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NQR Studies on Magnetism and Superconductivity of Oxides Superconductors

Research Project

Project/Area Number 63540267
Research Category

Grant-in-Aid for General Scientific Research (C)

Allocation TypeSingle-year Grants
Research Field 物性一般(含極低温・固体物性に対する理論)
Research InstitutionFaculty of Science, Hokkaido University

Principal Investigator

KUMAGAI Ken-ichi  Hokkaido Univ., Dept. of Physics, Associate Professor, 理学部, 助教授 (70029560)

Co-Investigator(Kenkyū-buntansha) NAKAJIMA Haruo  Hokkaido Univ., Dept. Physics, Professor, 理学部, 教授 (10000796)
Project Period (FY) 1988 – 1989
Project Status Completed (Fiscal Year 1989)
Budget Amount *help
¥2,000,000 (Direct Cost: ¥2,000,000)
Fiscal Year 1989: ¥300,000 (Direct Cost: ¥300,000)
Fiscal Year 1988: ¥1,700,000 (Direct Cost: ¥1,700,000)
KeywordsNuclear Magnetic Resonance / Nuclear Spin-Lattice Relaxation Time / High-T_c Superconductor / Antiferromagnetism / 磁気秩序
Research Abstract

Nuclear quadrupole resonances (NQR) of ^<139>La and ^<63,65>Cu have been investigated in the wide range of x in hole-doped La_<2-x>M_xCuO_4 (M=Sr, Ba). The divergence of the nuclear relaxation rate of ^<139>La at T_c*-10K indicates the existence of the peculiar frustrated magnetic phase between the 3D-antiferro- magnetic and superconducting phases. The spin echo signals of ^<63,65>Cu are observed between 30-50KHz in zero external field. The spectra consist of the two component of the Cu-NQR lines for x<0.4, of which origin is still unclear. Relaxation rates, 1/T_1 and 1/T_2 are much enhanced with decreasing x. The temperature dependence of 1/T_1 for x>0.4 obeys the Korringa relation, T_1T=const., below 200K.
We have confirmed the antiferromagntic order of Cu moments in the electron-doped Ln_<2-x>Ce_xCuO_4 (Ln =Nd, Pr, Sm). Unexpected observation of nuclear magnetic resonance (NMR) with vanishingly small quadrupole interactions in the Ce-doped samples suggests that the local electronic properties at Cu site in the electron-doped oxides differ from the hole-doped ones.

Report

(3 results)
  • 1989 Annual Research Report   Final Research Report Summary
  • 1988 Annual Research Report
  • Research Products

    (12 results)

All Other

All Publications (12 results)

  • [Publications] 熊谷健一: "Absence of the Linear-Temperature Term in Heat Cpapacity of the Bi-Sr-Ca-Cu-O System" Physica. 152C. 286-288 (1988)

    • Related Report
      1989 Annual Research Report
  • [Publications] 渡辺功雄: "Effects of Oxygen and Magnetic Imputies on Nuclear Relaxation Anomalies in La-M-Cu-O System." J.Magnetism and Magnetic Materials. 76&77. 599-600 (1988)

    • Related Report
      1989 Annual Research Report
  • [Publications] 熊谷健一: "^<139>La-NQR and Heat Capacity of La_<2-x>M_xCuO_4(M=Ba,Sr)" Jpn.J.Appl.Phys.Series 1. 1. 37-41 (1988)

    • Related Report
      1989 Annual Research Report
  • [Publications] 熊谷健一: "Evidence of Magnetic Order of Cu-Moments in the Superconducting and Nornal Region of La_<2-x>Sr_xCuO_4:Observstion of Cu-NQR" Physica. 157C. 307-314 (1989)

    • Related Report
      1989 Annual Research Report
  • [Publications] 大芦敏行: "Observation of Cu-NQR in Bi_2Sr_2(Ca_<1-x>Y_x)Cu_2O_<8+y>" Physica. 157C. 315-319 (1989)

    • Related Report
      1989 Annual Research Report
  • [Publications] 和田信雄: "Observation of the Static Magnetic Moment on the Cupper Site in the Superconducting La_<2-x>Sr_4CuO_4:Nuclear Heat Capacity Measurement" Physica. 157C. (1989)

    • Related Report
      1989 Annual Research Report
  • [Publications] 熊谷健一: Physica. 152C. 286-288 (1988)

    • Related Report
      1988 Annual Research Report
  • [Publications] 渡辺功雄: J.Magnetism and Magnetic Materials. 76&77. 599-600 (1988)

    • Related Report
      1988 Annual Research Report
  • [Publications] 熊谷健一: Jpn.J.Appl.Phys.Series 1. 1. 37-41 (1988)

    • Related Report
      1988 Annual Research Report
  • [Publications] 熊谷健一: Physica. 157C. 307-314 (1989)

    • Related Report
      1988 Annual Research Report
  • [Publications] 大芦敏行: Physica. 157C. 315-319 (1989)

    • Related Report
      1988 Annual Research Report
  • [Publications] 和田信雄: Physica. 157C. (1989)

    • Related Report
      1988 Annual Research Report

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Published: 1988-04-01   Modified: 2016-04-21  

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