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X ray inelastic scattering spectroscopy for electron momentum density in solids

Research Project

Project/Area Number 62460031
Research Category

Grant-in-Aid for General Scientific Research (B)

Allocation TypeSingle-year Grants
Research Field 固体物性
Research Institution東京水産大学 (1989)
The Institute of Physical and Chemical Research (1987-1988)

Principal Investigator

SHIOTANI Nobuhiro  Tokyo University of Fisheries, Faculty of Fisheries, Professor, 水産学部, 教授 (30087415)

Co-Investigator(Kenkyū-buntansha) ITOH Fumitake  Gunma University, Faculty of Engineering, Professor, 工学部, 教授 (60005907)
SAKAI Nobuhiko  Institute of Physical and Chemical Research, Senior Researcher, 磁性研究室, 副主任研究員 (60013497)
Project Period (FY) 1987 – 1989
Project Status Completed (Fiscal Year 1989)
Budget Amount *help
¥6,300,000 (Direct Cost: ¥6,300,000)
Fiscal Year 1989: ¥400,000 (Direct Cost: ¥400,000)
Fiscal Year 1988: ¥1,000,000 (Direct Cost: ¥1,000,000)
Fiscal Year 1987: ¥4,900,000 (Direct Cost: ¥4,900,000)
KeywordsCompton scattering / Synchrotron radiation / Electron momentum density / Spin-dependent momentum density / Fermi surface / Band theory / Bonding electron / Elliptically polarized X rays / 放射光 / 二重湾曲モノクロメ-タ- / 耐熱特性 / 電子運動量分布 / 直線偏光X線 / コンプトニプロファイル / 円偏光X線 / 超イオン電導 / フェルミモメンタム / 位置敏感X線検出器 / 軌道放射光 / 磁気コンプトン散乱
Research Abstract

Compton scattering measurement is a unique method to study electron momentum density distributions in matter. This work has been done mostly at Photon Factory, National Laboratory for High Energy Physics. The results obtained are as follows;
1. A high resolution Comptonspectrometer for 29.5keV incident X rays.has been constructed at Beam Line 14C. It consists of a bent crystal monochromator, a Cauchois type crystal analyzer for energy analysis of Compton scattered X rays and a sheet of Imaging Plate as a position sensitive detector. The momentum resolution is 0.09 atomic units. With this Compton profiles of Si, Al and liquid Li, Na, Li-Na alloy were measured. Information on the band structure and the effects of electron-electron correlation has been obtained. The Compton profiles of LiH, Li_2O,and Li_3N were also measured and information on the bonding electrons in these compounds has been obtained.
2. At Beam Line AR-NE1 another more advanced spectrometer has been constructed. This one is for 40-80keV incident X rays and consists of a quasi doubly bent monochromator and four pairs of Cauchois type analyzer and Imaging Plate. With this Compton profiles along four different crystalline axes can be measured simultaneously. The three dimensional electron momentum density map can be reconstructed from the profiles taken along various crystalline axes to get much detailed information on the band structure and the Fermi surface geometry in metals and alloys.
3. Electron-spin dependent Compton profiles of Fe and Ni single crystals were measured and compared with the band theoretical results. One of the conclusions obtained is that the momentum-wavefunctions of the magnetic electrons in these metals are well described by the band theory. It has been demonstrated that elliptically polarized synchrotron radiation X rays are quite useful to study magnetic properties of ferromagnetic materials.

Report

(4 results)
  • 1989 Annual Research Report   Final Research Report Summary
  • 1988 Annual Research Report
  • 1987 Annual Research Report
  • Research Products

    (41 results)

All Other

All Publications (41 results)

  • [Publications] N.Shiotani: "An X-Ray Spectrometer for Compton Scattering Experiments with Synchrotron Radiation" Nucl.Instrum and Method. A275. 447-452 (1989)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1989 Final Research Report Summary
  • [Publications] N.Shiotani: "Compton Profiles of Aluminuum and Silion" J.phys.:Condens.Matter. 1. SA27-SA31 (1989)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1989 Final Research Report Summary
  • [Publications] S.Yamamoto: "First Production of Intense Circularly Polarized Hard X Rays from a Novel Multipole Wiggler in an Accumulation Ring" Phys.Rev.Lett.62. 2672-2675 (1989)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1989 Final Research Report Summary
  • [Publications] N.Sakai: "High-Resolution Compton Profile of Si Using 29.5 keV Synchrotron-Radiation X-Rays'" J.Phys.Soc.Jpn.58. 3270-3279 (1989)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1989 Final Research Report Summary
  • [Publications] N.Sakai: "Challenge to Precise Magnetic Compton-Profile Measurements" Rev.Sci.Instrum.60. 1666-1670 (1989)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1989 Final Research Report Summary
  • [Publications] F.Itoh: "High-Rssolution Compton Profile Spectrometer for 29.5keV X-Rays' with a Combination of Crystal Analyser and Imaging Plate" Rev.Sci.Instrum.60. 2402-2405 (1989)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1989 Final Research Report Summary
  • [Publications] F.Itoh: "High Resolution Compton Profile of Liquid Li,Na and Li-Na Alloys'" J.Non-Cryst.Solids. in press.

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1989 Final Research Report Summary
  • [Publications] N.Sakai: "Compton-Profile Observation of Negative Spin Polarization of Conduction Electrons in Ferromagnetic Ni Metal" Photon Factory Activity Report. in press.

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1989 Final Research Report Summary
  • [Publications] N.Sakai: "Improved Measurement of Magnetic-Electron Compton Profile of Ferromagnetic Fe" Photon Factory Activity Report. in press.

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1989 Final Research Report Summary
  • [Publications] Y.Sakurai: "High Resolution Compton Spectrometer at AR" Photon Factory Activity Report. in press.

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1989 Final Research Report Summary
  • [Publications] N.Shiotani: "Electron Momentum Density Studied by High Energy X-Ray Compton Scattering" Postitron Annihilation(eds.L.Dorikens-Vanpraet,M.Dorikens and D.Segers,World Scientific). 122-124 (1989)

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1989 Final Research Report Summary
  • [Publications] N.Sakai: "Compton-Profile Investigation on Magnetic Electrons in Ferromagnetic Fe+3%Si and Single Crystals" Phys.Rev.Lett.(to be submitted).

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      1989 Final Research Report Summary
  • [Publications] N. Shiotani: "An X-ray Spectrometer for Compton Scattering Experiments with Synchrotron Radiation" Nucl. Instrum. and Methods, A275, 447-452, 1989.

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1989 Final Research Report Summary
  • [Publications] N. Shiotani: "Compton Profiles of Aluminum and Silicon" J. Phys. : Condens. Matter, 1, SA27-SA31, 1989.

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1989 Final Research Report Summary
  • [Publications] S. Yamamoto: "First Production of Circularly Polarized Hard X Rays from a Novel Multipole Wiggler in an Accumulation Ring" Phys. Rev. Lett., 62, 2672-2675, 1989.

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1989 Final Research Report Summary
  • [Publications] N. Sakai: "High-Resolution Compton Profile of Si Using 29.5keV Synchrotron-Radiation X-Rays" J. Phys. Soc. Jpn., 58, 3270-3279, 1989.

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1989 Final Research Report Summary
  • [Publications] N. Sakai: "Challenge to Precise Magnetic Compton-Profile Measurements" Rev. Sci. Instrum., 60, 1666-1670, 1989.

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1989 Final Research Report Summary
  • [Publications] F. Itoh: "High-Resolution Compton Profile Spectrometer for 29.5 keV X-Rays with a Combination of Crystal Analyzer and Imaging Plate" Rev. Sci. Instrum., 60, 2402-2405 1989.

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1989 Final Research Report Summary
  • [Publications] F. Itoh: "High Resolution Compton Profiles of Liquid Li, Na and Li-Na alloy" J. Non-Cryst. Solids, in press. 1990.

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1989 Final Research Report Summary
  • [Publications] N. Sakai: "Compton-Profile Observation of Negative Spin Polarization in Ferromagnetic Ni metal" Photon Factory Activity Report, in press. 1990.

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1989 Final Research Report Summary
  • [Publications] N. Sakai: "Improved Measurement of Magnetic-Electron Compton Profiles of Ferromagnetic Fe" ibid.

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1989 Final Research Report Summary
  • [Publications] Y. Sakurai: "High Resolution Compton Spectrometer at AR" ibid.

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1989 Final Research Report Summary
  • [Publications] N. Shiotani: "Electron Momentum Density Studied by High Energy X-Ray Compton Scattering" Positron Annihilation, eds. L. Dorikens-Vanpraet et al. World Scientific, 122-124, 1989.

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1989 Final Research Report Summary
  • [Publications] N. Sakai: "Compton-Profile investigation on Magnetic Electrons in Ferromagnetic Fe+3%Si and Ni Single Crystals" To be submitted to Phys. Rev. Lett.

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      1989 Final Research Report Summary
  • [Publications] N.Shiotani: "An X-Ray Spectrometer for Compton Scattering Experiments with Synchrotron Radiation" Nucl.Instrum.and Methods. A275. 447-452 (1989)

    • Related Report
      1989 Annual Research Report
  • [Publications] N.Shiotani: "Compton Profiles of Aluminium and Silicon" J.Phys.:Condens.Matter. 1. SA27-SA31 (1989)

    • Related Report
      1989 Annual Research Report
  • [Publications] S.Yamamoto: "First Production of Intense Circularly Polarized Hard X Rays from a Novel Multipole Wiggler in an Accumulation Ring" Phys,Rev.Lett.62. 2672-2675 (1989)

    • Related Report
      1989 Annual Research Report
  • [Publications] N.Sakai: "High-Resolution Compton Profile of Si Using 29.5 keV Synchrotron-Radiation X-Rays" J.Phys.Soc.Jpn.58. 3270-3279 (1989)

    • Related Report
      1989 Annual Research Report
  • [Publications] N.Sakai: "Challenge to Precise Magnetic Compton-Profile Measurements" Rev.Sci.Instrum.60. 1666-1670 (1989)

    • Related Report
      1989 Annual Research Report
  • [Publications] F.Itoh: "High-Resolution Compton Profile Spectrometer for 29.5keV X-Rays with a Combination of Crystal Analyzer and Imaging Plate" Rev.Sci.Instrum.60. 2402-2405 (1989)

    • Related Report
      1989 Annual Research Report
  • [Publications] F.Itoh: "High Resolution Compton Profiles of Liquid Li,Na and Li-Na Alloys" J.Non-Cryst.Solids. in press.

    • Related Report
      1989 Annual Research Report
  • [Publications] N.Sakai: "Compton-Profile Observation of Negative Spin Polarization of Conduction Electrons in Ferromagnetic Ni Metal" Photon Factory Activity Report.

    • Related Report
      1989 Annual Research Report
  • [Publications] N.Sakai: "Improved Measurement of Magnetic-Electron Compton Profitas of Ferromagnetic Fe" Photon Factory Activity Report.

    • Related Report
      1989 Annual Research Report
  • [Publications] Y.Sakurai: "High Resolution Compton Spectrometer at AR" Photon Factory Activity Report.

    • Related Report
      1989 Annual Research Report
  • [Publications] N.Shiotani: "Electron Momentum Density Studied by High Energy X-Ray Compton Scattering" Positron Annihilation eds.L.Dorikens-Vanpraet,(World Scientific) M.Dorikens and D.Segers. 122-124 (1989)

    • Related Report
      1989 Annual Research Report
  • [Publications] N.Shiotani 他: Nucl.Instr.and Methods. A275. 447-452 (1989)

    • Related Report
      1988 Annual Research Report
  • [Publications] N.Sakai 他: Rew.scien.Instr.(1989)

    • Related Report
      1988 Annual Research Report
  • [Publications] F.Itoh 他: Rew.Scien.Instr.(1989)

    • Related Report
      1988 Annual Research Report
  • [Publications] N.Shiotani 他: J.Phys.C Condensed Matter. (1989)

    • Related Report
      1988 Annual Research Report
  • [Publications] N.Shiotani 他: Proc.8th Int.Cont.Positron Annihilation. (1989)

    • Related Report
      1988 Annual Research Report
  • [Publications] S.Yamamoto 他: Phys.Rew.Lett.

    • Related Report
      1988 Annual Research Report

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Published: 1987-04-01   Modified: 2016-04-21  

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