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1998 Fiscal Year Final Research Report Summary

Theoretical Study of Quantum Transport Phenomena through an Atom Sized Contact.

Research Project

Project/Area Number 08650032
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeSingle-year Grants
Section一般
Research Field 表面界面物性
Research InstitutionOsaka University

Principal Investigator

KASAI Hideaki  Osaka University, Department of Applied Physics, Professor, 大学院・工学研究科, 教授 (00177354)

Co-Investigator(Kenkyū-buntansha) NAKANISHI Hiroshi  Osaka University, Department of Material & Life Science, Reseach Associate, 大学院・工学研究科, 助手 (40237326)
Project Period (FY) 1996 – 1998
Keywordsquantized conductance / STM / atom bridge / electron correlation / Hubbard model / metal surface
Research Abstract

When the tip of a scanning tunneling microscope is brought into contact with a metal surface and then lifted up slowly, an atom-sized contact is formed between the tip and the surface. An atom-sized bridge is thus formed and its cross section consists of a few atoms to a few tens of atoms. Conductance of the bridge is measured as a function of the stretching length of the bridge, while the tip is lifted up. A stepwise variation of the conductance is experimentally observed roughly in units of 2e^<>h. In order to satisfy requirements for downsizing from mesoscopic scale to atomic scale in electronics, it is necessary to examine various phenomena occurring in such atom-sized systems. With this in mind, we examine the effects of the constricted structure of the atom-sized bridge and the effects of the Coulomb interaction between electrons on the quantized conductance through an atom-sized bridge. The obtained results are summarized as follows.
1. The effects of the constricted structure of … More the atom-sized bridge :
Stepwise variation of the conductance is disturbed by the broken symmetry of the shape of the atom-sized bridge.
2. The effects of the intra-site Coulomb interaction between electrons :
At finite temperatures, the Coulomb interaction causes various types of electron-electron scattering processes, inter-subband as well as intra-subband scattering processes and Umklapp as well as normal scattering processes, and strongly affects the quantum transport property of an atom-sized bridge. As a result, the following are derived.
(1) At the conductance plateau, the deviation of the conductance value from multiples of the universal value of 2e2/h grows as the temperature is decreased. This temperature dependence is stronger for stronger Coulomb interactions.
(2) Near the step, a valley structure appears as a function of the stretching length of the bridge. As the temperature is decreased, the valley gets narrower. The depth of the valley grows significantly, as the Coulomb interaction becomes stronger. Less

  • Research Products

    (45 results)

All Other

All Publications (45 results)

  • [Publications] W.A.Dino: "Combined Effect of Molecular Rotational-and Surface Vibrational-Excitations on the Dissociative Adsorption Dynamics of D_2/Cu(111)" Surface Science. 363. 52-61 (1996)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] H.Kasai: "A Microscopic Theory of Desorption Induced by Electronic Transitions" Surface Science. 363. 214-222 (1996)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] H.Tsuchiura: "Effects of Electronic Excitations on Potential Energy Surfaces : Simple Model Calculations" Surface Science. 363. 274-280 (1996)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] A.Okiji: "The effects of the Electronic Excitation on the Behaviour of Particles Scattered by Metal Surfaces" Springer Series in Solid-State Sciences(Springer,Berlin). 121. 138-146 (1996)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] H.Kasai: "On the Molecular Orientation Dependence of Dynamical Processes on Solid Surfaces : Dissociative Adsorption and Scattering" Springer Series in Solid-State Sciences(Springer,Berlin). 121. 99-111 (1996)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] W.A.Dino: "Role of the Rotational Motion in the Dissociative Adsorption and Associative Desorption Dynamics of D_2/Cu(111)" Physical Review Letters. 78. 286-289 (1997)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] H.Tsuchiura: "A.Model Calculation for Photo-Stimulated Desorption" Journal of the Physical Society of Japan. 66. 2805-2810 (1997)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] W.A.Dino: "Rotational Effects in the Dissociative Adsorption Dynamics of Hydrogen on a Pd Surface" Journal of the Physical Society of Japan. 66. 3344-3347 (1997)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] 笠井秀明: "解離と会合-飛来する水素と離れ去る水素の金属表面での挙動-" 日本物理学会誌. 52. 824-830 (1997)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] M.Sakaue: "Transient Population of Photoexcited Electrons in a Localized State at a Metal Surface" Journal of the Physical Society of Japan. 66. 3718-3721 (1997)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] A.Okiji: "Molecular Orientation Dependence of Dynamical Processes on Metal Surfaces : Dissociative Adsorption and Scattering,and Associative Desorption" Proceedings of International Workshop on the Current Problems in Condensed Matter : Theory and Experiments(Plenum Press,).275-282 (1998)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] W.A.Dino: "Rotational Alignment in the Associative Desorption Dynamics of Hydrogen Molecules from Metal Surfaces" Journal of the Physical Society of Japan. 67. 1517-1520 (1998)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] M.Sakaue: "The Effect of Interband Excitations on Time-Resolved Two-Photon Photoemission via a Localized State at a Metal Surface" Journal of the Physical Society of Japan. 67. 2058-2066 (1998)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] Y.Kawahito: "Effects of Intra-site Coulomb Interaction on Quantized Conductance in a Quantum wire between an STM-tip and a Metal Surface" Surface Science. 409. L709-L714 (1998)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] T.Kawasaka: "Adsorbate-Induced Charge Density Oscillations and Many-Body Effects in STM Image" Physics Letters A. 250. 403-407 (1998)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] A.Fukui: "A Model Calculation for Dissociative Scattering of Hydrogen Molecules from Metal Sufaces" Journal of the Physical Society of Japan. 67. 4201-4208 (1998)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] K.Hasegawa: "Dynamics of STM-Induced CO Desorption from Cu(111)" Journal of the Physical Society of Japan. 67. 4018-4021 (1998)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] W.A.Dino: "Dynamical Quantum Filtering in Hydrogen-Surface Reactions" Surface Science Letters. 418. L39-L44 (1998)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] Y.Kawahito: "Quantum Transport in an Atom-sized Bridge between a Metal Surface and a Tip of a Scanning Tunneling Microscope at Finite Temperatures" Journal of Applied Physics. 85. 947-952 (1999)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] 笠井秀明: "日独科学協力事業「表面動的過程の物理に関するセミナー」" 表面科学. 19. 210-212 (1998)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] 笠井秀明: "金属表面での電子遷移誘起脱離" 表面科学. 19. 629-634 (1998)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] Y.Miura: "Rotational and Vibrational Coupling Effects on the Dissociative Adsorption and Associative Desorption Dynamics of D_2/Cu(111)" Journal of the Physical Society of Japan. 68・3. (1999)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] M.Sakaue: "Effect of Coulomb Interactions between Photoexcited Electrons and Holes on Time-Resolved Two-Photon Photoemission from a Metal Surface" Journal of the Physical Society of Japan. 68・3. (1999)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] A.Okiji: "Proceedings of the International Symposium on Dynamical Quantum Processes on Solid Surfaces" North-Holland(Surface Science 363), 456 (1996)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] A.Okiji: "Elementary Processes in Excitations and Reactions on Solid Surfaces" Springer Verlag(Springer Series in Solid-State Sciences 121), 243 (1996)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] W.A.Dino: "Combined Effect of Molecular Rotational-and Surface Vibrational-Excitations on the Dissociative Adsorption Dynamics of D_2/Cu (111)" Surface Science. 363. 52-61 (1996)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] H.Kasai: "A Microscopic Theory of Desorption Induced by Electronic Transitions" Surface Science. 363. 214-222 (1996)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] H.Tsuchiura: "Effects of Electronic Excitations on Potential Energy Surfaces : Simple Model Calculations" Surface Science. 363. 274-280 (1996)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] A.Okiji: "The Effects of the Electronic Excitation on the Behavior of Particles Scattered by Metal Surfaces" Springer Series in Solid-State Sciences. 121 (Springer, Berlin). 138-146 (1996)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] H.Kasai: "On the Molecular Orientation Dependence of Dynamical Processor on Solid surfaces : Dissociative Adsorption and Scattering" Springer Series in Soild-State Sciences. 121 (Springer, Berlin). 99-111 (1996)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] W.A.Dino: "Role of the Rotational Motion in the Dissociative Adsorption and Associative Desorption Dynamics of D_2/Cu (111)" Physical Review Letters. 78. 286-289 (1997)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] H.Tsuchiura: "A.Model Calculation for Photo-Stimulated Desorption" Journal of the Physical Society of Japan. 66. 2805-2810 (1997)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] W.A.Dino: "Rotational Effects in the Dissociative Adsorption Dynamics of Hydrogen on a Pd Surface" Journal of the Physical Society of Japan. 66. 33344-3347 (1997)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] M.Sakaue: "Transient Population of Photoexcited Electrons in a Localized State at a Metal Surface" Journal of the Physical Society of Japan. 66. 3718-3721 (1997)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] A.Okiji: "Molecular Orientation Dependence of Dynamical Processes on Metal Surfaces : Dissociative Adsorption and Scattering, and Associative Desorption" Proceedings of International Workshop on the Current Problems in Condensed Matter : Theory and Experiments (plenum Press). 275-282 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] W.A.Dino: "Rotational Alignment in the Associative Desorption Dynamics of Hydrogen Molecules from Metal Surfaces" Journal of the Physical Society of Japan. 67. 1517-1520 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] M.Sakaue: "The Effect of Interband Excitations on Time-Resolved Tow-Photon Photoemission via a Localized State at a Metal Surface" Journal of the Physical Society of Japan. 67. 2058-2066 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] Y.Kawahito: "Effects of Intra-site Coulomb Interaction on Quantized Conductance in a Quantum wire between an STM-tip and a Metal Surface" Surface Science Letters. 409. L709-L714 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] T.Kawasaka: "Adsorbate-Induced Charge Density Oscillations and Many-Body Effects in STM Image" Physics Letters A. 250. 403-407 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] A.Fukui: "A Model Calculation for Dissociative Scattering of Hydrogen Molecules from Metal Surfaces" Journal of the Physical Society of Japan. 67. 4201-4208 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] K.Hasegawa: "Dynamics of STM-Induced CO Desorption from Cu(111)" Journal of the Physical Society of Japan. 67. 4018-4021 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] W.A.Dino: "Dynamical Quantum Filtering in Hydrogen-Surface Reactions" Surface Sicence Letters. 418. L39-L44 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] Y.Kawahito: "Quantum Transport in an Atom-sized Bridge between a Metal Surface and a Tip of a Scanning Tunneling Microscope at Finite Temperatures" Journal of Applied Physics. 85. 947-952 (1999)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] Y.Miura: "Rotational and Vibrational Coupling Effects on the Dissociative Adsorption and Associative Desorption Dynamics of D_2/Cu (111)" Journal of the Physical Society of Japan. 68(in press). (1999)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] M.Sakaue: "Effect of Coulomb Interactions between Photoexcited Electrons and Holes on Time-Resolved Tow-Photon Photomission from a Metal Surface" Journal of the Physical Society of japan. 68(in press). (1999)

    • Description
      「研究成果報告書概要(欧文)」より

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Published: 1999-12-08  

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