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2010 Fiscal Year Final Research Report

Assessment and control of radiative/nonradiative recombination processes in In-rich InGaN and in Al-rich AlGaN

Planned Research

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Project AreaOptoelectronics Frontier by Nitride Semiconductor -Ultimate Utilization of Nitride Semiconductor Material Potential-
Project/Area Number 18069007
Research Category

Grant-in-Aid for Scientific Research on Priority Areas

Allocation TypeSingle-year Grants
Review Section Science and Engineering
Research InstitutionKyoto University

Principal Investigator

KAWAKAMI Yoichi  Kyoto University, 大学院・工学研究科, 教授 (30214604)

Co-Investigator(Kenkyū-buntansha) FUNATO Mitsuru  京都大学, 大学院・工学研究科, 准教授 (70240827)
Project Period (FY) 2006 – 2010
KeywordsInGaN / AlGaN / 輻射再結合 / 非輻射再結合 / 発光機構解明
Research Abstract

For high In-content InGaN, we proposed to use {11-22} semipolar planes and demonstrated high radiative recombination probabilities in semipolar InGaN quantum wells (QWs). Furthermore, LEDs emitting in the blue to red spectral region were fabricated on this semipolar {11-22} plane. In addition, to assess optical properties in InGaN QWs, a scanning near-field optical microscope that uses two independent fiber probes was developed, by which carrier dynamics were visualized. For high Al-content AlGaN, we first established the growth method to obtain high quality films on sapphire (0001) substrates. The guideline to extract intense emission from AlGaN QWs grown on the (0001) plane was clarified. Based on this guideline, high power efficiency (max. 40%) and high emission power (max 100mW) were achieved at ~240nm from an AlGaN QW pumped by an electron beam.

  • Research Products

    (42 results)

All 2010 2009 2008 2007 2006 Other

All Journal Article (22 results) (of which Peer Reviewed: 22 results) Presentation (13 results) Book (4 results) Remarks (1 results) Patent(Industrial Property Rights) (2 results) (of which Overseas: 1 results)

  • [Journal Article] All deformation potentials in GaN determined by reflectance spectroscopy under uniaxial stress: definite breakdown of the quasicubic approximation2010

    • Author(s)
      R.Ishii, A.Kaneta, M.Funato, Y.Kawakami, A.A.Yamaguchi
    • Journal Title

      Phys.Rev.B 81

      Pages: 155202/1-155202/11

    • Peer Reviewed
  • [Journal Article] Strain states in semipolar III-nitride semiconductor quantum wells2010

    • Author(s)
      M.Funato, D.Inoue, M.Ueda, Y.Kawakami, Y.Narukawa, T.Mukai
    • Journal Title

      J.Appl.Phys. 107

      Pages: 123501/1-123501/5

    • Peer Reviewed
  • [Journal Article] Valence band effective mass of non-c-plane nitride heterostructures2010

    • Author(s)
      K.Kojima, M.Funato, Y.Kawakami, S.Noda
    • Journal Title

      J.Appl.Phys. 107

      Pages: 123105/1-123105/7

    • Peer Reviewed
  • [Journal Article] 100 mW deep ultraviolet emission from aluminum nitride based quantum wells pumped by an electron beam2010

    • Author(s)
      T.Oto, R.G.Banal, K.Kataoka, M.Funato, Y.Kawakami
    • Journal Title

      NaturePhotonics 4

      Pages: 767-771

    • Peer Reviewed
  • [Journal Article] Characteristics of high Al-content AlGaN/AlN quantum wells fabricated by modified migration enhanced epitaxy2010

    • Author(s)
      R.G.Banal, M.Funato, Y.Kawakami
    • Journal Title

      Phys.Stat.Solidi (C) 7

      Pages: 2111-2114

    • Peer Reviewed
  • [Journal Article] Visualization of the local carrier dynamics in an InGaN quantum well using dual-probe scanning near-field optical microscopy2010

    • Author(s)
      A.Kaneta, T, Hashimoto, K.Nishimura, M.Funato, Y.Kawakami
    • Journal Title

      Appl.Phys.Exp. 3

      Pages: 102102/1-102102/3

    • Peer Reviewed
  • [Journal Article] Positive binding energy of a biexciton confined in a localization center formed in a single InxGa1-xN/GaN quantum disk2009

    • Author(s)
      R.Bardoux, A.Kaneta, M.Funato, Y.Kawakami, A.Kikuchi, K.Kishino
    • Journal Title

      Phys.Rev.B 79

      Pages: 155307/1-155307/6

    • Peer Reviewed
  • [Journal Article] Growth characteristics of AlN on sapphire substrates by modified migration-enhanced epitaxy2009

    • Author(s)
      R.G.Banal, M.Funato, Y.Kawakami
    • Journal Title

      J.Cryst.Growth 311

      Pages: 2834-2836

    • Peer Reviewed
  • [Journal Article] Optical anisotropy control of non-c-plane InGaN quantum wells2009

    • Author(s)
      K.Kojima, H.Kamon, M.Funato, Y.Kawakami
    • Journal Title

      Jpn.J.Appl.Phys. 48

      Pages: 080201/1-080201/3

    • Peer Reviewed
  • [Journal Article] Excitonic properties of polar, semipolar, and nonpolar InGaN/GaN strained quantum wells with potential fluctuations2008

    • Author(s)
      M.Funato, Y.Kawakami
    • Journal Title

      J.Appl.Phys. 103,

      Pages: 093501/1-093501/7

    • Peer Reviewed
  • [Journal Article] Nanoscopic recombination processes InGaN/GaN quantum wells emitting violet, blue, and green spectra2008

    • Author(s)
      A.Kaneta, M.Funato, Y.Kawakami
    • Journal Title

      Phys.Rev.B 78

      Pages: 125317/1-125317/7

    • Peer Reviewed
  • [Journal Article] Polarization switching phenomena in semipolar InxGa1-xN/GaN quantum well active layers2008

    • Author(s)
      M.Ueda, M.Funato, K.Kojima, Y.Kawakami, Y.Narukawa, T.Mukai
    • Journal Title

      Phys.Rev.B 78

      Pages: 233303/1-233303/4

    • Peer Reviewed
  • [Journal Article] Monolithic polychromatic light-emitting diodes based on InGaN microfacet quantum wells toward tailor-made solid-state lighting2008

    • Author(s)
      M.Funato, T.Kondou, K.Hayashi, S.Nishiura, M.Ueda, Y.Kawakami, Y.Narukawa, T.Mukai
    • Journal Title

      Appl.Phys..Exp. 1

      Pages: 011106/1-011106/3

    • Peer Reviewed
  • [Journal Article] Initial nucleation of AlN grown directly on sapphire substrates by metal-organic vapor phase epitaxy2008

    • Author(s)
      R.G.Banal, M.Funato, Y.Kawakami
    • Journal Title

      Appl.Phys.Lett. 92

      Pages: 241905/1-241905/3有

    • Peer Reviewed
  • [Journal Article] Emission color tunable light-emitting diodes composed of InGaN multifacet quantum wells2008

    • Author(s)
      M.Funato, K.Hayashi, M.Ueda, Y.Kawakami, Y.Narukawa, T.Mukai
    • Journal Title

      Appl.Phys.Lett. 93

      Pages: 021126/1-021126/3

    • Peer Reviewed
  • [Journal Article] Optical gain spectra for near UV to aquamarine (A1,In) GaN laser diodes2007

    • Author(s)
      K.Kojima, U.T.Schwarz, M.Funato, Y.Kawakami, S.Nagahama, T.Mukai
    • Journal Title

      Opt.Exp. 15

      Pages: 7730-7736

    • Peer Reviewed
  • [Journal Article] Efficient green emission from (11-22)InGaN/GaN quantum wells on GaN microfacets probed by scanning near field optical microscopy2007

    • Author(s)
      Y.Kawakami, K.Nishizuka, D.Yamada, A.Kaneta, M.Funato, Y.Narukawa, T.Mukai
    • Journal Title

      Appl.Phys.Lett. 90

      Pages: 261912/1-261912/3

    • Peer Reviewed
  • [Journal Article] Blue, green, and amber InGaN/GaN light-emitting diodes on semipolar (11-22) GaN bulk substrates2006

    • Author(s)
      M.Funato, M.Ueda, Y.Kawakami, Y.Narukawa, T.Kosugi, M.Takahashi, T.Mukai
    • Journal Title

      Jpn.J.Appl.Phys 45

      Pages: L659-L662

    • Peer Reviewed
  • [Journal Article] Epitaxial growth and optical properties of semipolar (11-22) GaN and InGaN/GaN quantum wells on GaN bulk substrates2006

    • Author(s)
      M.Ueda, K.Kojima, M.Funato, Y.Kawakami, Y.Narukawa, T.Mukai
    • Journal Title

      Appl.Phys.Lett. 89

      Pages: 211907/1-211907/3

    • Peer Reviewed
  • [Journal Article] Tailored emission color synthesis using microfacet quantum wells consisting of nitride semiconductors without phosphors2006

    • Author(s)
      M.Funato, T.Kotani, T.Kondou, Y.Kawakami, Y.Narukawa, T.Mukai
    • Journal Title

      Appl.Phys.Lett. 88

      Pages: 261920/1-261920/3

    • Peer Reviewed
  • [Journal Article] Direct correlation between nonradiative recombination centers and threading dislocations in InGaN quantum wells by near-field photoluminescence spectroscopy2006

    • Author(s)
      A, Kaneta, M.Funato, Y.Narukawa, T.Mukai, Y.Kawakami
    • Journal Title

      Phys.Stat.Solidi (C) 3

      Pages: 1897-1901

    • Peer Reviewed
  • [Journal Article] Gain suppression phenomena observed in InxGa1-xN quantum well laser diodes emitting at 470 nm2006

    • Author(s)
      K.Kojima, M.Funato, Y.Kawakami, S.Nagahama, T.Mukai, H.Braun, U.T.Schwarz
    • Journal Title

      Appl.Phys.Lett. 89

      Pages: 241127/1-241127/3

    • Peer Reviewed
  • [Presentation] Visualization of the local carrier dynamics in InGaN SQW using dual probe scanning near field optical microscope, Intern.2010

    • Author(s)
      A.Kaneta, T.Hashimoto, K.Nishimura, M.Funato, Y.Kawakami
    • Organizer
      Workshop on Nitride Semicond.
    • Place of Presentation
      Tampa, Florida, USA(Invited)
    • Year and Date
      2010-09-21
  • [Presentation] Impact of breakdown of the quasi-cubic approximation in GaN on the optical polarization properties of nonpolar and semipolar GaN/AlGaN quantum wells, The 37th Intern.2010

    • Author(s)
      R.Ishii, A.Kaneta, M.Funato, Y.Kawakami
    • Organizer
      Symp.on Compound Semicond.
    • Place of Presentation
      Takamatsu, Japan(Invited)
    • Year and Date
      2010-06-01
  • [Presentation] Mapping of efficiency droop in InGaN quantum wells studied by scanning near-field optical microscopy, The 8th Intern.2010

    • Author(s)
      Y.Kawakami, A.Hashiya, A.Kaneta, M.Funato
    • Organizer
      Symp.on Semicond.Light Emitting Devices
    • Place of Presentation
      Beijing, China(Invited)
    • Year and Date
      2010-05-17
  • [Presentation] Semipolar (11-22)-oriented InGaN/GaN LEDs and their optical properties, The 2nd Intern.2009

    • Author(s)
      Y.Kawakami, M.Ueda, A.Kaneta, M.Funato
    • Organizer
      Conf.on White LEDs and Solid State Lighting
    • Place of Presentation
      Taipei, Taiwan(Invited)
    • Year and Date
      2009-12-16
  • [Presentation] Semipolar (11-22)-oriented InGaN/GaN quantum wells, Asia Communications and Photonics Conf.2009

    • Author(s)
      M.Funato, Y.Kawakami
    • Organizer
      and Exhibition
    • Place of Presentation
      Shanghai, China(Invited)
    • Year and Date
      2009-11-03
  • [Presentation] Polarization anisotropy in semipolar/polar nitride semiconductor quantum wells, 8th Intern.Conf.2009

    • Author(s)
      M.Funato, Y.Kawakami
    • Organizer
      on Nitride Semicond.
    • Place of Presentation
      Jeju, Korea(Invited)
    • Year and Date
      2009-10-23
  • [Presentation] Recombination dynamics in semi-polar {11-22} InGaN/GaN quantum wells, 6th Intern.2009

    • Author(s)
      Y.Kawakami
    • Organizer
      Workshop on Bulk Nitride Semicond.
    • Place of Presentation
      Galindia Mazurski Eden, Poland(Invited)
    • Year and Date
      2009-08-25
  • [Presentation] Characterization and control of recombination process in nitride semiconductors2009

    • Author(s)
      Y.Kawakami, A.Kaneta, M.Ueda, M.Funato
    • Organizer
      E-MRS Spring meeting 2009
    • Place of Presentation
      Strasbourg, France(Invited)
    • Year and Date
      2009-06-11
  • [Presentation] Multi-color light-emitting diodes based on GaN micro-structures2009

    • Author(s)
      M.Funato, Y.Kawakami, Y.Narukawa, T.Mukai
    • Organizer
      SPIE Photonics West
    • Place of Presentation
      San Jose, California, USA(Invited)
    • Year and Date
      2009-01-29
  • [Presentation] Monolithic polychromatic InGaN light-emitting diodes based on micro-facet structures, Intern.2008

    • Author(s)
      M.Funato, Y.Kawakami
    • Organizer
      Meeting on Information Display 2008
    • Place of Presentation
      Ilsan, Korea(Invited)
    • Year and Date
      2008-10-16
  • [Presentation] Polarization anisotropy in semipolar InGaN/GaN quantum well active layers, Intern.2008

    • Author(s)
      M.Ueda, M.Funato, Y.Narukawa, T.Mukai, Y.Kawakami
    • Organizer
      Workshop on Nitride Semicond.
    • Place of Presentation
      Montreux, Switzerland(Invited)
    • Year and Date
      2008-10-09
  • [Presentation] Characterization and Control of recombination dynamics in low-dimensional InGaN-based semiconductors, The 3rd Intern.Conf.2008

    • Author(s)
      Kawakami, A.Kaneta, M.Funato, Y.Narukawa, T.Mukai
    • Organizer
      Smart Materials Structures Systems
    • Place of Presentation
      Acireale, Sicily, Italy(Invited)
    • Year and Date
      2008-06-09
  • [Presentation] Local Spectroscopic Investigations on Semipolar InGaN-Based Nanostructures and Their Application to LEDs, 7th Intern.Conf.2007

    • Author(s)
      Y.Kawakami, A.Kaneta, K.Nishizuka, M.Ueda, K.Kojima, M.Funato, Y.Narukawa, T.Mukai
    • Organizer
      on Nitride Semicond.
    • Place of Presentation
      Las Vegas, USA(Invited)
    • Year and Date
      2007-07-10
  • [Book] 窒化物基板および格子整合基板の成長とデバイス特性2009

    • Author(s)
      船戸充, 川上養一
    • Total Pages
      104-118
    • Publisher
      シーエムシー出版
  • [Book] Nitrides with Nonpolar Surfaces : Growth, Properties, and Devices edited by T.Paskova, WILEY-VCH2008

    • Author(s)
      M.Funato, Y.Kawakami, Y.Narukawa, T.Mukai(分担執筆)
    • Total Pages
      385-411
    • Publisher
      Semipolar InGaN/GaN quantum wells for highly functional light emitters
  • [Book] Materials Science Forum 590, Trans Tech Publications2008

    • Author(s)
      Y.Kawakami, A.Kaneta, M.Funato(分担執筆)
    • Total Pages
      249-274
    • Publisher
      Assessment and Modification of Recombination Dynamics in InxGa1-xN-Based Quantum Wells Advances in Light Emitting Materials
  • [Book] 発光と受光の物理と応用2,3章2007

    • Author(s)
      川上養一
    • Total Pages
      22-35
    • Publisher
      培風館
  • [Remarks] ホームページ

    • URL

      http://www.optomater.kuee.kyoto--u.ac.jp/

  • [Patent(Industrial Property Rights)] 紫外線照射装置2010

    • Inventor(s)
      川上養一, 船戸充, 大音隆男, R.G.Banal, 外3名
    • Industrial Property Rights Holder
      京都大学, ウシオ電機(株)
    • Industrial Property Number
      特許,2010-128252
    • Filing Date
      2010-06-03
  • [Patent(Industrial Property Rights)] 紫外線照射装置2010

    • Inventor(s)
      岡本晃一, 船戸充, 川上養一, 外2名
    • Industrial Property Rights Holder
      京都大学, ウシオ電機(株), 外5名
    • Industrial Property Number
      特許,PCT/JP2010/063102
    • Filing Date
      2010-08-03
    • Overseas

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Published: 2012-02-13   Modified: 2016-04-21  

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