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Study of alcohol soluble organic precursor and solution-processed organic semiconductor devices

Research Project

Project/Area Number 26810107
Research Category

Grant-in-Aid for Young Scientists (B)

Allocation TypeMulti-year Fund
Research Field Organic and hybrid materials
Research InstitutionKyushu University

Principal Investigator

Watanabe Motonori  九州大学, カーボンニュートラル・エネルギー国際研究所, 助教 (60700276)

Project Period (FY) 2014-04-01 – 2016-03-31
Project Status Completed (Fiscal Year 2015)
Budget Amount *help
¥4,030,000 (Direct Cost: ¥3,100,000、Indirect Cost: ¥930,000)
Fiscal Year 2015: ¥910,000 (Direct Cost: ¥700,000、Indirect Cost: ¥210,000)
Fiscal Year 2014: ¥3,120,000 (Direct Cost: ¥2,400,000、Indirect Cost: ¥720,000)
Keywords酸素センサー / インジゴ / 有機半導体 / 溶液プロセス / 酸素ー光応答型電極 / インディゴ / 有機材料化学 / 有機電界効果トランジスタ / センサー / 構造有機化学
Outline of Final Research Achievements

This project of final goal is development of novel solution-processed organic semiconductor devices that can be converted from alcohol soluble organic precursor. To develop this purpose, novel organic materials and a series of substituent group were investigated in this project. 5,5'-Alkylsubsituted leucoindigo could soluble to alcohol such as ethanol with high solubility, and it could convert to corresponding indigo by oxygen as chemical oxidant. This leuco structure material could allow to fabricate for thin-film structure device by solution-process, also converted to indigo by oxygen. The film device showed opt-electronic response and showed current, suggested this system can be used for oxygen chemical sensor under opt-electronic measurement condition.

Report

(3 results)
  • 2015 Annual Research Report   Final Research Report ( PDF )
  • 2014 Research-status Report
  • Research Products

    (27 results)

All 2016 2015 2014 Other

All Int'l Joint Research (2 results) Journal Article (7 results) (of which Int'l Joint Research: 1 results,  Peer Reviewed: 7 results,  Acknowledgement Compliant: 6 results,  Open Access: 2 results) Presentation (15 results) (of which Int'l Joint Research: 2 results,  Invited: 5 results) Book (1 results) Remarks (2 results)

  • [Int'l Joint Research] 台湾中央研究院/台湾大学/東海大学(台湾)

    • Related Report
      2015 Annual Research Report
  • [Int'l Joint Research] イリノイ大学/マサチューセッツ工科大学(米国)

    • Related Report
      2015 Annual Research Report
  • [Journal Article] Effect of porphyrin molecular structure on water splitting activity of a KTaO3 photocatalyst2016

    • Author(s)
      H. Hagiwara, K. Higashi, M. Watanabe, R. Kakigi, S. Ida, T. Ishihara
    • Journal Title

      Catalysts

      Volume: 3 Issue: 3 Pages: 42-42

    • DOI

      10.3390/catal6030042

    • Related Report
      2015 Annual Research Report
    • Peer Reviewed / Open Access / Acknowledgement Compliant
  • [Journal Article] Synthesis of Dibromo[3.3]paracyclophanes2016

    • Author(s)
      Masahiko Shibahara, Motonori Watanabe, Takaaki Miyazaki, Kenta Goto, Taisuke Matsumoto, Teruo Shinmyozu
    • Journal Title

      Synthesis

      Volume: 48 Issue: 08 Pages: 1197-1201

    • DOI

      10.1055/s-0035-1560421

    • Related Report
      2015 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Impact of Alkoxy Chain Length on Carbazole-based, Visible Light-driven, Dye Sensitized Photocatalytic Hydrogen Production2015

    • Author(s)
      Motonori Watanabe, Hidehisa Hagiwara, Yudai Ogata, Aleksandar Staykov, Sean R. Bishop, Nicola H. Perry, Yuan Jay Chang, Shintaro Ida, Keiji Tanaka, Tatsumi Ishihara
    • Journal Title

      Journal of Materials Chemistry A

      Volume: 3 Issue: 43 Pages: 21713-21721

    • DOI

      10.1039/c5ta04991a

    • Related Report
      2015 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Synthesis and Investigation of the Effect of Substitution on the Structure, Physical Properties, and Electrochemical Properties of Anthracenodifuran Derivatives2015

    • Author(s)
      Motonori Watanabe, Yasutaka Doi, Hidehisa Hagiwara, Aleksandar Tsekov Staykov, Shintaro Ida, Taisuke Matsumoto, Teruo Shinmyozu, and Tatsumi Ishihara
    • Journal Title

      The Journal of Organic Chemistry

      Volume: 80 Issue: 18 Pages: 91599166-91599166

    • DOI

      10.1021/acs.joc.5b01525

    • Related Report
      2015 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Synthesis and electronic properties of ferrocene-containing organic dyads2015

    • Author(s)
      Motonori Watanabe,* Yuan Jay Chang, Po-ting Chou, Aleksandar Staykov, Masahiko Shibahara, Katsuya Sako, Tatsumi Ishihara, Tahsin J Chow
    • Journal Title

      Tetrahedron Letteers

      Volume: 56 Issue: 12 Pages: 1548-1551

    • DOI

      10.1016/j.tetlet.2015.02.012

    • Related Report
      2014 Research-status Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Crystal structure of (E)-2-cyano-3-(12-methyl-12H-benzo[b]pheno­thia­zin-11-yl)acrylic acid2014

    • Author(s)
      Motonori Watanabe,Tatsumi Ishihara
    • Journal Title

      Acta Crystallographica Section E: Crystallographic Communications

      Volume: E70 Issue: 9 Pages: o1026-o1027

    • DOI

      10.1107/s1600536814018388

    • Related Report
      2014 Research-status Report
    • Peer Reviewed / Open Access / Acknowledgement Compliant
  • [Journal Article] Spacer Effects in Metal-Free Organic Dyes for Visible-Light-Driven Dye-Sensitized Photocatalytic Hydrogen Production2014

    • Author(s)
      Motonori Watanabe, Hidehisa Hagiwara, Iribe Aoi, Yudai Ogata, Kenta Shiomi, Aleksandar Staykov, Shintaro Ida, Keiji Tanaka, Tatsumi Ishihara
    • Journal Title

      Journal of Materials Chemistry A

      Volume: 2 Pages: 12952-12961

    • Related Report
      2014 Research-status Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Presentation] Synthesis, structure, and physical properties of the 5,5’-position alkylated indigo2016

    • Author(s)
      WATANABE, Motonori; UEMURA, Naoki; GOTO, Kenta; HAGIWARA, Hidehisa; IDA, Shintaro; ISHIHARA, Tatsumi
    • Organizer
      日本化学会 第96春季年会 (2016)
    • Place of Presentation
      同志社大学京田辺キャンパス、京田辺、京都
    • Year and Date
      2016-03-24
    • Related Report
      2015 Annual Research Report
  • [Presentation] Small Band-Gap Organic Materials for Opt-Electronic Application and Energy Conversion2016

    • Author(s)
      Motonori Watanabe
    • Organizer
      The 3rd CMS International Symposium
    • Place of Presentation
      Kyushu University, IMCE, Japan
    • Year and Date
      2016-01-22
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] mpact of Alkoxy Chain Length on Carbazole-based, Visible Light-driven, Dye Sensitized Photocatalytic Hydrogen Production2015

    • Author(s)
      Motonori Watanabe, Hidehisa Hagiwara, Yudai Ogata, Aleksandar Staykov, Sean R. Bishop, Nicola H. Perry, Yuan Jay Chang, Shintaro Ida, Keiji Tanakaa, Tatsumi Ishihara
    • Organizer
      第9回有機π電子系シンポジウム
    • Place of Presentation
      レイクサイド入鹿、犬山、愛知
    • Year and Date
      2015-11-20
    • Related Report
      2015 Annual Research Report
  • [Presentation] Furan-contained oligoacene and opt-electronic application2015

    • Author(s)
      Motonori Watanabe, Yuan Jay Chang, Kenta Goto, Masahiko Shibahara, Teruo Shinmyozu, Tatsumi Ishihara, and Tahsin J Chow
    • Organizer
      International Symposium on Construction and Application of Functional Molecules/System
    • Place of Presentation
      Yilan County, Hotel Royal Chiaoshi, Taiwan
    • Year and Date
      2015-10-18
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Synthesis of the Ethynyl-substituent functionalized difuranoanthracene and physical property2015

    • Author(s)
      Motonori Watanabe, Yasutaka Doi, Hidehisa Hagiwara, Aleksandar Staykov, Taisuke Matsumoto, Teruo Shinmyozu, Shintaro Ida, Tatsumi Ishihara
    • Organizer
      第26回基礎有機化学討論会 26th Symposium on Physical Organic Chemistry
    • Place of Presentation
      愛媛大学、松山、愛媛
    • Year and Date
      2015-09-24
    • Related Report
      2015 Annual Research Report
  • [Presentation] Organic dye modified visible light driven photocatalytic water decomposition for hydrogen production2015

    • Author(s)
      Motonori Watanabe
    • Organizer
      2015 Fall Symposium of Photochemistry Association in Taiwan
    • Place of Presentation
      Tung-Hai University, Taiwan
    • Year and Date
      2015-09-05
    • Related Report
      2015 Annual Research Report
    • Invited
  • [Presentation] Visible light driven photocatalytic water decomposition for hydrogen production2015

    • Author(s)
      Motonori Watanabe
    • Organizer
      構造有機若手の会2015
    • Place of Presentation
      九州大学伊都キャンパス、福岡、福岡
    • Year and Date
      2015-08-31
    • Related Report
      2015 Annual Research Report
  • [Presentation] Synthesis, Structure, and Physical Property of Novel Difuranoacene2015

    • Author(s)
      Motonori Watanabe, Yasutaka Doi, Hidehisa Hagiwara ,Shintaro Ida, Tatsumi Ishihara
    • Organizer
      第52回化学関連支部合同九州大会
    • Place of Presentation
      北九州国際会議場、小倉、福岡
    • Year and Date
      2015-07-27
    • Related Report
      2015 Annual Research Report
  • [Presentation] Novel Metal-Free Donor-Spacer-Acceptor Dyads for Visible Light Driven Dye-Sensitized Water Splitting Hydrogen Production2014

    • Author(s)
      Motonori Watanabe
    • Organizer
      The 8th Taiwan-Japan Bilateral Symposium on Architecture of Functional Organic Molecules
    • Place of Presentation
      Kyushu University (Hakozaki Campus), Fukuoka
    • Year and Date
      2014-11-27
    • Related Report
      2014 Research-status Report
    • Invited
  • [Presentation] An impact of alkyl chain length for water splitting performance in carbazole-based visible light driven dye-sensitized wate r splitting hydrogen production2014

    • Author(s)
      Motonori WATANABE, Hidehisa HAGIWARA, Yudai OGATA, Shen BISHOP, Shintaro IDA, Tanaka KEIJI, Tatsumi ISHIHARA
    • Organizer
      International Conference on Artificial Photosynthesis (ICARP2014)
    • Place of Presentation
      Awaji Yumebutai International Conference Center, Awaji City, Hyogo
    • Year and Date
      2014-11-23
    • Related Report
      2014 Research-status Report
  • [Presentation] Synthesis, Structure, and Physical Property of Novel Difuranoacene2014

    • Author(s)
      Motonori Watanabe, Yasutaka Doi, Hidehisa Hagiwara ,Shintaro Ida, Tatsumi Ishihara
    • Organizer
      The 8th Symposium on Organic π-Electron Systems
    • Place of Presentation
      Ryutouen Hotel, Saga
    • Year and Date
      2014-11-21
    • Related Report
      2014 Research-status Report
  • [Presentation] An Impact of Alkyl Chain Effect in Metal-Free Organic Dyes for Visible-Light-Driven Dye-Sensitized Photocatalytic Hydrogen Production2014

    • Author(s)
      Motonori Watanabe, Hidehisa Hagiwara Yudai Ogata, Aleksandar Staykov, Shintaro Ida, Keiji Tanaka, Tatsumi Ishihara
    • Organizer
      25th Symposium on Physical Organic Chemistry
    • Place of Presentation
      Touhoku Univ. Sendai
    • Year and Date
      2014-09-08
    • Related Report
      2014 Research-status Report
  • [Presentation] Benzophenothiazine containing Donor-Acceptor Dyads for Photocatalytic Water Splitting Hydrogen Production Reaction2014

    • Author(s)
      Motonori Watanabe, Hidehisa Hagiwara, Aoi Iribe, Yudai Ogata, Kenta Shiomi, Aleksandar Staykov, Shintaro Ida, Keiji Tanaka, Tatsumi Ishihara
    • Organizer
      51th Kitakytushu Symposium on Related with Chemistry-Associated Branch
    • Place of Presentation
      Kitakyushu International Conference Center
    • Year and Date
      2014-07-28
    • Related Report
      2014 Research-status Report
  • [Presentation] Novel Donor-Acceptor Organic Molecules for Visible Light Driven Photocatalytic Dye-Sensitized Water Splitting Hydrogen Production2014

    • Author(s)
      Motonori Watanabe
    • Organizer
      International Conference for Top and Emerging Materials Scientists
    • Place of Presentation
      Downtown Hotel Zhuhai, Zhuhai, China
    • Year and Date
      2014-07-23
    • Related Report
      2014 Research-status Report
    • Invited
  • [Presentation] Spacer Effects in Metal-Free Organic Dyes for Visible-Light Driven Dye-Sensitized Photocatalytic Hydrogen Production2014

    • Author(s)
      Motonori Watanabe, Hidehisa Hagiwara, Aoi Iribe, Yudai Ogata, Kenta Shiomi, Aleksandar Staykov, Shintaro Ida, Keiji Tanaka, Tatsumi Ishihara
    • Organizer
      Pre-symposium TOCAT7 in Fukuoka
    • Place of Presentation
      Fukuoka, Kyushu University (Kasuga campus)
    • Year and Date
      2014-05-30
    • Related Report
      2014 Research-status Report
  • [Book] Hydrogen Energy Engineering: A Japanese Perspective (Green Energy and Technology)2016

    • Author(s)
      Aleksandar STAYKOV, Stephen M. LYTH, and Motonori WATANABE
    • Total Pages
      300
    • Publisher
      Hydrogen Energy Engineering
    • Related Report
      2015 Annual Research Report
  • [Remarks] Kyushu University I2CNER Motonori Watanabe Lab

    • URL

      http://homepage1.canvas.ne.jp/orgchem/publication.html

    • Related Report
      2015 Annual Research Report
  • [Remarks] 渡邊源規研究室

    • URL

      http://homepage1.canvas.ne.jp/orgchem/index.html

    • Related Report
      2014 Research-status Report

URL: 

Published: 2014-04-04   Modified: 2022-02-16  

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