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1995 Fiscal Year Final Research Report Summary

Geochemical Study on Mantle-derived Hydrocarbons.

Research Project

Project/Area Number 05403002
Research Category

Grant-in-Aid for General Scientific Research (A)

Allocation TypeSingle-year Grants
Research Field 地球化学
Research InstitutionUniversity of Tokyo

Principal Investigator

WAKITA Hiroshi  Univ.of.Tokyo, Earthquake Chem., Professor, 理学部, 教授 (40011689)

Co-Investigator(Kenkyū-buntansha) ISHIBASHI Jun-ichiro  Univ.of.Tokyo, Earthquake Chem., Res.Associ, 理学部, 助手 (20212920)
NAKAI Shun'ichi  Univ.of .Tokyo, Earthquake Chem., Assoc.Prof., 理学部, 助教授 (50188869)
Project Period (FY) 1993 – 1995
KeywordsCarbon Compound / Carbon Isotope / Mantle / volcanic Gas / Natural Gas / Submarine Hydrothermal System
Research Abstract

This study aims at revealing origins, distributions and transportation mechanisms of carbon compounds in the Earth, using samples of natural gases, high temperature volcanic gases and hydrothermal vents from seafloor.
We succeeded in carbon isotopic measurement of methane of 10nM with a precision of 5 per mil with a GasChromatograph/Combustion/Mass Spectrometer system combined with a methane concentration line.
Most of natural gases from China showed a carbon isotopic distribution among hydrocarbons (C1-C5) wherein delta^<13>C becomes more negative with decreasing molecular weight of hydrocarbons, i.e.delta^<13>C1<delta^<13>C2<delta^<13>C3<delta^<13>C4, which suggests than most of natural gases formed by pyrolysys of organic matters in sediments. High temperature fumaroles collected in Satsuma-iojima contain methane formed by pyrolysys of organic matters in aquifer, which indicates difficulty to detect magma-derived methane without contamination. However, we developed a new methane extraction and concentration line for water samples and detected methane formed by an inorganic reaction in hydrothermal vent fluids collected in East Pacific Rise.
This study showed the developed concentration method combined with the GC/C/MS enabled us to investigate carbon compound in mantle. We will continue to imporve our methane concentration method and will apply the technique to other samples such as fluid inclusions in rocks.

  • Research Products

    (14 results)

All Other

All Publications (14 results)

  • [Publications] J.Ishibashi: "Helium and carbon geochemistry of hydrothemal fields from the North Fiji Basi sprending ridge(southwest Pacific)" Earth Planerury Science Letters. 128. 183-197 (1994)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] U. Tsunogai: "Peculiar features of Suiyo seamount hydrthermal fluids,Izu-Bonin Are:Differences from Subaevial volcarism" Earth Planerary Science Letters. 126. 289-301 (1994)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] S. Xu: "Helium isotopic compositions in Quarternary volcanic geothermal area near Indo Eurasian collisional Murgin Tengchary,China." In:Noble Gas Geochemistry and Cosmochemistry,Ed j. Matsuda (Terra Pub. Co,Tokyo). 305-313 (1994)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] J.Ishibasi: "Helium and carbon geochemistry of hydrochemical fluids from the Okinawa Trough Back Arc Basin,southwest Japan." Chemical Geology. 123. 1-15 (1995)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] S. Xu: "Mantle derived noble guses in natural gases from Songino Basin,China.21GC05:Geochimica et. Cosmochimica Acta" 59. 4675-4683 (1995)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] S. Xu: "Helium isotope compositions in sedimentary basins in China" Applied Geochemistry. 10. 643-656 (1995)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] U. Tsunogai: "Fresh water seepage on the seafbor:Sagami trough subduction zone,Japan" Earth Planetary Science Letters. (in press). (1996)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] J.Ishibashi: "Helium and carbon geochemistry of hydrothermal fluids form the North Fiji Basin spreading ridge (southwest Pacific)" Earth Planet.Sci.Lett.128. 183-197 (1994)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] U.Tsunogai: "Peculiar features of Suiyo seamount hydrothermal fluids, Izu-Bonin Arc : Differences from subaerial volcanism" Earth Planet.Sci.Lett.126. 289-301 (1994)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] J.Ishibashi: "Helium and carbon geochemistry of hydrothermal fluids from the Mid-Okinawa Trough Back Arc Basin, southwest of Japan" Chem.Geol.123. 1-15 (1995)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] S.Xu: "Mantle-derived noble gases in natural gases from Songliao Basin, china" Geochim.Cosmochim.Acta. 59. 4675-4683 (1995)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] S.Xu: "Helium isotope compositions in sedimentary basins in China" Appl.Geochem.10. 643-656 (1995)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] U.Tsunogai: "Fresh water seepage on the seafloor : Sagami trough subduction zone, Japan." Earth Planet.Sci.Lett.(in press).

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] S.Xu: Helium isotopic compositions in Quaternary volcanic geothermal area near Indo-Eurasian Collisional Margin at Tengchong, China. In Noble Gas Geochemistry and Cosmochemistry, Ed.J.Matsuda. Terra Sci.Publ.Co., Tokyo, 305-313 (1994)

    • Description
      「研究成果報告書概要(欧文)」より

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Published: 1997-03-04  

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