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Revealing the near-field properties of coupled plasmonic systems by photoemission electron microscopy

Research Project

Project/Area Number 26870014
Research Category

Grant-in-Aid for Young Scientists (B)

Allocation TypeMulti-year Fund
Research Field Physical chemistry
Nanostructural physics
Research InstitutionHokkaido University

Principal Investigator

SUN QUAN  北海道大学, 創成研究機構, 特任助教 (90727463)

Project Period (FY) 2014-04-01 – 2016-03-31
Project Status Completed (Fiscal Year 2015)
Budget Amount *help
¥4,030,000 (Direct Cost: ¥3,100,000、Indirect Cost: ¥930,000)
Fiscal Year 2015: ¥1,300,000 (Direct Cost: ¥1,000,000、Indirect Cost: ¥300,000)
Fiscal Year 2014: ¥2,730,000 (Direct Cost: ¥2,100,000、Indirect Cost: ¥630,000)
KeywordsSurface plasmon / Plasmon coupling / Near field / Dephasing time / PEEM / Plasmaon coupling / Dephasing
Outline of Final Research Achievements

We investigated the near-field properties of several coupled plasmonic systems using photoemission electron microscropy (PEEM). The PEEM measurements allow to obtain near-field mapping and spectral response of plasmonic nanostructures. With this technique we revealed near-field plasmon coupling in one dimensional gold nanochains and observed the energy transport along the nanochians. We also explored plasmon hybridization in gold dolmen nanostructures. Especially, the hybridized bonding and anti-bonding plasmon modes were explored in near field, and the dramatic evolution of near field intensity distribution between bonding and anti-bonding modes was observed. Furthermore, we established a time-resolved PEEM setup to investigate the dynamics of plasmon resonances, and we experimentally demonstrated for the first time that the quadrupole mode in Au nanoblocks has longer dephasing time than that of the dipole mode.

Report

(3 results)
  • 2015 Annual Research Report   Final Research Report ( PDF )
  • 2014 Research-status Report
  • Research Products

    (17 results)

All 2016 2015 2014

All Journal Article (3 results) (of which Int'l Joint Research: 1 results,  Peer Reviewed: 2 results,  Open Access: 1 results,  Acknowledgement Compliant: 1 results) Presentation (14 results) (of which Int'l Joint Research: 5 results,  Invited: 2 results)

  • [Journal Article] Dissecting the few-femtosecond dephasing time of dipole and quadrupole modes in gold nanoparticles using polar-ized photoemission electron microscopy2016

    • Author(s)
      Q. Sun, H. Yu, K. Ueno, A. Kubo, Y. Matsuo, H. Misawa
    • Journal Title

      ACS Nano

      Volume: 10 Issue: 3 Pages: 3835-3842

    • DOI

      10.1021/acsnano.6b00715

    • Related Report
      2015 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Robust and Versatile Light Absorption at Near Infrared Wavelengths by Plasmonic Aluminum Nanorods2014

    • Author(s)
      O. Lecarme, Q. Sun, K. Ueno, H. Misawa
    • Journal Title

      ACS Photonics

      Volume: 1 Issue: 6 Pages: 538-546

    • DOI

      10.1021/ph500096q

    • Related Report
      2014 Research-status Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Construction of Plasmon-Induced Artificial Photosynthesis and its Dynamics Measured by PEEM2014

    • Author(s)
      上野 貢生, 孫 泉, 三澤 弘明
    • Journal Title

      Hyomen Kagaku

      Volume: 35 Issue: 12 Pages: 668-673

    • DOI

      10.1380/jsssj.35.668

    • NAID

      130004785030

    • ISSN
      0388-5321, 1881-4743
    • Related Report
      2014 Research-status Report
  • [Presentation] Spectral response and spatial evolution of plasmonic near field in coupled gold nanostructures2016

    • Author(s)
      Han Yu, Quan Sun, Tomoya Oshikiri, Kosei Ueno, Yasutaka Matsuo, Atsushi Kubo and Hiroaki Misawa
    • Organizer
      日本化学会第96春季年会
    • Place of Presentation
      同志社大学(京都)
    • Year and Date
      2016-03-24
    • Related Report
      2015 Annual Research Report
  • [Presentation] Exploring plasmonic hot spots and their dynamics by photoemission electron microscopy2015

    • Author(s)
      Quan Sun, Han Yu, Kosei Ueno, Atsushi Kubo, Yasutaka Matsuo, and Hiroaki Misawa
    • Organizer
      The 2015 International Chemical Congress of Pacific Basin Societies (Pacifichem 2015)
    • Place of Presentation
      Honolulu, USA
    • Year and Date
      2015-12-15
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Fano resonances on gold nano dolmen structures probed by photoemission electron microscopy2015

    • Author(s)
      Han Yu, Quan Sun, Kosei Ueno, Yasutaka Matsuo, Atsushi Kubo, and Hiroaki Misawa
    • Organizer
      The 2015 International Chemical Congress of Pacific Basin Societies (Pacifichem 2015)
    • Place of Presentation
      Honolulu, USA
    • Year and Date
      2015-12-15
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Time-resolved Photoemission Electron Microscopy: a Versatile Tool for Accessing the Near Field and Dynamics of Plasmonic Antennae2015

    • Author(s)
      Quan Sun, Han Yu, Kosei Ueno, Atsushi Kubo, Yasutaka Matsuo, and Hiroaki Misawa
    • Organizer
      The 27th International Conference on Photochemistry (ICP 2015)
    • Place of Presentation
      Jeju, Korea
    • Year and Date
      2015-06-28
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Higher-order Localized Surface Plasmon Resonances on Gold Nanostructures Probed by Photoemission Electron Microscopy2015

    • Author(s)
      Han Yu, Quan Sun, Kosei Ueno, Atsushi Kubo, Yasutaka Matsuo, and Hiroaki Misawa
    • Organizer
      The 27th International Conference on Photochemistry (ICP 2015)
    • Place of Presentation
      Jeju, Korea
    • Year and Date
      2015-06-28
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Near-field plasmon coupling in gold nanochains revealed by photoemission electron microscopy2015

    • Author(s)
      Quan Sun, Han Yu, Kosei Ueno, Atsushi Kubo, Yasutaka Matsuo, and Hiroaki Misawa
    • Organizer
      The 7th International Conference on Surface Plasmon Photonics (SPP7)
    • Place of Presentation
      Jerusalem, Israel
    • Year and Date
      2015-05-31
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Exploring the Fano resonance of dolmen structures in near field by PEEM2015

    • Author(s)
      H. Yu, Q. Sun, K. Ueno, Y. Matsuo, A. Kubo and H. Misawa
    • Organizer
      2015年第62回応用物理学会春季学術講演会
    • Place of Presentation
      東海大学湘南キャンパス (神奈川)
    • Year and Date
      2015-03-11 – 2015-03-14
    • Related Report
      2014 Research-status Report
  • [Presentation] Probing the near field of bright and dark surface plasmon modes in gold nanoparticles by photoemission electron microscopy2014

    • Author(s)
      H. Yu, Q. Sun, A. Kubo, Y. Matsuo, K. Ueno and H. Misawa
    • Organizer
      The 15th Ries-Hokudai International Symposium
    • Place of Presentation
      Gateaux Kingdom, Sapporo (Japan)
    • Year and Date
      2014-12-16 – 2014-12-17
    • Related Report
      2014 Research-status Report
  • [Presentation] Femtosecond laser direct writing of 3D photonic crystals with stop gaps in the visible regime2014

    • Author(s)
      Q. Sun, T. Tokiwa, K. Ueno and H. Misawa
    • Organizer
      The 4th International Conference on Manipulation, Manufacturing and Measurement on the Nanoscale (3M Nano 2014)
    • Place of Presentation
      Academia Sinica, Taipei (Taiwan)
    • Year and Date
      2014-10-27 – 2014-10-31
    • Related Report
      2014 Research-status Report
    • Invited
  • [Presentation] Near field and dynamics of surface plasmon dark states in gold nanoblocks revealed by PEEM2014

    • Author(s)
      H. Yu, Q. Sun, A. Kubo, Y. Matsuo, K. Ueno and H. Misawa
    • Organizer
      2014年光化学討論会
    • Place of Presentation
      北海道大学 (札幌)
    • Year and Date
      2014-10-11 – 2014-10-13
    • Related Report
      2014 Research-status Report
  • [Presentation] Watching the near field of localized surface plasmon resonances and their dynamics by photoemission electron microscopy2014

    • Author(s)
      Q. Sun, H. Yu, K. Ueno, A. Kubo, Y. Matsuo and H. Misawa
    • Organizer
      Belgium and Japan Joint Symposium on Nanoplasmonics and Nanoimaging Chemistry
    • Place of Presentation
      Hokkaido University, Sapporo (Japan)
    • Year and Date
      2014-10-10
    • Related Report
      2014 Research-status Report
  • [Presentation] Exploring quadrupole and higher order surface plasmon resonances in individual plasmonic nanoantennas by PEEM2014

    • Author(s)
      Q. Sun, H. Yu, K. Ueno, A. Kubo, Y. Matsuo and H. Misawa
    • Organizer
      The 9th conference on LEEM/PEEM (LEEM/PEEM-9)
    • Place of Presentation
      Best Western Plus Hotel Steglitz International, Berlin (Germany)
    • Year and Date
      2014-09-14 – 2014-09-18
    • Related Report
      2014 Research-status Report
  • [Presentation] Near field and dynamics in gold nanoparticles probed by photoemission electron microscopy2014

    • Author(s)
      H. Yu, Q. Sun, A. Kubo, Y. Matsuo, K. Ueno and H. Misawa
    • Organizer
      The 1st Korea-Japan Bilateral Workshop on Functional Materials Science
    • Place of Presentation
      Hokkaido University, Sapporo (Japan)
    • Year and Date
      2014-08-01
    • Related Report
      2014 Research-status Report
  • [Presentation] Applications of photoemission electron microscopy in plasmonics2014

    • Author(s)
      Q. Sun, H. Yu, K. Ueno and H. Misawa
    • Organizer
      Light Conference-Young Scientists Forum 2014
    • Place of Presentation
      CIOMP, Changchun (China)
    • Year and Date
      2014-07-04 – 2014-07-05
    • Related Report
      2014 Research-status Report
    • Invited

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Published: 2014-04-04   Modified: 2017-05-10  

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