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Development of micrometer-scaled ion beam analysis technique for the evaluation of environmental dynamics of individual aerosol particles

Research Project

Project/Area Number 26706025
Research Category

Grant-in-Aid for Young Scientists (A)

Allocation TypePartial Multi-year Fund
Research Field Quantum beam science
Research InstitutionGunma University

Principal Investigator

Kada Wataru  群馬大学, 大学院理工学府, 助教 (60589117)

Project Period (FY) 2014-04-01 – 2017-03-31
Project Status Completed (Fiscal Year 2016)
Budget Amount *help
¥24,570,000 (Direct Cost: ¥18,900,000、Indirect Cost: ¥5,670,000)
Fiscal Year 2016: ¥3,250,000 (Direct Cost: ¥2,500,000、Indirect Cost: ¥750,000)
Fiscal Year 2015: ¥3,900,000 (Direct Cost: ¥3,000,000、Indirect Cost: ¥900,000)
Fiscal Year 2014: ¥17,420,000 (Direct Cost: ¥13,400,000、Indirect Cost: ¥4,020,000)
KeywordsIBIL / 荷電粒子誘起発光 / イオンマイクロビーム / 化学形態分析 / イメージング / PIXE / エアロゾル / イオンビーム誘起発光 / スペクトロスコピー / 環境動態解析
Outline of Final Research Achievements

In this study, we have developed a new ion beam analytical technology of charged particle induced luminescence(IBIL) for individual analysis of airborne particles. IBIL has the possibility to visualize the distribution of organic and inorganics in compounds or on the surface of particles in scale of several micrometers. To enhance its applicability under general microbeam scanning condition, we developed a high resolution type visible light detector based on photo-multiplier tube array. Continuous analysis of IBIL disclosed significant change in the emission wavelength of IBIL from particulate targets as well as organic standards. Based on these experimental results, IBIL spectroscopy and imaging technique enabled to analyze or identify the chemical composition and changes in micrometer-scale targets.

Report

(4 results)
  • 2016 Annual Research Report   Final Research Report ( PDF )
  • 2015 Annual Research Report
  • 2014 Annual Research Report
  • Research Products

    (34 results)

All 2017 2016 2015 2014

All Journal Article (12 results) (of which Peer Reviewed: 10 results,  Acknowledgement Compliant: 11 results,  Open Access: 1 results) Presentation (19 results) (of which Int'l Joint Research: 7 results,  Invited: 1 results) Patent(Industrial Property Rights) (3 results) (of which Overseas: 1 results)

  • [Journal Article] Development of a high-speed wavelength-dispersive IBIL analysis and imaging system using a multi-channel photon-counting spectrometer2017

    • Author(s)
      Wataru Kada, Shunsuke Kawabata, Takahiro Satoh, Raj Kumar Parajuli, Naoto Yamada, Masashi Koka, Kenta Miura, Osamu Hanaizumi, Tomihiro Kamiya
    • Journal Title

      Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms

      Volume: 印刷中

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Observation of changes in ion beam induced luminescence spectra from organics during focused microbeam irradiation2017

    • Author(s)
      Wataru Kada, Shunsuke Kawabata, Takahiro Satoh, Makoto Sakai, Raj Kumar Parajuli, Naoto Yamada, Masashi Koka, Kenta Miura, Osamu Hanaizumi, Tomihiro Kamiya
    • Journal Title

      Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms

      Volume: 印刷中 Pages: 100-105

    • DOI

      10.1016/j.nimb.2017.01.025

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Micro-PIXE analysis and imaging of radio-photoluminescence glass bead microdosimeters2017

    • Author(s)
      S. Kawabata, W. Kada, Y. Matsubara, T. Satoh, M. Sakai, R.K. Parajuli, N. Yamada, M. Koka, K. Miura, O. Hanaizumi, T. Kamiya
    • Journal Title

      Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms

      Volume: 印刷中 Pages: 139-143

    • DOI

      10.1016/j.nimb.2017.04.017

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Electrode Spacing Effect on Ultraviolet Photoconductivity of Metal-Semiconductor-Metal Detectors with ZnO Nanorod Arrays Grown by Hydrothermal Method2016

    • Author(s)
      R. K. Parajuli, W. Kada, S. Kawabata, Y. Matsubara, M. Sakai, K. Miura, T. Satoh, M. Koka, N. Yamada, T. Kamiya, and O. Hanaizumi
    • Journal Title

      Sensors and Materials

      Volume: 28 Pages: 1

    • DOI

      10.18494/SAM.2016.1242

    • ISSN
      0914-4935, 2435-0869
    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Open Access / Acknowledgement Compliant
  • [Journal Article] 鉱物内部の微視的な化学組成分布可視化のためのイオンマイクロビーム誘起 発光分析法の開発2016

    • Author(s)
      加田 渉, 川端駿介, Parajuli Raj Kumar, 江夏昌志, 山田尚人, 横山彰人, 佐藤隆博, 三浦健太, 神谷富裕, 花泉修
    • Journal Title

      Geo-Pollution Science, Medical Geology and Urban Geology

      Volume: 12 Pages: 5-9

    • NAID

      40021464907

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Ionoluminescence analysis of glass scintillators and application to single-ion-hit real-time detection2016

    • Author(s)
      A. Yokoyama, W. Kada, T. Satoh, M. Koka, K. Shimada, Y. Yokoata, K. Miura, and O. Hanaizumi
    • Journal Title

      Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms

      Volume: 371 Pages: 340-343

    • DOI

      10.1016/j.nimb.2015.10.024

    • Related Report
      2015 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Evaluation of Radio-photoluminescence Spectra of Copper-doped Phosphate Glass Dosimeter Irradiated with Ionized Particles2016

    • Author(s)
      R. K. Parajuli, W. Kada, S. Kawabata, Y. Matsubara, K. Miura, A. Yokoyama, M. Haruyama, M. Sakai, and O. Hanaizumi
    • Journal Title

      Key Engineering and Materials

      Volume: 698 Pages: 163-170

    • DOI

      10.4028/www.scientific.net/kem.698.163

    • Related Report
      2015 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] In situ ion-beam-induced luminescence analysis for evaluating a micrometer-sized radio-photoluminescence glass dosimeter2016

    • Author(s)
      S. Kawabata, W. Kada, R. K. Parajuli, Y. Matsubara, K. Miura, T. Satoh, M. Koka, N. Yamada, T. Kamiya, and O. Hanaizumi
    • Journal Title

      Japanese Journal of Applied Physics

      Volume: 55

    • Related Report
      2015 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Continuous observation of ion beam induced luminescence spectra from organic standard targets2015

    • Author(s)
      W. Kada, A. Yokoyama, M. Koka, K. Miura, T. Satoh, O. Hanaizumi and T. Kamiya
    • Journal Title

      International Journal of PIXE

      Volume: 25 Issue: 01n02 Pages: 127-134

    • DOI

      10.1142/s0129083515500138

    • Related Report
      2015 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Continuous Observation of Ion Beam Induced Luminescence Spectra from Organic Standard Targets2015

    • Author(s)
      Wataru Kada, Akihito Yokoyama, Masashi Koka, Kenta Miura, Takahiro Satoh, Osamu Hanaizumi, and Tomihiro Kamiya
    • Journal Title

      International Journal of PIXE

      Volume: -

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] イオンビーム励起発光を利用した分析技術の開発とその応用2015

    • Author(s)
      加田 渉、 横山 彰人、江夏 昌志、佐藤 隆博、神谷 富裕
    • Journal Title

      自動制御連合講演会講演論文集

      Volume: -

    • Related Report
      2014 Annual Research Report
    • Acknowledgement Compliant
  • [Journal Article] イオン励起発光顕微イメージング分光と大気マイクロPIXEを組み合わせたシステムによる大気中微粒子の分析2014

    • Author(s)
      加田 渉, 横山 彰人, 佐藤 隆博, 江夏 昌志, 神谷 富裕
    • Journal Title

      放射線と産業

      Volume: 136 Pages: 40-46

    • NAID

      40020125409

    • Related Report
      2014 Annual Research Report
  • [Presentation] 荷電粒子誘起発光分析を利用したミクロスケール粒子からの蛍光連続取得と大気中微粒子分析への応用2017

    • Author(s)
      加田渉, 川端 駿介, 佐藤 隆博, 江夏 昌志, 山田 尚人, 三浦 健太, 花泉修, 神谷 富裕
    • Organizer
      第10回大気バイオエアロゾルシンポジウム
    • Place of Presentation
      金沢大学サテライト・プラザ
    • Year and Date
      2017-02-19
    • Related Report
      2016 Annual Research Report
  • [Presentation] 微粒子や鉱物微小領域評価のためのイオンマイクロビーム発光連続分析技術2016

    • Author(s)
      加田渉, 川端駿介, 佐藤隆博, 江夏昌志, 山田尚人, 三浦健太1 神谷富裕, 村尾智, 花泉修
    • Organizer
      第26回環境地質学シンポジウム
    • Place of Presentation
      日本大学文理学部
    • Year and Date
      2016-11-25
    • Related Report
      2016 Annual Research Report
  • [Presentation] 荷電粒子誘起発光多波長同時分析・イメージングを目的とした フォトンカウンティング型分光器の開発2016

    • Author(s)
      加田 渉, 川端 駿介, 佐藤 隆博, 江夏 昌志, 山田 尚人, 三浦 健太, 花泉修, 神谷 富裕
    • Organizer
      第32回PIXEシンポジウム
    • Place of Presentation
      サン・リフレ函館(函館市勤労者総合福祉センター)
    • Year and Date
      2016-11-09
    • Related Report
      2016 Annual Research Report
  • [Presentation] Development of combined focused ion beam microprobe analysis and imaging techniques for chemical composition characterization of microscopic targets2016

    • Author(s)
      Wataru Kada, Shunsuke Kawabata, Takahiro Satoh, Masashi Koka, Naoto Yamada, Makoto Sakai, Parajuli Raj Kumar, Kenta Miura, Osamu Hanaizumi, and Tomihiro Kamiya
    • Organizer
      International Conference on Advanced Engineering and Its Education in 2016 (ICAEE16)
    • Place of Presentation
      Kiryu Chamber of Commerce and Industry, Keivick Hall
    • Year and Date
      2016-10-13
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Observation of the changes in IBIL spectra from organics during focused microbeam irradiation2016

    • Author(s)
      Wataru Kada, Shunsuke Kawabata, Takahiro Satoh, Makoto Sakai, Parajuli Raj Kumar, Naoto Yamada, Masashi Koka, Kenta Miura, Osamu Hanaizumi, and Tomihiro Kamiya
    • Organizer
      15th International Conference on Nuclear Microprobe Technology and Applications (ICNMTA2016)
    • Place of Presentation
      Institute of Modern Physics, Chinese Academy of Sciences (IMP-CAS) , Lanzhou, China
    • Year and Date
      2016-07-31
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Development of high-speed wavelength-dispersive IBIL analysis and imaging system using multi-channel photon-counting spectrometer2016

    • Author(s)
      Wataru Kada, Shunsuke Kawabata, Takahiro Satoh, Parajuli Raj Kumar, Naoto Yamada, Masashi Koka, Kenta Miura, Osamu Hanaizumi, and Tomihiro Kamiya
    • Organizer
      12th European Conference on Accelerators in Applied Research and Technology (ECAART12)
    • Place of Presentation
      University of Jyvaskyla
    • Year and Date
      2016-07-03
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Micro-PIXE analysis and imaging of Radio-photoluminescence glass beads dosimeter designed for micro-dosimetry2016

    • Author(s)
      Shunsuke Kawabata, Wataru Kada, Yoshinori Matsubra , Takahiro Satoh, Makoto Sakai, Parajuli Raj Kumar, Naoto Yamada, Masashi Koka, Kenta Miura, Osamu Hanaizumi, and Tomihiro Kamiya
    • Organizer
      12th European Conference on Accelerators in Applied Research and Technology (ECAART12)
    • Place of Presentation
      University of Jyvaskyla
    • Year and Date
      2016-07-03
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 集束イオンビームを利用した光材料開発と その場分析技術の開発2016

    • Author(s)
      加田渉
    • Organizer
      荷電粒子ビームの工業への応用第132委員会 第223回研究会
    • Place of Presentation
      東京理科大学森戸記念館
    • Related Report
      2016 Annual Research Report
  • [Presentation] Fabrication and in situ evaluation of integrated micro-optical devices by a focused proton microbeam technique2015

    • Author(s)
      W. Kada, R. Saruya, H. Kato, K. Miura, S. Kawabata, Y. Matsubara, P. Raj Kumar, A. Yokoyama, M. Koka, T. Satoh, Y. Ishii, T. Kamiya, H. Nishikawa, and O. Hanaizumi
    • Organizer
      International Symposium on Innovative Material Technologies Utilizing Ion Beams, The 25th annual meeting of MRS-J
    • Place of Presentation
      Industrial & trade center building, Yokohama, Japan
    • Year and Date
      2015-12-08
    • Related Report
      2015 Annual Research Report
    • Invited
  • [Presentation] Complex System of MicrometerSized Material Modification and In-Situ Elemental and Luminescence Analysis Using Proton Microbeam Probe2015

    • Author(s)
      S. Kawabata, W. Kada, Y.Matsubara, K. Miura, T. Satoh, M. Koka, N. Yamada, T. Kamiya, and O. Hanaizumi,
    • Organizer
      28th International Microprocesses and Nanotechnology Conference (MNC2015)
    • Place of Presentation
      Toyama International Conference Center, Toyama, Japan
    • Year and Date
      2015-11-10
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research
  • [Presentation] イオンマイクロビーム誘起発光分光装置を利用したβSiAlON:Euシンチレータの荷電粒子モニタとしての評価2015

    • Author(s)
      加田 渉、Raj Kumar Parajuli、川端 駿介、松原 良典、江夏 昌志、山田 尚人、 神谷 富裕、三浦 健太、 花泉 修
    • Organizer
      第31回 PIXEシンポジウム
    • Place of Presentation
      日本原子力研究開発機構高崎量子応用研究所、群馬
    • Year and Date
      2015-10-28
    • Related Report
      2015 Annual Research Report
  • [Presentation] イオンマイクロビーム誘起発光分光装置の開発とこれを利用した新規シンチレータの評価2015

    • Author(s)
      加田 渉,佐藤 隆博,川端 駿介, 江夏 昌志, 山田 尚人, 横山 彰人, 神谷 富裕, 三浦 健太, 花泉 修
    • Organizer
      第 9 回次世代先端光科学研究会
    • Place of Presentation
      静岡大学、静岡
    • Year and Date
      2015-09-24
    • Related Report
      2015 Annual Research Report
  • [Presentation] イオンマイクロビーム誘起発光分析による自作ガラス線量計素子の評価2015

    • Author(s)
      川端 駿介、加田 渉、松原 良典、三浦 健太、佐藤 隆博、江夏 昌志、山田 尚人、 神谷 富裕、花泉 修
    • Organizer
      2015 年(平成27 年) 第76 回応用物理学会秋季学術講演会
    • Place of Presentation
      名古屋国際会議場、愛知
    • Year and Date
      2015-09-13
    • Related Report
      2015 Annual Research Report
  • [Presentation] Radiation tolerability evaluation of SiAlON scintillator using Ion Beam Induced Luminescence (IBIL) Analysis2015

    • Author(s)
      R. K. Parajuli, S. Kawabata, Y. Matsubara, W. Kada, M. Sakai, K. Miura, T. Satoh, M. Koka, N. Yamada, T. Kamiya, and O. Hanaizumi
    • Organizer
      2015 年(平成27 年) 第76 回応用物理学会秋季学術講演会
    • Place of Presentation
      名古屋国際会議場、愛知
    • Year and Date
      2015-09-13
    • Related Report
      2015 Annual Research Report
  • [Presentation] Continuous observation of IBIL spectra obtained from microscopic targets2015

    • Author(s)
      W. Kada, T. Satoh, S. Kawabata, A. Yokoyama, M. Koka, N. Yamada, K. Miura, O. Hanaizumi ,and T. Kamiya
    • Organizer
      22nd International Conference on Ion Beam Analysis(IBA2015)
    • Place of Presentation
      Milenij Grand Hotel 4 opatijska cvijeta, Opatija, Croatia
    • Year and Date
      2015-06-14
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research
  • [Presentation] In-situ luminescence analysis and imaging of G2000 glass scintillator fabricated for real-time measurement of heavy ion microbeam2015

    • Author(s)
      A. Yokoyama, W. Kada, T. Satoh, M. Koka, K. Miura, and O. Hanaizumi
    • Organizer
      22nd International Conference on Ion Beam Analysis(IBA2015)
    • Place of Presentation
      Milenij Grand Hotel 4 opatijska cvijeta, Opatija, Croatia
    • Year and Date
      2015-06-14
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research
  • [Presentation] イオンマイクロビーム励起発光を利用した分析技術の開発とその応用2014

    • Author(s)
      加田渉,横山彰人,江夏昌志,佐藤隆博,神谷富裕
    • Organizer
      第57回自動制御連合講演会
    • Place of Presentation
      ホテル天坊,群馬県渋川市
    • Year and Date
      2014-11-10 – 2014-11-12
    • Related Report
      2014 Annual Research Report
  • [Presentation] イオン誘起発光分光による微量有機物分析の試み2014

    • Author(s)
      加田 渉, 佐藤 隆博,横山 彰人, 山田 尚人, 江夏 昌志, 神谷 富裕, 花泉 修
    • Organizer
      第30 回PIXE シンポジウム
    • Place of Presentation
      岩手医科大学附属循環器医療センター,岩手県盛岡市
    • Year and Date
      2014-10-22 – 2014-10-24
    • Related Report
      2014 Annual Research Report
  • [Presentation] 陽子マイクロビームプローブによるイオン誘起発光顕微分光分析 を可能にする高分解能顕微光学系の開発2014

    • Author(s)
      加田渉,横山彰人 ,江夏昌志, 山田 尚人, 佐藤隆博, 神谷富裕
    • Organizer
      第75回応用物理学会秋季学術講演会
    • Place of Presentation
      北海道大学,北海道札幌市
    • Year and Date
      2014-09-17 – 2014-09-20
    • Related Report
      2014 Annual Research Report
  • [Patent(Industrial Property Rights)] 荷電粒子放射線計測方法および荷電粒子放射線計測装置2017

    • Inventor(s)
      加田渉,三浦健太,花泉修,山田鈴弥,須崎純一,田中基
    • Industrial Property Rights Holder
      加田渉,三浦健太,花泉修,山田鈴弥,須崎純一,田中基
    • Industrial Property Rights Type
      特許
    • Industrial Property Number
      2017-036154
    • Filing Date
      2017-02-28
    • Related Report
      2016 Annual Research Report
  • [Patent(Industrial Property Rights)] 荷電粒子放射線計測方法および荷電粒子放射線計測装置2016

    • Inventor(s)
      加田渉,三浦健太,花泉修,神谷富裕,佐藤隆博,須崎純一,山田鈴弥
    • Industrial Property Rights Holder
      加田渉,三浦健太,花泉修,神谷富裕,佐藤隆博,須崎純一,山田鈴弥
    • Industrial Property Rights Type
      特許
    • Filing Date
      2016-08-25
    • Related Report
      2016 Annual Research Report
    • Overseas
  • [Patent(Industrial Property Rights)] 荷電粒子放射線計測方法および荷電粒子放射線計測装置2015

    • Inventor(s)
      加田渉 三浦健太 花泉修 神谷富裕 佐藤隆博 須崎純一 山田鈴弥
    • Industrial Property Rights Holder
      加田渉 三浦健太 花泉修 神谷富裕 佐藤隆博 須崎純一 山田鈴弥
    • Industrial Property Rights Type
      特許
    • Filing Date
      2015-08-28
    • Related Report
      2015 Annual Research Report

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Published: 2014-04-04   Modified: 2018-03-22  

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