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1997 Fiscal Year Final Research Report Summary

Proton Polarization at Room Temperature wih Laser and it's application

Research Project

Project/Area Number 07554006
Research Category

Grant-in-Aid for Scientific Research (A)

Allocation TypeSingle-year Grants
Section展開研究
Research Field 素粒子・核・宇宙線
Research InstitutionKYOTO UNIVERSITY

Principal Investigator

MASAIKE Akira  Kyoto Univ., Graduate School of Science, Professor, 大学院・理学研究科, 教授 (40022587)

Co-Investigator(Kenkyū-buntansha) SHIMIZU Hirohiko  The Institute of Physical and Chemical Reserach, Research Assoicate, 研究員 (50249900)
FUNAHASHI Haruhiko  Kyoto Univ., Graduate School of Science, Research Assoicate, 大学院・理学研究科, 助手 (00283581)
ENYO Hideto  Kyoto Univ., Graduate School of Science, Associate Professor, 大学院・理学研究科, 助教授 (30213606)
TERASHIMA Masahide  Kyoto Univ., Graduate School of Science, Associate Professor, 大学院・理学研究科, 助教授 (00188674)
HIROTA Noboru  Kyoto Univ., Graduate School of Science, Professor, 大学院・理学研究科, 教授 (90093301)
Project Period (FY) 1995 – 1997
Keywordspolarized proton / triplet state / naphthalene / pentacene / dye-laser / solid sffect / relaxation time
Research Abstract

We have polarized protons in molecular crystals of naphthalene doped with pentacene using a dye laser in 3 KGauss at the temperature higher than 77 Kelvin. In this new method electrons are excited to high singlet states with the laser beam, where the spin-orbit interaction causes the transition from singlet states to intermediate triplet states. The populations of the Zeeman sublevels of the lowest triplet states with Z-components of the total electron spin+1,0, -1 are 12,76 and 12% respectively. During the lifetime of the triplet state (some 20 microsec) microwave irradiation occurs and the external field is swept simultaneously to transfer the population difference of electrons between two Zeeman sublevels to the proton polarization by means of the integrated solid effect. Electrons on the triplet states decay to the ground state, where the proton spin remains polarized for a long time.
We have tried to polarize protons in naphthalene doped with pentacene (0.01 mol%) with a high-power pulsed dye-laser (lambda=590-605nm) and got about 34% polarization at liquid nitrogen temperature. The enhancement factor corresponding to this value is 8*10^4. The relaxation times of protons are about 1,000 and 160 minutes in hte field of 3KG and 7G respectively. The method is applicable to the wide fields of spin physics. Since the target has no heating problem and no serious problem of radiation damage, it can be used for high-intensity beams of hadrons and electrons. Secondly, the target is useful for experiments with very low-momentum charged particles, since the necessary magnetci field to keep the polatization is extremely low.

  • Research Products

    (11 results)

All Other

All Publications (11 results)

  • [Publications] M.Iinuma, et al,: "High proton polarization in crystalline naphthalene by dynamic unclear polarization with laser excitation at room temperature and liquid nitrogen temperature" Phy.Lett.A. 208. 251-256 (1995)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] M.Daigo, et al.: "Proton polarization at room temterature" AIP Conf.Proc.343. 567-571 (1995)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] M.Terazima, et al.: "Photoexcited triplet states of fullerenes studied by the time-resolved EPR method" Proc.of Fullerenes : Chemistry,physics and New Directions VII. 16-21 (1995)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] T.Maekawa, et al.: "A large nuclear polarization of ^<139>La in Nd^<3+> : LaAlO_3 for testing the time reversal invariance" Nucl.Instrum.Methods A. 366. 115-119 (1995)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] E.I.Sharapov and H.M.Shimizu: "Experimental study of time-reversal invariance in neutron-nucleus interactions" Phys.Part.Nucl.27. 651-666 (1996)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] 飯沼 昌隆, 政池 明: "レーザー光による陽子スピンの偏極" パリティ. 12. 43-47 (1997)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] M.Iinuma, et al.: "High proton polarization in cyrstalline naphthalene by dynamic nuclear polarization with laser excitation at room temperature and liquid nitrogen temperature" Phys.Lett.A208. 251-256 (1995)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] M.Daigo, et al.: "Proton polarization at room temperature" AIP Conf.Proc.343. 567-571 (1995)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] M.Terazima, et al.: "Photoexcited triplet states of fullerenes studied by the time-resolved EPR method" Proc.of Fullerenes : Chemistry, Physics and New Directions. VII. 16-21 (1995)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] T.Maekawa, et al.: "A large nuclear polarization of ^<139>La in Nd^<3+> : LaAlO_3 for testing the time reversal invariance" Nucl.Instrum.Methods. A366. 115-119 (1995)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] E.I.Sharapov and H.M.Shimizu: "Experimental study of time-reversal invariance in neutron-nucleus interactions" Phys.Part.Nucl.27. 651-666 (1996)

    • Description
      「研究成果報告書概要(欧文)」より

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Published: 1999-03-16  

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