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2001 Fiscal Year Final Research Report Summary

Charge-Orbital Ordered States in Manganese Oxides studied by High Resolution Electron Microscopy

Research Project

Project/Area Number 11440104
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Research Field 固体物性Ⅱ(磁性・金属・低温)
Research InstitutionTokyo Institute of Technology

Principal Investigator

YAMAMOTO Naoki  Tokyo Institute of Technology, Physics Department, Assoc. Professor, 大学院・理工学研究科, 助教授 (90108184)

Co-Investigator(Kenkyū-buntansha) MORI Shigeo  Osaka Prefecture University, Dept. Materials Science, Assoc. Professor, 総合科学部, 助教授 (20251613)
Project Period (FY) 1999 – 2001
KeywordsManganese oxides / Correlated electron system / transition metal oxide / Nano-structure / Charge order / colossal magneto resistance / Lorenz electron microscopy / magnetic structure
Research Abstract

Manganese oxides show several characteristic properties such as metal-insulator phase transition, colossal magneto resistance and charge-orbital ordered phases due to strong interactions among charge/orbitals of d electrons, their spin system, and lattice system, Recently by transmission electron microscopy we found the coexistence of the charge ordered (CO) phase and ferromagnetic metal (FM) phase, which are closely related to the colossal magneto resistance and charge-orbital ordered phases. In the present study we investigated nano-structure of the phase separated state and charge/orbital ordered structure using a high resolution transmission electron microscope and Lorenz electron microscope. We observed the coexistence of the CO phase and FM phase in La_<1-x>Ca_xMnO_3, and found that the paired Jahn-Teller stripes (PJTS) play an important role in forming nano-structures of the coexistence state. The effect of substitution of the Mn site with Cr ion is also studied. Lorenz electron microscope reveals that large domains of FM phase and CO phase coexist on a micrometer scale in (La_<5/8-x>Pr_x)Ca_<3/8>MnO_3.

  • Research Products

    (23 results)

All Other

All Publications (23 results)

  • [Publications] R.Shoji, S.Mori, N.Yamamoto, A.Machida, Y.Moritom: "Phase separation and destabilization in the charge ordered state of the Cr-doped manganites"J.Phys.Soc.Jpn. 70. 267 (2001)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] K.Matsuno, T.Katsufuji, S.Mori, Y.Moritomo, et al.: "Charge ordering in the geometrically frustrated spinelAlV_2O_4"J.Phys.Soc.Jpn. 70,No.6. 4801 (2001)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] T.Katsufuji, S Mori, M.Masaki, Y.Moritomo, et al.: "Dielectric and magnetic anomalies and spin frustration in hexagonal RMnO3(R=Y, Yb, and Lu)"Phys.Rev.B. 64. 104419 (2001)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] A.Machida, Y.Moritomo, S.Mori, N.Yamamoto et al.: "Microscopic charge separation in Tb_<1-X>Ca_xMnO_3 (x〜1)"J.Phys.Soc.Jpn.. 71. 27 (2002)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] S.Mori, R.Shoji, N.Yamamoto, T.Katsufuji, A.Machda et al.: "Charge ordered state in the impurity-doped manganites"J.Phys.Soc.Jpn. (In press).

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] S.Mori, R.Shoji, N.Yamamoto, T.Katsufuji: "Impurity effect on the charge ordered state in mangnaites"J. Phys.and Chem. of Solids. (In press).

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] 山本直紀: "実験物理学講座5「構造解析」3-2節"丸善(株). 54 (2001)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] S.Mori, C.H.Chen and S-W. Cheong: "Pairing of charge-ordered stripes in La_<1-x>Ca_xMnO_3"Nature. 392. 473 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] S.Mori, C.H.Chen and S-W. Cheong: "Paired and unpaired charge stripes in the ferromagnetic phase of La_<0.5>Ca_<0.5>MnO_3"Phys. Rev. Lett.. 81. 3972 (1998)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] Y.Moritomo, A.Machida, S.Mori, N.Yamamoto and A.Nakamura: "Electronic phase diagram of Cr-doped manganites"Phys. Rev.. B60. 9220 (1999)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] S.Mori, T.Katsufuji, N.Yamamoto, C.H.Chen, and S-W.Cheong: "Microstructure related to charge and orbital ordering in Pr_<0.5>Ca_<0.5>MnO_3"Phys. Rev.. B59. 13573 (1999)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] T.Katsufuji, S-W.Cheong, S.Mori and C.H.Chen: "Impurity effects on the Electronic/Magnetic ground states of Perovskite Manganites"J. Phys. Soc. Jpn.. 68. 1090 (1999)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] N.Fukumoto, S.Mori, N.Yamamoto, Y.Moritomo, T.Katsufuji, C.H.Chen and S-W.Cheong: "Structural feature related to charge ordering and metal-insulator transition in Nd_<0.5>Sr_<0.5>MnO_3"Phys. Rev. B60. 12963 (1999)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] M.Uehara, S.Mori, C.H.Chen and S-W.Cheong: "Percolative phase separation and Colossal Magnetroresistance in mixed-valence manganites"Nature. 399. 560 (1999)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] C.H.Chen, S.Mori and S-W.Cheong: "Anomalous melting transition of the charge-ordered state in manganites"Phys. Rev. Lett.. 83. 4792 (1999)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] A.Machida, Y.Moritomo, N.Nishibori, M.Tanaka, M.Sakata, K.Ohyama, S.Mori, N.Yamamoto and A.Nakamura: "Phase separation and insulator-metal behavior of doped manganites"Phys. Rev.. B62. 3883-3887 (2000)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] A.Machida, M.Itoh, Y.Moritomo, S.Mori, N.Yamamoto, K.Ohoyama and A.Nakamura: "Electronic phase diagram in bandwidth controlled manganites"Physica. B281&282. 524 (2000)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] R.Shoji, S.Mori, N.Yamamoto, A.Machida and Y.Moritomi: "Phase separation and destabilization in the charge ordered state of the Cr-doped manganites"J. Phys. Soc. Jpn.. 70. 267 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] K.Matsuno, T.Katsufuji, S.Mori, Y.Moritomo, A.Machida, and H.Takagi: "Charge ordering in the geometrically frustrated spinelAlV_2O_4"J. Phys. Soc. Jpn.. 70, No.6. 4801-4804 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] T. Katsufuji, S. Mori, M. Masaki, Y. Moritomo, N. Yamamoto, and H. Takagi: "Dielectric and magnetic anomalies and spin frustration in hexagonal RMnO3(R=Y, Yb, and Lu)"Phys. Rev.. B64. 104419 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] A. Machida, Y. Moritomo, S. Mori, N. Yamamoto, K. Ohoyama, E. Nishibori, M. Takata, M. Sakata, T. Otomo, and A. Nakamura: "Microscopic charge separation in Tb_<1-x>Ca_xMnO_3 (x〜1)"J. Phys. Soc. Jpn.. 71, 27. (2002)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] S.Mori, R.Shoji, N.Yamamoto, T.Katsufuji, A.Machida and Y. Moritomo: "Charge ordered state in the impurity-doped manganites"J. Phys. Soc. Jpn.. (in press).

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] S.Mori, R.Shoji, N.Yamamoto, T.Katsufuji: "Impurity effect on the charge ordered state in mangnaites"J. Phys. and Chem. of Solids. (in press).

    • Description
      「研究成果報告書概要(欧文)」より

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Published: 2003-09-17  

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