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1992 Fiscal Year Final Research Report Summary

Chemical composition of fog water classified according to their sizes and their formation process.

Research Project

Project/Area Number 03804024
Research Category

Grant-in-Aid for General Scientific Research (C)

Allocation TypeSingle-year Grants
Research Field 気象・海洋・陸水学
Research InstitutionNagoya University

Principal Investigator

ISHIZAKA Yutaka  Water Research Institute Associate Professor., 水圏科学研究所, 助教授 (50022710)

Co-Investigator(Kenkyū-buntansha) TSURUTA Haruo  National Institute of Agro-Environmental Sciences Head of Environmental Survey L, 環境管理部, 室長
Project Period (FY) 1991 – 1992
Keywordsacidic fog / pH of fog water / chemical composition of fog water / SO_2 / HNO_3 / sulfate ion / nitrate ion
Research Abstract

In order to study the formation process of acidic fog, chemical composition of fog water was examined simultaneously with chemical analysis of gaseous and particulate materials near the top of Mt. Norikura (Height of observation site:2770m). In this experiment, fog water was classified into four size classes and sampled with a newly made string-type cloud collector, in addition to bulk fog water sampling.
Acidity measurement showed that acidic fogs are often formed in the summer seasons and minimum pH of fog water reached 3.30. It was also found that change in pH is a function of the droplet size and minimum pH of the smallest droplets(mean diameter(] SY.simeq.[)3.6um) was 3.03. Main anions in fog water were sulfate and nitrate and concentration of many constituents increased generally with decreasing fog droplet size. On the other hand, chemical composition of particulate materials suggested that aerosol particles consisted mainly of ammonium sulfate. Therefore, we assumed that ammonium in fog water was originated from aerosols captured into fog droplets. It was estimated from the assumption that sulfate produced within fog droplets by absorption of sulfur dioxide exceed 50 % of sulfate in the smallest fog droplets. Based on our observations, three processes were suggested for the formation of acidic fogs: nucleation of acidic particles such as ammonium sulfate, sulfate produced in fog droplets and absorption of nitric acid vapor.

  • Research Products

    (10 results)

All Other

All Publications (10 results)

  • [Publications] Qian,G.W.,Y.Ishizaki,Y.Minami,Y.Kurahashi,I.T.Bernadis: "Transfomation of individual aerosol particles in acidic fogevolution." Journ.Meteor.Soc.Japan.70. 711-722 (1992)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] 銭 公望、石坂 隆、鶴田 治雄: "酸性霧発生前後における個々のエアロゾル粒子と霧粒の成分の変化に関する観測." 日本化学会誌(化学と工業化学). (5). 690-697 (1991)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] 鶴田 治雄,太田 正雄: "乗鞍岳におけるガス・霧水・雨水中の化学成分の測定-アルデヒド類、オゾン、過酸化水素の挙動-." 日本気象学会春季大会講演予稿集. 167. (1991)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] 石坂 隆、銭 公望、皆己 幸也、倉橋 佳伸、大和 政彦、鶴田 治雄: "硝酸アンモニウム粒子による酸性霧粒の形成の可能性について." 日本気象学会春季大会講演予稿集. 224. (1991)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] 皆己 幸也、竹中 千里、Bernadia I.Irawati、石坂 隆: "乗鞍岳における霧水の粒径別化学組成に関する観測-霧水の酸性化過程に着目して-." 日本気象学会秋季大会講演予稿集. 167. (1991)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] 鶴田 治雄、太田 正雄、石坂 隆: "乗鞍岳における夏期の霧水、霧水と雨水中の水溶性成分とガス(SO_2,O_3)の測定(第3報)." 日本気象学会秋季大会講演予稿集. 168. (1991)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] Ishizaka,Y.,and G.W.Qian(edited by Fukuta,N.and P.E.Wagner): "Internally mixed particles of sulfate and nitrate in acidic fogs.(Nuceation and Atmospheric Aerosols)" A.Deepak Publishing, 403-406. (1992)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] Oian, G. W., Y.Ishizaka & T. Haruo: "Chemical change of aerosol particles during the formation of acidic fog droplets." Journ. Chem. Soc. Japan Chemistry and Industrial Chemistry.No.5. 690-697 (1991)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] Qian, G. W., Y. Ishizaka, Y. Minami, Y. Kurahashi, I.T. Bernadia: "Transformation of individual aerosol particles in acidic fog evolution." Journ. Meteor. Soc. Japan. 70. 711-722 (1992)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] Ishizaka, Y., and G. W. Qian,: "Internally mixed particles of sulfate and nitrate in acidic fogs." Nucleation and Atmospheric Aerosols (edited by Fukuta, N. and P. E. Wagner), A. Deepak Publishing.403-406 (1992)

    • Description
      「研究成果報告書概要(欧文)」より

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Published: 1994-03-24  

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