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La-Ba and La-Ce geochronometers and Ce-138 as a geochemical tracer, developed to study origin and evolution of terrestrial materials

Research Project

Project/Area Number 58065003
Research Category

Grant-in-Aid for Specially Promoted Research

Allocation TypeSingle-year Grants
Research InstitutionThe University of Tokyo

Principal Investigator

MASUDA Akimasa  The University of Tokyo, Faculty of Science, Professor, 理学部, 教授 (40030788)

Co-Investigator(Kenkyū-buntansha) TANAKA Tsuyoshi  Geological Survey of Japan, Senior Reseacher, 主任研究官 (00236605)
NAKAI Shun'ichi  The University of Tokyo, Faculty of Science, Research Associate, 理学部, 助手 (50188869)
AKAGI Tasuku  The University of Tokyo, Faculty of Science, Research Associate, 理学部, 助手 (80184076)
SHIMIZU Hiroshi  The University of Tokyo, Faculty of Science, Lecturer, 理学部, 講師 (60090544)
Project Period (FY) 1983 – 1986
Project Status Completed (Fiscal Year 1986)
Budget Amount *help
¥265,000,000 (Direct Cost: ¥265,000,000)
Fiscal Year 1986: ¥5,000,000 (Direct Cost: ¥5,000,000)
Fiscal Year 1985: ¥10,000,000 (Direct Cost: ¥10,000,000)
Fiscal Year 1984: ¥30,000,000 (Direct Cost: ¥30,000,000)
Fiscal Year 1983: ¥220,000,000 (Direct Cost: ¥220,000,000)
KeywordsLa-Ce geochronometer / La-Ba geochronometer / <^(138)Ce> isotope tracer / Re-Os geochronometer / Decay constant of <^(138)La> / REE pattern / Ce anomaly / 希土鉱物 / アミツォーク片麻岩 / 南極隕石 / Os同位体トレーサ
Research Abstract

two new geochronometers, <^(138)La> - <^(138)Ce> and <^(138)La> - <^(138)Ba> systems, have been developed in this study, with some technical and/or scientific achievments in other geochronometers, Re-Os, Rb-Sr and Sm-Nd.
1. La-Ce systematics: (1) The <beta^-> decay constant of <^(138)La> was calculated to be 2.94x <10^(-12)> <yr^(-1)> by fitting of La-Ce ages to Sm-Nd ages for the Amitsoq gneiss, Greenland, and the Mustikkamaki pegmatite, Finland. (2) Ce isotopic study suggested that the positive Ce anomaly observed for lunar sample 14310 is considered to have been subjected to some oxic (hydrothermal/aqueous/ice) alteration in the early stage of the lunar history. (3) The Archean Amitsoq gneisses have been analyzed for Ce and Nb isotopic ratios and REE abundances. It was suggested that parent material of the Amitsoq gneisses had Ce and Nd isotopic ratios close to chondritic values at the time of their formation (ca. 3,800 Ma). (4) <^(138)Ce> / <^(142)Ce> and <^(143)Nd> / <^(144)Nd> rat … More ios in nineteen terrestrial rocks including MORB and metamorphic rocks from continental crust have been determined. It was disclosed that the rocks from continental crust were derived directly from the source with chondritic or liquid-type REE patterns. (5) Nd and Ce isotopic ratios for ferromanganese nodules from various Pacific regions indicate that the major source of Nd in these ferromanganese nodules is continental, while Ce is supplied mainly from abyssal volcanics. 2. La-Ba systematics: The geochronological utility of the <^(138)La> - <^(138)Ba> decay has been demonstrated for REE-rich minerals such as allanite, monazite and epidote. Fitting of La-Ba ages to Sm-Nb ages for Korsnas galena mine samples and Mustikkamaki pegmatite samples yielded the <lambda> <_(EC)> <^(138)La> value of 4.15x <10^(-12)> <yr^(-1)> . 3. Re-Os systematics: Osmium isotopes in three Os reagents, four terrestrial Os-Ir alloys (iridosmines) and five iron meteorites have been measured on the inductively coupled plasma mass spectrometer, with the precision of around 1% for <^(187)Os> / <^(192)Os> . Our studies on iron meteorites suggest that the formation ages for iron meteorites merit re-examination. Further, Re-Os ages were reported for molybdenite samples. 4. Rb-Sr systematics: Rb-Sr age for diogenite have been determined to be 4,400Ma which is 100Ma younger than the formation age of eucrite. Less

Report

(2 results)
  • 1986 Final Research Report Summary
  • 1985 Annual Research Report
  • Research Products

    (36 results)

All Other

All Publications (36 results)

  • [Publications] T.Tanaka;A.Masuda: Nature. 300. 515-518 (1982)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1986 Final Research Report Summary
  • [Publications] H.Shimizu;A.Masuda;T.Tanaka: Mem.Natl Inst.Polar Res.,No.30Spec.Issue. 341-348 (1983)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1986 Final Research Report Summary
  • [Publications] A.Masuda;S.Nakai: Geochem.J.17. 313-314 (1983)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1986 Final Research Report Summary
  • [Publications] T.Tanaka:A.Masuda: Nature. 306. 503-504 (1983)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1986 Final Research Report Summary
  • [Publications] H.Shimizu;T.Tanaka;A.Masuda: Nature. 307. 251-252 (1984)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1986 Final Research Report Summary
  • [Publications] 増田彰正,高橋和也: 月刊「地球」. 7. 498-505 (1985)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1986 Final Research Report Summary
  • [Publications] S.Nakai;H.Shimizu;A.Masuda: Nature. 320. 433-435 (1986)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1986 Final Research Report Summary
  • [Publications] K.Takahashi;A.Masuda;H.Shimizu: Mem.Natl Inst.Polar Res.No.41. 96-105 (1986)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1986 Final Research Report Summary
  • [Publications] 清水洋: 月刊「地球」. 8. 493-496 (1986)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1986 Final Research Report Summary
  • [Publications] H.Shimizu;A.Masuda: Geochim.Cosmochim.Acta. 50. 2453-2460 (1986)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1986 Final Research Report Summary
  • [Publications] A.Masuda,T.Hirata and H.Shimizu: Geochem.J.20. 233-239 (1986)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1986 Final Research Report Summary
  • [Publications] K.Takahashi;A.Masuda: Mem.Natl Inst.Polar Res.

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1986 Final Research Report Summary
  • [Publications] S.Hishita;A.Masuda: Naturwissenschaften.

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1986 Final Research Report Summary
  • [Publications] A.Makishima;H.Shimizu;A.Masuda: Mass Spectroscopy.

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1986 Final Research Report Summary
  • [Publications] T.Tanaka;H.Shimizu;Y.Kawata;A.Masuda: Nature.

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1986 Final Research Report Summary
  • [Publications] H.Hidaka;A.Masuda: Earth Planet.Sci.Lett.

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1986 Final Research Report Summary
  • [Publications] 高橋和也,増田彰正: ""南極の科学6-南極いん石",第9章,"南極いん石の化学",国立極地研究所編" 古今書院,

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1986 Final Research Report Summary
  • [Publications] T. Tanaka and A. Masuda: "The La-Ce geochronometer: A new dating method" Nature. 300. 515-518 (1982)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1986 Final Research Report Summary
  • [Publications] H. Shimizu, A. Masuda and T. Tanaka: "Cerium anomaly in REE pattern of Antarctic eucrite" Mem. Natl Inst. Polar Res.Spec. Issue No. 30. 341-348 (1983)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1986 Final Research Report Summary
  • [Publications] A. Masuda and S. Nakai: "An examination of Geochronological utility of electron capture decay of La-138" Geochem. J.17. 313-314 (1983)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1986 Final Research Report Summary
  • [Publications] T. Tanaka and A. Masuda: "On the half life of <^(138)La> " Nature. 306. 503-504 (1983)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1986 Final Research Report Summary
  • [Publications] H. Shimizu, T. Tanaka-and A. Masuda: "Meteoritic <^(138)Ce> / <^(142)Ce> ratio and its evolution" Nature. 307. 251-252 (1984)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1986 Final Research Report Summary
  • [Publications] A. Masuda and K. Takahashi: "The Differentiated Meteorites, Viwed from REE and Isotopic Cosmochemistry (in Japanese)" The Earth Monthly. 7. 498-505 (1985)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1986 Final Research Report Summary
  • [Publications] S. Nakai, H. Shimizu and A. Masuda: "A new geochronometer using lanthanum-138" Nature. 320. 433-435 (1986)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1986 Final Research Report Summary
  • [Publications] K. Takahashi, A. Masuda and H. Shimizu: "REE abundances and Rb-Sr geochronology of Yamato-791197" Mem. Natl Inst. Polar Res.Spec. Issue No. 41. 96-105 (1986)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1986 Final Research Report Summary
  • [Publications] H. Shimizu: "Re-Os system as a new method in geochemical study of oceanic crust (in Japanese)" The Earth Monthly. 8. 493-496 (1986)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1986 Final Research Report Summary
  • [Publications] H. Shimizu and A. Masuda: "REE patterns of eucrites and their genetic implications" Geochim. Cosmochim. Acta. 50. 2453-2460 (1986)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1986 Final Research Report Summary
  • [Publications] A. Masuda, T. Hirata and H. Shimizu: "Determinations of osmium isotope ratios in iron meteorites and iridosmines by ICP-MS" Geochem. J.20. 233-239 (1986)

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1986 Final Research Report Summary
  • [Publications] K. Takahashi and A. Masuda: "Two lunar meteorites, Y-791197 and Y-82192: REE abundances and geochronological dating" Mem. Natl Inst. Polar Res.

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1986 Final Research Report Summary
  • [Publications] S. Hishita and A. Masuda: "Thousandfold variation in <^(235)U> / <^(238)U> ratios observed in a uranium sample from Oklo: Evidence for Pu segregation" Naturwissenschaften.

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1986 Final Research Report Summary
  • [Publications] A. Makishima, H. Shimizu and A. Masuda: "Precise measurement of cerium and lanthanum isotope ratios" Mass Spectroscopy.

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1986 Final Research Report Summary
  • [Publications] T. Tanaka, H. Shimizu, Y. Kawata and A. Masuda: "La-Ce and Sm-Nd combined isotopic systematics, with theoretical considerations and observed data" Nature.

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1986 Final Research Report Summary
  • [Publications] H. Hidaka and A. Masuda: "Nuclide analyses of rare-earth elements of the Oklo uranium ore samples: ore formation and reactor working conditions" Earth Planet. Sci. Lett.Submitted.

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1986 Final Research Report Summary
  • [Publications] K. Takahashi and A. Masuda: Kokin Shoin. Chemistry of Antarctic meteorites (in "Science of the Antarctic Vol.6 Antarctic meteorites"),

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1986 Final Research Report Summary
  • [Publications] Nature. (1986)

    • Related Report
      1985 Annual Research Report
  • [Publications] Proc 10th Symposium on Antarctic Meteorites. (1985)

    • Related Report
      1985 Annual Research Report

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Published: 1987-03-31   Modified: 2016-04-21  

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