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2000 Fiscal Year Final Research Report Summary

Study of the Ultra Sensitive Detection of Hydrogen Isotope by the intense Lyman-α resonant ionization

Research Project

Project/Area Number 11650052
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeSingle-year Grants
Section一般
Research Field Applied optics/Quantum optical engineering
Research InstitutionHigh Energy Accelerator Research Organization(KEK)

Principal Investigator

MIYAKE Yasuhiro  KEK, Associate Professor, 物質構造科学研究所, 助教授 (80209882)

Co-Investigator(Kenkyū-buntansha) NISHIYAMA Kusuo  KEK, Professor, 物質構造科学研究所, 教授 (50164611)
SHIMOMURA Koichiro  KEK, Research Associate, 物質構造科学研究所, 助手 (60242103)
NAGAMINE Kanetada  KEK, Professor, 物質構造科学研究所, 教授 (50010947)
MATSUDA Yasuyuki  RIKEN, Researcher, ミュオン科学, 研究員
Project Period (FY) 1999 – 2000
KeywordsHyrdorgen / Lymanα Light / Lemanα / Difference Frequency / Resonant Ionization / Wave mixing / Deuterium / VUV / Laser
Research Abstract

We have been pursuing an ultra-sensitive method for detecting and extracting hydrogen isotopes by utilizing a resonant ionization cheme via the {1S→2P→unbound} transition. A time-of-flight measurement using the pulsed lasers coupled with a mass separation device enables us to distinguish any hydrogen isotope with a very low background. By preparing a new "Slow Ion Optics" set-up to extract hydrogen isotope ions efficiently, the detection limit of the present method was improved to be much better than 3x10^3 cm^<-3>.
In the case of the laser induced fluorescence technique using Lyman-α or Balmer-α photons, the lowest detection limit is reported to be as low as the order of 10^7-10^9 cm^<-3>, or 10^7 cm^<-3>, respectively. In the case of the two-phone induced Balmer-α emission the detection limit is reported to be same order as that by three photon ionization, 3 X 10^9 cm^<-3>.
The detection limit of the present Lyman-α resonant ionization method can be evaluated by the following procedure … More . Assuming the probability of H_2 dissociation at the W surface at 2000 K to be 10% in 9.5 x 10^<-8> mbar of H_2 gas, about 3 x 10^7 H atoms exist in a volume of about 0.6 cm^3, which is the effective volume of extraction along the laser passage. Since we obtained an MCP signal of 4.5V with a temporal width of 80 ns at 2000 K, in contrast with that of 2 mV with 20 ns for a signle event, we can evaluate the number of 9000 H atoms per laser pulse that are extracted at 2000 K.From this, the extraction and detection efficiency is calculated to be 3 x 10^<-4>. Since the residual gas is not likely to be completely consisted of hydrogen molecules, the detection limit of the present Lyman-α resonant ionization method is estimated to be better than 3 x 10^3 cm^<-3>. It is thus 3 - 5 orders of magnitude better than the other methods. And also it is improved at least more than 2.5 times compared with that of our previous report and it is highest that we know of. The method of applying Lyman-α resonant ionization spectroscopy can be recognized as an ultra sensitive and efficient mass-selection technique. Less

  • Research Products

    (16 results)

All Other

All Publications (16 results)

  • [Publications] Y.Miyake et al.: "Thermionic Emission of Mu, H, D and T from hot W"Surface Science. 433-435. 785-789 (1999)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] Y.Miyake et al.: "Construction of the experimental set-up for ultra slow muon generation by thermal Mu ionization method at RIKEN-RAL"Physica B. 289-290. 666-669 (2000)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] 三宅 康博: "超低速ミュオンの発生法の開発と、関連して得られたタングステン表面における水素原子同位体脱離過程の研究"真空 J.Vac.Soc.Jpn.. 43,2. 126-134 (2000)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] 三宅 康博: "英国理研・ラザフォード研究施設に於けるライマンαを用いた超低速ミュオン研究"光学. 29,11. 696-701 (2000)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] Y.Miyake et al.: "ULTRA SLOW MUON GENERATION BY LASER RESONANT IONIZATION TOWARDS THE 21ST CENTURY"Rad.Phys.Chem.. 60・4-5. 521-524 (2001)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] Y.Miyake et al.: "Improvement of the detection limit of hydrogen by Lyman-α RIS"Resonant Ionization Spectroscopy(2000). (2001)

    • Description
      「研究成果報告書概要(和文)」より
  • [Publications] Y.Miyake, K.Shimomura, P.Strasser, Y.Matsuzaki, S.N.Nakamura, K.Ishida, T.Matuszaki, I.Watanabe, S.Makimura, J.P.Marangos, R.Scheuermann, P.Bakule and K.Nagamine: "Ultra slow muon generation by laser resonant ionization at the RIKEN-RAL Muon Facility"RIKEN Review. No.20. 55-57 (1999)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] Y.Miyake, K.Shimomura, A.P.Mills, Jr., J.P.Marangos and K.Nagamine: "Therminic Emission of Mu, H, D and T from hot W"Surface Science. 433-435. 785-789 (1999)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] Y.Miyake ; Muon Science in Japan: "Muon Science in the joint project"ENERGY REVIEW. 12. 16-17 (1999)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] Y.Miyake, K.Shimomura, A.P.Mills, Jr., J.P.Marangos and K.Nagamine, ; Therminic Emission of Mu, H, D and from hot W: "MSL99 KEK Proceedins 99-11"HJHF99-5. 1656-168 (1999)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] Y.Miyake, K.Shimomura, Y.Matsuda, R.J.Scheuermann, P.Bakule, S.Makimura, P.Strasser, S.N.Nakamura, K.Ishida, T.Matuszaki, I.Watanabe, and K.Nagamine: "Construction of the experimental set-up for ultra slow muon generation by Thermal Mu ionization method at RIKEN-RAL"Physica B. 289-290. 666-669 (2000)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] Y.Miyake: "Ultra Slow Muon Generation and Thermionic Emission of Hydorogen Isotopes From tungsten surface(in Japanese)"J.Vac. Soc. Jpn.. 43, 2. 126-134 (2000)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] Y.Miyake: "Ultra slow muon generationby Lyman-a resonant ionization method at RIKEN/RAL facility"KOGAKU. 29, 11. 696-701 (2000)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] Y.Miyake, K.Shimomura, S.Makimura, Y.Matsuda, P.Bakule, R.J.Scheuermann, and K.Nagamine: "ULTRA SLOW MUON GENERATION BY LASER RESONANT IONIZATION TOWARDS THE 21ST CENTURY"Rad. Phys. Chem.. 60/4-5. 521-524 (2001)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] Y.Miyake, S.Makimura, K.Shimomura, Y.Matsuda, P.Bakule, P.Strasser R.J.Scheuermann, and K.Nagamine: "Improvement of the detection limit of hydrogen by Lyman-α RIS"Resonant Ionization Spectroscopy. (in press). (2001)

    • Description
      「研究成果報告書概要(欧文)」より
  • [Publications] Y.Miyake, S.Makimura, K.Shimomura, Y.Matsuda, P.Bakule, R.J.Scheuermannm, and K.Nagamine: "A new method to obtain a 212 nm laser source for Lyman-α light with CLBO crystals"Resonant Ionization Spectroscopy. (in press). (2001)

    • Description
      「研究成果報告書概要(欧文)」より

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Published: 2002-03-26  

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