• Search Research Projects
  • Search Researchers
  • How to Use
  1. Back to previous page

Development of functional carbon materials based on two-dimensional organic frameworks

Research Project

Project/Area Number 26886011
Research Category

Grant-in-Aid for Research Activity Start-up

Allocation TypeSingle-year Grants
Research Field Nanomaterials chemistry
Research InstitutionKyushu University

Principal Investigator

SHIRAKI Tomohiro  九州大学, 工学(系)研究科(研究院), 助教 (10508089)

Project Period (FY) 2014-08-29 – 2016-03-31
Project Status Completed (Fiscal Year 2015)
Budget Amount *help
¥2,470,000 (Direct Cost: ¥1,900,000、Indirect Cost: ¥570,000)
Fiscal Year 2015: ¥1,170,000 (Direct Cost: ¥900,000、Indirect Cost: ¥270,000)
Fiscal Year 2014: ¥1,300,000 (Direct Cost: ¥1,000,000、Indirect Cost: ¥300,000)
Keywords共有結合性有機構造体 / 結晶性 / 炭化 / 窒素ドープカーボン / ナノ材料 / 超分子化学 / ナノ粒子 / ナノカーボン
Outline of Final Research Achievements

In this study, development of functional carbon materials was examined through carbonization of covalent organic frameworks (COFs) that are constructed by crystalline molecular networks composed of covalently-linked organic molecules. At first, we succeeded in development of a room temperature synthesis method that provided highly-crystalline COFs compared to the reported ones prepared by solvothermal methods. The nitrogen atom-containing COFs were carbonized to synthesize graphitic carbon materials. Importantly, we found that crystallinity of COFs strongly effects on the resulting graphitic carbon structures and nitrogen-doped conditions that are related to functionalities as fuel cell catalysts and super capacitors.

Report

(3 results)
  • 2015 Annual Research Report   Final Research Report ( PDF )
  • 2014 Annual Research Report
  • Research Products

    (18 results)

All 2016 2015 Other

All Journal Article (6 results) (of which Int'l Joint Research: 1 results,  Peer Reviewed: 6 results,  Acknowledgement Compliant: 1 results,  Open Access: 1 results) Presentation (11 results) (of which Int'l Joint Research: 3 results) Remarks (1 results)

  • [Journal Article] Determination of Precise Redox Properties of Oxygen-Doped Single-Walled Carbon Nanotubes Based on in Situ Photoluminescence Electrochemistry2016

    • Author(s)
      Tomonari Shiraishi, Gergely Juhasz, Tomohiro Shiraki, Naoto Akizuki, Yuhei Miyauchi, Kazunari Matsuda, Naotoshi Nakashima
    • Journal Title

      The Journal of Physical Chemistry

      Volume: 120 Issue: 14 Pages: 4774-4779

    • DOI

      10.1002/chem.201504533

    • Related Report
      2015 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Room-temperature Synthesis of a Covalent Organic Framework with Enhanced Surface Area and Thermal Stability and Application to Nitrogen-doped Graphite Synthesis2015

    • Author(s)
      Tomohiro Shiraki, Gayoung Kim, Naotoshi Nakashima
    • Journal Title

      Chemistry Letters

      Volume: 44 Issue: 11 Pages: 1488-1490

    • DOI

      10.1246/cl.150678

    • NAID

      130005108069

    • ISSN
      0366-7022, 1348-0715
    • Related Report
      2015 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Synthesis of porous gold nanoparticles/MoS2 nanocomposites based on redox reaction2015

    • Author(s)
      Xiaojing Yu, Tomohiro Shiraki, Shengchun Yang, Bingjun Ding, Naotoshi Nakashima
    • Journal Title

      RSC advances

      Volume: 5 Issue: 105 Pages: 86558-86563

    • DOI

      10.1039/c5ra15421a

    • Related Report
      2015 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Strong Main-Chain Length-Dependence for the ß-Phase Formation of Oligofluorenes2015

    • Author(s)
      Tomohiro Shiraki, Shoichiro Shindome, Fumiyuki Toshimitsu, Tsuyohiko Fujigaya, Naotoshi Nakashima
    • Journal Title

      Polymer Chemistry

      Volume: 6 Issue: 28 Pages: 5103-5109

    • DOI

      10.1039/c5py00385g

    • Related Report
      2015 Annual Research Report
    • Peer Reviewed
  • [Journal Article] In Situ Photoluminescence Spectroelectrochemistry for Determination of Electronic States of Single-walled Carbon Nanotubes2015

    • Author(s)
      Tomohiro Shiraki and Naotoshi Nakashima
    • Journal Title

      e-Journal of Surface Science and Nanotechnology

      Volume: 13 Issue: 0 Pages: 179-184

    • DOI

      10.1380/ejssnt.2015.179

    • NAID

      130005065389

    • Related Report
      2015 Annual Research Report 2014 Annual Research Report
    • Peer Reviewed
  • [Journal Article] In Situ Synthesis of Covalent Organic Frameworks (COFs) on Carbon Nanotubes and Graphenes by Sonochemical Reaction for CO2 Adsorbents2015

    • Author(s)
      JongTae Yoo, SuHyun Lee, Shinsuke Hirata, ChaeRin Kim, Chang Kee Lee, Tomohiro Shiraki, Naotoshi Nakashima, and Jin Kie Shim
    • Journal Title

      Chemistry Letters

      Volume: 44 Issue: 4 Pages: 560-562

    • DOI

      10.1246/cl.141194

    • NAID

      130005062110

    • Related Report
      2015 Annual Research Report 2014 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Presentation] Covalent Organic Frameworks Carbonized for Synthesis of Functional Carbon Materials2016

    • Author(s)
      Tomohiro Shiraki, Gayoung Kim, Naotoshi Nakashima
    • Organizer
      第65回高分子学会年次大会 高分子学会
    • Place of Presentation
      神戸国際会議場・展示場
    • Year and Date
      2016-05-25
    • Related Report
      2015 Annual Research Report
  • [Presentation] 分子が規則配列した有機構造体の炭化による窒素ドープカーボンの調製2016

    • Author(s)
      白木 智丈, キム ガヨン, 中嶋 直敏
    • Organizer
      第50回 フラーレン・ナノチューブ・グラフェン総合シンポジウム
    • Place of Presentation
      東京大学 伊藤国際学術研究センター 伊藤謝恩ホール(東京)
    • Year and Date
      2016-02-20
    • Related Report
      2015 Annual Research Report
  • [Presentation] Characterization of Covalent Organic Framework Synthesized in a Mild Reaction Condition2015

    • Author(s)
      Gayoung Kim, Tomohiro Shiraki, Naotoshi Nakashima
    • Organizer
      2015 Pusan-Gyeongnam/Kyushu-Seibu Joint Symposium on High Polymers (17th) and Fibers (15th) (2015 PGKS)
    • Place of Presentation
      Dong-A University Bumin Campus, Busan
    • Year and Date
      2015-11-12
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research
  • [Presentation] A two-dimensional organic layered material with high crystallinity by a room temperature synthesis2015

    • Author(s)
      Gayoung Kim, Tomohiro Shiraki, Naotoshi Nakashima
    • Organizer
      6th A3 Symposium on Emerging Materials
    • Place of Presentation
      Chikushi Hall (C-CUBE), Chikushi Campus, Kyushu University
    • Year and Date
      2015-11-09
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 室温合成による共有結合性有機フレームワークの高結晶化とグラファイト型カーボンの作製2015

    • Author(s)
      キムガヨン・白木智丈・中嶋直敏
    • Organizer
      第5回 CSJ化学フェスタ2015
    • Place of Presentation
      タワーホール船堀
    • Year and Date
      2015-10-13
    • Related Report
      2015 Annual Research Report
  • [Presentation] Room temperature synthesis of two-dimensional organic framework materials2015

    • Author(s)
      キム ガヨン, 白木 智丈, 中嶋 直敏
    • Organizer
      第49回 フラーレン・ナノチューブ・グラフェン 総合シンポジウム
    • Place of Presentation
      北九州国際会議場
    • Year and Date
      2015-09-07
    • Related Report
      2015 Annual Research Report
  • [Presentation] 共有結合性有機フレームワークの室温合成と構造評価2015

    • Author(s)
      キム ガヨン・白木 智丈 ・中嶋 直敏
    • Organizer
      第52回化学関連支部合同九州大会
    • Place of Presentation
      北九州国際会議場
    • Year and Date
      2015-06-27
    • Related Report
      2015 Annual Research Report
  • [Presentation] Characterization of Covalent Organic Framework Synthesized in a Mild Reaction Condition2015

    • Author(s)
      Gayoung Kim, Tomohiro Shiraki, Naotoshi Nakashima
    • Organizer
      The 2nd Symposium of Korea-Japan joint Project for Carbon Nanotube Electro-Optical Study
    • Place of Presentation
      Pukyong National Univ., Korea
    • Year and Date
      2015-06-12
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research
  • [Presentation] ジオクチルフルオレンオリゴマーの鎖長に依存したベータ相形成挙動の変化と半導体性カーボンナノチューブの可溶化能2015

    • Author(s)
      白木 智丈・新留 頌一郎・利光 史行・藤ヶ谷 剛彦・中嶋 直敏
    • Organizer
      第64回高分子学会年次大会
    • Place of Presentation
      札幌コンベンションセンター
    • Year and Date
      2015-05-27 – 2015-05-29
    • Related Report
      2014 Annual Research Report
  • [Presentation] 室温合成法により得られた共有結合性有機フレームワークの構造と機能2015

    • Author(s)
      金 佳怜・白木 智丈 ・中嶋 直敏
    • Organizer
      第64回高分子学会年次大会
    • Place of Presentation
      札幌コンベンションセンター
    • Year and Date
      2015-05-27
    • Related Report
      2015 Annual Research Report 2014 Annual Research Report
  • [Presentation] 鎖長制御されたオリゴフルオレンのベータ相形成に基づく光学特性変化とカーボンナノチューブの選択的可溶化機能2015

    • Author(s)
      白木 智丈・新留 頌一郎・利光 史行・藤ヶ谷 剛彦・中嶋 直敏
    • Organizer
      日本化学会 第95春季年会
    • Place of Presentation
      日本大学 理工学部船橋キャンパス/薬学部
    • Year and Date
      2015-03-26 – 2015-03-29
    • Related Report
      2014 Annual Research Report
  • [Remarks] 研究室ホームページ

    • URL

      http://nakashima.cstm.kyushu-u.ac.jp/jp/index.html

    • Related Report
      2015 Annual Research Report

URL: 

Published: 2014-09-09   Modified: 2017-05-10  

Information User Guide FAQ News Terms of Use Attribution of KAKENHI

Powered by NII kakenhi