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Hydrogen Production by Water Splitting Using Metallic Nanoparticle Composite Photoelectrode for Effective Utilization of Solar Energy

Research Project

Project/Area Number 26810105
Research Category

Grant-in-Aid for Young Scientists (B)

Allocation TypeMulti-year Fund
Research Field Energy-related chemistry
Research InstitutionNational Institute of Advanced Industrial Science and Technology

Principal Investigator

FUKU KOJIRO  国立研究開発法人産業技術総合研究所, 太陽光発電研究センター, 研究員 (10711765)

Project Period (FY) 2014-04-01 – 2016-03-31
Project Status Completed (Fiscal Year 2015)
Budget Amount *help
¥3,120,000 (Direct Cost: ¥2,400,000、Indirect Cost: ¥720,000)
Fiscal Year 2015: ¥1,430,000 (Direct Cost: ¥1,100,000、Indirect Cost: ¥330,000)
Fiscal Year 2014: ¥1,690,000 (Direct Cost: ¥1,300,000、Indirect Cost: ¥390,000)
Keywords光電極 / 水素 / 過酸化水素 / 水 / 太陽光 / 半導体 / 酸素 / ナノ粒子 / 太陽光エネルギー / 酸化物半導体 / 金属ナノ粒子 / LSPR誘起反応 / 高付加価値酸化生成物
Outline of Final Research Achievements

The production of hydrogen peroxide was investigated using water as the raw material to effectively utilize oxidative reactions in the photoelectrochemical production of hydrogen by water splitting. The oxidative production and accumulation of hydrogen peroxide were achieved with high photocurrent property and selectivity under irradiation of simulated solar light by combining a composite photoanode using bismuth vanadium oxide and electrolyte of hydrogen carbonate. Design of photoelectrode system specialized to production of hydrogen peroxide was also achieved by introducing reductive production of hydrogen peroxide from oxygen as a cathode reaction.

Report

(3 results)
  • 2015 Annual Research Report   Final Research Report ( PDF )
  • 2014 Research-status Report
  • Research Products

    (20 results)

All 2016 2015 2014

All Journal Article (2 results) (of which Peer Reviewed: 2 results,  Acknowledgement Compliant: 1 results) Presentation (14 results) (of which Int'l Joint Research: 4 results) Patent(Industrial Property Rights) (4 results)

  • [Journal Article] Efficient oxidative hydrogen peroxide production and accumulation in photoelectrochemical water splitting using a tungsten trioxide/bismuth vanadate photoanode2016

    • Author(s)
      Kojiro Fuku, Kazuhiro Sayama
    • Journal Title

      Chemical Communications

      Volume: 52 Issue: 31 Pages: 5406-5409

    • DOI

      10.1039/c6cc01605g

    • Related Report
      2015 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Photoelectrochemical Reaction for the Efficient Production of Hydrogen and High-Value-Added Oxidation Reagents2015

    • Author(s)
      Kojiro Fuku, Nini Wang, Yugo Miseki, Takashi Funaki, Kazuhiro Sayama
    • Journal Title

      ChemSusChem

      Volume: 印刷中 Issue: 9 Pages: 1593-1600

    • DOI

      10.1002/cssc.201403463

    • Related Report
      2014 Research-status Report
    • Peer Reviewed
  • [Presentation] 酸化反応において高選択的に過酸化水素を生成する光電極システムの設計2016

    • Author(s)
      宮瀬 雄太、福 康二郎、三石 雄悟、郡司 天博、佐山 和弘
    • Organizer
      日本化学会第96春季年会
    • Place of Presentation
      同志社大学 京田辺キャンパス(京都府・京田辺市)
    • Year and Date
      2016-03-25
    • Related Report
      2015 Annual Research Report
  • [Presentation] Photoelectrode system for the production of hydrogen and high-value-added oxidation reagents2015

    • Author(s)
      Kazuhiro Sayama, Kojiro Fuku, Yugo Miseki, Takashi Funaki
    • Organizer
      The International Chemical Congress of Pacific Basin Societies 2015 (Pacifichem)
    • Place of Presentation
      Hyatt Regency Waikiki, Honolulu, Hawaii, USA
    • Year and Date
      2015-12-20
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Design of photoelectrode system for oxidative production of hydrogen peroxide in water splitting2015

    • Author(s)
      Kojiro Fuku, Kazuhiro Sayama
    • Organizer
      The International Chemical Congress of Pacific Basin Societies 2015 (Pacifichem)
    • Place of Presentation
      Hyatt Regency Waikiki, Honolulu, Hawaii, USA
    • Year and Date
      2015-12-16
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 酸化物光電極システムにおける酸化反応の有効利用の検討2015

    • Author(s)
      宮瀬 雄太、福 康二郎、三石 雄悟、郡司 天博、佐山 和弘
    • Organizer
      第22回シンポジウム「光触媒反応の最近の展開」
    • Place of Presentation
      東京理科大学 野田キャンパス カナル会館(千葉県・野田市)
    • Year and Date
      2015-12-04
    • Related Report
      2015 Annual Research Report
  • [Presentation] 水を酸化して過酸化水素を製造できる光電極システムの設計2015

    • Author(s)
      福 康二郎、佐山 和弘
    • Organizer
      第116回触媒討論会
    • Place of Presentation
      三重大学(三重県・津市)
    • Year and Date
      2015-09-17
    • Related Report
      2015 Annual Research Report
  • [Presentation] 光電極を用いた水素製造をともなう過酸化物合成2015

    • Author(s)
      宮瀬 雄太、福 康二郎、三石 雄悟、郡司 天博、佐山 和弘
    • Organizer
      第116回触媒討論会
    • Place of Presentation
      三重大学(三重県・津市)
    • Year and Date
      2015-09-16
    • Related Report
      2015 Annual Research Report
  • [Presentation] Oxidative production of peroxides using WO3/BiVO4 photoanode2015

    • Author(s)
      Yuta Miyase, Kojiro Fuku, Yugo Miseki, Takahiro Gunji, Kazuhiro Sayama
    • Organizer
      First International Symposium on Recent Progress of Energy and Environmental Photocatalysis (Photocatalysis 1)
    • Place of Presentation
      東京理科大学 野田キャンパス カナル会館(千葉県・野田市)
    • Year and Date
      2015-09-03
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Efficient production of hydrogen peroxide using BiVO4 photoelectrode for effective utilization of oxidative reaction in water splitting2015

    • Author(s)
      Kojiro Fuku, Kazuhiro Sayama
    • Organizer
      7th International Conference on Green and Sustainable Chemistry, 4th JACI/GSC Symposium
    • Place of Presentation
      一橋大学 一橋講堂(東京都・千代田区)
    • Year and Date
      2015-07-07
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Efficient production of hydrogen peroxide using BiVO4 photoelectrode for effective utilization of oxidative reaction in water splitting2015

    • Author(s)
      Kojiro Fuku, Kazuhiro Sayama
    • Organizer
      第4回JACI/GSCシンポジウム・第7回GSC東京国際会議
    • Place of Presentation
      一橋大学 一橋講堂
    • Year and Date
      2015-07-05 – 2015-07-08
    • Related Report
      2014 Research-status Report
  • [Presentation] BiVO4を用いた酸化的な過酸化水素製造2015

    • Author(s)
      福 康二郎、佐山 和弘
    • Organizer
      第34回光がかかわる触媒化学シンポジウム
    • Place of Presentation
      東京工業大学 蔵前会館 くらまえホール(東京都・目黒区)
    • Year and Date
      2015-06-19
    • Related Report
      2015 Annual Research Report
  • [Presentation] 水素および高付加価値酸化生成物の効率的製造を目指した光電極システムの設計2015

    • Author(s)
      福 康二郎、三石 雄悟、舩木 敬、佐山 和弘
    • Organizer
      日本化学会第95春季年会
    • Place of Presentation
      日本大学 理工学部船橋キャンパス
    • Year and Date
      2015-03-28
    • Related Report
      2014 Research-status Report
  • [Presentation] WO3/BiVO4光電極を用いた酸化的な化合物合成2015

    • Author(s)
      宮瀬 雄太、福 康二郎、三石 雄悟、郡司 天博、佐山 和弘
    • Organizer
      日本化学会第95春季年会
    • Place of Presentation
      日本大学 理工学部船橋キャンパス
    • Year and Date
      2015-03-26
    • Related Report
      2014 Research-status Report
  • [Presentation] WO3光電極による酸化反応の有効利用を目指した水分解水素製造2015

    • Author(s)
      佐山 和弘、福 康二郎、Wang Nini、三石 雄悟
    • Organizer
      電気化学会第82回大会
    • Place of Presentation
      横浜国立大学
    • Year and Date
      2015-03-17
    • Related Report
      2014 Research-status Report
  • [Presentation] BiVO4光電極による酸化反応の有効利用を目指した水分解水素製造2015

    • Author(s)
      福 康二郎、宮瀬 雄太、Wang Nini、三石 雄悟、郡司 天博、佐山 和弘
    • Organizer
      電気化学会第82回大会
    • Place of Presentation
      横浜国立大学
    • Year and Date
      2015-03-17
    • Related Report
      2014 Research-status Report
  • [Patent(Industrial Property Rights)] 過酸化水素の製造方法および製造装置2016

    • Inventor(s)
      福 康二郎、草間 仁、佐山 和弘
    • Industrial Property Rights Holder
      福 康二郎、草間 仁、佐山 和弘
    • Industrial Property Rights Type
      特許
    • Industrial Property Number
      2016-062043
    • Filing Date
      2016-03-25
    • Related Report
      2015 Annual Research Report
  • [Patent(Industrial Property Rights)] 過酸化水素の製造方法および製造装置2015

    • Inventor(s)
      福 康二郎、草間 仁、佐山 和弘
    • Industrial Property Rights Holder
      福 康二郎、草間 仁、佐山 和弘
    • Industrial Property Rights Type
      特許
    • Industrial Property Number
      2015-163005
    • Filing Date
      2015-08-20
    • Related Report
      2015 Annual Research Report
  • [Patent(Industrial Property Rights)] 光エネルギーの利用方法および光エネルギーの利用装置2014

    • Inventor(s)
      佐山 和弘、福 康二郎、三石 雄悟
    • Industrial Property Rights Holder
      佐山 和弘、福 康二郎、三石 雄悟
    • Industrial Property Rights Type
      特許
    • Industrial Property Number
      2014-227980
    • Filing Date
      2014-11-10
    • Related Report
      2014 Research-status Report
  • [Patent(Industrial Property Rights)] 光エネルギーの利用方法および光エネルギーの利用装置2014

    • Inventor(s)
      佐山 和弘、福 康二郎、三石 雄悟
    • Industrial Property Rights Holder
      佐山 和弘、福 康二郎、三石 雄悟
    • Industrial Property Rights Type
      特許
    • Industrial Property Number
      2014-227981
    • Filing Date
      2014-11-10
    • Related Report
      2014 Research-status Report

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Published: 2014-04-04   Modified: 2017-05-10  

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