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1995 Fiscal Year Final Research Report Summary

Spin fluctuation in frustrated antiferromagnets

Research Project

Project/Area Number 06640474
Research Category

Grant-in-Aid for General Scientific Research (C)

Allocation TypeSingle-year Grants
Research Field 固体物性Ⅱ(磁性・金属・低温)
Research InstitutionKYOTO UNIVERSITY

Principal Investigator

MAEGAWA Satoru  Kyoto University, Graduate school of human and environmental studies, Associate Professor, 大学院人間・環境学研究科, 助教授 (40135489)

Project Period (FY) 1994 – 1995
KeywordsFrustration / Triangular Lattice Antiferromagnet / Kagome Lattice Antiferromagnet / Spin Fluctuation / Successive Phase Transition / Nuclear Magnetic Resonance / Nuclear Magnetic Relaxation / Relaxation Time
Research Abstract

The NMR spectrum and the nuclear magnetic relaxation time have been measured to investigate the phase transition, the spin structure and the fluctuation in frustrated antiferromagnets.
1. Magnetic properties in the triangular lattice Heisenberg antiferromagnet, RbNiCl_3.
(1) Successive phase transitions were confirmed and the temperature range of the intermediate phase is found to be only 0.2K.
(2) The NMR splitting of ^<87>Rb is explained by the electric quadrupole interaction including up to the second-order perturbation.
(3) A new model was proposed about the spin structure in the low temperature phase and the interactions between spins.
(4) A characteristic fluctuation in the frustrated antiferromagnets has been clarified by the measurement of the relaxation times in each phase.
2. Spin-lattice relaxation time and electron spin fluctuation in the triangular lattice Heisenberg antiferromagnet with a small easy-axis anisotropy, CsNiBr_3
(1) Spin-lattice relaxation times have been measured in the paramagnetic phase, the component disordered phase and the triangular ordered phase.
(2) It was found that the swinging fluctuation exists in the triangular ordered phase and the two-magnon process of this fluctuation contributes to the nuclear relaxation.
(3) The characteristic fluctuation in the paramagnetic phase was revealed from the relaxation time.
3. Magnetic properties and fluctuation in Kagome Lattice Antiferromagnets AFe_3(OH)_6(SO_4)_2 (A=NH_4, Na, K).
(1) Successive phase transitions were observed for the first time in the Kagome Lattice Antiferromagnets.
(2) Spin structure in each phase was considered by the measurement of the NMR spectra of^1H nad ^<23> Na.
(3) The characteristic fluctuation in Kagome Lattice Antiferromagnet was found.

  • Research Products

    (18 results)

All Other

All Publications (18 results)

  • [Publications] 前川覚: "Observation of Successive Phase Transitions in the Kagome Lattice Antiferromagnets AFe3(OH)6(SO4)_2 (A=NH4,Na,K)" Journal of Physical Society of Japan. (発表予定). (1996)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] 前川覚: "かごめ格子反強磁性体の磁性と相転移" 物性研だより. (印刷中). (1996)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] 河本敏郎: "Sublattice Switching in the Three-Dimensional Ordered Phase of the Triangular-Lattice Antiferromagnet CsCoCl_3" Physical Review B. 52. 12526-12529 (1995)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] 前川覚: "かごめ格子反強磁性体RFe_3(OH)_6(SO_4)_2 (R=Na,NH_4)の磁性と緩和" 物性研究. 64. 518-521 (1995)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] 前川覚: "Nuclear Magnetic Relaxation and Electron-Spin Fluctuation in a Triangular-Lattice Heisenberg Antiferromagnet CsNiBr_3" Physical Review B. 51. 15979-15985 (1995)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] 宗田悟志: "^<87>Rb NMR Study of the Triangular Lattice Antiferromagnet RbNiCl_3" Journal of Magnetism and Magnetic Materials. 140. 1787-1788 (1995)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] 前川覚: "Spin Fluctuation in a Trangular Lattice Aniferromagnet CsNiBr_3 Studied by NMR" Journal of Magnetism and Magnetic Materials. 140. 1789-1790 (1995)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] 小山田明: "NQR Studies of the Structural Instabilities in CePb_2Al_3" Physica B. 206. 237-239 (1995)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] 鈴木孝: "Anomalous Physical Properies of the low Carrier Concentration state in f-electron Systems" Physica B. 206. 771-779 (1995)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] S.MAEGAWA: "Observation of Successive Phase Transitions in Kagome Lattice Antiferromagnets AFe_3(OH)_6(SO_4)_2 (A=NH_4, Na, K)" Journal of Physical Society of Japan. (submitted to). (1996)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] S.MAEGAWA: "Magnetic Properties and Phase Transition in Kagome Lattice Antiferromagnets" Report of the Institute of Solid State Physics. (in press). (1996)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] T.KOHMOTO: "Sublattice Switching in the Three-Dimensional Ordered Phase of the Triangular-Lattice Antiferromagnet CsCoCl_3" Physical Review B. Vol.52, No.17. 12526-12529 (1995)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] S.MAEGAWA: "Magnetic Properties and Relaxation in Kagome Lattice Antiferromagnets RFe_3(OH)_6(SO_4)_2 (R=NH_4, Na)" Research on Solid State Physics. Vol.64, No.5. 518-521 (1995)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] S.MAEGAWA: "Nuclear Magnetic Relaxation and Electron-Spin Fluctuation in a Triangular-Lattice Heisenberg Antiferromagnet CsNiBr_32" Physical Review B. Vol.51, No.22. 15979-15985 (1995)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] S.MUNETA: "^<87>Rb NMR Study of the Triangular Lattice Antiferromagnet RbNiCl_3" Journal of Magnetism and Magnetic Materials. Vol.140. 1787-1788 (1995)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] S.MAEGAWA: "Spin Fluctuation in a Triangular Lattice Antiferromagnet CsNiBr_3 Studied by NMR" Journa of Magnetism and Magnetic Materials. Vol.140. 1789-1790 (1995)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] A.OYAMADA: "NQR Studies of the Structural Instabilities in CePb_2Al_3" Physica B. Vol.206. 237-239 (1995)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] T.SUZUKI: "Anomalous Physical Properties of the Low Carrier Concentration State in f-electron Systems" Physica B. Vol.206. 771-779 (1995)

    • Description
      「研究成果報告書概要(欧文)」より

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Published: 1997-03-04  

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