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Analysis of multielectron dynamics in intense laser fields

Research Project

Project/Area Number 26600111
Research Category

Grant-in-Aid for Challenging Exploratory Research

Allocation TypeMulti-year Fund
Research Field Optical engineering, Photon science
Research InstitutionThe University of Tokyo

Principal Investigator

Ishikawa Kenichi  東京大学, 大学院工学系研究科(工学部), 教授 (70344025)

Co-Investigator(Renkei-kenkyūsha) SATO Takeshi  東京大学, 大学院工学系研究科, 特任講師 (30507091)
Project Period (FY) 2014-04-01 – 2017-03-31
Project Status Completed (Fiscal Year 2016)
Budget Amount *help
¥3,900,000 (Direct Cost: ¥3,000,000、Indirect Cost: ¥900,000)
Fiscal Year 2016: ¥780,000 (Direct Cost: ¥600,000、Indirect Cost: ¥180,000)
Fiscal Year 2015: ¥780,000 (Direct Cost: ¥600,000、Indirect Cost: ¥180,000)
Fiscal Year 2014: ¥2,340,000 (Direct Cost: ¥1,800,000、Indirect Cost: ¥540,000)
Keywordsアト秒科学 / 量子エレクトロニクス / 強光子場科学 / 高強度場物理 / 第一原理計算
Outline of Final Research Achievements

We have analyzed multielectron dynamics in molecules under intense laser fields calculated with ab initio methods. By analyzing the enhanced ionization of hydrogen molecules using Bohmian trajectories, we have revealed, contrary to what was previously believed, that the ejection from the up-field and down-field cores are comparable. Moreover, we have numerically implemented multiconfiguration time-dependent Hartree-Fock method for molecules, we have successfully simulated high-harmonic generation from a water molecule and charge migration in LiH and water molecules, for the first time.

Report

(4 results)
  • 2016 Annual Research Report   Final Research Report ( PDF )
  • 2015 Research-status Report
  • 2014 Research-status Report
  • Research Products

    (39 results)

All 2017 2016 2015 2014 Other

All Int'l Joint Research (3 results) Journal Article (9 results) (of which Int'l Joint Research: 2 results,  Peer Reviewed: 9 results,  Acknowledgement Compliant: 9 results) Presentation (24 results) (of which Int'l Joint Research: 11 results,  Invited: 11 results) Book (1 results) Remarks (2 results)

  • [Int'l Joint Research] ウィーン工科大学(オーストリア)

    • Related Report
      2016 Annual Research Report
  • [Int'l Joint Research] ウィーン工科大学(オーストリア)

    • Related Report
      2015 Research-status Report
  • [Int'l Joint Research] ミュンヘン工科大学(ドイツ)

    • Related Report
      2015 Research-status Report
  • [Journal Article] High-order harmonic generation enhanced by dynamical electron correlation2017

    • Author(s)
      Iliya Tikhomirov, Takeshi Sato, and Kenichi L. Ishikawa
    • Journal Title

      Phys. Rev. Lett.

      Volume: 印刷中

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Trajectory analysis of high-order-harmonic generation from periodic crystals2017

    • Author(s)
      T. Ikemachi, Y. Shinohara, T. Sato, J. Yumoto, M. Kuwata-Gonokami, and K. L. Ishikawa
    • Journal Title

      Physical Review A

      Volume: 95 Issue: 4 Pages: 043416-043416

    • DOI

      10.1103/physreva.95.043416

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] High-harmonic spectra from time-dependent two-particle reduced-density-matrix theory2017

    • Author(s)
      F. Lackner, I. Bresinova, T. Sato, K. L. Ishikawa, and J. Burgdorfer
    • Journal Title

      Physical Review A

      Volume: 95 Issue: 3

    • DOI

      10.1103/physreva.95.033414

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Int'l Joint Research / Acknowledgement Compliant
  • [Journal Article] Time-dependent complete-active-space self-consistent-field method for atoms: Application to high-harmonic generation2016

    • Author(s)
      T. Sato and K. L. Ishikawa
    • Journal Title

      Physical Review A

      Volume: 94 Issue: 2

    • DOI

      10.1103/physreva.94.023405

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Int'l Joint Research / Acknowledgement Compliant
  • [Journal Article] Implementation of the multiconfiguration time-dependent Hartree-Fock method for general molecules on a multi-resolution Cartesian grid2016

    • Author(s)
      R. Sawada, T. Sato, and K. L. Ishikawa
    • Journal Title

      Physical Review A

      Volume: 93 Issue: 2 Pages: 023434-023434

    • DOI

      10.1103/physreva.93.023434

    • Related Report
      2015 Research-status Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] A Review on Ab Initio Approaches for Multielectron Dynamics2015

    • Author(s)
      K. L. Ishikawa and T. Sato
    • Journal Title

      IEEE J. Sel. Topics Quantum Electron.

      Volume: 21 Pages: 1-1

    • DOI

      10.1109/jstqe.2015.2438827

    • Related Report
      2015 Research-status Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] ime-dependent multiconfiguration self-consistent-field method based on occupation restricted multiple active space model for multielectron dynamics in intense laser fields2015

    • Author(s)
      T. Sato and K. L. Ishikawa
    • Journal Title

      Phys. Rev. A

      Volume: 91 Issue: 2

    • DOI

      10.1103/physreva.91.023417

    • Related Report
      2014 Research-status Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] The structure of approximate two electron wavefunction in intense laser driven ionization dynamics2014

    • Author(s)
      T. Sato and K. L. Ishikawa
    • Journal Title

      J. Phys. B

      Volume: 47 Issue: 20 Pages: 204031-204031

    • DOI

      10.1088/0953-4075/47/20/204031

    • Related Report
      2014 Research-status Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Ryohto Sawada, Takeshi Sato, and Kenichi L. Ishikawa2014

    • Author(s)
      Ryohto Sawada, Takeshi Sato, and Kenichi L. Ishikawa
    • Journal Title

      Physical Review A

      Volume: 90 Issue: 2 Pages: 023404-023404

    • DOI

      10.1103/physreva.90.023404

    • Related Report
      2014 Research-status Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Presentation] Strong-field phenomena from the first principles2017

    • Author(s)
      Kenichi L. Ishikawa
    • Organizer
      The 8th Asian Workshop on Generationand Application of Coherent XUV and X-ray Radiation
    • Place of Presentation
      Hsinchu, Taiwan
    • Year and Date
      2017-03-27
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Time-dependent ab initio wavefunction methods for multielectron dynamics of atoms and molecules in intense laser fields2017

    • Author(s)
      Takeshi Sato
    • Organizer
      Okazaki conference: International Symposium on Ultrafast Dynamics in Molecular and Material Sciences
    • Place of Presentation
      自然科学研究機構岡崎コンファレンスセンター
    • Year and Date
      2017-03-06
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Development and applications of time-dependent ab initio wavefunction methods for intense-laser driven multielectron dynamics of atoms and molecule2017

    • Author(s)
      Takeshi Sato
    • Organizer
      3rd China-Japan-Korea Workshop on Theoretical and Computational Chemistry
    • Place of Presentation
      Daejeon, Korea
    • Year and Date
      2017-01-10
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] 第一原理計算で探る高強度レーザー場と原子・分子の相互作用2016

    • Author(s)
      石川顕一
    • Organizer
      原子衝突学会第41回年会
    • Place of Presentation
      富山大学五福キャンパス
    • Year and Date
      2016-12-10
    • Related Report
      2016 Annual Research Report
    • Invited
  • [Presentation] Strong-Fileld Phenomena from the First Principles2016

    • Author(s)
      Kenichi L. Ishikawa
    • Organizer
      9th Asian Symposium on Intense Laser Science (ASILS9)
    • Place of Presentation
      Ninh Binh, Vietnam
    • Year and Date
      2016-12-06
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Time-Dependent Multiconfiguration Self-Consistent-Field(TD-MCSCF) Approaches for Multielectron Dynamis in Intense Laser Fields2016

    • Author(s)
      Kenichi L. Ishikawa
    • Organizer
      ITAMP Workshop on the Electronic-Structure Problem in Theoretical Strong-Field Physics
    • Place of Presentation
      Cambridge, MA, USA
    • Year and Date
      2016-10-10
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] 第一原理強光子場物理2016

    • Author(s)
      石川顕一
    • Organizer
      第6回光科学異分野横断萌芽研究会
    • Place of Presentation
      静岡県伊東市
    • Year and Date
      2016-08-17
    • Related Report
      2016 Annual Research Report
    • Invited
  • [Presentation] Implementation and applications of time-dependent multiconfiguration methods for laser-driven multielectron dynamics of atoms2016

    • Author(s)
      T. Sato and K. Ishikawa
    • Organizer
      International Conference on Ultrafast Phenomena 2016
    • Place of Presentation
      Santa Fe, USA
    • Year and Date
      2016-07-17
    • Related Report
      2015 Research-status Report
    • Int'l Joint Research
  • [Presentation] First-principles Simulations of General Molecules in Intense Laser Fields2016

    • Author(s)
      R. Sawada, T. Sato, and K. L. Ishikawa
    • Organizer
      International Conference on Ultrafast Phenomena 2016
    • Place of Presentation
      Santa Fe, USA
    • Year and Date
      2016-07-17
    • Related Report
      2015 Research-status Report
    • Int'l Joint Research
  • [Presentation] First-principles simulations of multielectron dynamics in intense laser field2016

    • Author(s)
      Kenichi L. Ishikawa
    • Organizer
      7th Shanghai-Tokyo Advanced Research Symposium on Ultrafast Intense Laser Science
    • Place of Presentation
      湘南国際村センター
    • Year and Date
      2016-05-20
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] 外部複素スケーリングを用いたコンパクトな強レーザー場第一原理計算2016

    • Author(s)
      織茂悠貴、佐藤健、澤田亮人、石川顕一
    • Organizer
      第63回応用物理学会春季学術講演会
    • Place of Presentation
      東京工業大学大岡山キャンパス
    • Year and Date
      2016-03-19
    • Related Report
      2015 Research-status Report
  • [Presentation] 非対称な系へのMulti-resolution MCTDHFの適用22016

    • Author(s)
      澤田亮人、佐藤健、石川顕一
    • Organizer
      第63回応用物理学会春季学術講演会
    • Place of Presentation
      東京工業大学大岡山キャンパス
    • Year and Date
      2016-03-19
    • Related Report
      2015 Research-status Report
  • [Presentation] アト秒パルスによるネオン原子のイオン化の第一原理シミュレーション2016

    • Author(s)
      岩津広大、佐藤健、石川顕一
    • Organizer
      第63回応用物理学会春季学術講演会
    • Place of Presentation
      東京工業大学大岡山キャンパス
    • Year and Date
      2016-03-19
    • Related Report
      2015 Research-status Report
  • [Presentation] Multielectron Dynamics in Intense Laser Fields2016

    • Author(s)
      K. L. Ishikawa
    • Organizer
      Computational Chemistry Symposium of ICCMSE 2016
    • Place of Presentation
      Athens, Greece
    • Year and Date
      2016-03-17
    • Related Report
      2015 Research-status Report
    • Int'l Joint Research / Invited
  • [Presentation] 高強度レーザー場中の多電子ダイナミクス2016

    • Author(s)
      佐藤健、石川顕一
    • Organizer
      電気学会 光・量子デバイス研究会
    • Place of Presentation
      富山県氷見市
    • Year and Date
      2016-01-24
    • Related Report
      2015 Research-status Report
  • [Presentation] 強光子場第一原理シミュレーションへの外部複素スケーリングの実装2016

    • Author(s)
      織茂悠貴、佐藤健、澤田亮人、石川顕一
    • Organizer
      レーザー学会学術講演会第36回年次大会
    • Place of Presentation
      名城大学天白キャンパス
    • Year and Date
      2016-01-11
    • Related Report
      2015 Research-status Report
  • [Presentation] Multi resolution MCTDHFによる高強度レーザーパルス下での分子計算2016

    • Author(s)
      澤田亮人、佐藤健、石川顕一
    • Organizer
      レーザー学会学術講演会第36回年次大会
    • Place of Presentation
      名城大学天白キャンパス
    • Year and Date
      2016-01-11
    • Related Report
      2015 Research-status Report
  • [Presentation] 非対称な系へのMulti-resolution MCTDHFの適用2015

    • Author(s)
      澤田亮人、佐藤健、石川顕一
    • Organizer
      第76回応用物理学会秋季学術講演会
    • Place of Presentation
      名古屋国際会議場
    • Year and Date
      2015-09-13
    • Related Report
      2015 Research-status Report
  • [Presentation] Time-dependent multiconfiguration self-consistent-field methods for multielectron dynamics in intense laser fields2015

    • Author(s)
      T. Sato and K. Ishikawa
    • Organizer
      XXIX International Conference on Photonic, Electronic, and Atomic Collisions (ICPEAC 2015)
    • Place of Presentation
      Toledo, Spain
    • Year and Date
      2015-07-22
    • Related Report
      2015 Research-status Report
    • Int'l Joint Research
  • [Presentation] Bohmian-trajectory Analysis of Enhanced Ionization of Molecules in Intense Laser Fields2015

    • Author(s)
      Ryohto Sawada, Takeshi Sato, Kenichi Ishikawa
    • Organizer
      CLEO-Europe 2015
    • Place of Presentation
      Munich, Germany
    • Year and Date
      2015-06-21
    • Related Report
      2015 Research-status Report
    • Int'l Joint Research
  • [Presentation] Multi Resolution TDSE/MCTDHF の開発2015

    • Author(s)
      澤田亮人、佐藤健、石川顕一
    • Organizer
      第62回応用物理学会春季学術講演会
    • Place of Presentation
      東海大学、神奈川県
    • Year and Date
      2015-03-11 – 2015-03-14
    • Related Report
      2014 Research-status Report
  • [Presentation] ボーム経路解析による高強度場現象の計算シミュレーション2014

    • Author(s)
      澤田亮人、佐藤健、石川顕一
    • Organizer
      第75回応用物理学会秋季学術講演会
    • Place of Presentation
      北海道大学、北海道
    • Year and Date
      2014-09-17 – 2014-09-20
    • Related Report
      2014 Research-status Report
    • Invited
  • [Presentation] Enhanced ionization のボーム経路解析2014

    • Author(s)
      澤田亮人、佐藤健、石川顕一
    • Organizer
      日本物理学会 2014 年 秋季大会
    • Place of Presentation
      中央大学、愛知県
    • Year and Date
      2014-09-07 – 2014-09-10
    • Related Report
      2014 Research-status Report
  • [Presentation] Bohmian-trajectory analysis of enhanced ionization of molecules in intense laser fields2014

    • Author(s)
      R. Sawada, T. Sato, K.L. Ishikawa
    • Organizer
      International workshop on theory for attsecond quantum dynamics
    • Place of Presentation
      電気通信大学、東京都
    • Year and Date
      2014-06-30
    • Related Report
      2014 Research-status Report
    • Invited
  • [Book] アト秒科学~1京分の1秒スケールの超高速現象を光で観測・制御する~2015

    • Author(s)
      大森賢治、石井順久、石川顕一、板谷治郎、香月浩之、森下亨、渡部俊太郎
    • Total Pages
      200
    • Publisher
      化学同人
    • Related Report
      2015 Research-status Report
  • [Remarks] 論文一覧

    • URL

      http://www.atto.t.u-tokyo.ac.jp/report/list/

    • Related Report
      2016 Annual Research Report
  • [Remarks] 東京大学 石川研究室の論文一覧

    • URL

      http://www.atto.t.u-tokyo.ac.jp/report/list/

    • Related Report
      2015 Research-status Report 2014 Research-status Report

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Published: 2014-04-04   Modified: 2018-03-22  

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