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2001 Fiscal Year Final Research Report Summary

Quantum Critical Phenomena in Heavy-Fermion System under Pressures

Research Project

Project/Area Number 11440111
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Research Field 固体物性Ⅱ(磁性・金属・低温)
Research InstitutionHIROSHIMA UNIVERSITY

Principal Investigator

TAKABATAKE Toshiro  Hiroshima University, Grad. School of Advanced Sciences of Matter, Prof., 大学院・先端物資科学研究科, 教授 (40171540)

Co-Investigator(Kenkyū-buntansha) IGA Fumitoshi  Hiroshima University, Grad. School of Advanced Sciences of Matter, Assoc. Prof., 大学院・先端物資科学研究科, 助教授 (60192473)
UMEO Kazunori  Hiroshima University, Grad. School of Advanced Sciences of Matter, Res. Assoc., 大学院・先端物資科学研究科, 助手 (10223596)
Project Period (FY) 1999 – 2001
KeywordsPressure / Quantum Critical Phenomena / Heavy Fermion System / Spin Fluctuation / Antiferromagnetism / Single Crystal / Uniaxial Pressure / Crystal Field
Research Abstract

We studied the quantum critical phenomena of heavy fermion systems under pressures by means of high-quality single crystals. New findings are as followings.
1. Hexagonal heavy fermion system Ce_7Ni_3 : Ce_7Ni_3 undergoes tow antiferromagnetic transitions at 1.8 K and 0.7 K. The antiferromagnetic order vanishes at B//c = 0.3 T. For B//c > 0.6 T, a new magnetic ordered phase appears below 0.5 K. For 0.3 T < B//c < 0.6 T, the specific heat C follows the form of C/T∝-lnT, so called non-Fermi-liquid behavior. The origin of the field-induced magnetic phase may be attributed to a geometrical frustration in the magnetic moment of Ce sites formed a quasi-regular tetrahedron
2 Uniaxial-pressure induced magnetic order in CeNiSn : CeNiSn is a paramagnetic semimetal with a pseudo-gap. By applying the uniaxial pressure of 0.13 GPa along the c axis, an antiferromagnetic order appears at around 3 K. For P//a, however, the density of carriers increases. The Kondo temperature for the crystal field ground state estimated by the resistivity for P//c is suppressed with pressure. Therefore, we may deduce that the formation of magnetic order is attributed to the weakened hybridization in a-b plane between the 4f electrons for the crystal field ground state and conduction electrons.
3 Non Fermi liquid behavior in Ce_2Rh_3Ge_5 under pressures : The critical pressure Pc where the antiferromagnetic order of orthorhombic Ce_2Rh_3Ge_5 with T_N = 4.9 vanishes was estimated to be 0.45 GPa. Even for P>3Pc, non-Fermi-liquid behavior is observed in both the resistivity ρ and the susceptibility χ : ρ ∝T^<1.45> and χ ∝1-T^<0.27>. Because the magnetization hardly decreases for P = 3Pc, the origin of the non-Fermi-liquid behavior may be due to a short-rang magnetic order of the remaining local moments.

  • Research Products

    (32 results)

All Other

All Publications (32 results)

  • [Publications] K.Umeo: "Magnetic instability in Ce_7Ni_3 studied by low-temperature specific heat and magnetic suscetibility"Physica B. 259-261. 407-408 (1999)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] K.Izawa: "Metallic ground state of CeNiSn"Phys.Rev.B. 59. 2599-2603 (1999)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] T.Takabatake: "Impurity-induced localization of quasiparticles in the presence of a pseudogap in CeNiSn"Phys.Rev.B. 59. 13878-13881 (1999)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] K.Umeo: "Uniaxial-Stress Induced Magnetic Order in CeNiSn"Phys.Rev.B. 60. R6957-R6960 (1999)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] Z.Hossain: "Antiferromagnetic Kondo-lattice systems Ce_2Ph_3Ge_5 and Ce_2Ir_3Ge_5 with moderate heavy-fermion behavior"Phys.Rev.B. 60. 10383-10387 (1999)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] Y.Echizen: "Effect of Kondo-hole impurity on the pseudogap in CeNiSn"Physica B. 259-261. 292-293 (1999)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] H.Kadowaki: "Incommensurate Magnetic Structure of the Heavy Fermion Antiferromagnet Ce_7Ni_3"J.Phts.Soc.Jpn.. 69. 2269-2279 (2000)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] S.Mishima: "Nuclear magnetic resonance and nuclear quadruple resonance studies of ^<61>Ni in heavy fermion compound Ce_7Ni_3"Solid State Communications. 87. 5134-5136 (2000)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] Y.Echizen: "Magnetic ordering in single crystal CeNi_<0.82>Cu_<0.18>Sn"Solid State Communications. 115. 587-591 (2000)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] T.Yoshino: "High-field susceptibility of Kondo semimetals CeNiSn and CeRhSb"Physica B. 281&282. 291-293 (2000)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] Y.Bando: "Thermoelectric power of CeNi_<1-x>T_xSn(T=Co, Cu, Pt) and Ce_<1-y>La_ySn(x, y=0.01 and 0.05)"Physica B. 281&282. 294-295 (2000)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] K.Motoya: "Neutron scattering study of heavy fermion antiferromagnet Ce_7Ni_3 under pressure"J.Magn.Magn.Mater.. 226-230. 137-138 (2001)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] A.Schenck: "Muon-spin-rotation study of Ce_7Ni_3:muon-related and intrinsic properties of the paramagnetic phase"J.Phys.: Cond.Matter. 13. 4277-4290 (2001)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] T.Terashima: "Magnetoresitance and magnetic susceptibility in CeNiSn"Physica B. 294-295. 245-248 (2001)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] K.Umeo: "Pressure-induced magnetic instability in Ce_2Ph_3Ge_5"Phys.Rev.B. 64. 144412-144419 (2001)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] K.Umeo: "Non-Fermi Liquid Behavior in Ce_2Ph_3Ge_5 above the Critical Pressure of the Antiferromagnetic Instability"Physica B. (in press). (2002)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] K. Umeo et al.: "Magnetic instability in Ce_7Ni_3 studied by low-temperature specific heat and magnetic susceptibility"Physica B. 259-261. 407-408 (1999)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] K. Izawa et al.: "Metallic ground state of CeNiSn"Phys. Rev. B. 59. 2599-2603 (1999)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] T. Takabatake et al.: "Impurity-induced localization of quasiparticles in the presence of a pseudogap in CeNiSn"Phys. Rev. B. 59. 13878-13881 (1999)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] K. Umeo et al.: "Uniaxial-Stress Induced Magnetic Order in CeNiSn"Phys. Rev. B. 60. R6957-R6960 (1999)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] Z. Hossain et al.: "Antiferromagnetic Kondo-lattice systems Ce_2Rh_3Ge_5 and Ce_2Ir_3Ge_5 with moderate heavy-fermion behavior"Phys. Rev. B. 60. 10383-10387 (1999)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] Y. Echizen et al.: "Effect of Kondo-hole impurity on the pseudogap in CeNiSn"Physica B. 259-261. 292-293 (1999)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] H. Kadowaki et al.: "Incommensurate Magnetic Structure of the Heavy Fermion Antiferromagnet Ce_7Ni_3"J. Phys. Soc. Jpn.. 69. 2269-2279 (2000)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] S. Mishima et al.: "Nuclear magnetic resonance and nuclear quadrupole resonance studies of ^<61>Ni in heavy fermion compound Ce_7Ni_3"J. Appl. Phys.. 87. 5134-5136 (2000)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] Y. Echizen et al.: "Magnetic ordering in single crystal CeNi_0 _<82>Cu_0 _<18>Sn"Solid State Commun.. 115. 587-591 (2000)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] T. Yoshino et al.: "High-field susceptibility of Kondo semimetals CeNiSn and CeRhSb"Physica B. 281&282. 291-293 (2000)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] Y. Bando et al.: "Thermoelectric power of CeNi_<1-x>T_xSn (T = Co, Cu, Pt) and CeNi_<1-y>La_ySn (x, y = 0.01and 0.05)"Physica B. 281&282. 294-295 (2000)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] K. Motoya et al.: "Neutron scattering study of heavy fermion antiferromagnet Ce_7Ni_3 under pressure"J. Magn. Magn. Mater.. 226-230. 137-138 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] A. Schenck et al.: "Muon-spin-rotation study of Ce_7Ni_3 : muon-related and intrinsic properties of the paramagnetic phase"J. Phys. : Cond. Matter. 13. 4277-4290 (2000)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] T. Terashima et al.: "Magnetoresitance and magnetic susceptibility in CeNiSn"Physica B. 294-295. 245-248 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] K. Umeo et al.: "Pressure-induced magnetic instability in Ce_2Rh_3Ge_5"Phys. Rev. B. 64. 144412-144419 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] K. Umeo et al.: "Non-Fermi Liquid Behavior in Ce_2Rh_3Ge_5 above the Critical Pressure of the Antiferromagnetic Instability"Physica B. (in press). (2002)

    • Description
      「研究成果報告書概要(欧文)」より

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Published: 2003-09-17  

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