Project/Area Number |
61540231
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Research Category |
Grant-in-Aid for General Scientific Research (C)
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Allocation Type | Single-year Grants |
Research Field |
固体物性
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Research Institution | Toyohashi University of Technology |
Principal Investigator |
OOTA Akio Associate Proceffor, Toyohashi University of Technology, 工学部, 助教授 (10124728)
|
Co-Investigator(Kenkyū-buntansha) |
NOGUCHI Seiichiro Professor, Toyohashi University of Technology, 工学部, 教授 (30023013)
KOYOMA Kuniyuki Research Associate, Toyohashi University of Technology, 工学部, 助手 (40170394)
|
Project Period (FY) |
1986 – 1987
|
Project Status |
Completed (Fiscal Year 1987)
|
Budget Amount *help |
¥1,900,000 (Direct Cost: ¥1,900,000)
Fiscal Year 1987: ¥300,000 (Direct Cost: ¥300,000)
Fiscal Year 1986: ¥1,600,000 (Direct Cost: ¥1,600,000)
|
Keywords | Ternary Silicides / Iron-Containing / Superconductivity / Stoichiometry / Electrical Resistivity / Magnetic Susceptibility / Pauli paramagnetism / Residual Resistivity Ratio / ホール係数 / 希土類化合物 / 鉄を含む化合物 |
Research Abstract |
Superconductivity has been studied through electrical resistivity, Hall coefficient and AC susceptibility on a series of iron-containing rare earth silicides Lu-Fe-Si around the stoichiometric composition Lu_2Fe_3Si_5. The superconducting transition temperature T_c shows a maximum (-6.0K) on the stoichiometry and decreases with a deviation from itespecially on the Fe-rich side. The upper critical field for Lu_2Fe_3Si_5 increases linearly with decreasing temperature with a slope of about 1.5 Tesla/K, which is nearly the same as the ones for other off-stoichiometic samples in spite of the difference in T_2. All samples show a monotonic increase in resistivity with temperature in the range between T_c and 300K. The resistivity ratio <vho>(300K)/<rho>(6K) equals to -16 for Lu_2Fe_3Si_5 and decreases with a deviation from the stoichiometry especially on the Fe-rich side, which indicates the appearance of disorder in the sample as expected from the result of T_c. All samples show T^2 dependence of resistivity at lowtemperatures, which is interpreted in terms of electron-electron scattering. The carrier concentration of Lu_2Fe_3 obtained from Hall coefficiet is independent of temperature between T_c ad 300K, and is estimated to be 6 x 10^<27> m^<-3>, which is compared with 1 x 10^<27> m^<-3> for another isostructural sample Y_2Fe_3Si_5 with T_c = 2.4K. The difference in T_c between them would be ascribed to the difference of carrier concentration.
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