY) 2014-04-01 – 2017-03-31
Project Status Completed (Fiscal Year 2016)
Budget Amount *help
¥3,900,000 (Direct Cost: ¥3,000,000、Indirect Cost: ¥900,000)
Fiscal Year 2015: ¥650,000 (Direct Cost: ¥500,000、Indirect Cost: ¥150,000)
Fiscal Year 2014: ¥3,250,000 (Direct Cost: ¥2,500,000、Indirect Cost: ¥750,000)
Keywords同位体 / 物質循環 / 環境動態 / 金属元素 / 質量分析 / 重金属
Outline of Final Research Achievements

Natural isotopic variations of metallic elements were determined among geological and environmental samples collected from the earth surface. Rapid and low blank chemical purification techniques were developed for some first transitional elements and light elements. Precise isotopic determination techniques with high sample throughput of the elements were also established by ICP-MS. Resultant isotopic variation observed for nickel among these samples was small compared to other transitional elements like copper and zinc. Wide isotopic variations of boron and lithium were also confirmed using the developed techniques. Their isotope ratios of some samples with anthropogenic origin have large isotopic shifts apart from those with natural origin. The application of the mass-dependent isotopic fractionation of metallic elements as the isotopic proxy may be possible for a better understanding of the anthropogenic input to the environment.

Report

(4 results)
  • 2016 Annual Research Report   Final Research Report ( PDF )
  • 2015 Research-status Report
  • 2014 Research-status Report
  • Research Products

    (38 results)

All 2017 2016 2015 2014 Other

All Journal Article (7 results) (of which Int'l Joint Research: 1 results,  Peer Reviewed: 6 results,  Open Access: 4 results,  Acknowledgement Compliant: 1 results) Presentation (29 results) (of which Int'l Joint Research: 6 results,  Invited: 4 results) Book (1 results) Remarks (1 results)

  • [Journal Article] A simple and rapid method for isotopic analysis of nickel, copper, and zinc in seawater using chelating extraction and anion exchange2017

    • Author(s)
      S. Takano, M. Tanimizu, T. Hirata, K.C. Shin, Y. Fukami, K. Suzuki, and Y. Sohrin
    • Journal Title

      Analytica Chimica Acta

      Volume: 967 Pages: 1-11

    • DOI

      10.1016/j.aca.2017.03.010

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Stable isotope fractionation of tungsten during adsorption on Fe and Mn (oxyhydr)oxides2017

    • Author(s)
      T. Kashiwabara, S. Kubo, M. Tanaka, R. Senda, T. Iizuka, M. Tanimizu, Y. Takahashi
    • Journal Title

      Geochimica. Cosmochimica. Acta

      Volume: 204 Pages: 52-67

    • DOI

      10.1016/j.gca.2017.01.031

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Cerium stable isotope ratios in ferromanganese deposits and their potential as a paleo-redox proxy2016

    • Author(s)
      R. Nakada, Y. Takahashi, and M. Tanimizu
    • Journal Title

      Geochimica Cosmochimica Acta

      Volume: 181 Pages: 89-100

    • DOI

      10.1016/j.gca.2016.02.025

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] 高感度無機質量分析法による極微量核種定量の試み2015

    • Author(s)
      谷水雅治
    • Journal Title

      放射線

      Volume: 40 Pages: 209-213

    • Related Report
      2015 Research-status Report
    • Peer Reviewed
  • [Journal Article] 重元素の質量に依存した安定同位体存在度変動の検出2015

    • Author(s)
      谷水雅治
    • Journal Title

      Isotope News

      Volume: 2015年9月号 Pages: 7-11

    • Related Report
      2015 Research-status Report
  • [Journal Article] Isotopic constraints on biogeochemical cycling of copper in the ocean2014

    • Author(s)
      Takano S, Tanimizu M, Hirata T, Sohrin Y
    • Journal Title

      Nature Communications

      Volume: 5 Issue: 1 Pages: 1-7

    • DOI

      10.1038/ncomms6663

    • NAID

      120005517897

    • Related Report
      2014 Research-status Report
    • Peer Reviewed / Open Access / Acknowledgement Compliant
  • [Journal Article] Hydrothermal carbonate chimneys from a continental rift (Afar Rift): mineralogy, geochemistry and mode of formation2014

    • Author(s)
      V.M. Dekov, N.M. Egueh, G.D. Kamenov, G. Bayon, S.V. Lalonde, M. Schmidt, V. Liebetrau, F. Munnik, Y. Fouquet, M. Tanimizu, M.O. Awaleh, I. Guirreh, B. Le Gall
    • Journal Title

      Chemical Geology

      Volume: 387 Pages: 87-100

    • DOI

      10.1016/j.chemgeo.2014.08.019

    • Related Report
      2014 Research-status Report
    • Peer Reviewed
  • [Presentation] Development of a rapid and quantitative nickel purification technique for accurate nickel isotopic analysis in geochemical reference materials2017

    • Author(s)
      Kobayashi, Y., Takano, S., and Tanimizu, M.
    • Organizer
      欧州冬季プラズマ分光化学会議2017
    • Place of Presentation
      オーストリア共和国ザンクトアントン
    • Year and Date
      2017-02-23
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Geochemical characteristics of hydrothermal fluids observed along Median Tectonic Line in Mie-Prefecture, Japan2017

    • Author(s)
      Tanimizu, M., Nakai, R., Sugimoto, N., and Mori, Y.
    • Organizer
      欧州冬季プラズマ分光化学会議2017
    • Place of Presentation
      オーストリア共和国ザンクトアントン
    • Year and Date
      2017-02-23
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 高分解能・高回収率の新たなNi単離法の確立と地球化学標準物質のNi高精度同位体分析(口頭発表)2016

    • Author(s)
      小林裕基・高野祥太朗・谷水雅治
    • Organizer
      2016年度日本質量分析学会同位体比部会
    • Place of Presentation
      秋田温泉さとみ(秋田県秋田市)
    • Year and Date
      2016-11-17
    • Related Report
      2016 Annual Research Report
  • [Presentation] プラズマイオン源質量分析法を用いた 元素同位体分析の海洋分野への応用展開(基調講演)2016

    • Author(s)
      谷水雅治
    • Organizer
      2016年度日本地球化学会年会
    • Place of Presentation
      大阪市立大学(大阪府大阪市)
    • Year and Date
      2016-09-16
    • Related Report
      2016 Annual Research Report
    • Invited
  • [Presentation] 2種類の固相抽出法を用いた地質学的試料からのNi単離法の確立及び同位体比の高精度測定2016

    • Author(s)
      小林裕基・高野祥太朗・谷水雅治
    • Organizer
      2016年度日本地球化学会年会
    • Place of Presentation
      大阪市立大学(大阪府大阪市)
    • Year and Date
      2016-09-15
    • Related Report
      2016 Annual Research Report
  • [Presentation] Distributions of Nickel, copper and zinc isotopes in the North Pacific Ocean2016

    • Author(s)
      Takano, S., Uehara, W., Shin, K.-C., Hirata, T., Tanimizu, M., and Sohrin, Y.
    • Organizer
      Goldschmidt 2016
    • Place of Presentation
      パシフィコ横浜(神奈川県横浜市)
    • Year and Date
      2016-06-29
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 3段階のイオン交換分離法による高分離能かつ高回収率の地質学的試料からの新たなNi単離法の確立2016

    • Author(s)
      小林裕基・高野祥太朗・谷水雅治
    • Organizer
      第64回質量分析総合討論会
    • Place of Presentation
      ホテル阪急エキスポパーク(大阪府吹田市)
    • Year and Date
      2016-05-20
    • Related Report
      2016 Annual Research Report
  • [Presentation] 海水中Ni、Cu、Zn同位体比一括分析法の開発と西部太平洋海水試料への応用2016

    • Author(s)
      高野祥太朗, 上原渉, 谷水雅治, 平田岳史, 申基澈, 宗林由樹
    • Organizer
      東京大学大気海洋研究所共同利用研究集会「GEOTRECE計画エンジン全開:太平洋・インド洋における微量元素・同位体の生物地球化学研究の進展」
    • Place of Presentation
      東京大学大気海洋研究所(千葉県・柏市)
    • Year and Date
      2016-03-29
    • Related Report
      2015 Research-status Report
  • [Presentation] 同位体マルチプロキシからみた三重県中部地域温泉水の地球化学的特徴2015

    • Author(s)
      仲井涼, 森康則, 谷水雅治
    • Organizer
      第5回同位体環境学シンポジウム
    • Place of Presentation
      総合地球環境学研究所(京都府・京都市)
    • Year and Date
      2015-12-25
    • Related Report
      2015 Research-status Report
  • [Presentation] 海水中Ni、Cu、Zn同位体比精密分析法の開発2015

    • Author(s)
      高野祥太朗, 上原渉, 宗林由樹, 平田岳史, 谷水雅治, 申基澈
    • Organizer
      第5回同位体環境学シンポジウム
    • Place of Presentation
      総合地球環境学研究所(京都府・京都市)
    • Year and Date
      2015-12-25
    • Related Report
      2015 Research-status Report
  • [Presentation] ICP-MSの高アバンダンス感度化による236U定量の試み2015

    • Author(s)
      谷水雅治, 杉山尚樹
    • Organizer
      日本質量分析学会同位体比部会2015
    • Place of Presentation
      湯の宿「木もれび」(滋賀県・大津市)
    • Year and Date
      2015-11-26
    • Related Report
      2015 Research-status Report
  • [Presentation] 地質学的試料からの新たなNi単離法の確立2015

    • Author(s)
      小林裕基, 高野祥太朗, 谷水雅治
    • Organizer
      日本質量分析学会同位体比部会2015
    • Place of Presentation
      湯の宿「木もれび」(滋賀県・大津市)
    • Year and Date
      2015-11-26
    • Related Report
      2015 Research-status Report
  • [Presentation] 三重県中部地方の温泉水および河川水の起源推定2015

    • Author(s)
      仲井涼, 森康則, 谷水雅治
    • Organizer
      日本質量分析学会同位体比部会2015
    • Place of Presentation
      湯の宿「木もれび」(滋賀県・大津市)
    • Year and Date
      2015-11-25
    • Related Report
      2015 Research-status Report
  • [Presentation] エアロゾル中の鉄の化学種および同位体比:海洋への水溶性鉄の供給に関連して2015

    • Author(s)
      高橋嘉夫
    • Organizer
      一般財団法人海洋化学研究所69周年秋季講演会
    • Place of Presentation
      京都大学(京都府・京都市)
    • Year and Date
      2015-11-13
    • Related Report
      2015 Research-status Report
    • Invited
  • [Presentation] ICP質量分析計を用いた地球化学標準試料(岩石・海水・炭酸塩)のリチウム同位体比迅速分析2015

    • Author(s)
      永石一弥, 谷水雅治, 石川剛志
    • Organizer
      2015年度日本地球化学会
    • Place of Presentation
      横浜国立大学(神奈川県・横浜市)
    • Year and Date
      2015-09-17
    • Related Report
      2015 Research-status Report
  • [Presentation] δ11B-δ7Li値からみた三重県温泉水の地球化学的特徴2015

    • Author(s)
      谷水雅治, 仲井涼, 小林裕基, 森康則, 木村浩之, 青常, 中村仁美
    • Organizer
      2015年度日本地球化学会
    • Place of Presentation
      横浜国立大学(神奈川県・横浜市)
    • Year and Date
      2015-09-16
    • Related Report
      2015 Research-status Report
  • [Presentation] 海水中ニッケル、銅、亜鉛同位体比の迅速・精密分析法の開発2015

    • Author(s)
      高野祥太朗, 宗林由樹, 上原渉, 申基澈, 谷水雅治, 平田岳史
    • Organizer
      2015年度日本地球化学会
    • Place of Presentation
      横浜国立大学(神奈川県・横浜市)
    • Year and Date
      2015-09-16
    • Related Report
      2015 Research-status Report
  • [Presentation] 様々な大気環境における塩素消失に関わる化学反応の推定2015

    • Author(s)
      坂田昂平, 坂口綾, 為則雄祐, 高橋嘉夫
    • Organizer
      2015年度日本地球化学会
    • Place of Presentation
      横浜国立大学(神奈川県・横浜市)
    • Year and Date
      2015-09-16
    • Related Report
      2015 Research-status Report
  • [Presentation] Boron isotope fractionation during transportation of sea-salt particle2015

    • Author(s)
      Sakata, S., A. Sakaguchi, Y. Takahashi, K. Nagaishi, and M. Tanimizu
    • Organizer
      Goldschmidt2015
    • Place of Presentation
      プラハ(チェコ共和国)
    • Year and Date
      2015-08-19
    • Related Report
      2015 Research-status Report
    • Int'l Joint Research
  • [Presentation] Reconstruction of heavy element emission history from a peat-rich pond in the western Pacific region2015

    • Author(s)
      Tanimizu, M., M. Kohno, Y. Asahara, M. Minami, and T. Hosono
    • Organizer
      Goldschmidt2015
    • Place of Presentation
      プラハ(チェコ共和国)
    • Year and Date
      2015-08-18
    • Related Report
      2015 Research-status Report
    • Int'l Joint Research
  • [Presentation] Determination of isotopic ratio of nickel, copper, and zinc in seawater using an ethylenediaminetriacetic acid chelating resin2015

    • Author(s)
      Takano, S., M. Tanimizu, T. Hirata, Y. Sohrin, S. Little, and C. Archer
    • Organizer
      Goldschmidt2015
    • Place of Presentation
      プラハ(チェコ共和国)
    • Year and Date
      2015-08-17
    • Related Report
      2015 Research-status Report
    • Int'l Joint Research
  • [Presentation] シュウ酸エアロゾルと金属元素の相互作用:その安定性と地球冷却効果との関連2015

    • Author(s)
      山川庸芝明, 坂田昂平, 宮原彩, 宮本千尋, 高橋嘉夫, 坂口 綾
    • Organizer
      日本地球惑星科学連合大会2015
    • Place of Presentation
      幕張メッセ(千葉県・千葉市)
    • Year and Date
      2015-05-28
    • Related Report
      2015 Research-status Report
  • [Presentation] 塩素消失の新しい指標としての主要イオン化学組成の利用法2015

    • Author(s)
      坂田昂平, 坂口綾, 為則雄祐, 小川雅裕, 高橋嘉夫
    • Organizer
      日本地球惑星科学連合大会2015
    • Place of Presentation
      幕張メッセ(千葉県・千葉市)
    • Year and Date
      2015-05-28
    • Related Report
      2015 Research-status Report
  • [Presentation] 21世紀のGoldschmidt的地球化学: 分子地球化学2015

    • Author(s)
      高橋嘉夫
    • Organizer
      日本地球惑星科学連合大会2015
    • Place of Presentation
      幕張メッセ(千葉県・千葉市)
    • Year and Date
      2015-05-26
    • Related Report
      2015 Research-status Report
    • Invited
  • [Presentation] ICP質量分析法を用いたd7Li値迅速分析法の確立2014

    • Author(s)
      谷水雅治、永石一弥
    • Organizer
      日本地球化学会2014年年会
    • Place of Presentation
      富山大学(富山県富山市)
    • Year and Date
      2014-09-18
    • Related Report
      2014 Research-status Report
  • [Presentation] ICP-MSの高アバンダンス感度化による新たなアプリケーションの展望2014

    • Author(s)
      谷水雅治
    • Organizer
      日本分析化学会2014年大会
    • Place of Presentation
      広島大学(広島県東広島市)
    • Year and Date
      2014-09-17
    • Related Report
      2014 Research-status Report
    • Invited
  • [Presentation] Accurate determination of trace elements in high-matrix samples by ICP-MS/MS2014

    • Author(s)
      M. Tanimizu
    • Organizer
      Asia Oceania Geosciences Society 11th Annual Meeting
    • Place of Presentation
      Royton Sapporo Hotel(北海道札幌市)
    • Year and Date
      2014-07-29
    • Related Report
      2014 Research-status Report
  • [Presentation] Biogeochemical Cycling of Copper Isotopes in the Ocean2014

    • Author(s)
      S. Takano, M. Tanimizu, T. Hirata, Y. Sohrin
    • Organizer
      Asia Oceania Geosciences Society 11th Annual Meeting
    • Place of Presentation
      Royton Sapporo Hotel(北海道札幌市)
    • Year and Date
      2014-07-29
    • Related Report
      2014 Research-status Report
  • [Presentation] 高精度ホウ素同位体比迅速分析法の地下水・火山岩への応用2014

    • Author(s)
      谷水雅治、永石一弥、石川剛志
    • Organizer
      日本地球惑星科学連合2014年大会
    • Place of Presentation
      パシフィコ横浜(神奈川県横浜市)
    • Year and Date
      2014-05-01
    • Related Report
      2014 Research-status Report
  • [Book] 第7.1章 鉛同位体と環境地球化学(書名: 地球のしくみを理解する)2015

    • Author(s)
      谷水雅治 (広島大学地球惑星システム学科編)
    • Total Pages
      20
    • Publisher
      広島大学出版会
    • Related Report
      2015 Research-status Report
  • [Remarks] 海洋における銅同位体比の分布を高精度で解明

    • URL

      http://www.jamstec.go.jp/j/about/press_release/20141205/

    • Related Report
      2014 Research-status Report

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Published: 2014-04-04   Modified: 2018-03-22  

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