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Advanced direct local structure determination of quasicrystals in physical space

Publicly Offered Research

Project AreaHypermaterials: Inovation of materials scinece in hyper space
Project/Area Number 22H04595
Research Category

Grant-in-Aid for Scientific Research on Innovative Areas (Research in a proposed research area)

Allocation TypeSingle-year Grants
Review Section Science and Engineering
Research InstitutionKyoto University

Principal Investigator

STELLHORN JENSRUEDIGER  京都大学, 工学研究科, 特定研究員 (90868431)

Project Period (FY) 2022-04-01 – 2024-03-31
Project Status Completed (Fiscal Year 2023)
Budget Amount *help
¥4,030,000 (Direct Cost: ¥3,100,000、Indirect Cost: ¥930,000)
Fiscal Year 2023: ¥1,950,000 (Direct Cost: ¥1,500,000、Indirect Cost: ¥450,000)
Fiscal Year 2022: ¥2,080,000 (Direct Cost: ¥1,600,000、Indirect Cost: ¥480,000)
Keywordshypermaterial / atomic structure / X-ray holography / local structure / quasicrystal / micro-focus / Quasicrystals / Hypermaterials / Atomic structure / X-ray Holography / hypermaterials / synchrotron methods / local order / x-ray holography
Outline of Research at the Start

The project contributes to understand complex atomic arrangements in hypermaterials using atomic resolution holography, in particular with low-temperature and nano-focus implementations. This will establish a new way to visualize aperiodic structures with a direct and element-selective approach.

Outline of Annual Research Achievements

This project was able to significantly widen the area of applicability of Atomic Resolution Holography (ARH) experiments for hypermaterials.
First experiments to test soft X-ray measurements were successfully conducted and show the feasibility for the detection of lighter elements, specifically Al, which is a significant building block in numerous hypermaterials. Moreover, micro-focus measurements were conducted with international collaboration at Japanese and European facilities, and were able to uncover a new phenomenon related to the ordering of icosahedral clusters within icosahedral quasicrystals and approximants.
The scientific results have been presented at various international conferences.
The results of this project open up the way for the investigation of the local atomic structure of other hypermaterials. The novel implementations developed in this project will also support investigations of other structurally complex systems, in particular those with large structural disorder. Furthermore, as a direct result of this project, it is also planned to evaluate how X-ray holography can complement the investigation of local disorder measured by Diffuse Scattering methods. The combination of both techniques may yield an accurate structural picture of the local atomic environment over several length scales from few atomic bonds (a few tenths of nm) to the nanoscale (a few dozen nm).

Research Progress Status

令和5年度が最終年度であるため、記入しない。

Strategy for Future Research Activity

令和5年度が最終年度であるため、記入しない。

Report

(2 results)
  • 2023 Annual Research Report
  • 2022 Annual Research Report
  • Research Products

    (9 results)

All 2023 2022 Other

All Int'l Joint Research (3 results) Presentation (6 results) (of which Int'l Joint Research: 4 results,  Invited: 1 results)

  • [Int'l Joint Research] Science and Engineering of Materials/and Processes/SIMAP(フランス)

    • Related Report
      2023 Annual Research Report
  • [Int'l Joint Research] Marburg University(ドイツ)

    • Related Report
      2023 Annual Research Report
  • [Int'l Joint Research] Science and Engineering of Materials/and Processes/SIMAP(フランス)

    • Related Report
      2022 Annual Research Report
  • [Presentation] Local Atomic Order in Hypermaterials and Hyperordered Structures2023

    • Author(s)
      Jens R. Stellhorn
    • Organizer
      International Conference on Complex Orders in Condensed Matter:aperiodic order, local order, electronic order, hidden order (ICOCCM)
    • Related Report
      2023 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Investigating the local structure of icosahedral phases by Atomic Resolution Holography2023

    • Author(s)
      Jens R. Stellhorn
    • Organizer
      IUCr conference
    • Related Report
      2023 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Investigation of the Local Atomic Structure of Quasicrystals by Atomic Resolution Holography2023

    • Author(s)
      Jens R. Stellhorn
    • Organizer
      International Conference on Quasicrystals, ICQ15
    • Related Report
      2023 Annual Research Report 2022 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Unravelling disorder in aperiodic systems by diffuse scattering and atomic resolution holography2023

    • Author(s)
      Jens R. Stellhorn
    • Organizer
      Quasicrystal meeting 2023
    • Related Report
      2023 Annual Research Report
  • [Presentation] Atomic Resolution Holography to Study the Local Structure in Quasicrystals2022

    • Author(s)
      Jens R. Stellhorn
    • Organizer
      European Crystallographic Meeting, ECM33
    • Related Report
      2022 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Recent progress of Atomic Resolution Holography for icosahedral systems2022

    • Author(s)
      Jens R. Stellhorn
    • Organizer
      8th Hypermaterials Meeting
    • Related Report
      2022 Annual Research Report

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Published: 2022-04-19   Modified: 2024-12-25  

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