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Ultimate limit of the compressed pulse duration from a time-delay compensated monochromator

Research Project

Project/Area Number 26600107
Research Category

Grant-in-Aid for Challenging Exploratory Research

Allocation TypeMulti-year Fund
Research Field Optical engineering, Photon science
Research InstitutionHokkaido University

Principal Investigator

Sekikawa Taro  北海道大学, 工学(系)研究科(研究院), 准教授 (90282607)

Research Collaborator IGARASHI Hironori  
MAKIDA Ayumu  
FUJIWARA Takehisa  
IIKUBO Ryo  
Project Period (FY) 2014-04-01 – 2016-03-31
Project Status Completed (Fiscal Year 2015)
Budget Amount *help
¥3,900,000 (Direct Cost: ¥3,000,000、Indirect Cost: ¥900,000)
Fiscal Year 2015: ¥780,000 (Direct Cost: ¥600,000、Indirect Cost: ¥180,000)
Fiscal Year 2014: ¥3,120,000 (Direct Cost: ¥2,400,000、Indirect Cost: ¥720,000)
Keywords高次高調波 / 光電子分光 / パルス圧縮 / 分子軌道 / 時間遅延補償分光器
Outline of Final Research Achievements

The purposes of this study are the generation and the characterization of 1-fs high harmonic pulses from the time-delay compensated monochromator and the study of photochemical reactions by time-resolved photoelectron spectroscopy. 10-fs laser pulses were produced by the hollow-fiber technique to produce 1-fs high harmonic pulses. The beam coupling to the hollow fiber was highly stabilized and was stable for more than 5 hours. However the energy loss during the pulse compression was so large that the characterization of the high harmonic pulses was not done. The optimization of the optical dispersion of the system improved the temporal resolution of the system to 55 fs. The dynamics of photochemical reactions were investigated.

Report

(3 results)
  • 2015 Annual Research Report   Final Research Report ( PDF )
  • 2014 Research-status Report
  • Research Products

    (21 results)

All 2016 2015 2014 Other

All Int'l Joint Research (1 results) Journal Article (4 results) (of which Int'l Joint Research: 1 results,  Peer Reviewed: 4 results,  Acknowledgement Compliant: 1 results) Presentation (15 results) (of which Int'l Joint Research: 3 results) Book (1 results)

  • [Int'l Joint Research] stockholm university(sweden)

    • Related Report
      2015 Annual Research Report
  • [Journal Article] Excited State Non-Adiabatic Dynamics of N-Methylpyrrole: A Time-Resolved Photoelectron Spectroscopy and Quantum Dynamics Study2016

    • Author(s)
      G. Wu, S. P. Neville, O. Schalk, T. Sekikawa, M. N. R. Ashfold, G. A. Worth, and A. Stolow
    • Journal Title

      Journal of Chemical Physics

      Volume: 144 Issue: 1 Pages: 2463-2468

    • DOI

      10.1063/1.4938423

    • Related Report
      2015 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] 単一次数高調波光源による気相分子の時間分解光電子分光2015

    • Author(s)
      関川太郎,飯窪亮,原渕祐,佐藤壮太,武次徹也,萱沼洋輔
    • Journal Title

      レーザー研究

      Volume: 43 Pages: 833-837

    • NAID

      130007957178

    • Related Report
      2015 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Excited State Non-Adiabatic Dynamics of Pyrrole: A Time-Resolved Photoelectron Spectroscopy and Quantum Dynamics Study2015

    • Author(s)
      G. Wu, S. Neville, O. Schalk, T. Sekikawa, M. Ashfold, G. Worth, and A. Stolow
    • Journal Title

      Journal of Chemical Physics

      Volume: 142 Issue: 7

    • DOI

      10.1063/1.4907529

    • Related Report
      2014 Research-status Report
    • Peer Reviewed
  • [Journal Article] Ultrafast relaxation dynamics in trans-1,3-butadiene studied by time-resolved photoelectron spectroscopy with high harmonic pulses2014

    • Author(s)
      A. Makida, H. Igarashi, T. Fujiwara, T. Sekikawa, Y. Harabuchi, and T. Taketsugu
    • Journal Title

      J. Phys. Chem. Lett.

      Volume: 5 Issue: 10 Pages: 1760-1765

    • DOI

      10.1021/jz5003567

    • Related Report
      2014 Research-status Report
    • Peer Reviewed
  • [Presentation] 1,4- シクロヘキサジエンにおける水素原子の脱離ダイナミクス2016

    • Author(s)
      荒木孝太郎,天宅建晴,跡部龍之介,関川太郎,原渕祐,佐藤 壮太,武次 徹也
    • Organizer
      応用物理学会春季学術講演会
    • Place of Presentation
      東京工業大学大岡山キャンパス(東京都目黒区)
    • Year and Date
      2016-03-21
    • Related Report
      2015 Annual Research Report
  • [Presentation] 時間分解光電子分光による1,2-ブタジエンの光化学反応ダイナミクスの研究2015

    • Author(s)
      飯窪亮, 藤原丈久, 関川太郎, 原渕祐, 佐藤壮太, 武次徹也, 萱沼洋輔
    • Organizer
      第9回分子科学討論会
    • Place of Presentation
      東京工業大学大岡山キャンパス(東京都目黒区)
    • Year and Date
      2015-09-19
    • Related Report
      2015 Annual Research Report
  • [Presentation] 共役系ジエンにおける超高速光励起緩和ダイナミクスの研究2015

    • Author(s)
      天宅建晴,荒木孝太郎,関川太郎
    • Organizer
      応用物理学会秋季学術講演会
    • Place of Presentation
      名古屋国際会議場(愛知県名古屋市)
    • Year and Date
      2015-09-13
    • Related Report
      2015 Annual Research Report
  • [Presentation] Ring-opening dynamics of 1,3-cyclohexadiene studied by time-resolved molecular orbital spectroscopy2015

    • Author(s)
      T. Sekikawa, R. Iikubo, Y. Harabuchi, and T. Taketsugu
    • Organizer
      The Hamburg Conference on Femtochemistry
    • Place of Presentation
      DESY, Hamburg (Germany)
    • Year and Date
      2015-07-15
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Photodissociation of 1,2-Butadiene Studied by Time-Resolved Molecular Orbital Spectroscopy Using Single-Order High Harmonic Pulses2015

    • Author(s)
      R. Iikubo, T. Fujiwara, ∙T. Sekikawa, Y. Harabuchi, T. Taketsugu, and Y. Kayanuma
    • Organizer
      Conference on Lasers and Electro-Optics Europe & European Quantum Electronics
    • Place of Presentation
      Munich(Germany)
    • Year and Date
      2015-06-21
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Photodissociation of 1,2-Butadiene Studied by Time-Resolved Molecular Orbital Spectroscopy Using Single-Order High Harmonic Pulses2015

    • Author(s)
      R. Iikubo, T. Fujiwara, T. Sekikawa, Y. Harabuchi, T. Taketsugu, and Y. Kayanuma,
    • Organizer
      4th Advanced Lasers and Photon Sources Conference ALPS’15
    • Place of Presentation
      Pacifico Yokohama(Yokohama, Kanagawa)
    • Year and Date
      2015-04-23
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Time-resolved molecular orbital spectroscopy using single-order high harmonic pulses2015

    • Author(s)
      T. Sekikawa, R. Iikubo, T. Fujiwara, Y. Harabuchi, and T. Taketsugu
    • Organizer
      Ultrafast Dynamic Imaging of Matter 2015
    • Place of Presentation
      Grindelwald (スイス)
    • Year and Date
      2015-03-11
    • Related Report
      2014 Research-status Report
  • [Presentation] 時間分解分子軌道分光による1,3-シクロヘキサジエンの光化学反応ダイナミクスの研究2015

    • Author(s)
      飯窪 亮,藤原丈久,関川太郎,原渕 祐,武次徹也
    • Organizer
      レーザー学会学術講演会第35回年次大会
    • Place of Presentation
      東海大学高輪校舎(港区)
    • Year and Date
      2015-01-12
    • Related Report
      2014 Research-status Report
  • [Presentation] 時間分解分子軌道分光による1,2-ブタジエンの光解離の研究2015

    • Author(s)
      飯窪 亮,藤原丈久,関川太郎,原渕 祐,武次徹也
    • Organizer
      レーザー学会学術講演会第35回年次大会
    • Place of Presentation
      東海大学高輪校舎(港区)
    • Year and Date
      2015-01-12
    • Related Report
      2014 Research-status Report
  • [Presentation] 時間分解光電子分光による1,3-シクロヘキサジエンの光開環反応の研究2014

    • Author(s)
      飯窪 亮, 藤原 丈久, 関川 太郎, 原渕 祐, ,武次 徹也
    • Organizer
      第8回分子科学討論会
    • Place of Presentation
      広島大学(東広島市)
    • Year and Date
      2014-09-24
    • Related Report
      2014 Research-status Report
  • [Presentation] 1,3-シクロヘキサジエンの開環反応の観測2014

    • Author(s)
      飯窪亮,藤原丈久,関川太郎,原渕祐,武次徹也
    • Organizer
      第 75 回応用物理学会秋季学術講演会
    • Place of Presentation
      北海道大学(札幌市)
    • Year and Date
      2014-09-19
    • Related Report
      2014 Research-status Report
  • [Presentation] 1,2-butadieneにおける化学結合切断の実時間観測2014

    • Author(s)
      飯窪亮,藤原丈久,関川太郎,原渕祐,武次徹也
    • Organizer
      第 75 回応用物理学会秋季学術講演会
    • Place of Presentation
      北海道大学(札幌市)
    • Year and Date
      2014-09-18
    • Related Report
      2014 Research-status Report
  • [Presentation] Ultrafast Relaxation and Photodissociation Dynamics of 1,3-Butadiene Studied by Probing Molecular Orbitals2014

    • Author(s)
      A. Makida, T. Fujiwara, T. Sekikawa, Y. Harabuchi, and T. Taketsugu,
    • Organizer
      19th International Conference on Ultrafast Phenomen
    • Place of Presentation
      沖縄コンベンションセンター(宜野湾市)
    • Year and Date
      2014-07-08
    • Related Report
      2014 Research-status Report
  • [Presentation] Ultrafast and Photodissociation Dynamics of 1,2-Butadiene Studied by Photoelectron Spectroscopy2014

    • Author(s)
      Iikubo, T. Fujiwara, T. Sekikawa, Y. Harabuchi, and T. Taketsugu
    • Organizer
      19th International Conference on Ultrafast Phenomen
    • Place of Presentation
      沖縄コンベンションセンター(宜野湾市)
    • Year and Date
      2014-07-07
    • Related Report
      2014 Research-status Report
  • [Presentation] Ultrafast Relaxation and Photodissociation Dynamics of 1,3-Butadiene Studied by Probing Molecular Orbitals2014

    • Author(s)
      A. Makida, T. Fujiwara, Y. Harabuchi, T. Taketsugu, and Taro Sekikawa
    • Organizer
      Conference on Lasers and Electro-Optics
    • Place of Presentation
      San Jose (USA)
    • Year and Date
      2014-06-09
    • Related Report
      2014 Research-status Report
  • [Book] Optical Technologies for Extreme-Ultraviolet and Soft X-ray Coherent Sources2015

    • Author(s)
      T. Sekikawa
    • Total Pages
      19
    • Publisher
      Springer
    • Related Report
      2015 Annual Research Report

URL: 

Published: 2014-04-04   Modified: 2017-05-10  

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