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2011 Fiscal Year Annual Research Report

多極子自由度に由来する秩序と揺らぎの研究

Planned Research

Project AreaEmergence of Heavy Electrons and Their Ordering
Project/Area Number 20102007
Research InstitutionThe University of Tokyo

Principal Investigator

榊原 俊郎  東京大学, 物性研究所, 教授 (70162287)

Co-Investigator(Kenkyū-buntansha) 吉澤 正人  岩手大学, 工学研究科, 教授 (30220619)
徳永 陽  日本原子力研究開発機構, 先端基礎研究センター, 研究員 (00354902)
青木 勇二  首都大学東京, 理工学研究科, 教授 (20231772)
Keywordsメタ磁性 / 超音波弾性定数測定 / NMR / 多極子 / 鉄砒素系超伝導体 / 高圧測定 / かご状物質 / 近藤効果
Research Abstract

1.PrT_2X_<20>系の四極子秩序と揺らぎ
PrTi_2Al_<20>においてAl-NMRによる核スピン-格子緩和率の温度および磁場依存性の詳細な測定を行い、低温の緩和率の特異な増大が増強Pr核スピンの揺らぎによるものではなく、Prのf電子の多極子揺らぎによるものであることを明らかにした(徳永)。中性子散乱およびμSR測定を行い、Γ_3二重項が基底状態で強的な四極子秩序を示すことを確認した(中辻)。高圧下電気抵抗測定の結果、四極子転移温度が7GPa以上の圧力下で低下する傾向を見出し、量子臨界点の存在が示唆される,(上床)。PrV_2Al_<20>について極低温磁化測定を行い、[100]方向の高磁場において新規の秩序相が存在することを発見した(榊原、中辻)。PrRh_2Zn_<20>について低温比熱測定をA02班と共同で行い、60mK付近に四極子転移の比熱異常を見出した(榊原)
2.鉄系超伝導体の軌道揺らぎ(吉澤)
Ba(Fe_<1-x>Co_x)_2As_2について面間の弾性定数C33の測定を行い、量子臨界点近傍の試料ではC33が超伝導転移温度の遙か高温から軟化し、構造相転移点でも異常を示さないことを見出した。このことは磁気的な面間の相関と超伝導との関わりを示唆し、この系の構造揺らぎと超伝導との相関関係に次ぐ重要な知見と考えている。
3.YbT_2Zn_<20>関係
YbIr_2Zn_<20>について極低温磁化測定を行い、メタ磁性転移磁場近傍で非フェルミ液体的な磁化の温度依存性を見出した(榊原)。YbCo_2Zn_<20>について圧力下磁場中比熱測定を行い、臨界点近傍において比熱がT^<-n>(0.44<n<0.54)に比例することを明らかにした。
4.新物質関係
新しく立方晶系SmTi_2Al_<20>,SmV_2Al_<20>の単結晶試料を作威し、それらがSm系では非常に珍しく近藤効果を示すこと、また磁場の影響を受けない磁気的秩序状態を示すことを発見した(青木、中辻)。PrNb_2Al_<20>において四極子自由度が関与した非フェルミ液体状態を示唆する極低温比熱発散を見出した(青木)。

Current Status of Research Progress
Current Status of Research Progress

2: Research has progressed on the whole more than it was originally planned.

Reason

PrT_2X_<20>については磁場温度相図に関して進展があり、また秩序状態の解明も進んだ。さらに圧力下で量子相転移が存在する可能性が出てきた。加えて、新規物質で興味深い性質を示すものが見つかった。鉄砒素系超伝導体についても、軌道揺らぎの重要性が明らかになったことが挙げられる。

Strategy for Future Research Activity

特に大きな変更点はないが、PrT2X20の低温高圧下の物性測定を行い、四極子秩序相から無秩序相への量子相転移が存在する証拠を得ること、および量子臨界点近傍で超伝導が出現するかどうかを探索することが今後の大きな目標である。

  • Research Products

    (40 results)

All 2012 2011

All Journal Article (22 results) (of which Peer Reviewed: 22 results) Presentation (18 results)

  • [Journal Article] Elastic Anomalies Associated with superconducting phase transitions in Iron-based Superconductor Ba(Fe_<1-x>Co_x)_2As_22012

    • Author(s)
      A.Ismayil
    • Journal Title

      J.Phys.Conf.Ser.

      Volume: (印刷中) Pages: 4

    • Peer Reviewed
  • [Journal Article] Structural Quantum Criticality and Superconductivity in Iron-Based Superconductor Ba(Fe_<1-x>Co_x)_2As_22012

    • Author(s)
      M.Yoshizawa
    • Journal Title

      J.Phys.Soc.Jpn.

      Volume: 81 Pages: 024604(6)

    • DOI

      10.1143/JPSJ.81.024604

    • Peer Reviewed
  • [Journal Article] Large elastic anomalies and strong electron-lattice coupling in iron-based superconductor Ba(Fel-xCox) 2As22012

    • Author(s)
      M.Yoshizawa
    • Journal Title

      Solid State Commun.

      Volume: 152 Pages: 680-687

    • DOI

      10.1016/j.ssc.2011.12.006

    • Peer Reviewed
  • [Journal Article] f-Electron-Nuclear Hyperfine-Coupled Multiplets in the Unconventional Charge Order Phase of Filled Skutterudite PrRu4P122011

    • Author(s)
      Y.Aoki
    • Journal Title

      J.Phys.Soc.Jpn.

      Volume: 80 Pages: 054704(7)

    • DOI

      10.1143/JPSJ.80.054704

    • Peer Reviewed
  • [Journal Article] Strong Effect of Yb Filling Fraction on the Magnetic Ground Sate of the Filled Skutterudite YbFe4Sb122011

    • Author(s)
      T.SAITO
    • Journal Title

      J.Phys.Soc.Jpn.

      Volume: 80 Pages: 063708(4)

    • DOI

      10.1143/JPSJ.80.063708

    • Peer Reviewed
  • [Journal Article] Unusual Field-Insensitive Phase Transition and Eondo Behavior in SmTi2Al202011

    • Author(s)
      R.Higashinaka
    • Journal Title

      J.Phys.Soc.Jpn.

      Volume: 80 Pages: 093703(4)

    • DOI

      10.1143/JPSJ.80.093703

    • Peer Reviewed
  • [Journal Article] Pressure-induced changes in the magnetic and valence state of EuFe2As22011

    • Author(s)
      K.Matsubayashi
    • Journal Title

      Phys.Rev.B

      Volume: 84 Pages: 024505(1-6)

    • DOI

      10.1103/PhysRevB.84.024502

    • Peer Reviewed
  • [Journal Article] Magnetic and transport properties of CeT2A110 (T=Fe, Ru, Os) under pressure2011

    • Author(s)
      Y.Kawamura
    • Journal Title

      J.Phys. : Conf.Ser.

      Volume: 273 Pages: 012038(1-5)

    • DOI

      10.1088/1742-6596/273/1/012038

    • Peer Reviewed
  • [Journal Article] Elastic Anomalies of TbB_4 in Pulsed High Magnetic Fields2011

    • Author(s)
      T.K.Fujita
    • Journal Title

      J.Phys, Soc.Jpn.

      Volume: 80 Pages: SA084(3)

    • DOI

      10.1143/JPSJS.80SA.SA084

    • Peer Reviewed
  • [Journal Article] Effect of Carrier Doping on Physical Properties of A-Site Ordered Perovskite CaCu_3Ti_4O_<12>2011

    • Author(s)
      A.Ismayil
    • Journal Title

      J.Phys, Soc.Jpn.

      Volume: 80 Pages: SA113(3)

    • DOI

      10.1143/JPSJS.80SA.SA113

    • Peer Reviewed
  • [Journal Article] NMR Determination of Noncollinear Antiferromagnetic Structure in TbCoGa2011

    • Author(s)
      Y.Tokunaga
    • Journal Title

      Physical Review B

      Volume: 84 Pages: 214403_1-7

    • DOI

      10.1103/PhysRevB.84.214403

    • Peer Reviewed
  • [Journal Article] 237Np nuclear relaxation rate in heavy fermion superconductor NpPd5Al22011

    • Author(s)
      H.Chudo
    • Journal Title

      Physical Review B

      Volume: 84 Pages: 094402_1-5

    • DOI

      10.1103/PhysRevB.84.094402

    • Peer Reviewed
  • [Journal Article] NMR Study on AmO2 : Comparison with UO2 and NpO22011

    • Author(s)
      Y.Tokunaga
    • Journal Title

      J.Phys.Soc.Jpn.Suppl.A

      Volume: 80 Pages: SA110_1-3

    • DOI

      10.1143/JPSJS.80SA.SA110

    • Peer Reviewed
  • [Journal Article] Low temperature magnetism of the metallic pyrochlore oxide Pr2+xIr2-xO7+δ2011

    • Author(s)
      K.Kimura
    • Journal Title

      Journal of Physics : Conference Series

      Volume: 320 Pages: 012079/1-4

    • DOI

      doi:10.1088/1742-6596/320/1/012079

    • Peer Reviewed
  • [Journal Article] Spontaneous Hall Effect in the Spin Liquid Phase of Pr2Ir2O72011

    • Author(s)
      S.Nakatsuji
    • Journal Title

      J.Phys. : Conf.Series (2011), in print

      Volume: 320 Pages: 012056/1-9

    • DOI

      doi:10.1088/1742-6596/320/1/012056

    • Peer Reviewed
  • [Journal Article] Anisotropic Hysteretic Hall Effect and Magnetic Control of Chiral Domains in the Chiral Spin States of Pr2Ir2O72011

    • Author(s)
      L.Balicas
    • Journal Title

      Phys.Rev.Lett.(2011)

      Volume: 106 Pages: 217204/1-4

    • DOI

      10.1103/PhysRevLett.106.217204

    • Peer Reviewed
  • [Journal Article] μSR Evidence of Nonmagnetic Order and 141Pr Hyperfine-Enhanced Nuclear Magnetism in the Cubic Γ3 Ground Doublet System PrTi2Al202011

    • Author(s)
      T.U.Ito
    • Journal Title

      J.Phys.Soc.Jpn.

      Volume: 80 Pages: 113703/1-4

    • DOI

      doi:10.1088/1742-6596/320/1/012079

    • Peer Reviewed
  • [Journal Article] Strong valence fluctuation effects in SmTr2Al20 (Tr=Ti,V,Cr)2011

    • Author(s)
      A.Sakai, S.Nakatsuji
    • Journal Title

      Phys.Rev.B (2011)

      Volume: 84 Pages: 201106/1-5

    • DOI

      DOI:10.1103/PhysRevB.84.201106

    • Peer Reviewed
  • [Journal Article] Evidence of a Field-Induced Ordering in YbCo2Zn20 in a [111] Magnetic Fie2011

    • Author(s)
      Y.Shimura
    • Journal Title

      J.Phys.Soc.Jpn.

      Volume: 80 Pages: 073707 1-4

    • DOI

      10.1143/JPSJ.80.073707

    • Peer Reviewed
  • [Journal Article] Low-Temperature Magnetization of the Metamagnetic Heavy Fermion Compound YbIr2Zn202011

    • Author(s)
      Y.Shimura
    • Journal Title

      J.Phys.Soc.Jpn.

      Volume: 80 Pages: SA051 1-3

    • DOI

      10.1143/JPSJS.80SA.SA051

    • Peer Reviewed
  • [Journal Article] Low Temperature Magnetic Properties of Pr Pr(Cu, Ga) 13 with Orbitally Degenerate Ground State2011

    • Author(s)
      Y.Shimura
    • Journal Title

      J.Phys.Soc.Jpn.

      Volume: 80 Pages: SA072 1-3

    • DOI

      10.1143/JPSJS.80SA.SA072

    • Peer Reviewed
  • [Journal Article] Low-temperature magnetic properties of Pr(Cu, Ga) 12.852011

    • Author(s)
      Y.Shimura
    • Journal Title

      J.Phys. : Conf.Ser.

      Volume: 273 Pages: 012054 1-4

    • DOI

      10.1088/1742-6596/273/1/012054

    • Peer Reviewed
  • [Presentation] 鉄系超伝導体の弾性的性質2012

    • Author(s)
      吉澤正人
    • Organizer
      日本物理学会第67回年次大会
    • Place of Presentation
      関西学院大学26pYD-7(シンポジウム講演)
    • Year and Date
      2012-03-26
  • [Presentation] 超音波測定における鉄系超伝導体Fe_<1.03>Te_<0.8>Se_<0.2>の弾性特性2012

    • Author(s)
      坂野幸平
    • Organizer
      日本物理学会第67回年次大会
    • Place of Presentation
      関西学院大学25aPS-84
    • Year and Date
      2012-03-25
  • [Presentation] Large elastic softening in heavy fermion superconductor Rh_<17>S_<15>2012

    • Author(s)
      Abdusalam Ismayil
    • Organizer
      日本物理学会第67回年次大会
    • Place of Presentation
      関西学院大学25aYH-4
    • Year and Date
      2012-03-25
  • [Presentation] Elastic properties of iron-based superconductor2011

    • Author(s)
      M.Yoshizawa
    • Organizer
      24th International Symposium on Superconductivity (ISS2012)
    • Place of Presentation
      Tokyo(招待講演)
    • Year and Date
      2011-10-25
  • [Presentation] Sign reversal of Field-Angle Resolved Heat Capacity Oscillations in a Heavy Fermion Superconductor CeCoIn5 and dx2-y2 Pairing Symmetry2011

    • Author(s)
      T.Sakakibara
    • Organizer
      The Korean Physical Society Autumn Meeting 2011
    • Place of Presentation
      Busan Exhibition Convention Center, Busan, Korea
    • Year and Date
      2011-10-20
  • [Presentation] Quantum Critical Behavior of Heavy Fermion Compound YbCo2Zn20 under Pressure and Magnetic Field2011

    • Author(s)
      R.Yamanaka
    • Organizer
      TOKIMEKI 2011 International workshop on heavy fermions
    • Place of Presentation
      Osaka University
    • Year and Date
      2011-09-24
  • [Presentation] NMRによる多極子秩序の観測2011

    • Author(s)
      徳永陽
    • Organizer
      日本物理学会2011年秋季大会
    • Place of Presentation
      富山大学,富山
    • Year and Date
      2011-09-22
  • [Presentation] 充填スクッテルダイトにおける磁場の影響を受けない重い電子状態2011

    • Author(s)
      青木勇二
    • Organizer
      日本物理学会2011年秋季大会
    • Place of Presentation
      富山大学五福キャンパス(企画講演)
    • Year and Date
      2011-09-21
  • [Presentation] 回転磁場中比熱測定によるCeIrIn5の超伝導ギャップ構造の研究2011

    • Author(s)
      橘高俊一郎
    • Organizer
      日本物理学会2011年秋季大会
    • Place of Presentation
      富山大学五福キャンパス
    • Year and Date
      2011-09-21
  • [Presentation] Quantum criticlaity without tuning and possible quantum critical phase in the mixed valent compound β-YbAlB42011

    • Author(s)
      Y.Matsmnoto
    • Organizer
      International Conference on Strongly Correlated Electron Systems (SCES 2011)
    • Place of Presentation
      Cambridge, England
    • Year and Date
      2011-09-02
  • [Presentation] Spin liquids, Quantum Criticality in Itinerant Magnets2011

    • Author(s)
      S.Nakatsuji
    • Organizer
      Tokyo-Cologne Workshop on Strongly Correlated Transition Metal Compounds
    • Place of Presentation
      Cologne, Germany
    • Year and Date
      2011-09-02
  • [Presentation] Field-induced ordering in the heavy fermion compound YbCo2Zn202011

    • Author(s)
      Y.Shimura
    • Organizer
      SCES 2011
    • Place of Presentation
      Cambridge, UK
    • Year and Date
      2011-09-02
  • [Presentation] NMR study of various actinides systems2011

    • Author(s)
      Y.Tokunaga, et al
    • Organizer
      J-ACTINET Meeting 2011
    • Place of Presentation
      Tohoku University-Tokyo office, Tokyo
    • Year and Date
      2011-09-01
  • [Presentation] Novel Quantum Phases in 4f based Kondo Lattice Systems2011

    • Author(s)
      E.C.T.O' Farrell
    • Organizer
      International Conference on Strongly Correlated Electron Systems (SCES 2011)
    • Place of Presentation
      Cambridge, England
    • Year and Date
      2011-08-31
  • [Presentation] Kondo Effects and Multipolar Order in cubic Γ3 systems PrTr2Al20 (Tr=Ti, V)2011

    • Author(s)
      A.Sakai
    • Organizer
      International Conference on Strongly Correlated Electron Systems (SCES 2011)
    • Place of Presentation
      Cambridge, England
    • Year and Date
      2011-08-31
  • [Presentation] Ultrasonic investigation on a cage structure compound PrV2Al202011

    • Author(s)
      Y.Nakanishi
    • Organizer
      International Conference on Strongly Correlated Electron Systems (SCES 2011)
    • Place of Presentation
      Cambridge, England
    • Year and Date
      2011-08-31
  • [Presentation] Quantum Criticality and Superconductivity in Ba(Fe_<1-x>Co_x)_2As_2 Investigated by Ultrasonic Measurements2011

    • Author(s)
      M.Yoshizawa
    • Organizer
      26th International Conference on Low Temperature Physics (LT26)
    • Place of Presentation
      Beijing International Convention Center (BICC), China(招待講演)
    • Year and Date
      2011-08-16
  • [Presentation] Quantum criticality without tuning in the intermediate valence material β-YbAlB42011

    • Author(s)
      S.Nakatsuji
    • Organizer
      International Conference on Low Temperature Physics
    • Place of Presentation
      LT26, Beijing, China
    • Year and Date
      2011-08-12

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Published: 2013-06-26  

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