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2011 Fiscal Year Final Research Report

Fabrication of functionalized materials by realizing appropriate doping technology

Planned Research

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Project AreaNano Materials Science for Atomic Scale Modification
Project/Area Number 19053008
Research Category

Grant-in-Aid for Scientific Research on Priority Areas

Allocation TypeSingle-year Grants
Review Section Science and Engineering
Research InstitutionNational Institute for Materials Science

Principal Investigator

TANIGUCHI Takashi  独立行政法人物質・材料研究機構, 先端材料プロセスユニット, グループリーダー (80354413)

Co-Investigator(Kenkyū-buntansha) HIRAGA Keijiro  北見工業大学, 工学部, 教授 (80354190)
YOSHIDA Hidehiro  物質・材料研究機構, 先端材料プロセスユニット, 主幹研究員 (80313021)
SAKAGUCHI Isao  物質・材料研究機構, 先端材料プロセスユニット, 主幹研究員 (20343866)
WADA Yoshiki  物質・材料研究機構, 先端材料プロセスユニット, 主幹研究員 (90343847)
OHASHI Naoki  物質・材料研究機構, 環境・エネルギー部門, 部門長 (60251617)
Project Period (FY) 2007 – 2011
Keywords機能性セラミックス / 超塑性 / 粒界構造制御 / 超硬質材料
Research Abstract

The aim of this study is to obtain high quality functionalized materials by realizing appropriate doping technology under the variety of synthesis process, including high pressure and high temperature process, solid-state reaction, and thin film growth technique. By cooperating with the researchers in theoretical and ultimate structural analysis field, we tried to control the effective doping technology for the functionalized nitride and oxide ceramic materials. Successful doping with large misfit in highly covalent rigid crystals was achieved. Theoretical and structural analyses clearly show the occupancy site in the crystal by defect complex model. This fact suggests the way of functionalization by doping in the large lattice misfit systems. New multifunctional oxide polycrystalline materials have been developed through the atomic modification which controls high temperature matter transport in grain boundary and interface. Synthesis and characterization of oxide semiconductor films were performed aiming to develop electronic devices by utilizing the advantages in the concept of Nano-Dopant.

  • Research Products

    (50 results)

All 2011 2010 2009 2008 2007

All Journal Article (29 results) (of which Peer Reviewed: 29 results) Presentation (17 results) Patent(Industrial Property Rights) (4 results)

  • [Journal Article] Hot Carrier-Assisted Intrinsic Photoresponse in Graphene2011

    • Author(s)
      N.M.Gabor, T.Taniguchi, P. Jarillo-Herrero, 計9名.
    • Journal Title

      Science

      Volume: 344 Pages: 648

    • Peer Reviewed
  • [Journal Article] Tunable metal-insulator transition in double-layer graphene heterostructures2011

    • Author(s)
      L.A.Ponomarenko, A.K.Geim, T.Taniguchi, 計13名.
    • Journal Title

      Nat.Phys.

      Volume: 7 Pages: 958

    • Peer Reviewed
  • [Journal Article] Spectroscopic analysis of Eu^<3+> in single-crystal hexagonal phase AlN2011

    • Author(s)
      J. B. Gruber, U. Vetter, T. Taniguchi, 計7名
    • Journal Title

      J.Appl.Phys.

      Volume: 110 Pages: 023104

    • Peer Reviewed
  • [Journal Article] Low Temperature Spark Plasma Sintering of Yttria Ceramics with Ultrafine Grain Size2011

    • Author(s)
      H. Yoshida, K. Hiraga, K. Yamanaka, 計7名
    • Journal Title

      J. Am. Cearm. Soc.

      Volume: 94 [10] Pages: 3301-3307

    • Peer Reviewed
  • [Journal Article] Fabrication of Transparent Yttria by High-Pressure Spark Plasma Sintering2011

    • Author(s)
      H. Zhang, B.-N.Kim, K.Morita, H.Yoshida, K.Hiraga, Y.Sakka
    • Journal Title

      J. Am. Cearm. Soc

      Volume: 94 Pages: 3206

    • Peer Reviewed
  • [Journal Article] High-Strain-Rate Superplasticity in Oxide Ceramics: a Trial of Microstructural Design Based on Creep-Cavitation Mechanisms2011

    • Author(s)
      K.Hiraga, H.Yoshida, 計6名
    • Journal Title

      Acta Metallurgica Sinica

      Volume: 24 Pages: 195

    • Peer Reviewed
  • [Journal Article] Photocatalytic Activity And Related Surface Properties of Transparent ZnO Films Prepared By A Low-Temperature Aqueous Route2011

    • Author(s)
      H. Wagata, N, Ohashi, 計8名
    • Journal Title

      Photochem, Photobio

      Volume: 87 Pages: 1009

    • Peer Reviewed
  • [Journal Article] Polarity Of Heavily Doped ZnO Films Grown On Sapphire And SiO_2 Glass Substrates By Pulsed LaserDeposition2011

    • Author(s)
      Y.Adachi, N. Ohashi, 計11名
    • Journal Title

      Thin Solid Films

      Volume: 519(18) Pages: 5875-5881

    • Peer Reviewed
  • [Journal Article] Polarity Determination Of Wurtzite-Type Crystals Using Hard X-Ray Photoelectron Diffraction2011

    • Author(s)
      J.R.Williams, N.Ohashi, 計7名
    • Journal Title

      Surface Science

      Volume: 605 (13-14) Pages: 1336-1340

    • Peer Reviewed
  • [Journal Article] Visualization Of Grain Boundary As Blocking Layer For Oxygen Tracer Diffusion And A Proposed Defect Model In Non Doped BaTiO_3 Ceramics2011

    • Author(s)
      K.Watanabe, N.Ohashi, 計10名
    • Journal Title

      Applied Physics Express

      Volume: 4 (5), AR 055801

    • Peer Reviewed
  • [Journal Article] Boron nitride substrates for high-quality graphene electronics2010

    • Author(s)
      C.R. Dean, T. Taniguchi, P. Kim, 計11名
    • Journal Title

      Nature Nanotechnology

      Volume: 5 Pages: 722-726

    • Peer Reviewed
  • [Journal Article] Doping of hexagonal boron nitride via intercalation: A theoretical prediction2010

    • Author(s)
      F.Oba, A.Togo, I.Taknaka, K.Watanabe, T.Taniguchi
    • Journal Title

      Phys.Rev.B

      Volume: 81 Pages: 075125

    • Peer Reviewed
  • [Journal Article] Mantle Superplasticity and Its Self-made Demise2010

    • Author(s)
      T. Hiraga, T. Miyazaki, M. Tasaka, and H. Yoshida
    • Journal Title

      Nature

      Volume: 468 Pages: 1091-1094

    • Peer Reviewed
  • [Journal Article] Doping Effect of Divalent Cations on Sintering of Polycrystalline Yttria2010

    • Author(s)
      M.Kodo, K.Soga, H.Yoshida, and T.Yamamoto
    • Journal Title

      J. Europ. Ceram Soc.

      Volume: 30 Pages: 2741

    • Peer Reviewed
  • [Journal Article] Phase-transformation and Grain-growth Kinetics in Yttria-stabilized Tetragonal Zirconia Polycrystal Doped with a Small Amount of Alumina2010

    • Author(s)
      K.Matsui, H.Yoshida, and Y.Ikuhara
    • Journal Title

      J. Euro. Ceram Soc

      Volume: 30 Pages: 1679

    • Peer Reviewed
  • [Journal Article] Investigations Of Growth Kinetics Of Pulsed Laser Deposition Of Tin Oxide Films By Isotope Tracer Technique2010

    • Author(s)
      Y.-H.Zhen, N.Ohashi, 計11名
    • Journal Title

      J. Appl. Phys.

      Volume: 108 Pages: AR 104901

    • Peer Reviewed
  • [Journal Article] Development of ultra-fine-grain binderless cBN tool for precision cutting of ferrous materials2009

    • Author(s)
      K.Fujisaki, H.Yokota, T.Taniguchi, 計8名
    • Journal Title

      J. Mater. Process. Technol.

      Volume: 209, 15-16 Pages: 5646-5652

    • Peer Reviewed
  • [Journal Article] Doping-amount and temperature dependence of superplastic flow in tetragonal ZrO_2 polycrystal doped with TiO_2 and/or GeO_22009

    • Author(s)
      H.Yoshida, K.Morita, B.-N.Kim, K.Hiraga, and T.Yamamoto
    • Journal Title

      Acta Materialia

      Volume: 57 Pages: 3029-3038

    • Peer Reviewed
  • [Journal Article] Densification Behavior of Ti-doped Polycrystalline Alumina in a Nitrogen-Hydrogen Atmosphere2009

    • Author(s)
      H.Yoshida, K.Hiraga, T.Yamamoto
    • Journal Title

      Materials Transactions

      Volume: 50 [5] Pages: 1032-1036

    • Peer Reviewed
  • [Journal Article] Isothermal Sintering Effects on Phase Separation and Grain Growth in Yttria-stabilized Tetragonal Zirconia Polycrystal2009

    • Author(s)
      K.Matsui, H.Yoshida, and Y.Ikuhara
    • Journal Title

      J. Am Ceram. Soc.

      Volume: 92 [2] Pages: 467

    • Peer Reviewed
  • [Journal Article] Ionic conductivity of tetragonal ZrO_2 polycrystal doped with TiO_2 and GeO_22009

    • Author(s)
      H.Yoshida, K.Morita, B.-N. Kim, and K. Hiraga,
    • Journal Title

      Journal of the European Ceramic Society

      Volume: 29 [2] Pages: 411-418

    • Peer Reviewed
  • [Journal Article] Synthesis And Characterization Of ZnO/Glass/ZnO Structures Showing Highly Nonlinear Current-Voltage Characteristics2009

    • Author(s)
      N.Ohashi, 計6名
    • Journal Title

      Materials Transactions

      Volume: 50 (5) Pages: 1060-1066

    • Peer Reviewed
  • [Journal Article] Polarity-Dependent Photoemission Spectra Of Wurtzite-Type Zinc Oxide2009

    • Author(s)
      N.Ohashi, 計9名
    • Journal Title

      Applied Physics Letters

      Volume: 94 (12) Pages: AR 122102

    • Peer Reviewed
  • [Journal Article] Hexagonal Boron Nitride Single Crystal Growth at Atmospheric Pressure Using Ni-Cr Solvent2008

    • Author(s)
      Y.Kubota, K.Watanabe, O.Tsuda, T.Taniguchi
    • Journal Title

      Chem.Mater.

      Volume: [20] Pages: 1661-1663

    • Peer Reviewed
  • [Journal Article] Misfit Dislocation Formation at the c/t Interphase Boundary in Y-TZP2008

    • Author(s)
      S.Ii, H.Yoshida, K.Matsui, Y.Ikuhara
    • Journal Title

      Journal of the American Ceramics Society

      Volume: 91 [11] Pages: 3810-3812

    • Peer Reviewed
  • [Journal Article] Densific ation of Nanocrystalline Yttria by Low Temperature Spark Plasma Sintering2008

    • Author(s)
      H.Yoshida, K. Hiraga, 計6名
    • Journal Title

      J. Am. Ceram. Soc

      Volume: 91, 1707

    • Peer Reviewed
  • [Journal Article] Hard X-Ray Photoemission Spectroscopy In Wurtzite-Type Zinc Magnesium Oxide Solid-Solution Films Grown By Pulsed-Laser Deposition2008

    • Author(s)
      T.Ohsawa, N.Ohashi, 計10名
    • Journal Title

      Applied Physics Letters

      Volume: 92 (23) Pages: AR 232108

    • Peer Reviewed
  • [Journal Article] Synthesis of high purity boron nitride single crystals under high pressure by using Ba-BN solvent2007

    • Author(s)
      T.Taniguchi, K.Watanabe
    • Journal Title

      J.Cryst.Growth

      Volume: [303] Pages: 525-529

    • Peer Reviewed
  • [Journal Article] High-strain-rate Superplasticity in Oxide Ceramics2007

    • Author(s)
      K. Hiraga, B.-N. Kim, K. Morita, H. Yoshida, T.S. Suzuki , and Y. Sakka
    • Journal Title

      Science and Technology of Advanced Materials

      Volume: 8 [7-8] Pages: 578-587

    • Peer Reviewed
  • [Presentation] High Temperature Plastic Flow Behavior and Related Grain Boundary Phenomena in Cation-doped Tetragonal Zirconia Polycrystal2011

    • Author(s)
      H. Yoshida, K. Morita, B.-N. Kim, K. Hiraga, and T. Yamamoto
    • Organizer
      THERMEC’2011 (International Conference on Processing & Manufacturing of Advanced Materials)
    • Place of Presentation
      Quebec city, Canada
    • Year and Date
      20110801-05
  • [Presentation] Characterization and Management of Defects in Oxides2011

    • Author(s)
      N.Ohashi
    • Organizer
      ICMAT2011, 主催: The Materials Research Society of Singapore
    • Place of Presentation
      シンガポール
    • Year and Date
      20110626-0701
  • [Presentation] Synthesis of hBN single crystals under high pressure and high temperature2011

    • Author(s)
      T.Taniguchi
    • Organizer
      第7回日米セミナー Nanoscale Transport Phenomena, JSPS(Japan)
    • Place of Presentation
      Ise-Shima, Japan
    • Year and Date
      2011-12-11
  • [Presentation] 超塑性セラミックスの開発-無機材料化学と金属学の観点から-2011

    • Author(s)
      平賀啓二郎, 金炳男, 森田孝治, 吉田英, 目義雄
    • Organizer
      日本化学会北海道支部北見地区講演会
    • Place of Presentation
      北見工業大学
    • Year and Date
      2011-11-22
  • [Presentation] 高純度窒化ホウ素単結晶及び焼結体の高圧合成と機能発現2011

    • Author(s)
      谷口 尚
    • Organizer
      先進セラミックス第124委員会 第136回会議,日本学術振興会
    • Place of Presentation
      東京
    • Year and Date
      2011-06-02
  • [Presentation] High purity boron nitride: synthesis under high pressure and 1atm, and their properties2011

    • Author(s)
      T.Taniguchi
    • Organizer
      NDNC2011
    • Place of Presentation
      Matsue, Japan
    • Year and Date
      2011-05-16
  • [Presentation] 高圧下温度差法による窒化ホウ素単結晶の合成と不純物制御2011

    • Author(s)
      谷口 尚
    • Organizer
      高圧を用いたワイドバンドギャップ半導体単結晶の育成と評価」応用物理学会 結晶工学分科会
    • Place of Presentation
      東京
    • Year and Date
      2011-04-21
  • [Presentation] Doping Effect on High-Temperature Plastic Flow in Fine-grained Alumina2010

    • Author(s)
      H. Yoshida, Y. Ikuhara, and T. Sakuma
    • Organizer
      2010 AGU (The American Geophysical Union) Fall Meeting
    • Place of Presentation
      San Francisco, California, USA
    • Year and Date
      20101213-17
  • [Presentation] High-purity boron nitrides single crystals and sintered bodies2010

    • Author(s)
      T.Taniguchi
    • Organizer
      CIMTEC 2010
    • Place of Presentation
      Florence, Italy
    • Year and Date
      20100606-11
  • [Presentation] Charge compensation in oxide semiconductors2010

    • Author(s)
      N.Ohashi
    • Organizer
      International Symposium on Compound Semiconductor Week 2010, 主催:Japan Society of Applied Physics
    • Place of Presentation
      高松
    • Year and Date
      20100531-0604
  • [Presentation] Development of zinc oxide and its related materials and structures2010

    • Author(s)
      N.Ohashi
    • Organizer
      Korea-Japan Joint Workshop on Semiconductor Physics and devices, 韓国物理学会・日本応用物理学会 共催, 韓国
    • Year and Date
      2010-04-21
  • [Presentation] 酸化物セラミックスのナノ粒界制御と高温物質輸送現象2010

    • Author(s)
      吉田英弘
    • Organizer
      日本金属学会2010年(第146回)春期大会
    • Place of Presentation
      筑波大学
    • Year and Date
      2010-03-28
  • [Presentation] 高純度窒化ホウ素単結晶の高圧・常圧合成2009

    • Author(s)
      谷口 尚
    • Organizer
      第22回 秋季シンポジウム,日本セラミックス協会
    • Place of Presentation
      松山
    • Year and Date
      20090916-18
  • [Presentation] Grain Boundary Nanostructure and High Temperature Plastic Flow in Polycrystalline Oxide Ceramics2009

    • Author(s)
      H.Yoshida, K.Morita, B.-N.Kim, K.Hiraga
    • Organizer
      THERMEC’ 2009 (International Conference on Processing & Manufacturing of Advanced Materials)
    • Place of Presentation
      Berlin, Germany
    • Year and Date
      20090825-29
  • [Presentation] ”高圧合成プロセスにおける機能元素制御による新機能材料の創製”日本金属学会セミナー「機能元素のナノ材料科学」2009

    • Author(s)
      谷口 尚
    • Organizer
      日本金属学会
    • Place of Presentation
      京都
    • Year and Date
      2009-07-24
  • [Presentation] 超高圧力下におけるIII族窒化物 結晶・焼結体の合成 ~高純度化と不純物添加による機能発現2008

    • Author(s)
      谷口 尚
    • Organizer
      日本金属学会 2008年秋季(第143回)大会
    • Place of Presentation
      熊本
    • Year and Date
      20080923-25
  • [Presentation] High Temperature Plastic Flow and Related Grain Boundary Matter Transport Phenomena in Polycrystalline Oxide Ceramics2008

    • Author(s)
      H. Yoshida, K. Morita, B.-N. Kim and K. Hiraga
    • Organizer
      Mechanics and Mechanisms of Finite Plastic Deformation
    • Place of Presentation
      Kauai, Hawaii, USA
    • Year and Date
      20080103-08
  • [Patent(Industrial Property Rights)] 高窒素含有遷移金属窒化物の製造方法及び高窒素含有遷移金属窒 化物2011

    • Inventor(s)
      川村史朗, 谷口 尚, 他
    • Industrial Property Rights Holder
      物質・材料研究機構
    • Industrial Property Number
      特許, 特願2011-155185:
    • Filing Date
      2011-07-13
  • [Patent(Industrial Property Rights)] 透光性YAG多結晶体とその製造方法2010

    • Inventor(s)
      吉田英弘, 曽我公平, 山本剛久
    • Industrial Property Rights Holder
      吉田英弘, 曽我公平, 山本剛久
    • Industrial Property Number
      特許, 特願2008-326477
    • Acquisition Date
      2010-06-10
  • [Patent(Industrial Property Rights)] 切削工具とこれを用いた切削方法2008

    • Inventor(s)
      横田秀夫, 藤崎和弘, 谷口 尚, 他
    • Industrial Property Rights Holder
      理化学研究所
    • Patent Publication Number
      特許, 特開 2009-214213:
    • Filing Date
      2008-03-10
  • [Patent(Industrial Property Rights)] 酸化イットリウム焼結体及び当該焼結体の製造方法2008

    • Inventor(s)
      曽我公平, 河道正泰, 山本剛久, 吉田英弘
    • Industrial Property Rights Holder
      東京理科大学
    • Industrial Property Number
      特許, 特願2008-021606
    • Acquisition Date
      2008-01-31

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Published: 2013-07-31  

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