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Photocatalytic CO2 reduction on Solid-Gas Interface: CO2 reduction films

Research Project

Project/Area Number 26620166
Research Category

Grant-in-Aid for Challenging Exploratory Research

Allocation TypeMulti-year Fund
Research Field Organic and hybrid materials
Research InstitutionNiigata University

Principal Investigator

Tatstuto Yui  新潟大学, 自然科学系, 准教授 (50362281)

Project Period (FY) 2014-04-01 – 2017-03-31
Project Status Completed (Fiscal Year 2016)
Budget Amount *help
¥3,640,000 (Direct Cost: ¥2,800,000、Indirect Cost: ¥840,000)
Fiscal Year 2016: ¥910,000 (Direct Cost: ¥700,000、Indirect Cost: ¥210,000)
Fiscal Year 2015: ¥1,690,000 (Direct Cost: ¥1,300,000、Indirect Cost: ¥390,000)
Fiscal Year 2014: ¥1,040,000 (Direct Cost: ¥800,000、Indirect Cost: ¥240,000)
Keywords膜状触媒 / CO2還元 / 新エネルギー / 層状半導体 / 金属錯体 / 界面化学 / 光触媒 / 半導体膜 / 金属ナノ粒子 / 固体膜 / レニウム錯体
Outline of Final Research Achievements

Synthesis of layered metal oxide semiconductors (LMOSs) and metal complexes, e.g. rhenium complexes, were investigated with the aim of constructing a CO2 reduction photocatalyst that can work under the gas phase. LMOSs have a stacking structure of the planner-shaped semiconductor crystals with several angstrom thick. LMOSs enable to produce a film structured and synergistic catalysts by modifying the functional molecules or chemical species. Among them, the following investigations were carried out on the hybrids of the LMOSs and various functional chemical species, and the following results were obtained. 1) Synthesis of transparent LMOS thin films, 2) Synthesis of metal particles within the interlayer space of the LMOS thin film, and 3) Synthesis of the powdered LMOSs and rhenium complexes. We will report details of these research results.

Report

(4 results)
  • 2016 Annual Research Report   Final Research Report ( PDF )
  • 2015 Research-status Report
  • 2014 Research-status Report
  • Research Products

    (31 results)

All 2017 2016 2015 2014

All Journal Article (8 results) (of which Peer Reviewed: 5 results,  Open Access: 2 results,  Acknowledgement Compliant: 3 results) Presentation (20 results) (of which Int'l Joint Research: 5 results,  Invited: 5 results) Book (3 results)

  • [Journal Article] In Situ Synthesis of Gold Nanoparticles without Aggregation in the Interlayer Space of Layered Titanate Transparent Films2017

    • Author(s)
      Sasaki, Kazuhisa Matsubara, Kazuki Kawamura, Shiori Saito, Kenji Yagi, Masayuki Yui, Tatsuto
    • Journal Title

      Journal of Visualized Experiments

      Volume: 119 Issue: 119 Pages: 1-10

    • DOI

      10.3791/55169

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Open Access / Acknowledgement Compliant
  • [Journal Article] Color tuning of cationic pyrene derivatives on a clay nanosheet: Retardation of gradual redshift on clay2017

    • Author(s)
      D. Morimoto, K. Sato, K. Saito, M. Yagi, S. Takagi, T. Yui
    • Journal Title

      J. Photochem. Photobiol., A, Chem.

      Volume: 337 Pages: 112-117

    • DOI

      10.1016/j.jphotochem.2017.01.023

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Light energy accumulation from pyrene derivative to tris(bipyridine)ruthenium on clay surface2017

    • Author(s)
      D. Morimoto, H. Yoshida, K. Sato, K. Saito, M. Yagi, S. Takagi, T. Yui
    • Journal Title

      Langmuir

      Volume: 印刷中 Issue: 15 Pages: 3680-3684

    • DOI

      10.1021/acs.langmuir.7b00512

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] 層状半導体薄膜を用いた光CO2還元触媒の構築2017

    • Author(s)
      由井樹人・斎藤弘夢・酒井創太郎・吉田晴也
    • Journal Title

      (財)日本板硝子材料工学助成会

      Volume: 印刷中

    • Related Report
      2016 Annual Research Report
  • [Journal Article] Synthesis of Copper Nanoparticles within the Interlayer Space of Titania Nanosheet Transparent Films2016

    • Author(s)
      Sasaki, K.; Matsubara, K.; Kawamura, S.; Saito, K.; Yagi, M.; Yui, T.
    • Journal Title

      J. Mater. Chem. C

      Volume: 4 Issue: 7 Pages: 1476-1481

    • DOI

      10.1039/c5tc03152d

    • Related Report
      2015 Research-status Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] 電荷分離状態の長寿命化と二酸化炭素の光資源化2015

    • Author(s)
      由井樹人、高木文彰、足立崇、斎藤弘夢
    • Journal Title

      ケミカルエンジニヤリング(化学工業社)

      Volume: 60 Pages: 779-783

    • NAID

      40020601295

    • Related Report
      2015 Research-status Report
  • [Journal Article] 人工光合成系構築に向けた光捕集システムと光CO2還元系の融合2015

    • Author(s)
      由井樹人、石谷治
    • Journal Title

      光有機材料・デバイス分科会光産業 2014技術動向調査

      Volume: なし Pages: 37-40

    • Related Report
      2015 Research-status Report
  • [Journal Article] A Novel Type of CO2 Reduction Photocatalyst with Visible-Light Harvesting Function2015

    • Author(s)
      Ueda, Y.; Takeda, H.; Yui, T.; Koike, K.; Goto, Y.; Inagaki, S.; Ishitani, O.
    • Journal Title

      ChemSusChem

      Volume: 8 Issue: 3 Pages: 439-442

    • DOI

      10.1002/cssc.201403194

    • Related Report
      2014 Research-status Report
    • Peer Reviewed / Open Access
  • [Presentation] Synthesis and Characterization of Metal Nanoparticle / Layered Semiconductor Hybrids2017

    • Author(s)
      Tatsuto Yui, Sotaro Sakai, Hiromu Saito, Wataru Norimatsu
    • Organizer
      International Conference on Materials and Systems for Sustainability 2017
    • Place of Presentation
      Nagoya University (Aichi, Nagoya, Jpn.)
    • Year and Date
      2017-09-30
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research
  • [Presentation] In-situ Synthesis of Metal Nanoparticles within the Interlayer Space of Inorganic Layered Material Transparent Films2017

    • Author(s)
      Tatsuto YUI, Shiori KAWAMURA, Kazuhisa SASAKI, Sotaro SAKAI, and Hiromu SAITO
    • Organizer
      International Symposium on Pure & Applied Chemistry
    • Place of Presentation
      Hotel Continental Saigon (Ho Chi Minh, Vietnam)
    • Year and Date
      2017-06-08
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] 層状化合物をテンプレートとする金属ナノ粒子の合成2017

    • Author(s)
      由井樹人
    • Organizer
      日本化学会低次元系光機能材料研究会 第6 回研究講演会
    • Place of Presentation
      化学会館(東京・千代田区)
    • Related Report
      2016 Annual Research Report
    • Invited
  • [Presentation] 無機層状化合物層間を利用した銀ナノ粒子の合成と特異挙動2016

    • Author(s)
      酒井創太郎・河村栞里・佐々木和久・齊藤健二・由井樹人
    • Organizer
      2016年光化学討論会
    • Place of Presentation
      東京大学(東京・目黒区)
    • Year and Date
      2016-09-06
    • Related Report
      2016 Annual Research Report
  • [Presentation] 配位化合物と無機層状化合物からなる複合系の特異的な光化学挙動2016

    • Author(s)
      由井樹人
    • Organizer
      第28回配位化合物の光化学討論会
    • Place of Presentation
      京都繊維工大(京都府・京都市)
    • Year and Date
      2016-08-08
    • Related Report
      2016 Annual Research Report
  • [Presentation] 光化学の基礎と人工光合成反応の課題2016

    • Author(s)
      由井樹人
    • Organizer
      公益法人新化学技術推進協会(JACI), 先端化学・材料技術部会 高選択性反応分科会講演会
    • Place of Presentation
      JACI会議室(東京・千代田区)
    • Related Report
      2016 Annual Research Report
    • Invited
  • [Presentation] X線を用いたラメラ積層体の構造解析2016

    • Author(s)
      由井樹人
    • Organizer
      第4回 機器分析センター研究会
    • Place of Presentation
      新潟大学VBL (新潟・新潟市)
    • Related Report
      2016 Annual Research Report
    • Invited
  • [Presentation] Synthesis of metal nanoparticles within interlayer space of titania nanosheet film2015

    • Author(s)
      K. Sasaki, K. Matsubara, S. Kawamura, K. Saito, M. Yagi, W. Norimatsu, R. Sasai, T. Yui
    • Organizer
      The International Chemcal Congress of Pacific Basin Societies 2015
    • Place of Presentation
      Honolulu, Hawai, USA
    • Year and Date
      2015-12-15
    • Related Report
      2015 Research-status Report
    • Int'l Joint Research
  • [Presentation] Synthesis of silver nanoparticle within interlayer space of layered semiconductor2015

    • Author(s)
      S. Kawamura, K. Sasaki, F. Takagi, K. Saito, M. Yagi, W. Norimatsu, R. Sasai, T. Yui
    • Organizer
      The International Chemcal Congress of Pacific Basin Societies 2015
    • Place of Presentation
      Honolulu, Hawai, USA
    • Year and Date
      2015-12-15
    • Related Report
      2015 Research-status Report
    • Int'l Joint Research
  • [Presentation] K4Nb6O17層間へのRe錯体の導入2015

    • Author(s)
      高木文彰・由井樹人
    • Organizer
      低次元系光機能研究会第4回サマーセミナー
    • Place of Presentation
      大阪市立大、大阪市
    • Year and Date
      2015-09-25
    • Related Report
      2015 Research-status Report
  • [Presentation] 層状半導体と金属ナノ粒子複合体の合成と光化学特性2015

    • Author(s)
      由井樹人・河村栞里・佐々木和久・高木文彰・齊藤健二・八木政行・乗松航・笹井亮
    • Organizer
      2015年光化学討論会
    • Place of Presentation
      大阪市立大学、大阪市
    • Year and Date
      2015-09-09
    • Related Report
      2015 Research-status Report
  • [Presentation] 層状半導体層間での銀ナノ粒子の合成と近赤外吸収特性2015

    • Author(s)
      河村栞里・佐々木和久・髙木文彰・笹井亮・乗松航・齊藤健二・八木政行・由井樹人
    • Organizer
      2015年光化学討論会
    • Place of Presentation
      大阪市立大学、大阪市
    • Year and Date
      2015-09-09
    • Related Report
      2015 Research-status Report
  • [Presentation] Unique Photochemical Properties of Inorganic Nanosheet and Coordination Compound Hybrid Materials2015

    • Author(s)
      Tatsuto Yui
    • Organizer
      4th International Mini-Symposium on Coordination Chemistry for Advanced Materials
    • Place of Presentation
      Aoyama Gakuin University (Tokyo)
    • Year and Date
      2015-04-10
    • Related Report
      2015 Research-status Report
    • Int'l Joint Research / Invited
  • [Presentation] Synthesis of Metal Nanoparticle within Interlayer Space of Layered Compounds and their Spectroscopic Studies2014

    • Author(s)
      K. Sasaki, S. Kawamura, F. Takagi, and T. Yui
    • Organizer
      The 10th SPSJ International Polymer Conference (ICP2014)
    • Place of Presentation
      Tsukuba, Ibaraki
    • Year and Date
      2014-12-02 – 2014-12-06
    • Related Report
      2014 Research-status Report
  • [Presentation] 層状半導体をテンプレートとする銅ナノ粒子の合成と光物性2014

    • Author(s)
      佐々木和久・河村栞里・松原一喜・齊藤健二・八木政行・由井樹人
    • Organizer
      2014年光化学討論会
    • Place of Presentation
      北海道大学
    • Year and Date
      2014-10-11 – 2014-10-13
    • Related Report
      2014 Research-status Report
  • [Presentation] ナノ構造積層膜の光化学挙動2014

    • Author(s)
      向井祥吾・佐藤充啓・松原一喜・齊藤健二・八木政行・由井樹人
    • Organizer
      2014年光化学討論会
    • Place of Presentation
      北海道大学
    • Year and Date
      2014-10-11 – 2014-10-13
    • Related Report
      2014 Research-status Report
  • [Presentation] チタニアナノシート/銀微小粒子複合膜の合成2014

    • Author(s)
      河村栞里・佐々木和久・齊藤健二・八木政行・由井樹人
    • Organizer
      低次元系光機能研究会第3回サマーセミナー
    • Place of Presentation
      佐渡島 グリーンホテルきらく
    • Year and Date
      2014-09-02 – 2014-09-03
    • Related Report
      2014 Research-status Report
  • [Presentation] 層状半導体の層空間を用いた金属ナノ粒子の合成と特性評価2014

    • Author(s)
      佐々木和久・松原一喜・齊藤健二・八木政行・由井樹人
    • Organizer
      低次元系光機能研究会第3回サマーセミナー
    • Place of Presentation
      佐渡島 グリーンホテルきらく
    • Year and Date
      2014-09-02 – 2014-09-03
    • Related Report
      2014 Research-status Report
  • [Presentation] 無機ナノ積層膜中におけるポルフィリンの光化学挙動2014

    • Author(s)
      佐藤充啓・松原一喜・齊藤健二・八木政行・由井樹人
    • Organizer
      低次元系光機能研究会第3回サマーセミナー
    • Place of Presentation
      佐渡島 グリーンホテルきらく
    • Year and Date
      2014-09-02 – 2014-09-03
    • Related Report
      2014 Research-status Report
  • [Presentation] SYNTHESES OF METAL NANOPARTICLES WITHIN INTERLAYER SPACE OF LAYERED SEMICONDUCTOR2014

    • Author(s)
      Kazuhisa Sasaki, Shiori Kawamura, Fumiaki Takagi, Kenji Saito, Masayuki Yagi, and Tatsuto Yui
    • Organizer
      XXV IUPAC Symposium on Photochemistry
    • Place of Presentation
      Bordeaux
    • Year and Date
      2014-07-13 – 2014-07-18
    • Related Report
      2014 Research-status Report
  • [Book] Dojin Bioscience series; 光合成のエネルギー・物質変換 - 人工光合成を目指して2015

    • Author(s)
      由井樹人・石谷治
    • Total Pages
      288
    • Publisher
      化学同人
    • Related Report
      2015 Research-status Report
  • [Book] 人工光合成による二酸化炭素還元と光資源化2015

    • Author(s)
      由井樹人・石谷治
    • Total Pages
      281
    • Publisher
      東京化学同人
    • Related Report
      2014 Research-status Report
  • [Book] 化学の要点シリーズ~層間化合物~2014

    • Author(s)
      松原一喜・由井樹人
    • Total Pages
      103
    • Publisher
      共立出版
    • Related Report
      2014 Research-status Report

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Published: 2014-04-04   Modified: 2018-03-22  

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