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Development of Post-ionization method for next-generatino in-situ U-Pb dating mass spectrometer

Research Project

Project/Area Number 26610183
Research Category

Grant-in-Aid for Challenging Exploratory Research

Allocation TypeMulti-year Fund
Research Field Geochemistry/Cosmochemistry
Research InstitutionOsaka University

Principal Investigator

Terada Kentaro  大阪大学, 理学(系)研究科(研究院), 教授 (20263668)

Co-Investigator(Kenkyū-buntansha) 石原 盛男  大阪大学, 理学(系)研究科(研究院), 准教授 (30294151)
中村 亮介  大阪大学, 産学連携本部, 講師 (70379147)
豊田 岐聡  大阪大学, 理学(系)研究科(研究院), 教授 (80283828)
青木 順  大阪大学, 理学(系)研究科(研究院), 助教 (90452424)
Project Period (FY) 2014-04-01 – 2016-03-31
Project Status Completed (Fiscal Year 2015)
Budget Amount *help
¥3,640,000 (Direct Cost: ¥2,800,000、Indirect Cost: ¥840,000)
Fiscal Year 2015: ¥1,820,000 (Direct Cost: ¥1,400,000、Indirect Cost: ¥420,000)
Fiscal Year 2014: ¥1,820,000 (Direct Cost: ¥1,400,000、Indirect Cost: ¥420,000)
Keywords局所分析 / 太陽系年代学 / 年代測定 / 同位体 / 局所同位体分析 / 隕石 / SIMS
Outline of Final Research Achievements

Secondary Ion Mass Spectrometers (SIMSs), which have high spacial resolution (1~10 micron), have been used for isotopic measurement of individual minerals and/or presolar grains. The weakest point of this analytical method is that secondary ion yield is very low (less than 1 %). As a result, a large amount of sputtered atoms and molecules that are neutral are wasted.
To overcome this weakness of SIMSs, we adopted the post-ionization method using high-intensity laser, and have developed a multi-turned TOF-SIMS with a femto-second laser for post-ionization. By optimizing the timing of irradiation/acceralation and/or position of laser, we currently attain the multiplication factor of c.a. 10000. As a result, we succeeded in detection of U and Pb ions from natural zircon of which U concentration is about 100 ppm.

Report

(3 results)
  • 2015 Annual Research Report   Final Research Report ( PDF )
  • 2014 Research-status Report
  • Research Products

    (12 results)

All 2016 2015 2014 Other

All Journal Article (1 results) (of which Peer Reviewed: 1 results,  Open Access: 1 results) Presentation (10 results) (of which Int'l Joint Research: 2 results) Remarks (1 results)

  • [Journal Article] A new X-ray fluorescence spectroscopy for extraterrestrial materials using a muon beam.2014

    • Author(s)
      K. Terada, K. Ninomiya, T. Osawa, S. Tachibana, Y. Miyake, M. K. Kubo6, N. Kawamura, W. Higemoto, A. Tsuchiyama, M. Ebihara and M. Uesugi
    • Journal Title

      Scientific Reports

      Volume: 4 Issue: 1 Pages: 5072-5077

    • DOI

      10.1038/srep05072

    • Related Report
      2014 Research-status Report
    • Peer Reviewed / Open Access
  • [Presentation] DEVELOPMENT ON MULTI-TURNED TOF SIMS WITH A FEMTO-SECOND LASER FOR POST-IONIZATION: FIRST APPICATION TO EXTRATERRESTRIAL MATERIALS2016

    • Author(s)
      Terada, K., Kawai, Y., Toyoda, M., Ishihara, M., Aoki, J., Yabuta, H., Suwa, T. and Nakamura, R.
    • Organizer
      47th Lunar and Planetary Science Conference
    • Place of Presentation
      ヒューストン(米国)
    • Year and Date
      2016-03-21
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research
  • [Presentation] サブミクロン局所同位体分析に向けたレーザーポストイオン化SNMSの開発2015

    • Author(s)
      河井 洋輔, 寺田 健太郎, 上岡 萌, 諏訪 太一, 松田 貴博, 豊田 岐聡, 石原 盛男, 青木 順, 中村 亮介
    • Organizer
      日本惑星科学会2015年秋季講演会
    • Place of Presentation
      東京工業大学大(東京都・目黒区)
    • Year and Date
      2015-10-14
    • Related Report
      2015 Annual Research Report
  • [Presentation] 局所同位体分析に向けたポストレーザーイオン化SNMSの開発2015

    • Author(s)
      河井 洋輔, 寺田 健太郎, 上岡 萌, 諏訪 太一, 松田 貴博, 豊田 岐聡, 石原 盛男, 青木 順, 中村 亮介
    • Organizer
      2015年度日本地球化学会第62回年会
    • Place of Presentation
      横浜国立大学(神奈川県・横浜市)
    • Year and Date
      2015-09-16
    • Related Report
      2015 Annual Research Report
  • [Presentation] Development on the Post-Ionization method for next-generation SIMS2015

    • Author(s)
      Terada, K., Kawai, Y., Toyoda, M., Ishihara, M., Aoki, J., Nakamura, R.
    • Organizer
      Japan-Korea SHRIMP workshop
    • Place of Presentation
      広島大学(広島県・東広島市)
    • Year and Date
      2015-09-14
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 局所同位体分析に向けたポストレーザーイオン化SNMSの開発2015

    • Author(s)
      河井 洋輔, 寺田 健太郎, 上岡 萌, 諏訪 太一, 豊田 岐聡, 石原 盛男, 青木 順, 中村 亮介
    • Organizer
      第63回質量分析総合討論
    • Place of Presentation
      つくば国際会議場(茨城県・つくば市)
    • Year and Date
      2015-06-17
    • Related Report
      2015 Annual Research Report
  • [Presentation] レーザーポストイオン化SNMSを用いたプレソーラーSiCの同位体分析手法の開発2015

    • Author(s)
      諏訪 太一, 寺田 健太郎, 河井 洋輔, 薮田 ひかる, 豊田 岐聡, 石原 盛男, 青木 順
    • Organizer
      日本地球惑星科学連合2015年大会
    • Place of Presentation
      幕張メッセ国際会議場(千葉県・千葉市)
    • Year and Date
      2015-05-22
    • Related Report
      2015 Annual Research Report
  • [Presentation] 局所U-Pb年代分析にむけたポストイオン化SNMSの 開発2014

    • Author(s)
      上岡萌ほか
    • Organizer
      日本地球化学会
    • Place of Presentation
      富山大学
    • Year and Date
      2014-09-28
    • Related Report
      2014 Research-status Report
  • [Presentation] フェムト秒レーザーによる ポストイオン化SNMSの開発2014

    • Author(s)
      寺田健太郎ほか
    • Organizer
      第11回原子・分子・光科学(AMO)討論会
    • Place of Presentation
      豊中市
    • Year and Date
      2014-06-06
    • Related Report
      2014 Research-status Report
  • [Presentation] レーザーイオン化SNMSによる局所U-Pb年代分析法の開発2014

    • Author(s)
      寺田健太郎ほか
    • Organizer
      質量分析討論会
    • Place of Presentation
      吹田市
    • Year and Date
      2014-05-14 – 2014-05-16
    • Related Report
      2014 Research-status Report
  • [Presentation] サブミクロン局所U-Pb年代分析に向けた レーザーイオン化SNMSの開発2014

    • Author(s)
      寺田健太郎ほか
    • Organizer
      連合大会
    • Place of Presentation
      横浜市
    • Year and Date
      2014-04-28 – 2014-05-02
    • Related Report
      2014 Research-status Report
  • [Remarks] 超高感度極微量質量分析装置 (MULTUM-SNMS) の開発

    • URL

      http://planet.ess.sci.osaka-u.ac.jp/contents/research/research3.html

    • Related Report
      2015 Annual Research Report

URL: 

Published: 2014-04-04   Modified: 2017-05-10  

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