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1998 Fiscal Year Final Research Report Summary

the search of the orbital ordering of the magnetic moment by using x-ray magnetic scattering

Research Project

Project/Area Number 09440128
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Research Field 固体物性Ⅱ(磁性・金属・低温)
Research InstitutionTohoku University

Principal Investigator

ENDOH Yasuo  Tohoku University, Department of Physics, Professor, 大学院・理学研究科, 教授 (00013483)

Co-Investigator(Kenkyū-buntansha) SATO Nariaki  Tohoku University, Department of Physics, Research Physicist, 大学院・理学研究科, 助手 (30170773)
YAMADA Kazuyoshi  Kyoto University, Institute for Chemical Research, Professor, 科学研究所, 教授 (70133923)
HIROTA Kazuma  Tohoku University, Department of Physics, Assistant Professor, 大学院・理学研究科, 助教授 (90272012)
MIZUKI Junichiro  Tohoku University, Department of Physics, Professor, 大学院・理学研究科, 教授
Project Period (FY) 1997 – 1998
Keywordsorbital ordering / x-ray magnetic scattering / ATS scattering / Jahn Teller effect / synchrotron radiation / manganites / neutron scattering / lift of orbital
Research Abstract

We have studied the "high temperature superconductivity " and /or "colossal magnetoresistance (CMR)" as the key phenomena in the strongly correlated electron systems. In order to explore this important issue, we initiated to investigate a novel degree of freedom of "order" by using new technique of the synchrotron x-ray scattering besides neutron scattering.
First we studied carefully the mechanism of the resonant x-ray scattering of the orbital order occurred at the energy of K edge of the magnetic metal element, actually Mn cations. Then we found the mechanism that the intra Coulomb interaction between 4p and 3d orbital which is in the orbital ordered state lifts the 4p degeneracy. Then it gives rise an enhancement or resonance. Then we deeply studied the orbital order in LaMnO_3 originated by the Jahn Teller effect by using this newly established technique of the synchrotron x-ray scattering.
Second, we also extend this technique to study the phase transition of metal insulator in the doped manganites as recognized the CMR materials. We found that the phase transition is triggered by the orbital order-disorder transition.
Third, we extend this project studied during the recent two years granted to a new project aiming the standard probe of studying the orbital fluctuations.

  • Research Products

    (37 results)

All Other

All Publications (37 results)

  • [Publications] K.Hirota, Y.Endoh et al.: "Neutron-Scattering Studies of Magnetic Excitations in La_<1-X>Sr_XMnO_3 : A Dimensional Crossover" Physica B. 237-238. 36-38 (1997)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] Y.Endoh et al.: "Polarized Neutron Studies for Cr Excitations" J.Phys.Soc.Jpn.66. 1615-1617 (1997)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] N.Sato, Y.Endoh et al.: "Spin Fluctuations in the Heavy Fermion Superconductor UPd_2Al_3 Studied by Neutron Inelastic Scattering" J.Phys.Soc.Jpn.66. 1884-1887 (1997)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] Y.Endoh and K.Hirota: "Scaling of Spin-Wave Stiffness Constant to Curie Temperature in the Colossal Magnetoresistance Material La_<1-X>Sr_xmnO_3" J.Phys.Soc.Jpn.66. 2264-2267 (1997)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] M.A.Kastner, Y.Endoh: "Magnetic, Transport. and Optical Properties of Monolayer Copper Oxides" Rev.Mod.Phys.70. 897-928 (1998)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] K.Yamada, Y.Endoh et al.: "Doping Dependence of the Spatially Modulated Dynamical Spin Correlations and the Superconducting-Transition Temperature in La_<2-x>Sr_xCuO_4" Phys.Rev.B57. 6165-6172 (1998)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] S.Mitsudo, Y.Endoh et al.: "Submillimeter Wave ESR Measurement of LaMnO_3" J.Magn.Magn.Mater.177-181. 877-878 (1998)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] K.Hirota, Y.Endoh et al.: "Magnetic Excitations of Bandwidth-Controlled Mn Perovskite(La_<1-x-y>Y_y)Sr_xMnO_3" J.Magn.Magn.Mater.177-181. 864-866 (1998)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] K.Hirota, Y.Endoh: "Neutron-Diffraction Studies on the Magnetic Ordering Process in the Layered Mn Perovskite La_<2-2x>Sr_<1+2x>Mn_2O_7(x=0.40, 0.45 and 0.48)" J.Phys.Soc.Jpn.67. 3380-3383 (1998)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] Y.Murakami, Y.Endoh et al.: "Resonant X-ray Scattering from Orbital Ordering in LaMnO_3" Phy.Rev.Lett.81. 582-585 (1998)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] N.Bernhoeft, Y.Endoh et al.: "Enhancement of Magnetic Fluctuations on Passing below T_c in the Heavy Fermion Superconductor UPd_2Al_3" Phy.Rev.Lett.81. 4244-4247 (1998)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] N.Sato, Y.Endoh et al.: "Observation of Two-Energy Responses in Upd2Al3-Interaction of Magnetism and Superconductivity?" J.Alloys Comp.271-273. 433-436 (1998)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] Y.Endoh, K.Hirota et al.: "Field Induced Transition from Metal to Insulator in the CMR Manganites" Mat.Sci.Eng.B in press. (1999)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] M.Takahasi and J.Mizuki: "An Additional Axis for the Surface X-ray Diffractometer" J.Synchrotron Rad.5. 893-895 (1998)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] M.Kubota, K.Hirota, Y.Endoh et al.: "Neutron Scattering Studies on Magnetic Structure of the Duble-Layered Manganite La_<2-2x>Sr_<1+2x>Mn_2O_7(0.30【less than or equal】x【less than or equal】0.50)" J.Phys.Chem.Solid.in press. (1999)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] M.Takata, J.Mizuki et al.: "The MEM Charge Density Study of Rb_2CsC_<60>, K_2RbC_<60> and Li_2CsC_<60> by Synchrotron Radiation Powder Method." Jpn.J.Appl.phys.in press. (1999)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] H.Fujioka, K.Hirota, Y.Endoh: "Spin Dynamical Properties of the Layered Perovskite La_<1.2>Sr_<1.8>Mn_2O_7" J.Phys.Chem.Solid.in press. (1999)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] Y.Endoh et al.: "Colossal Magnetoresistive Oxides in Advances in condensed Matter Science" Elsevier, 432 (1999)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] 遠藤康夫 他編: "電子と物理" 丸善, 200 (1998)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] K.Hirota, Y.Endoh et al.: "Neutron-Scattering Studies of Magnetic Excitations in La_<1-x>Sr_xMnO_3 : ADimensional Crossover" Physica B. 237-238. 36-38 (1997)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] Y.Endoh et al.: "Polarized Neutron Studies for Cr-Excitations" J.Phys.Soc.Jpn.66. 1615-1617 (1997)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] Y.Endoh and K.Hirota: "Scaling of Spin-Wave Stiffness Constant to Curie Temperature in the Colossal Magnetoresistance Material La_<1-x>Sr_xMnO_3" J.Phys.Soc.Jpn.66. 2264-2267 (1997)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] N.Sato, Y.Endoh et al.: "Spin Fluctuations in the Heavy Fermion Superconductor Dpd_2Al_3 Studied by Neutron Inelastinc Scattering" J.Phys.Soc.66. 1884-1887 (1997)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] M.A.Kastner, Y.Endoh et al.: "Magnetic, Transport and Optical Properties of Monolayer Copper Oxides" Rev.Mod.Phys.70. 897-928 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] K.Yamada, Y.Endoh et al.: "Doping Dependence of the Spatially Modulated Dynamical Spin Correlations and the Superconducting-Transition Temperature in La_<2-x>Sr_xCuO_4" Phys.Rev.B57. 6165-6172 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] S.Mitsudo, Y.Endoh et al.: "Submillimeter wave ESR measurement of LaMnO_3" J.Magn.Magn.Mater.177-181. 877-878 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] K.Hirota, Y.Endoh et al.: "Magnetic excitations of bandwidth-controlled Mn Perovskite (La_<1-x-y>Y_y) Sr_xMnO_3" J.Magn.Magn.Mater.177-181. 864-866 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] K.Hirota, Y.Endoh et al.: "Neutron-Diffraction Studies on the Magnetic Ordering Process in the Layered Mn Perovskite La_<2-2x>Sr_<1+2x>Mn_2o_7 (x=0.40,0.45 and 0.48)" J.Phys.Soc.Jpn.67. 3380-3383 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] Y.Murakami, Y.Endoh et al.: "Resonant X-ray Scattering from Orbital Ordering in LaMnO_3" Phy.Rev.Lett.81. 582-585 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] "Observation of Two-Energy Responses in Upd_2Al_3-Interaction of Magnetism and Superconductivity?" J.Alloys Comp.271-273. 433-436 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] N.Bernhoeft, Y.Endoh et al.: "Enhancement of Magnetic Fluctuations on Passing below T_c in the Heavy Fermion Superconductor UPd_2 Al_3" Phys.Rev.Lett.81. 4244-4247 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] M.Takahasi, J.Mizuki: "An Additional Axis for the Surface X-ray Diffractometer" J.Synchrotron Rad.5. 893-895 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] Y.Endoh, K.Hirota et al.: "Field induced transition from metal to insulator in the CMR manganites" Mat.Sci.Eng.B. (in press).

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] M.Kubota, K.Hirota, Y.Endoh et al: "Neutron Scattering Studies on Magnetic Structure of the Duble-Layered Manganite La_<2-2x>Sr_<1+2x>Mn_2O_7 (0.30<less than or equal>x<less than or equal>0.50)" J.Phys.Chem.Solid. (in press).

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] H.Fujioka, K.Hirota, Y.Endoh et al.: "Spin Dynamical Properties of the Layered Perovskite La_<1.2>Sr_<1.8>Mn_2O_7" J.Phys.Chem.Solid. (in press).

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] M.Takata, J.Mizuki et al.: "The MEM Charge Density Study of Rb_2CsC_<60>, K_2RbC_<60> and Li_2CsC_<60> by Synchrotron Radiation Powder Method" Jpn.J.Appl.Phys.(in press).

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] Y.Endoh et al.: "Colossal Magnetoresistive Oxides in Advances in condensed Matter Science, "Review of Spin Dynamics and Orbital Ordering"" Elsevier. 432 (1999)

    • Description
      「研究成果報告書概要(欧文)」より

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Published: 1999-12-08  

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