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Catalytic reactions for mimicking processes in the fixation of carbon dioxide and methanogenesis by methanogenic bacteria

Research Project

Project/Area Number 26550054
Research Category

Grant-in-Aid for Challenging Exploratory Research

Allocation TypeMulti-year Fund
Research Field Environmental engineering and reduction of environmental burden
Research InstitutionHokkaido University

Principal Investigator

FUKUSHIMA Masami  北海道大学, 工学(系)研究科(研究院), 准教授 (40344113)

Project Period (FY) 2014-04-01 – 2016-03-31
Project Status Completed (Fiscal Year 2015)
Budget Amount *help
¥2,600,000 (Direct Cost: ¥2,000,000、Indirect Cost: ¥600,000)
Fiscal Year 2015: ¥910,000 (Direct Cost: ¥700,000、Indirect Cost: ¥210,000)
Fiscal Year 2014: ¥1,690,000 (Direct Cost: ¥1,300,000、Indirect Cost: ¥390,000)
Keywords環境技術 / 環境材料 / 触媒・化学プロセス / 超分子化学 / 生体機能利用
Outline of Final Research Achievements

In the methanogenesis by methanogenic bacteria, CO2 is fixed as N-formyl to methanofuran (MF). To mimic such processes chemically, catalytic systems were searched, in terms of the N-formylation of benzylamine as a model of MF. The Cu-diphosphine complex/polymethylhydrosiloxane system was found to be effective. In addition, the effects of humic substances, which are distributed in habitat of the bacteria, on the efficiency of N-formylation were also investigated.

Report

(3 results)
  • 2015 Annual Research Report   Final Research Report ( PDF )
  • 2014 Research-status Report
  • Research Products

    (5 results)

All 2016 2015 2014

All Journal Article (2 results) (of which Peer Reviewed: 2 results) Presentation (3 results)

  • [Journal Article] Effects of humic acids derived from lignite and cattle manure on antioxidant enzymatic activities of barley root.2016

    • Author(s)
      K. Nagasawa, B. Wang, K. Nishiya, K. Ushijima, Q. Zhu, M. Fukushima, T. Ichijo
    • Journal Title

      Journal of Environmental Science and Health, Part B: Pesticides, Food Contaminants, and Agricultural Wastes

      Volume: 51 Issue: 2 Pages: 81-89

    • DOI

      10.1080/03601234.2015.1080516

    • Related Report
      2015 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Monopersulfate oxidation of Acid Orange 7 with an iron(III)-tetrakis(N-methylpyridinium-4-yl)porphyrin intercalated into the layers of montmorillonite and pillared clay2015

    • Author(s)
      Ryo Nishimoto, Qianqian Zhu, Takafumi Miyamoto, Tsutomu Sato, Xuefei Tu, Apichaya Aneksampant, Masami Fukushima
    • Journal Title

      Journal of Molecular Catalysis A: Chemical

      Volume: 396 Pages: 84-89

    • DOI

      10.1016/j.molcata.2014.09.035

    • Related Report
      2014 Research-status Report
    • Peer Reviewed
  • [Presentation] 有機リン金属触媒によるCO2のN-ホルミル化に及ぼす腐植物質前駆体の影響2016

    • Author(s)
      五十嵐真美、福嶋正巳
    • Organizer
      日本化学会第96春季年会
    • Place of Presentation
      同志社大学京田辺キャンパス (京都)
    • Year and Date
      2016-03-24
    • Related Report
      2015 Annual Research Report
  • [Presentation] メタン生成細菌による二酸化炭素固定を模倣した触媒反応に関する研究2016

    • Author(s)
      福嶋正巳、五十嵐真美
    • Organizer
      日本化学会第96春季年会
    • Place of Presentation
      同志社大学京田辺キャンパス (京都)
    • Year and Date
      2016-03-24
    • Related Report
      2015 Annual Research Report
  • [Presentation] モンモリロナイトに担持された鉄ポルフィリン触媒の活性評価2014

    • Author(s)
      西本遼、宮本貴文、朱倩倩、佐藤努、福嶋正巳
    • Organizer
      日本分析化学会第63年会
    • Place of Presentation
      広島大学(広島)
    • Year and Date
      2014-09-18
    • Related Report
      2014 Research-status Report

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Published: 2014-04-04   Modified: 2017-05-10  

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